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Development of eco-friendly and low cost process for the production of bioethanol

Research Project

Project/Area Number 17K00669
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Design and evaluation of sustainable and environmental conscious system
Research InstitutionThe University of Tokushima

Principal Investigator

SASAKI Chizuru  徳島大学, 大学院社会産業理工学研究部(生物資源産業学域), 准教授 (50452652)

Co-Investigator(Kenkyū-buntansha) ALCANTARA J.RAFAEL (アルカンタラ アビラ・ラファエル)  京都大学, 工学研究科, 講師 (50709219)
Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2019: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2018: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2017: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Keywordsリグノセルロース / バイオマス / 加水分解 / 水熱処理 / バイオエタノール / 蒸留 / セルロース / 糖化 / グルコース
Outline of Final Research Achievements

To produce bioethanol at low cost and low energy, direct hydrolysis of cellulose (cotton towel) to glucose was investigated using microwave-assisted treatment. We found the optimal direct hydrolysis condition using diluted sulfuric acid as catalyst. Next, novel direct hydrolysis method for cotton towel was investigated using microwave combined with impregnation in concentrated fulsufic acid before the micowave treatment. This combination method proposed had some advantages such as higher hydrolysis glucose recovery yield and low input energy. Moreover, extractive distillation of bioethanol with addiive was investigated, ethanol was concentrated at high purity (98mol%).

Academic Significance and Societal Importance of the Research Achievements

リグノセルロース系バイオマスを原料としたバイオエタノール生産プロセスの実現に向けて、環境低負荷やコストダウンに繋がる研究の進展に寄与した。セルロースを酵素加水分解する方法の代替法として、水熱処理による直接糖化法を開発し、また、バイオエタノールの精製法として環境低負荷な物質を添加する方法を見出した。

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (22 results)

All 2020 2019 2018 2017

All Journal Article (9 results) (of which Peer Reviewed: 9 results) Presentation (12 results) (of which Int'l Joint Research: 4 results) Book (1 results)

  • [Journal Article] Microwave-assisted hydrolysis of cotton waste to glucose in combination with the concentrated sulfuric acid impregnation method2020

    • Author(s)
      Chizuru Sasaki, Tomoya Nakagawa, Chikako Asada, Yoshitoshi Nakamura
    • Journal Title

      Waste and Biomass Valorization

      Volume: -

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ethanol Production from Sugarcane Bagasse Using Pressurized Microwave Treatment with Inorganic Salts and Salt-Tolerant Yeast2020

    • Author(s)
      Chikako Asada, Chizuru Sasaki, Chihiro Oka and Yoshitoshi Nakamura
    • Journal Title

      Waste and Biomass Valorization

      Volume: 11 Pages: 2001-2007

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Microwave-assisted glucose production from bode (Styrax tonkinensis) woody biomass for bioethanol production2019

    • Author(s)
      Chizuru Sasaki, Haruka Negoro, Chikako Asada, Yoshitoshi Nakamura
    • Journal Title

      Journal of Material Cycles and Waste Management

      Volume: 21 Pages: 201-204

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Glucose and Valuable chemicals production from cotton waste using hydrothermal method2019

    • Author(s)
      Chizuru Sasaki, Ami Kiyokawa, Chikako Asada and Yoshitoshi Nakamura
    • Journal Title

      Waste and Biomass Valorization

      Volume: 10 Pages: 599-607

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Production of cellulose nanofibers from Aspen and Bode chopsticks using a high temperature and high pressure steam treatment combined with milling2018

    • Author(s)
      A. Suzuki, C. Sasaki, C. Asada, Y. Nakamura
    • Journal Title

      Carbohydrate Polymers

      Volume: - Pages: 303-310

    • DOI

      10.1016/j.carbpol.2018.04.047

    • Related Report
      2018 Research-status Report
    • Peer Reviewed
  • [Journal Article] Total Biorefinery Process of Lignocellulosic Waste Using Steam Explosion Followed by Water and Acetone Extractions2018

    • Author(s)
      Asada C.、Sasaki C.、Suzuki A.、Nakamura Y.
    • Journal Title

      Waste and Biomass Valorization

      Volume: 印刷中 Issue: 12 Pages: 2423-2432

    • DOI

      10.1007/s12649-017-0157-x

    • Related Report
      2018 Research-status Report 2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Glucose and Valuable Chemicals Production from Cotton Waste Using Hydrothermal Method2018

    • Author(s)
      Chizuru Sasaki, Ami Kiyokawa, Chikako Asada and Yoshitoshi Nakamura
    • Journal Title

      Waste and Biomass Valorization

      Volume: 印刷中 Issue: 3 Pages: 599-607

    • DOI

      10.1007/s12649-017-0084-x

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] High concentration ethanol production from mixed softwood sawdust waste2018

