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Cooperative monopole dynamics in spin ice

Research Project

Project/Area Number 17H04849
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Condensed matter physics II
Research InstitutionKyoto University

Principal Investigator

Takatsu Hiroshi  京都大学, 工学研究科, 講師 (60585602)

Project Period (FY) 2017-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥25,090,000 (Direct Cost: ¥19,300,000、Indirect Cost: ¥5,790,000)
Fiscal Year 2020: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Fiscal Year 2019: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Fiscal Year 2018: ¥7,410,000 (Direct Cost: ¥5,700,000、Indirect Cost: ¥1,710,000)
Fiscal Year 2017: ¥12,220,000 (Direct Cost: ¥9,400,000、Indirect Cost: ¥2,820,000)
Keywordsスピンアイス / カゴメアイス / 量子スピンアイス / 磁気モノポール / Dy2Ti2O7 / Tb2Ti2O7 / Ho2Ti2O7 / 磁性 / 物性実験 / 低温物性
Outline of Final Research Achievements

An elementary excitation in spin ice shows similar properties of the Dirac monopole that interacts with magnetic Coulomb forces. However, it has not been clarified whether the excitation manifests itself as a magnetic relaxation phenomenon or it can behave like a quasiparticle with a cooperative phenomenon. In this study, we have focused on Dy2Ti2O7and Tb2Ti2O7, and studied novel elementary excitation phenomena in spin ice, such as two-dimensional (2D) monopoles and quantum monopoles. We have found that the ac frequency dependent magnetic susceptibility in the 2D spin ice of Dy2Ti2O7 shows a single scaling form, which can be understood in terms of the dynamical scaling low for 2D Coulomb gas system (Phys. Rev. B 90, 144428 (2014).). We also realized for Tb2Ti2O7 that the behavior of the monopole characterized by a quantum spin ice could be clarified as information on thermal excitation. These studies shed light on the novel dynamics of monopole phenomenon in condensed matter physics.

Academic Significance and Societal Importance of the Research Achievements

本研究の結果、モノポールの2次元ダイナミクスは2次元XYモデルの理想的な実験系であること、そしてモノポール対間の相関長が重要な物理量であることが明らかになった。これは、スピンアイスにおけるモノポールのダイナミクスに関する新しい実験事実であり、固体凝縮相における新奇な素励起の実態を明らかにした点で学術的に非常に重要な成果である。また、Tb2Ti2O7でも量子スピンアイスを特徴づけるモノポールの振る舞いを熱励起の情報として明らかにでき、今後の研究につながる研究成果をあげることができた。

Report

(5 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • Research Products

    (34 results)

All 2021 2020 2019 2018 2017 Other

All Int'l Joint Research (3 results) Journal Article (11 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 10 results,  Open Access: 2 results) Presentation (19 results) (of which Int'l Joint Research: 3 results,  Invited: 2 results) Book (1 results)

  • [Int'l Joint Research] NIST(米国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] NCNR(米国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] NCNR, NIST(米国)

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Epitaxial Stabilization of SrCu3O4 with Infinite Cu3/2O2 Layers2020

    • Author(s)
      Takatsu Hiroshi、Ochi Masayuki、Yamashina Naoya、Namba Morito、Kuroki Kazuhiko、Terashima Takahito、Kageyama Hiroshi
    • Journal Title

      Inorganic Chemistry

      Volume: 59 Issue: 14 Pages: 10042-10047

    • DOI

      10.1021/acs.inorgchem.0c01213

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Hidden Ladder in SrMoO3/SrTiO3 Superlattices: Experiments and Theoretical Calculations2020

    • Author(s)
      Takatsu Hiroshi、Yamashina Naoya、Ochi Masayuki、Huang Hsin-Hui、Kobayashi Shunsuke、Kuwabara Akihide、Terashima Takahito、Kuroki Kazuhiko、Kageyama Hiroshi
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 89 Issue: 7 Pages: 074801-074801

    • DOI

      10.7566/jpsj.89.074801

    • NAID

      40022283455

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Molecular beam epitaxy growth of the highly conductive oxide SrMoO32020

    • Author(s)
      H. Takatsu, N. Yamashina, D. Shiga, R. Yukawa, K. Horiba, H. Kumigashira, T. Terashima, H. Kageyama
    • Journal Title

      J. Cryst. Growth

      Volume: in press Pages: 125685-125685

    • DOI

      10.1016/j.jcrysgro.2020.125685

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] A Partial Anion Disorder in SrVO2H Induced by Biaxial Tensile Strain2020

    • Author(s)
      M. Namba, H. Takatsu, W. Yoshimune, A. Daniel, S. Itoh, T. Terashima, and H. Kageyama
    • Journal Title

