• Search Research Projects
  • Search Researchers
  • How to Use
  1. Back to previous page

Development of atomic-scale characterization for low-dimensional materials

Research Project

Project/Area Number 17H04797
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Nanostructural physics
Research InstitutionNational Institute of Advanced Industrial Science and Technology

Principal Investigator

Senga Ryosuke  国立研究開発法人産業技術総合研究所, 材料・化学領域, 主任研究員 (80713221)

Project Period (FY) 2017-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥25,480,000 (Direct Cost: ¥19,600,000、Indirect Cost: ¥5,880,000)
Fiscal Year 2020: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2019: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2018: ¥4,030,000 (Direct Cost: ¥3,100,000、Indirect Cost: ¥930,000)
Fiscal Year 2017: ¥13,390,000 (Direct Cost: ¥10,300,000、Indirect Cost: ¥3,090,000)
Keywordsナノ材料 / 透過電子顕微鏡 / 電子エネルギー損失分光 / カーボンナノチューブ / グラフェン / 励起子 / フォノン / 低次元材料 / 光学特性 / 振動特性 / 電子線分光 / 物性評価 / 電子顕微鏡 / ナノ光物性 / 分散関係 / 光物性 / 原子層物質
Outline of Final Research Achievements

The optical absorption of a single carbon nanotube has been successfully measured by high-energy-resolution electron energy-loss spectroscopy. We have also established an analytical method to quantitatively link the electron valence excitation spectrum with the optical absorption spectrum. Then we have quantitatively clarified the modulation of optical conductivity at a local defect in a single carbon nanotube. Furthermore, we have developed a technique to investigate vibrational properties using angle-resolved electron energy loss spectroscopy and demonstrated for the first time to measure the phonon dispersion of a single layer graphene. These results were published in eight international journals including Nature, Nanoletters and Physical Review Letters, as well as in seven domestic and international invited talks.

Academic Significance and Societal Importance of the Research Achievements

本研究によって低次元材料の物性を決める励起子やフォノンといった準粒子の振る舞いを原子構造と一対一で結び付けることができた。これらの成果は基礎学術的な理解を深めるだけでなく、低次元材料の応用展開を考えるうえでも重要な知見である。例えば微小光源、単一光子エミッタ、高感度光センサーといったデバイスに関して、許容できる欠陥の種類や個数などの指針を与え最適な構造設計に貢献できる。またこれまで理論計算が先行していたナノ材料の格子振動の計測に成功したことも、材料科学分野に大きなインパクトを与える成果であり、熱電素子や光電子デバイス、超電導体などの今後の研究開発への貢献が期待できる。

Report

(5 results)
  • 2021 Final Research Report ( PDF )
  • 2020 Annual Research Report
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • Research Products

    (35 results)

All 2021 2020 2019 2018 2017 Other

All Int'l Joint Research (12 results) Journal Article (12 results) (of which Int'l Joint Research: 11 results,  Peer Reviewed: 12 results,  Open Access: 1 results,  Acknowledgement Compliant: 1 results) Presentation (11 results) (of which Int'l Joint Research: 7 results,  Invited: 9 results)

  • [Int'l Joint Research] University of Vienna(オーストリア)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Universita di Roma La Sapienza(イタリア)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] University of Vienna(オーストリア)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] c/o Universita G. D’Annunzio/Universita di Roma La Sapienza(イタリア)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Aalto University(フィンランド)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] National University of Singapore(シンガポール)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Aalt University(フィンランド)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Helmholtz-Zentrum Dresden- Rossendorf(ドイツ)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] University of Vienna(オーストリア)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Aalt University(フィンランド)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] Helmholtz-Zentrum Dresden-Rossendorf(ドイツ)

    • Related Report
      2017 Annual Research Report
  • [Int'l Joint Research] University of Vienna(オーストリア)

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Toward Confined Carbyne with Tailored Properties2021

    • Author(s)
      Shi Lei、Senga Ryosuke、Suenaga Kazu、Kataura Hiromichi、Saito Takeshi、Paz Alejandro Perez、Rubio Angel、Ayala Paola、Pichler Thomas
    • Journal Title

      Nano Letters

      Volume: 21 Issue: 2 Pages: 1096-1101

    • DOI

      10.1021/acs.nanolett.0c04482

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Deciphering the Intense Postgap Absorptions of Monolayer Transition Metal Dichalcogenides2021

    • Author(s)
      Hong Jinhua、Koshino Masanori、Senga Ryosuke、Pichler Thomas、Xu Hua、Suenaga Kazu
    • Journal Title

      ACS Nano

      Volume: 15 Issue: 4 Pages: 7783-7789

    • DOI

      10.1021/acsnano.1c01868

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Photothermal synthesis of confined carbyne2021

    • Author(s)
      Shi Lei、Senga Ryosuke、Suenaga Kazu、Chimborazo Johnny、Ayala Paola、Pichler Thomas
    • Journal Title

      Carbon

      Volume: 182 Pages: 348-353

    • DOI

      10.1016/j.carbon.2021.05.058

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Thermal management function of graphene under cryogenic temperature2021

    • Author(s)
      Kato Ryuichi、Naya Masami、Kasahata Naoki、Senga Ryosuke、Sato Chikara、Koshino Masanori、Suenaga Kazu、Hasegawa Masataka
    • Journal Title

      Carbon

      Volume: 183 Pages: 970-976

    • DOI

      10.1016/j.carbon.2021.07.077

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Probing Exciton Dispersions of Freestanding Monolayer WSe2 by Momentum-Resolved Electron Energy-Loss Spectroscopy2020

    • Author(s)
      Hong Jinhua、Senga Ryosuke、Pichler Thomas、Suenaga Kazu
    • Journal Title

