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Femtosecond gas electron diffraction by THz-wave-assisted electron diffraction

Research Project

Project/Area Number 17H03004
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Physical chemistry
Research InstitutionTokyo Metropolitan University (2019-2020)
The University of Tokyo (2017-2018)

Principal Investigator

Kanya Reika  東京都立大学, 理学研究科, 教授 (10401168)

Project Period (FY) 2017-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥18,850,000 (Direct Cost: ¥14,500,000、Indirect Cost: ¥4,350,000)
Fiscal Year 2020: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2019: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2018: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000)
Fiscal Year 2017: ¥8,970,000 (Direct Cost: ¥6,900,000、Indirect Cost: ¥2,070,000)
Keywords反応動力学 / 分子構造 / 電子回折法 / 強光子場科学 / 電子散乱
Outline of Final Research Achievements

A theoretical framework of laser-assisted electron scattering induced by single-cycle laser pulses and a protocol of THz-wave-assisted electron diffraction method were developed, and their feasibilities were confirmed by numerical simulations. In order to demonstrate THz-wave-assisted electron diffraction method experimentally, optical systems for the tilted-pulse-front pumping method and the electro-optical sampling method were constructed. An apparatus for THz-assisted electron scattering was constructed by incorporating the optical systems into a laser-assisted electron scattering apparatus. Furthermore, a hollow-core-fiber type pulse compressor was developed for generation of few-cycle laser pulses in the near-infrared region, and few-cycle laser assisted electron scattering processes were observed for the first time.

Academic Significance and Societal Importance of the Research Achievements

本研究課題で開発した理論の適用範囲は、テラヘルツ波によるレーザーアシステッド電子散乱過程に留まらず、近赤外領域の数サイクル・単一サイクルパルスによるレーザーアシステッド電子散乱過程にも渡り、数サイクルレーザーアシステッド電子散乱過程の初観測の成果とともにアト秒領域のダイナミクス研究への応用の可能性を示すものである。本課題は、テラヘルツ波アシステッド電子散乱過程を探求する初めての試みであり、テラヘルツ波の新たな利用法の創出につながる学術的基盤を確立することとなった。

Report

(5 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • Research Products

    (51 results)

All 2021 2020 2019 2018 2017

All Journal Article (4 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 3 results,  Open Access: 1 results) Presentation (47 results) (of which Int'l Joint Research: 34 results,  Invited: 21 results)

  • [Journal Article] Absolute carrier-envelope-phase dependences of single and double ionization of methanol in a near-IR few-cycle laser field2020

    • Author(s)
      Q. Zhang, S. Fukahori, T. Ando, R. Kanya, A. Iwasaki, T. Rathje, G. G. Paulus, K. Yamanouchi
    • Journal Title

      The Journal of Chemical Physics

      Volume: 152 Issue: 19

    • DOI

      10.1063/5.0006485

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Femtosecond Laser-Assisted Electron Scattering for Ultrafast Dynamics of Atoms and Molecules2019

    • Author(s)
      Kanya Reika、Yamanouchi Kaoru
    • Journal Title

      Atoms

      Volume: 7 Issue: 3 Pages: 85-85

    • DOI

      10.3390/atoms7030085

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Determination of the absolute carrier-envelope phase by angle-resolved photoelectron spectra of Ar by intense circularly polarized few-cycle pulses2017

    • Author(s)
      Shinichi Fukahori, Toshiaki Ando, Shun Miura, Reika Kanya, Kaoru Yamanouchi, Tim Rathje, and Gerhard G. Paulus
    • Journal Title

      Physical Review A

      Volume: 95 Issue: 5

    • DOI

      10.1103/physreva.95.053410

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Laser-Assisted Electron Scattering and Diffraction for Ultrafast Imaging of Atoms and Molecules2017

    • Author(s)
      Yuya Morimoto, Reika Kanya, Kaoru Yamanouchi
    • Journal Title

      Progress in Photon Science, Springer Series in Chemical Physics

      Volume: 115 Pages: 47-52

    • DOI

      10.1007/978-3-319-52431-3_5

    • ISBN
      9783319524306, 9783319524313
    • Related Report
      2017 Annual Research Report
  • [Presentation] Development of single-cycle THz light source for THz-wave-assisted electron diffraction2021

    • Author(s)
      Michihiro Kitanaka, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      Symposium on Recent Development in Ultrafast Intense Laser Science 2
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Measurements of two-dimensional differential cross section of femtosecond LAES signals of Ar atoms2021

    • Author(s)
      Motoki Ishikawa, Kakuta Ishida, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      Symposium on Recent Development in Ultrafast Intense Laser Science 2
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Development of a photocathode-type pulsed electron gun for time-resolved electron diffraction measurements2021

    • Author(s)
      Shuhei Sudo, Motoki Ishikawa, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      日本化学会 第101春季年会 (2021)
    • Related Report
      2020 Annual Research Report
  • [Presentation] Measurements of two-dimensional differential cross section of femtosecond LAES signals of Ar atoms2021