    • Author(s)
      Chikako Asada, Chizuru Sasaki, Yoshitoshi Nakamura
    • Journal Title

      Waste and Biomass Valorization

      Volume: 印刷中 Issue: 2 Pages: 433-439

    • DOI

      10.1007/s12649-017-0073-0

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Characterization of cellulose nanofiber from steam exploded Japanese cedar2017

    • Author(s)
      Akihiro Suzuki, Chizuru Sasaki, Chikako Asada, Yoshitoshi Nakamura
    • Journal Title

      BioResources

      Volume: 12 Pages: 7628-7641

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Presentation] 塩による効果を用いたエタノール精製プロセスの開発2020

    • Author(s)
      中村友紀, アルカンタラアヴィラ ヘスース ラファエル, 佐々木千鶴
    • Organizer
      化学工学会第85年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 塩含有溶媒を用いた抽出蒸留によるバイオエタノール脱水プロセスに関する研究2020

    • Author(s)
      トマ ガブリエル, アルカンタラアヴィラ ヘスース ラファエル, 佐々木千鶴
    • Organizer
      化学工学会第85年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] アルカリ凍結融解と水熱処理を併用した木質バイオマス中のセルロースの糖化に関する研究2019

    • Author(s)
      小田島海, 佐々木千鶴, 淺田元子, 中村嘉利
    • Organizer
      2019年度日本化学会中国四国支部大会徳島大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 高活性水蒸気処理を用いたセルロースナノファイバーの製造とバイオマスコンポジットへの応用2018

    • Author(s)
      橋本和紀、淺田元子、佐々木千鶴、中村嘉利
    • Organizer
      生物工学会
    • Related Report
      2018 Research-status Report
  • [Presentation] 高活性水蒸気処理と粉砕処理を併用したバイオリファイナリーシステムの開発2018

    • Author(s)
      鈴木昭浩、淺田元子、佐々木千鶴、中村嘉利
    • Organizer
      生物工学会
    • Related Report
      2018 Research-status Report
  • [Presentation] Synthesis of ecomaterial from plant biomass and its physical properties2017

    • Author(s)
      Akihiro Suzuki, Chikako Asada, Chizuru Sasaki, Yoshitoshi Nakamura
    • Organizer
      International Conference on Ecomaterials
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Comparison of steam explosion and steaming followed by milling treatment for bioethanol production from woody baiomss2017

    • Author(s)
      Yuta Danura, Chikako Asada, Chizuru Sasaki, Yoshitoshi Nakamura
    • Organizer
      International Conference on Ecomaterials
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Organosolv lignin extracted from hydrolyzed residue of steam exploded hardwood: a potential candidate for epoxy resin2017

    • Author(s)
      Takuya Yamamoto, Chikako Asada, Chizuru Sasaki, Yoshitoshi Nakamura
    • Organizer
      International Conference on Ecomaterials
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Glucose production from cotton-waste using hydrothermal methods2017

    • Author(s)
      Chizuru Sasaki, Chikako Asada, Yoshitoshi Nakamura
    • Organizer
      The 4th International Cellullose Conference
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] バイオマスへの応用を考慮した耐熱性セルラーゼ利用のための酵素カクテルの相乗効果検討2017

    • Author(s)
      髙田弥生、淺田元子、佐々木千鶴、中村嘉利
    • Organizer
      第9回日本醸造学会 若手シンポジウム
    • Related Report
      2017 Research-status Report
  • [Presentation] ファルカタを原料としたバイオエタノール製造のための水蒸気爆砕前処理の最適条件の検討2017

    • Author(s)
      妹尾政都、浅田元子、佐々木千鶴、中村嘉利
    • Organizer
      第9回日本醸造学会 若手シンポジウム
    • Related Report
      2017 Research-status Report
  • [Presentation] バイオエタノール残渣となるモデルリグニンを用いたエポキシ樹脂合成の抽出溶媒検討2017

    • Author(s)
      藤井萌、浅田元子、佐々木千鶴、中村嘉利
    • Organizer
      第9回日本醸造学会 若手シンポジウム
    • Related Report
      2017 Research-status Report
  • [Book] 枯渇資源と技術開発, --- 徳島大学における分野融合型枯渇資源対応技術の開発 ---2020

    • Author(s)
      杉山茂、森賀 俊広, 加藤 雅裕, 村井 啓一郎, 堀河 俊英, 霜田 直宏, 古部 昭広, 柳谷 伸一郎, 小笠原 正道, 山本 孝, 中村 嘉利, 浅田 元子, 佐々木 千鶴、田中 秀治, 竹内 政樹, 竹谷 豊, 奥村 仙示, 増田 真志, 岡本 敏弘
    • Total Pages
      5
    • Publisher
      徳島大学産業院出版部
    • Related Report
      2019 Annual Research Report

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Published: 2017-04-28   Modified: 2021-02-19  

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