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Exploring extreme response of solids exposed to intense few-cycle mid-infrared electric fields

Research Project

Project/Area Number 17H04816
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Optical engineering, Photon science
Research InstitutionThe University of Tokyo

Principal Investigator

Ishii Nobuihsa  東京大学, 物性研究所, 助教 (40586898)

Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥25,350,000 (Direct Cost: ¥19,500,000、Indirect Cost: ¥5,850,000)
Fiscal Year 2018: ¥8,840,000 (Direct Cost: ¥6,800,000、Indirect Cost: ¥2,040,000)
Fiscal Year 2017: ¥12,480,000 (Direct Cost: ¥9,600,000、Indirect Cost: ¥2,880,000)
Keywords超高速赤外レーザー / 固体 / 非線形効果 / 高次高調波 / 赤外フェムト秒光源 / 高次高調波発生 / 高強度赤外光源 / 非線形光学
Outline of Final Research Achievements

We have explored extremely nonlinear response of solid. We have developed an intense femtosecond laser in the mid-infrared region of the spectrum, allowing the application of more than 10 MV/cm electric fields in solids without optical damage. As a result, the response of electrons in solids exhibits extremely nonlinearity, generating high harmonics up to the ultraviolet region, which consist of comb-like spectral components that have integer multiple of the laser frequency. The polarization resolved study of the high harmonics directly allows us to determine the band curvature of the lowest conduction band of solids. In other experiments, we have demonstrated the selection rules in solid high harmonics generation experimentally for the first time. Additionally, we have detected the reflected high harmonics from solid interfaces, which reveals the propagation effect of intense mid-infrared pulses on high harmonic generation in solids.

Academic Significance and Societal Importance of the Research Achievements

高強度電界下の物質応答やその絶縁破壊は、近年の高速エレクトロニクスやスイッチング、並びにリーク電流問題と密接にかかわっており、これからさらなる高速化が進む、情報社会基盤における先駆的な研究であると思われる。
また光学分野においても、紫外線領域では物質の屈折率が低く透過率が低いために、偏光光学素子を作成することが非常に困難である。極限的非線形光学効果を用いて赤外光源の制御と固体高調波発生媒質の人工構造成型により、紫外高調波の偏光制御が可能となり、紫外の分光実験への適応が可能となる。

Report

(3 results)
  • 2019 Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • Research Products

    (28 results)

All 2019 2018 2017 Other

All Journal Article (11 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 11 results,  Open Access: 7 results,  Acknowledgement Compliant: 1 results) Presentation (16 results) (of which Int'l Joint Research: 4 results,  Invited: 4 results) Remarks (1 results)

  • [Journal Article] High-order harmonic generation from hybrid organic-inorganic perovskite thin films2019

    • Author(s)
      Hirori Hideki、Xia Peiyu、Shinohara Yasushi、Otobe Tomohito、Sanari Yasuyuki、Tahara Hirokazu、Ishii Nobuhisa、Itatani Jiro、Ishikawa Kenichi L.、Aharen Tomoko、Ozaki Masashi、Wakamiya Atsushi、Kanemitsu Yoshihiko
    • Journal Title

      APL Materials

      Volume: 7 Issue: 4 Pages: 041107-041107

    • DOI

      10.1063/1.5090935

    • NAID

      120006712768

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] All-optical characterization of the two-dimensional waveform and the Gouy phase of an infrared pulse based on plasma fluorescence of gas2018

    • Author(s)
      Saito Nariyuki, Ishii Nobuhisa, Kanai Teruto, Itatani Jiro
    • Journal Title

      Optics Express

      Volume: 26 Issue: 19 Pages: 24591-24591

    • DOI

      10.1364/oe.26.024591

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Polarization-Resolved Study of High Harmonics from Bulk Semiconductors2018

    • Author(s)
      Kaneshima Keisuke、Shinohara Yasushi、Takeuchi Kengo、Ishii Nobuhisa、Imasaka Kotaro、Kaji Tomohiro、Ashihara Satoshi、Ishikawa Kenichi L.、Itatani Jiro
    • Journal Title

      Physical Review Letters

      Volume: 120 Issue: 24 Pages: 243903-243903

    • DOI

      10.1103/physrevlett.120.243903

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Generation of sub-two-cycle CEP-stable optical pulses at 3.5 μm from a KTA-based optical parametric amplifier with multiple-plate compression2018