    • Author(s)
      Motoki Ishikawa, Kakuta Ishida, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      日本化学会 第101春季年会 (2021)
    • Related Report
      2020 Annual Research Report
  • [Presentation] Determination of collision times in laser-assisted electron scattering for ultrafast imaging of atoms and molecules2020

    • Author(s)
      Reika Kanya
    • Organizer
      The 6th Quantum Science (QS) symposium
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Progress of THz-wave-assisted electron diffraction apparatus2020

    • Author(s)
      Michihiro Kitanaka, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      Symposium on Recent Development in Ultrafast Intense Laser Science
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Laser-assisted electron scattering by Ar in a femtosecond intense laser field2020

    • Author(s)
      Motoki Ishikawa, Kakuta Ishida, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      Symposium on Recent Development in Ultrafast Intense Laser Science
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Femtosecond laser-assisted electron scattering and diffraction ─ old stories and future prospects ─2020

    • Author(s)
      Reika Kanya
    • Organizer
      Symposium on Recent Development in Ultrafast Intense Laser Science
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Attosecond streaking of electron diffraction patterns by laser-assisted electron scattering2019

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      第13回分子科学討論会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Attosecond streaking of electron diffraction patterns by laser-assisted electron scattering2019

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 18th International Symposium on Ultrafast Intense laser Science (ISUILS 2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Observation of laser-assisted electron scattering signals with sub-10 fs laser pulses2019

    • Author(s)
      Kota Kumakura, Motoki Ishikawa, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 20th International Symposium on Correlation, Polarization and Ionization in Atomic and Molecular Collisions
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Determination of collision times in laser-assisted electron scattering for ultrafast imaging of atoms and molecules2019

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      XXXIst International Conference on Photonic, Electronic, and Atomic Collisions
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Determination of collision times in laser-assisted electron scattering for ultrafast imaging of atoms and molecules2019

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      28th Annual International Laser Physics Workshop
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Laser-assisted streaking of electron diffraction patterns for ultrafast molecular imaging2019

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      International Symposium on Ultrafast Molecular Dynamics
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] CEP dependence of the dissociative ionization of methanol in the intense few-cycle laser fields2019

    • Author(s)
      Qiqi Zhang, Shinichi Fukahori, Toshiaki Ando, Reika Kanya, Atsushi Iwasaki, Tim Rathje, Gerhard G. Paulus, Kaoru Yamanouchi
    • Organizer
      3rd ETH Zurich-UTokyo Strategic Partnership Symposium on the UN Sustainable Development Goals and Innovation
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Ultrafast streaking of electron diffraction patterns by laser-assisted electron scattering2019

    • Author(s)
      Reika Kanya
    • Organizer
      International Symposium on Ultrafast Electronic and Structural Dynamics
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Photoionization of excited states of rare gas atoms prepared by electron impact excitation2019

    • Author(s)
      Takashi Hiroi, Yuya Morimoto, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      日本化学会第99春季年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Electron impact excitation spectroscopy of highly excited H22019

    • Author(s)
      Takashi Hiroi, Yuya Morimoto, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 4th STEPS Symposium on Photon Science
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Ultrafast streaking of scattered electrons by single-cycle IR-laser-assisted electron scattering2018

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 9th Shanghai-Tokyo Advanced Research on Ultrafast Intense Laser Science Symposium
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 多サイクル、および、単一サイクルレーザーパルスによるレーザーアシステッド電子散乱過程における衝突時刻のアト秒精度での決定2018

    • Author(s)
      歸家令果, 石田角太, 森本裕也, 山内 薫
    • Organizer
      第15回 AMO討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Development of an apparatus for femtosecond laser-assisted (e,2e) experiments2018

    • Author(s)
      Takashi Hiroi, Yuya Morimoto, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The XXI International Conference on Ultrafast Phenomena
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 多サイクル、および、単一サイクルレーザーパルスによるレーザーアシステッド電子散乱過程における衝突時刻のアト秒精度での決定2018

    • Author(s)
      歸家令果, 石田角太, 森本裕也, 山内 薫
    • Organizer
      第12回分子科学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] sub-10 fsレーザーパルスによるレーザーアシステッド電子散乱の観測2018

    • Author(s)
      熊倉洸太, 石川源基, 歸家令果, 山内 薫
    • Organizer
      第12回分子科学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Ultrafast streaking of electron diffraction patterns by laser-assisted electron scattering2018

    • Author(s)
      Reika Kanya
    • Organizer
      The 5th Ultrafast Dynamic Imaging of Matter
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Development of an apparatus for femtosecond laser-assisted (e,2e) experiments2018

    • Author(s)
      Takashi Hiroi, Yuya Morimoto, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 17th International Symposium on Ultrafast Intense laser Science
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Observation of laser-assisted electron scattering signals with sub-10 fs laser pulses2018

    • Author(s)
      Kota Kumakura, Motoki Ishikawa, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 17th International Symposium on Ultrafast Intense laser Science
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Determination of collision times with attosecond precision in laser-assisted electron scattering by multi-cycle and single-cycle laser pulses2018

