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Active control of lubrication properties of concentrated polymer brushes based on self assembly and stimuli-response

Research Project

Project/Area Number 17H04902
Research Category

Grant-in-Aid for Young Scientists (A)

Allocation TypeSingle-year Grants
Research Field Design engineering/Machine functional elements/Tribology
Research InstitutionTsuruoka National College of Technology

Principal Investigator

arafune hiroyuki  鶴岡工業高等専門学校, その他部局等, 准教授 (90707811)

Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥24,050,000 (Direct Cost: ¥18,500,000、Indirect Cost: ¥5,550,000)
Fiscal Year 2019: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2018: ¥10,010,000 (Direct Cost: ¥7,700,000、Indirect Cost: ¥2,310,000)
Fiscal Year 2017: ¥11,830,000 (Direct Cost: ¥9,100,000、Indirect Cost: ¥2,730,000)
Keywordsポリマーブラシ / トライボロジー / イオン液体 / 界面分析
Outline of Final Research Achievements

Development of low frictional materials are important issue to shift from mass consumption society to circular one because 75% of the degradation or breakdown are related to friction and wear of contact surface. In this research, we pursued improving the robustness of concentrated polymer brushes (CPB) by supplying brush resources from inside of lubrication layer to form loop-shaped CPB by self-aggregation.
Applying ABA-type triblock coplymer PBMA-PEG-PBMA into PBMA as loop-shaped CPB resources effectively reduced friction and improved robustness in glycerol solution. This concept was also confirmed in ionic liquids system, which means that it is expected to be applied for high temperature or vacuum.

Academic Significance and Societal Importance of the Research Achievements

機械機器の性能劣化の75%を占める表面・接触面の劣化改善に寄与する低摩擦材料の開発 は、消費型から循環型への社会移行において重要な課題である。低摩擦材料として期待される濃厚ポリマーブラシ(CPB)は不活性雰囲気でのコーティングが必要であり、また耐久性の向上が課題となっていた。
本研究は自己偏析によりループ型CPBを形成する技術であり、大気下でのCPB形成を可能とし、また従来の直鎖型CPBよりも高い耐久性を示す。本研究はCPBの低摩擦材料への展開における設計指針に資するとともに、自動車や家電製品の省エネ化・長寿化に寄与することが期待される。

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Annual Research Report
  • 2017 Annual Research Report
  • Research Products

    (15 results)

All 2020 2019 2018 2017 Other

All Int'l Joint Research (1 results) Journal Article (1 results) (of which Peer Reviewed: 1 results,  Acknowledgement Compliant: 1 results) Presentation (12 results) (of which Int'l Joint Research: 4 results,  Invited: 1 results) Patent(Industrial Property Rights) (1 results)

  • [Int'l Joint Research] Ecole Centrale de Lyon(フランス)

    • Related Report
      2017 Annual Research Report
  • [Journal Article] Highly robust and low frictional double-network ion gel2017

    • Author(s)
      Hiroyuki Arafune, Saika Honma, Toshio Kamijo, Takashi Morinaga, Miki Miura, Hidemitsu Furukawa, Takaya Sato
    • Journal Title

      Advanced Materials Interfaces

      Volume: 5 Issue: 9 Pages: 1700741-5

    • DOI

      10.1002/admi.201700074

    • Related Report
      2017 Annual Research Report
    • Peer Reviewed / Acknowledgement Compliant
  • [Presentation] Characterization of mechanical and frictional properties of ionic liquid-type double network gels2020

    • Author(s)
      Hiroyuki Arafune, Toshio Kamijo, Saika Honma, Takashi Morinaga, Takaya Sato
    • Organizer
      Polymer science conference
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Lubrication properties of double network gels composed of ionic liquids2020

    • Author(s)
      Hiroyuki Arafune, Toshio Kamijo, Takashi Morinaga and Takaya Sato
    • Organizer
      ICKEM2020
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 表面偏析により形成したポリマーブラシの潤滑特性評価2019

    • Author(s)
      荒船博之、上條利夫、本間彩夏、森永隆志、佐藤貴哉
    • Organizer
      第29回日本MRS年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 共振ずり測定を利用したイオン液体界面の潤滑挙動解析2019

    • Author(s)
      荒船博之
    • Organizer
      第35回緑陰セミナー
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Characterization of soft polymer interface lubricated by ionic liquids2019

    • Author(s)
      Hiroyuki Arafune, Toshio Kamijo, Takashi Morinaga, Takaya Sato
    • Organizer
      ITC 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] A robust lubrication system based on ionic liquid-type polymer materials2018

    • Author(s)
      Hiroyuki Arafune
    • Organizer
      2018 International conference of young researchers on advanced materials
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] イオン液体を用いたソフトトライボロジー材料2018

    • Author(s)
      佐藤 貴哉
    • Organizer
      第28回日本MRS年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] イオン液体型濃厚ポリマーブラシにおける潤滑特性解析2018

    • Author(s)
      荒船博之、本間彩夏、森永隆志、上條利夫、佐藤貴哉
    • Organizer
      第28回日本MRS年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] イオン液体型濃厚ポリマーブラシによる低摩擦系の構築2017

    • Author(s)
      荒船博之、上條利夫、森永隆志、佐藤貴哉
    • Organizer
      日本MRS年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] 親水性イオン液体置換型ダブルネットワークゲルの潤滑特性2017

    • Author(s)
      武藤史弥、荒船博之、上條利夫、佐藤貴哉
    • Organizer
      日本MRS年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] ロバストな低摩擦系を指向したイオン液体型濃厚ポリマーブラシと平滑膜の複合2017

    • Author(s)
      荒船博之、上條利夫、森永隆志、佐藤貴哉
    • Organizer
      繊維学会年次大会
    • Related Report
      2017 Annual Research Report
  • [Presentation] イオン液体型濃厚ポリマーブラシと平滑ガラスの複合系における潤滑特性2017

    • Author(s)
      荒船博之,上條利夫,森永隆志,本間彩夏,中野健,辻井敬亘,佐藤貴哉
    • Organizer
      トライボロジー会議2017春
    • Related Report
      2017 Annual Research Report
  • [Patent(Industrial Property Rights)] ポリマーブラシ層の形成方法2017

    • Inventor(s)
      佐藤貴哉 他6名
    • Industrial Property Rights Holder
      佐藤貴哉 他6名
    • Industrial Property Rights Type
      特許
    • Filing Date
      2017
    • Related Report
      2017 Annual Research Report

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Published: 2017-04-28   Modified: 2021-02-19  

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