    • Author(s)
      Lu Faming, Xia Peiyu, Matsumoto Yoshiyuki, Kanai Teruto, Ishii Nobuhisa, Itatani Jiro
    • Journal Title

      Optics Letters

      Volume: 43 Issue: 11 Pages: 2720-2723

    • DOI

      10.1364/ol.43.002720

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nonlinear propagation effects in high harmonic generation in reflection and transmission from gallium arsenide2018

    • Author(s)
      Xia Peiyu, Kim Changsu, Lu Faming, Kanai Teruto, Akiyama Hidefumi, Itatani Jiro, Ishii Nobuhisa
    • Journal Title

      Optics Express

      Volume: 26 Issue: 22 Pages: 29393-29393

    • DOI

      10.1364/oe.26.029393

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Photo-induced semimetallic states realised in electron-hole coupled insulators2018

    • Author(s)
      Kozo Okazaki, Yu Ogawa, Takeshi Suzuki, Takashi Yamamoto, Takashi Someya, Shoya Michimae, Mari Watanabe, Yangfan Lu, Minoru Nohara, Hidenori Takagi, Naoyuki Katayama, Hiroshi Sawa, Masami Fujisawa, Teruto Kanai, Nobuhisa Ishii, Jiro Itatani, Takashi Mizokawa, Shik Shin
    • Journal Title

      Nature Communications

      Volume: 9:4322 Issue: 1 Pages: 1-6

    • DOI

      10.1038/s41467-018-06801-1

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Resonant magneto-optical Kerr effect measurement system with polarization analysis using a high harmonic generation laser2018

    • Author(s)
      Yamamoto Sh.、Oumbarek D.、Fujisawa M.、Someya T.、Takahashi Y.、Yamamoto T.、Ishii N.、Yaji K.、Yamamoto S.、Kanai T.、Okazaki K.、Kotsugi M.、Itatani J.、Shin S.、Matsuda I.
    • Journal Title

      Journal of Electron Spectroscopy and Related Phenomena

      Volume: 222 Pages: 68-73

    • DOI

      10.1016/j.elspec.2017.09.001

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Observation of selection rules for circularly polarized fields in high-harmonic generation from a crystalline solid2017

    • Author(s)
      Saito Nariyuki、Xia Peiyu、Lu Faming、Kanai Teruto、Itatani Jiro、Ishii Nobuhisa
    • Journal Title

      Optica

      Volume: 4 Issue: 11 Pages: 1333-1333

    • DOI

      10.1364/optica.4.001333

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Generation of sub-two-cycle millijoule infrared pulses in an optical parametric chirped-pulse amplifier and their application to soft x-ray absorption spectroscopy with high-flux high harmonics2017

    • Author(s)
      Ishii Nobuhisa、Kaneshima Keisuke、Kanai Teruto、Watanabe Shuntaro、Itatani Jiro
    • Journal Title

      Journal of Optics

      Volume: 20 Issue: 1 Pages: 014003-014003

    • DOI

      10.1088/2040-8986/aa99ed

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Suppression of supercollision carrier cooling in high mobility graphene on SiC(0001)2017

    • Author(s)
      Takashi Someya, Hirokazu Fukidome, Hiroshi Watanabe, Takashi Yamamoto, Masaru Okada, Hakuto Suzuki, Yu Ogawa, Takushi Iimori, Nobuhisa Ishii, Teruto Kanai, Keiichiro Tashima, Baojie Feng, Susumu Yamamoto, Jiro Itatani, Fumio Komori, Kozo Okazaki, Shik Shin, and Iwao Matsuda
    • Journal Title

      PHYSICAL REVIEW B

      Volume: 95 Issue: 16 Pages: 165303-165303

    • DOI

      10.1103/physrevb.95.165303

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] 3.Ultrafast Melting of Spin DensityWave Order in BaFe2As2 Observed by Time- and Angle-Resolved Photoemission Spectroscopy with Extreme-Ultraviolet Higher Harmonic Generation2017

    • Author(s)
      H. Suzuki, K. Okazaki, T. Yamamoto, T. Someya, M. Okada, K. Koshiishi, M. Fujisawa, T. Kanai, N. Ishii, M. Nakajima, H. Eisaki, K. Ono, H. Kumigashira, J. Itatani, A. Fujimori and S. Shin
    • Journal Title