    • Author(s)
      Reika Kanya
    • Organizer
      International Workshop Attosecond Physics at the Nanoscale
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Laser-assisted electron scattering for ultrafast imaging of atoms and molecules2018

    • Author(s)
      Reika Kanya
    • Organizer
      The 13th Asian International Seminar on Atomic and Molecular Physics
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Laser-assisted Electron Scattering and Diffraction2018

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The Third STEPS Symposium on Photon Science
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Laser-assisted electron impact ionization2018

    • Author(s)
      Takashi Hiroi, Yuya Morimoro, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The Third STEPS Symposium on Photon Science
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Femtosecond gas electron diffraction by THz-wave assisted electron scattering: Numerical simulations of time-resolved electron diffraction patterns2017

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 3rd Computational Chemistry (CC) Symposium
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] テラヘルツ波アシステッド気体電子回折法:時間依存電子回折パターンの数値シミュレーション2017

    • Author(s)
      歸家令果, 山内 薫
    • Organizer
      第14回原子・分子・光科学(AMO)討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] レーザーアシステッド電子衝突イオン化の観測のための装置開発2017

    • Author(s)
      廣井卓思, 森本裕也, 歸家令果, 山内 薫
    • Organizer
      第14回原子・分子・光科学(AMO)討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Light-dressing effect in atoms and molecules in laser-assisted elastic electron scattering2017

    • Author(s)
      Reika Kanya, Yuya Morimoto, Kaoru Yamanouchi
    • Organizer
      XIX International Workshop on Low Energy Positron and Positronium Physics and XX International Symposium on Electron Molecule Collisions and Swarms (POSMOL 2107)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Ultrafast gas electron diffraction by THz-wave assisted electron scattering: Numerical simulations of time-resolved electron diffraction patterns2017

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 30th International Conference on Photonic, Electronic and Atomic Collisions (ICPEAC 2107)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Laser-assisted electron scattering and diffraction for ultrafast molecular imaging2017

    • Author(s)
      Reika Kanya, Yuya Morimoto, Kakuta Ishida, Kaoru Yamanouchi
    • Organizer
      International Symposium on (e,2e), Double Photoionization and Related Topics, 19th International Symposium on Polarization and Correlation in Electronic and Atomic Collisions ((e,2e) 2107)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Ultrafast gas electron diffraction by THz-wave-assisted electron scattering: Numerical simulations of time-resolved electron diffraction patterns2017

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 2nd International Symposium on Attosecond Science
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Observation of laser-assisted electron scattering processes by an angle-resolved time-of-flight type electron analyzer2017

    • Author(s)
      Motoki Ishikawa, Kakuta Ishida, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 2nd International Symposium on Attosecond Science
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] レーザーアシステッド電子衝突イオン化の観測装置の開発2017

    • Author(s)
      廣井卓思, 森本裕也, 歸家令果, 山内 薫
    • Organizer
      原子衝突学会第42回年会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 角度分解飛行時間型電子分析器によるレーザーアシステッド電子散乱過程の観測2017

    • Author(s)
      石川源基, 石田角太, 歸家令果, 山内 薫
    • Organizer
      第11回分子科学討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] レーザーアシステッド電子衝突イオン化観測装置の開発2017

    • Author(s)
      廣井卓思, 森本裕也, 歸家令果, 山内 薫
    • Organizer
      第11回分子科学討論会
    • Related Report
      2017 Annual Research Report
  • [Presentation] Numerical simulation of ultrafast gas electron diffraction by THz-wave-assisted electron scattering2017

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 14th International Conference on Multiphoton Processes
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Observation of laser-assisted electron scattering processes by an angle-resolved time-of-flight type electron analyzer2017

    • Author(s)
      Motoki Ishikawa, Kakuta Ishida, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 16th International Symposium on Ultrafast Intense laser Science (ISUILS2017)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of an apparatus for electron impact ionization in an intense laser field2017

    • Author(s)
      Takashi Hiroi, Yuya Morimoto, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 16th International Symposium on Ultrafast Intense laser Science (ISUILS2017)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] High-order multiphoton laser-assisted elastic electron scattering by Xe in a femtosecond near-infrared intense laser field: Plateau in energy spectra of scattered electrons2017

    • Author(s)
      Kakuta Ishida, Yuya Morimoto, Reika Kanya, Kaoru Yamanouchi
    • Organizer
      The 16th International Symposium on Ultrafast Intense laser Science (ISUILS2017)
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] THz-wave-assisted electron diffraction: Numerical simulations of time-resolved electron diffraction patterns2017

    • Author(s)
      Reika Kanya, Kaoru Yamanouchi
    • Organizer
      シンポジウム テラヘルツ科学の最前線Ⅳ
    • Related Report
      2017 Annual Research Report
  • [Presentation] Ultrafast molecular imaging by laser-assisted electron scattering2017

    • Author(s)
      Reika Kanya
    • Organizer
      The 21st East Asian Workshop on Chemical Dynamics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited

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Published: 2017-04-28   Modified: 2022-01-27  

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