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Investigation of photo-induced carrier dynamics in solar cells consisting of multinary compound semiconductors using photo-assisted nanoprobes

Research Project

Project/Area Number 17H02783
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Thin film/Surface and interfacial physical properties
Research InstitutionThe University of Tokyo

Principal Investigator

Takahashi Takuji  東京大学, 生産技術研究所, 教授 (20222086)

Project Period (FY) 2017-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥17,550,000 (Direct Cost: ¥13,500,000、Indirect Cost: ¥4,050,000)
Fiscal Year 2020: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Fiscal Year 2019: ¥3,900,000 (Direct Cost: ¥3,000,000、Indirect Cost: ¥900,000)
Fiscal Year 2018: ¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2017: ¥5,980,000 (Direct Cost: ¥4,600,000、Indirect Cost: ¥1,380,000)
Keywordsナノプローブ / 多元系化合物半導体 / 太陽電池 / 光励起キャリア / 光起電力 / 再結合プロセス
Outline of Final Research Achievements

Photo-assisted nanoprobe methods such as photo-assisted Kelvin probe force microscopy (P-KFM) and photothermal mode atomic force microscopy (PT-AFM) have been developed and improved. By means of them, in addition, photo-induced carrier dynamics, especially their recombination property, in solar cells consisting of multinary compound semiconductor like Cu(In,Ga)(S,Se)2 have been investigated. Furthermore, the electrostatic force microscopy with multi-frequency bias modulation method which becomes a base of optical capacitance AFM (PCap-AFM) has been developed, and its validity has been confirmed through actual measurements on similar solar cells.

Academic Significance and Societal Importance of the Research Achievements

多くの場合に微結晶系となる太陽電池用多元系化合物半導体に対して、局所計測が可能な光援用ナノプローブ技術を適用することによって、結晶粒界が光励起キャリアの再結合プロセスに与える影響などの微視的な知見を得るといった学術的な成果を上げた。また、それらの知見は、同種太陽電池の将来的な特性改善への貢献が期待されるといった社会的な意義も持っている。

Report

(5 results)
  • 2021 Final Research Report ( PDF )
  • 2020 Annual Research Report
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • Research Products

    (54 results)

All 2022 2021 2020 2019 2018 2017

All Journal Article (7 results) (of which Peer Reviewed: 5 results) Presentation (47 results) (of which Int'l Joint Research: 29 results,  Invited: 10 results)

  • [Journal Article] Multi-pulse modulation method in photothermal atomic force microscopy for variable frequency modulation of incident light2021

    • Author(s)
      Yamada Ayaka、Takahashi Takuji
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 60 Issue: SE Pages: SE1003-SE1003

    • DOI

      10.35848/1347-4065/abf07b

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Direct imaging method of frequency response of capacitance in dual bias modulation electrostatic force microscopy2020

    • Author(s)
      Fukuzawa Ryota, Takahashi Takuji
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 59 Issue: 7 Pages: 078001-078001

    • DOI

      10.35848/1347-4065/ab9ae0

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dual Bias Modulation Electrostatic Force Microscopy on Cu(In, Ga)Se22020

    • Author(s)
      Fukuzawa Ryota, Minemoto Takashi, Takahashi Takuji
    • Journal Title

      Proceedings of 2020 47th IEEE Photovoltaic Specialists Conference (PVSC)

      Volume: 00 Pages: 0394-0396

    • DOI

      10.1109/pvsc45281.2020.9300457

    • Related Report
      2020 Annual Research Report
  • [Journal Article] Development of dual bias modulation electrostatic force microscopy for variable frequency measurements of capacitance2020

    • Author(s)
      Fukuzawa Ryota, Takahashi Takuji
    • Journal Title

      Review of Scientific Instruments

      Volume: 91 Issue: 2 Pages: 023702-023702

    • DOI

      10.1063/1.5127219

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photovoltage Decay Measurements by Photo-Assisted Kelvin Probe Force Microscopy on Cu(In,Ga)Se2 Solar Cells2019

    • Author(s)
      Hyeondeuk Yong, Takashi Minemoto, Takuji Takahashi
    • Journal Title

      IEEE Journal of Photovoltaics

      Volume: 9 Issue: 2 Pages: 483-491

    • DOI

      10.1109/jphotov.2018.2885835

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dependence of Photovoltage on Incident Photon Energies Investigated by Photo-assisted Kelvin Probe Force Microscopy on Cu(In,Ga)Se2 Solar Cells2018