      Inorganics

      Volume: 8 Issue: 4 Pages: 26-26

    • DOI

      10.3390/inorganics8040026

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High Pressure Synthesis of Non-Stoichiometric LixWO3(0.5 < x < 1.0) with LiNbO3 Structure2019

    • Author(s)
      Kohdai Ishida, Yuya Ikeuchi, Cedric Tassel, Hiroshi Takatsu, Craig M. Brown, and Hiroshi Kageyama
    • Journal Title

      Inorganics

      Volume: 7 Issue: 5 Pages: 63-63

    • DOI

      10.3390/inorganics7050063

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Rattling Behavior in a Simple Perovskite NaWO32019

    • Author(s)
      Y. Ikeuchi, H. Takatsu, C. Tassel, C. M. Brown, T. Murakami, Y. Matsumoto, Y. Okamoto, and H. Kageyama
    • Journal Title

      Inorg. Chem.

      Volume: *** Issue: 10 Pages: 6790-6795

    • DOI

      10.1021/acs.inorgchem.9b00248

    • NAID

      130007735193

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] High-Pressure Synthesis of A2NiO2Ag2Se2 (A=Sr, Ba) with a High-Spin Ni2+ in Square-Planar Coordination2018

    • Author(s)
      Matsumoto Yuki、Yamamoto Takafumi、Nakano Kousuke、Takatsu Hiroshi、Murakami Taito、Hongo Kenta、Maezono Ryo、Ogino Hiraku、Song Dongjoon、Brown Craig M.、Tassel Cedric、Kageyama Hiroshi
    • Journal Title

      Angewandte Chemie International Edition

      Volume: 58 Issue: 3 Pages: 756-759

    • DOI

      10.1002/anie.201810161

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Field-rotational Magnetocaloric Effect: A New Experimental Technique for Accurate Measurement of the Anisotropic Magnetic Entropy2018

    • Author(s)
      Kittaka Shunichiro、Nakamura Shota、Kadowaki Hiroaki、Takatsu Hiroshi、Sakakibara Toshiro
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 87 Issue: 7 Pages: 073601-073601

    • DOI

      10.7566/jpsj.87.073601

    • NAID

      210000134879

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Continuum excitation and pseudospin wave in quantum spin-liquid and quadrupole ordered states of Tb2+xTi2-xO7+y2018

    • Author(s)
      H. Kadowaki, M. Wakita, B. Fak, J. Ollivier, S. Ohira-Kawamura, K. Nakajima, H. Takatsu and M. Tamai
    • Journal Title

      J. Phys. Soc. Jpn

      Volume: 87 Issue: 6 Pages: 0647041-6

    • DOI

      10.7566/jpsj.87.064704

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] パイロクロア磁性体Tb2Ti2O7における隠れた秩序と量子スピン液体状態2017

    • Author(s)
      高津 浩
    • Journal Title

      波紋

      Volume: 27 Pages: 140-143

    • NAID

      130007510649

    • Related Report
      2017 Annual Research Report
  • [Journal Article] High Pressure Synthesis of Fully Occupied Tetragonal and Cubic Tungsten Bronze Oxides2017

    • Author(s)
      Yuya Ikeuchi, Hiroshi Takatsu, Cedric Tassel, Yoshihiro Goto, Taito Murakami, and Hiroshi Kageyama*
    • Journal Title

      Angew.Chem.

      Volume: 56 Issue: 21 Pages: 5770-5773

    • DOI

      10.1002/anie.201701732

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed
  • [Presentation] 新規酸水素化物EuVO2Hの合成と基板応力による物性制御2020

    • Author(s)
      難波 杜人, 高津 浩, 北川 俊作, 三木田 梨歩, 姚 思伽, 石田 憲二, 寺嶋 孝仁, 陰山 洋, 木本 浩司, 片山 真祥, 伊奈 稔哲, 加藤 和男, 丸山 敬裕, 近松 彰, 長谷川 哲也
    • Organizer
      本セラミックス協会 第33回秋季シンポジウム
    • Related Report
      2020 Annual Research Report
  • [Presentation] 高圧・薄膜合成で開拓する定比組成タングステンブロンズおよび複合アニオン化合物2020

    • Author(s)
      高津 浩
    • Organizer
      第16回 新機能無機物質探索研究センターシンポジウム
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] 複合アニオン磁性体AVO2H (A = Sr, Eu)のV-NMR2020

    • Author(s)
      北川俊作, 金城克樹, 石田憲二, 難波杜人, 高津浩, 陰山洋
    • Organizer
      日本物理学会 第75回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Incipient narrow bandをもった‘隠れた梯子格子’の酸化物人工超格子薄膜2019