      Phys. Rev. B

      Volume: 95 Issue: 16 Pages: 165112-165112

    • DOI

      10.1103/physrevb.95.165112

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] 固体における強光子場科学のための中赤外光源開発2019

    • Author(s)
      石井順久
    • Organizer
      第39回レーザー学会学術講演会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 固体のサブサイクル分光に向けての3.5um帯CEP安定中赤外パルスの電気光学サンプリング2019

    • Author(s)
      夏 沛宇、Lu Faming、金島 圭佑、石井 順久、金井 輝人、板谷 治郎
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 高次高調波を用いた400 eVにおける窒素分子の時間分解軟X線吸収分光2019

    • Author(s)
      齋藤 成之、三戸 宏樹、石井 順久、金井 輝人、板谷 治郎
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Polarization properties of high harmonics in solids using linearly and circularly polarized infrared optical pulses2018

    • Author(s)
      Nobuhisa Ishii
    • Organizer
      The 9th Asian Workshop on Generation and Application of Coherent XUV and X-ray Radiation
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Complete characterization of an optical waveform by luminescence from gas plasma2018

    • Author(s)
      Nariyuki Saito, Nobuhisa Ishii, Teruto Kanai, and Jiro Itatani,
    • Organizer
      The 7th Advanced Lasers and Photon Sources
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 「水の窓」全域にわたる軟Ⅹ線高調波発生2018

    • Author(s)
      三戸宏樹、齋藤成之、石井順久、金井輝人、板谷治郎
    • Organizer
      第79回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 反射配置でのGaAsからの高次高調波発生と伝搬効果の評価2018

    • Author(s)
      夏沛宇、金昌秀、Faming Lu、石井順久、金井輝人、秋山英文、板谷治郎
    • Organizer
      第79回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 高強度赤外電場による光電子放出過程の搬送波包絡線位相依存性2018

    • Author(s)
      水野智也、Dagar Ritika、竹内健悟、石井順久、金井輝人、板谷治郎
    • Organizer
      第79回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 固体高調波分光における偏光とサブサイクル時間分解2018

    • Author(s)
      石井 順久
    • Organizer
      日本物理学会第73回年次大会
    • Related Report
      2017 Annual Research Report
    • Invited
  • [Presentation] Ellipsometry of high harmonics generated from gallium selenide irradiated by mid-infrared pulses2017

    • Author(s)
      Nobuhisa Ishii, Keisuke Kaneshima, Yasushi Shinohara, Kengo Takeuchi, Kenichi L. Ishikawa, Jiro Itatani
    • Organizer
      6th International Conference on Attosecond Physics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Polarization property of high harmonics generated from crystalline semiconductors excited by mid-infrared pulses2017

    • Author(s)
      Nobuhisa Ishii, Keisuke Kaneshima, Yasushi Shinohara, Kengo Takeuchi, Kenichi L. Ishikawa, Jiro Itatani
    • Organizer
      The European Conference on Lasers and Electro-Optics
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Ellipsometry of high harmonics in GaSe pumped by 3.3 μm optical parametric amplifiers2017

    • Author(s)
      Faming Lu, Teruto Kanai, Peiyu Xia, Nobuhisa Ishii, Jiro itatani
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] ナノチップにおける中赤外電場増強と光電子放出2017

    • Author(s)
      竹内 健悟、水野 智也、金島 圭佑、金井 輝人、石井 順久、板谷 治郎
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 固体結晶GaSeにおける深紫外域の高次高調波発生2017

    • Author(s)
      梶 智博、今坂 光太郎、金島 圭佑、石井 順久、板谷 治郎、芦原 聡
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 結晶対称性によって制御された固体からの円偏光高調波発生2017

    • Author(s)
      齋藤 成之、石井 順久、金井 輝人、渡部 俊太郎、板谷 治郎
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 高エネルギー光電子用運動量画像計測装置の開発と高強度赤外電場中での光イオン化過程2017

    • Author(s)
      水野 智也、竹内 健悟、Geiseler Henning、石井 順久、金井 輝人、板谷 治郎
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Annual Research Report
  • [Remarks] 固体結晶からの高次高調波発生の偏光分解測定 高調波の偏光に電子状態の異方性が映し出されることを実証

    • URL

      http://www.issp.u-tokyo.ac.jp/maincontents/news2.html?pid=5281

    • Related Report
      2018 Annual Research Report

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Published: 2017-04-28   Modified: 2021-02-19  

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