    • Author(s)
      Hyeondeuk Yong, Takashi Minemoto, Takuji Takahashi
    • Journal Title

      2018 IEEE 7th World Conference on Photovoltaic Energy Conversion (WCPEC)

      Volume: 1 Pages: 1966-1969

    • DOI

      10.1109/pvsc.2018.8547957

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Local Measurements of Surface Capacitance by Electrostatic Force Microscopy on Cu(In,Ga)Se2 Materials2017

    • Author(s)
      Tomoaki Ishii, Takashi Minemoto, and Takuji Takahashi
    • Journal Title

      Proceedings of 2017 IEEE 44th Photovoltaic Specialist Conference (PVSC)

      Volume: 1 Pages: 455-458

    • DOI

      10.1109/pvsc.2017.8366110

    • Related Report
      2017 Annual Research Report
  • [Presentation] Cu(In,Ga)(S,Se)2太陽電池に対するCs処理効果の光熱モードAFMによる検討2022

    • Author(s)
      山田 綾果、高橋 琢二
    • Organizer
      第69回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 周波数変調型静電引力顕微鏡法によるキャリア密度の定量測定2022

    • Author(s)
      福澤 亮太, 梁 剣波, 重川 直輝, 高橋 琢二
    • Organizer
      第69回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 二重バイアス変調静電引力顕微鏡による直接貼り合わせp-n接合の断面解析2021

    • Author(s)
      福澤 亮太, 梁 剣波, 重川 直輝, 高橋 琢二
    • Organizer
      第68回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Multi-pulse変調を用いた光熱モードAFMによる非発光再結合の変調周波数依存性測定2021

    • Author(s)
      山田 綾果、高橋 琢二
    • Organizer
      第68回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 周波数変調型静電引力顕微鏡における静電容量の定量測定に向けた金属-半導体間の静電引力と周波数シフト量の関係の定式化2021

    • Author(s)
      福澤 亮太、高橋 琢二
    • Organizer
      第82回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] ジュール熱の外部変調を利用した非接触型抵抗原子間力顕微鏡法2021

    • Author(s)
      福澤 亮太、高橋 琢二
    • Organizer
      第82回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 光照射ケルビンプローブフォース顕微鏡によるCu(In,Ga)Se2太陽電池での時間分解光起電力計測2021

    • Author(s)
      黒岩 朋恵、高橋 琢二
    • Organizer
      第82回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Time-resolved Photovoltaic Measurements by Photo-assisted Kelvin Probe Force Microscopy2021

    • Author(s)
      Tomoe Kuroiwa, Ryota Ishibashi, Takuji Takahashi
    • Organizer
      The 5th international symposium on “Elucidation of Next Generation Functional Materials・Surface and Interface Properties"
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 原子間力顕微鏡を用いた静電引力検出による局所静電容量の定量測定2021

    • Author(s)
      福澤 亮太、高橋 琢二
    • Organizer
      応用物理学会 KOSEN SC 第3回 VR学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Quantitative Capacitance Measurements in Frequency Modulation Electrostatic Force Microscopy2021

    • Author(s)
      Ryota Fukuzawa, Takuji Takahashi
    • Organizer
      29th International Colloquium on Scanning Probe Microscopy (ICSPM29)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Time-resolved photo-assisted Kelvin probe force microscopy on Cu(In,Ga)Se2 solar cells2021

    • Author(s)
      Tomoe Kuroiwa, Takuji Takahashi
    • Organizer
      29th International Colloquium on Scanning Probe Microscopy (ICSPM29)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dual Bias Modulation Electrostatic Force Microscopy on Cu(In,Ga)Se22020

    • Author(s)
      Ryota Fukuzawa, Takashi Minemoto, Takuji Takahashi
    • Organizer
      2020 47th IEEE Photovoltaic Specialists Conference (PVSC)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 導電性ナノプローブ用いた静電引力測定によるCu(In,Ga)Se2中のCd拡散効果の解析2020

    • Author(s)
      福澤 亮太、峯元 高志、高橋 琢二
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 光熱モードAFMによる非発光再結合局所分布計測を用いたCu(In,Ga)(S,Se)2に対するCs処理効果の検討2020

    • Author(s)
      山田 綾果、高橋 琢二
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 間欠バイアス印加ケルビンプローブフォース顕微鏡による時間分解計測2020