      Physical Review Letters

      Volume: 124 Issue: 8 Pages: 0-0

    • DOI

      10.1103/physrevlett.124.087401

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Layer Rotation-Angle-Dependent Excitonic Absorption in van der Waals Heterostructures Revealed by Electron Energy Loss Spectroscopy2019

    • Author(s)
      Gogoi Pranjal Kumar、Lin Yung-Chang、Senga Ryosuke、Komsa Hannu-Pekka、Wong Swee Liang、Chi Dongzhi、Krasheninnikov Arkady V.、Li Lain-Jong、Breese Mark B. H.、Pennycook Stephen J.、Wee Andrew T. S.、Suenaga Kazu
    • Journal Title

      ACS Nano

      Volume: 13 Issue: 8 Pages: 9541-9550

    • DOI

      10.1021/acsnano.9b04530

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Position and momentum mapping of vibrations in graphene nanostructures2019

    • Author(s)
      Senga Ryosuke、Suenaga Kazu、Barone Paolo、Morishita Shigeyuki、Mauri Francesco、Pichler Thomas
    • Journal Title

      Nature

      Volume: 573 Issue: 7773 Pages: 247-250

    • DOI

      10.1038/s41586-019-1477-8

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Direct Proof of a Defect-Modulated Gap Transition in Semiconducting Nanotubes2018

    • Author(s)
      Senga Ryosuke、Pichler Thomas、Yomogida Yohei、Tanaka Takeshi、Kataura Hiromichi、Suenaga Kazu
    • Journal Title

      Nano Letters

      Volume: 18 Issue: 6 Pages: 3920-3925

    • DOI

      10.1021/acs.nanolett.8b01284

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Depth sensitive imaging of graphene with an atomic resolution microscope2018

    • Author(s)
      Shigeyuki Morishita, Ryosuke Senga, Yung-Chang Lin, Ryuichi Kato, Hidetaka Sawada, and Kazutomo Suenaga
    • Journal Title

      Applied Physics Letters

      Volume: 113 Issue: 23 Pages: 233101-233101

    • DOI

      10.1063/1.5053926

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Structural analysis and oxygen reduction reaction activity in bamboo-like nitrogen-doped carbon nanotubes containing localized nitrogen in nodal regions2017

    • Author(s)
      Aoki Kaede、Senga Ryosuke、Suga Yosuke、Totani Kenro、Maki Tei、Itoh Hiroshi、Shinokura Kiichiro、Suenaga Kazutomo、Watanabe Toshiyuki
    • Journal Title

      Carbon

      Volume: 123 Pages: 99-105

    • DOI

      10.1016/j.carbon.2017.03.087

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Single-atom detection of light elements: Imaging or spectroscopy?2017

    • Author(s)
      Ryosuke Senga, Kazu Suenaga
    • Journal Title

      Ultramicroscopy

      Volume: 印刷中 Pages: 150-155

    • DOI

      10.1016/j.ultramic.2016.12.007

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Journal Article] Structural Distortions and Charge Density Waves in Iodine Chains Encapsulated inside Carbon Nanotubes2017

    • Author(s)
      Komsa Hannu-Pekka、Senga Ryosuke、Suenaga Kazutomo、Krasheninnikov Arkady V.
    • Journal Title

      Nano Letters

      Volume: 17 Issue: 6 Pages: 3694-3700

    • DOI

      10.1021/acs.nanolett.7b00969

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] Nanoscale optical and vibrational spectroscopy of low-dimensional materials in electron microscope2020

    • Author(s)
      Ryosuke Senga, Thomas Pichler, and Kazu Suenaga
    • Organizer
      2020 MRS Fall Meeting Symposium
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Ryosuke Senga, Thomas Pichler, and Kazu Suenaga2020

    • Author(s)
      Nanoscale optical and vibrational spectroscopy of low-dimensional materials in electron microscope
    • Organizer
      European Microscopy Congress 2020
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 電子顕微鏡を用いた低次元材料の局所物性評価2020

    • Author(s)
      千賀 亮典
    • Organizer
      2020年第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Nanoscale optical and vibrational spectroscopy of low-dimensional materials in electron microscope2020

    • Author(s)
      千賀 亮典
    • Organizer
      第58回 フラーレン・ナノチューブ・グラフェン 総合シンポジウム
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Nanoscale vibrational spectroscopy of graphene by large-q EELS2019

    • Author(s)
      千賀 亮典
    • Organizer
      M&M 2019 Microscopy & MicroAnalysis
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Nanoscale optical and vibrational spectroscopy of low-dimensional materials2019

    • Author(s)
      千賀亮典
    • Organizer
      1&2D Conference and Exhibition
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Characterization of Exciton Behavior in Low-Dimensional Materials by using monochromated EELS2018

    • Author(s)
      千賀亮典
    • Organizer
      Microscopy & Microanalysis 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Advanced STEM-EELS characterization of low-dimensional materials2018

    • Author(s)
      千賀亮典
    • Organizer
      The Fullerenes, Nanotubes and Graphene Research Society
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 高分解能EELSを用いた低次元材料物性評価2018

    • Author(s)
      千賀 亮典
    • Organizer
      日本顕微鏡学会 第42回関東支部講演会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] Direct measurement of a locally modulated gap transition at defects in carbon nanotubes2018

    • Author(s)
      千賀 亮典
    • Organizer
      International Winterschool on Electronic Properties of Novel Materials
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Characterization of individual 1D materials by monochromated STEM2017

    • Author(s)
      千賀亮典
    • Organizer
      8th International Workshop on Electron Energy Loss Spectroscopy and Related Techniques
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research

URL: 

Published: 2017-04-28   Modified: 2023-01-30  

Information User Guide FAQ News Terms of Use Attribution of KAKENHI

Powered by NII kakenhi