    • Author(s)
      高津 浩, 山科 直也, 越智 正之, 黒木 和彦, 寺嶋 孝仁, 陰山 洋
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Rattling Behavior in a Simple Perovskite NaWO32019

    • Author(s)
      Hiroshi Takatsu
    • Organizer
      International Conference on Strongly Correlated Electron Systems, SCES 2019
    • Related Report
      2019 Annual Research Report
  • [Presentation] XANESで明らかにする新規ユウロピウム酸水素化物の価数状態2019

    • Author(s)
      高津 浩, 難波 杜人, 陰山 洋, 片山 真祥
    • Organizer
      立命館SRセンター成果報告会
    • Related Report
      2019 Annual Research Report
  • [Presentation] スピンアイスDy2Ti2O7の気相液相転移の本質的転移幅について2019

    • Author(s)
      元木 大介, 河野 洋平, 橘高 俊一郎, 榊原 俊郎, 高津 浩, 門脇 広明
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] キタエフスピン液体候補物質alpha-RuCl3の単層薄膜作製II2019

    • Author(s)
      成塚 政裕,高津 浩,笠原 成, 笠原 裕一, 寺嶋 孝仁, 陰山 洋, 松田 祐司
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 巨大磁気異方性を有する酸水素化物EuVO2Hの単結晶薄膜2019

    • Author(s)
      難波 杜人, 高津 浩, 三木田 梨歩, 姚 思伽, 片山 真祥, 伊奈 稔哲, 加藤 和男, 寺嶋 孝仁, 陰山 洋
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 新しい層状銅酸化物の薄膜合成と低温物性2019

    • Author(s)
      Hiroshi Takatsu
    • Organizer
      日本物理学会 第74年回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] キタエフスピン液体候補物質α-RuCl3の単層薄膜作製2019

    • Author(s)
      成塚 政裕,高津 浩,笠原 成, 笠原 裕一, 寺嶋 孝仁, 陰山 洋, 松田 祐司
    • Organizer
      日本物理学会 第74年回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] モリブデン系酸化物人工超格子による超伝導の理論的検討2019

    • Author(s)
      山科 直也,高津 浩,黒木 和彦, 越智 正之, 陰山 洋
    • Organizer
      応用物理学会 春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] High Pressure Synthesis of Oxides and Mixed-anion Oxides with Novel Magnetic and Transport Properties2018

    • Author(s)
      H. Takatsu, H. Kageyama
    • Organizer
      14th International Ceramics Congress, CIMTEC 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 単純なペロブスカイト構造をもつNaWO3に見られるラットリング現象2018

    • Author(s)
      高津 浩,池内 勇哉,Cedric Tassel,Craig Brown, 村上 泰斗,松本 勇輝, 岡本 佳比古,陰山 洋
    • Organizer
      日本物理学会 2018年秋大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] LaドープしたSrVO2H薄膜の合成と低温物性2018

    • Author(s)
      高津 浩,Daniel Aurelien,三木田 梨歩,吉宗 航,寺嶋 孝仁,陰山 洋
    • Organizer
      日本物理学会 2018年秋大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] スピンアイスDy2Ti2O7の気相液相転移再考2018

    • Author(s)
      元木 大介, 河野 洋平, 橘高 俊一郎, 榊原 俊郎, 高津 浩, 門脇 広明
    • Organizer
      日本物理学会 2018年秋大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Quadrupole order and quantum spin liquid states in Tb2+xTi2-xO7+y2017

    • Author(s)
      Hiroshi Takatsu
    • Organizer
      International Conference on Strongly Correlated Electron Systems, SCES 2017
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Two dimensional monopole dynamics in spin ice2017

    • Author(s)
      Hiroshi Takatsu
    • Organizer
      JSPS Core-to-Core Workshop
    • Related Report
      2017 Annual Research Report
    • Int'l Joint Research
  • [Presentation] K0.6-xWO3(0.0 < x < 0.22)の異常金属相における電子状態2017

    • Author(s)
      池内勇哉, 高津浩, Cedric Tassel,村上泰斗, 陰山洋
    • Organizer
      日本物理学会 2017年秋大会
    • Related Report
      2017 Annual Research Report
  • [Book] 複合アニオン化合物の科学2021

    • Author(s)
      陰山 洋(編集), 荻野 拓(編集), 長谷川 哲也(編集) : 高津 浩 3.3節・分光法、3.4節・組成分析、付録A, B 担当
    • Total Pages
      264
    • Publisher
      丸善出版
    • ISBN
      9784621306109
    • Related Report
      2020 Annual Research Report

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Published: 2017-04-28   Modified: 2022-05-23  

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