    • Author(s)
      石橋 亮太、高橋 琢二
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 走査プローブ顕微鏡の基礎と応用2020

    • Author(s)
      高橋 琢二
    • Organizer
      応用物理学会 KOSEN SC 第1回 VR学術講演会
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] 光熱モードAFMによる非発光再結合特性評価を通じたCu(In,Ga)(S,Se)2に対するCs処理効果の検討2020

    • Author(s)
      山田 綾果、高橋 琢二
    • Organizer
      応用物理学会 KOSEN SC 第1回 VR学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 二重バイアス変調静電引力顕微鏡における可変周波数静電容量測定2020

    • Author(s)
      福澤 亮太、高橋 琢二
    • Organizer
      応用物理学会 KOSEN SC 第1回 VR学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Investigation on local non-radiative recombination property in Cu(In,Ga)(S,Se)2 by photothermal AFM2020

    • Author(s)
      Ayaka Yamada, Takuji Takahashi
    • Organizer
      2020 NAMIS MARATHON WORKSHOP
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Time-resolved measurements by Kelvin probe force microscopy with intermittent bias application2020

    • Author(s)
      Ryota Ishibashi, Takuji Takahashi
    • Organizer
      2020 NAMIS MARATHON WORKSHOP
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Time resolved Kelvin Probe Force Microscopy with Intermittent Bias Application Method2020

    • Author(s)
      Ryota Ishibashi, Takuji Takahashi
    • Organizer
      28th International Colloquium on Scanning Probe Microscopy (ICSPM28)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Multi-pulse Modulation Method in Photothermal Atomic Force Microscopy2020

    • Author(s)
      Ayaka Yamada, Takuji Takahashi
    • Organizer
      28th International Colloquium on Scanning Probe Microscopy (ICSPM28)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photo-assisted Scanning Probe Microscopy on Solar Cell Materials2020

    • Author(s)
      Takuji Takahashi
    • Organizer
      Seoul National Univ.(SNU)/IIS, The Univ.of Tokyo Joint Woprkshop on Innovative Micro/Nano systems
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 二重バイアス変調静電引力顕微鏡によるCu(In,Ga)Se2上での局所的容量測定2020

    • Author(s)
      福澤亮太, 峯元高志, 高橋琢二
    • Organizer
      第67回 応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Dual Bias Modulation Method for Variable Frequency Measurements in Electrostatic Force Microscopy2019

    • Author(s)
      Ryota Fukuzawa and Takuji Takahashi
    • Organizer
      The 21th International Scanning Probe Microscopy Conference (ISPM 2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dual Bias Modulation Electrostatic Force Microscopy for Variable Frequency2019

    • Author(s)
      Ryota Fukuzawa and Takuji Takahashi
    • Organizer
      NAMIS Marathon Workshop
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Investigation on Non-radiative Recombination Property in Cu(In,Ga)(S,Se)2 by Photothermal AFM2019

    • Author(s)
      Ayaka Yamada and Takuji Takahashi
    • Organizer
      NAMIS Marathon Workshop
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photo-assisted Scanning Probe Methods on Solar Cell Materials2019

    • Author(s)
      Takuji Takahashi
    • Organizer
      The 8th LIA NextPV International Workshop
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Direct Imaging Method of Frequency Response in Dual Bias Modulation Electrostatic Force Microscopy2019

    • Author(s)
      Ryota Fukuzawa and Takuji Takahashi
    • Organizer
      The 27th International Colloquium on Scanning Probe Microscopy (ICSPM27)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Non-radiative Recombination Properties in Cu(In,Ga)(S,Se)2 Investigated by Photothermal AFM2019

    • Author(s)
      Ayaka Yamada and Takuji Takahashi
    • Organizer
      The 27th International Colloquium on Scanning Probe Microscopy (ICSPM27)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dual Bias Modulation Electrostatic Force Microscopy for Variable Frequency Analyses2019

    • Author(s)
      Takuji Takahashi
    • Organizer
      The 4th International Symposium on "Elucidation of Property of Next Generation Functional Materials and Surface/Interface"
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 光熱モードAFMによるCu(In,Ga)(S,Se)2における非発光再結合特性の評価2019

    • Author(s)
      山田綾果, 高橋琢二
    • Organizer
      第80回 応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 二重バイアス変調静電引力顕微鏡による周波数応答の直接画像化2019

    • Author(s)
      福澤亮太, 高橋琢二
    • Organizer
      第80回 応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 二重バイアス変調静電引力顕微鏡における可変周波数測定2019

    • Author(s)
      福澤亮太, 高橋琢二
    • Organizer
      第80回 応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Valuable Frequency Measurements of dC/dV by Electrostatic Force Microscopy on Cu(In,Ga)(S,Se)22019

    • Author(s)
      Ryota Fukuzawa and Takuji Takahashi
    • Organizer
      LIMMS-Next PV Joint Energy Workshop
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photo-assisted Scanning Probe Methods on Solar Cell Materials2019

    • Author(s)
      Takuji Takahashi
    • Organizer
      LIMMS-Next PV Joint Energy Workshop
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Photo-assisted Kelvin Probe Force Microscopy on Cu(In,Ga)Se2 Solar Cells under Light with Various Photon Energies2018

    • Author(s)
      Hyeondeuk Yong, Takashi Minemoto, and Takuji Takahashi
    • Organizer
      The 20th International Scanning Probe Microscopy Conference (ISPM 2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dependence of Photovoltage on Incident Photon Energies Investigated by Photo-assisted Kelvin Probe Force Microscopy on Cu(In,Ga)Se2 Solar Cells2018

    • Author(s)
      Hyeondeuk Yong, Takashi Minemoto, and Takuji Takahashi
    • Organizer
      The 7th Edition of the World Conference on Photovoltaic Energy Conversion (WCPEC-7)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photo-assisted Kelvin Probe Force Microscopy on Cu(In,Ga)Se2 Solar Cells2018

    • Author(s)
      Takuji Takahashi
    • Organizer
      The 3rd international symposium on “Recent Trends in Elucidation and Function Discovery on Next Generation Functional Materials ・ Surface/Interface Properties”
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Photo-assisted Scanning Probe Microscopy on Cu(In,Ga)Se2 Solar Cells2018

    • Author(s)
      Takuji Takahashi
    • Organizer
      CNRS GDRe Thermal Nanosciences and Nano Engineering
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Dual Bias Modulation in EFM for Vanable Frequency Measurements of dC/dV2018

    • Author(s)
      Ryota Fukuzawa and Takuji Takahashi
    • Organizer
      14th International Conference on Atomically Controlled Surfaces, Interfaces and Nanostructures (ACSIN-14) & 26th International Colloquium on Scanning Probe Microscopy (ICSPM26)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photo-assisted Scanning Probe Methods on Solar Cells2018

    • Author(s)
      Takuji Takahashi
    • Organizer
      LIMMS/CNRS-IIS and UTC Joint Workshop
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Photothermal Measurements by AFM on Cu(In,Ga)Se2 Materials2017

    • Author(s)
      Risa Komatsu, Yasushi Hamamoto, Takashi Minemoto, and Takuji Takahashi
    • Organizer
      International Scanning Probe Microscopy Conference (Kyoto 2017)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photovoltaic Measurements on Cu(In,Ga)Se2 Solar Cells by Photo-assisted KFM under Various Illumination Conditions2017

    • Author(s)
      Hyeondeuk Yong, Takashi Minemoto, and Takuji Takahashi
    • Organizer
      International Scanning Probe Microscopy Conference (Kyoto 2017)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Local Measurements of Surface Capacitance by Electrostatic Force Microscopy on Cu(In,Ga)Se2 Materials2017

    • Author(s)
      Tomoaki Ishii, Takashi Minemoto, and Takuji Takahashi
    • Organizer
      2017 IEEE 44th Photovoltaic Specialist Conference (PVSC)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photo-carrier Recombination Properties in Cu(In,Ga)Se2 Solar Cells Investigated by Photo-assisted KFM under Various Illumination Conditions2017

    • Author(s)
      Hyeondeuk Yong, Takashi Minemoto, and Takuji Takahashi
    • Organizer
      25th International Colloquium on Scanning Probe Microscopy (ICSPM25)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photothermal-mode AFM on Cu(In,Ga)Se2 Materials2017

    • Author(s)
      Risa Komatsu, Takashi Minemoto, and Takuji Takahashi
    • Organizer
      25th International Colloquium on Scanning Probe Microscopy (ICSPM25)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research

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Published: 2017-04-28   Modified: 2023-01-30  

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