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Electronic states of bismuth layered materials with black-phosphorus-like structure

Research Project

Project/Area Number 17K05493
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Condensed matter physics I
Research InstitutionTokyo Institute of Technology

Principal Investigator

Nakatsuji Kan  東京工業大学, 物質理工学院, 准教授 (80311629)

Co-Investigator(Kenkyū-buntansha) 平山 博之  東京工業大学, 理学院, 教授 (60271582)
Project Period (FY) 2017-04-01 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2019: ¥1,040,000 (Direct Cost: ¥800,000、Indirect Cost: ¥240,000)
Fiscal Year 2018: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2017: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywords表面電子状態 / ビスマス超薄膜 / 光電子分光 / 走査トンネル顕微鏡 / 表面・界面物性
Outline of Final Research Achievements

Bi(110) ultra-thin films with black-phosphorous-like (BP-like) structure attract much interest as a candidate of two-dimensional topological insulator. In the present study, the atomic and electronic structures of Bi(110) ultra-thin films grown on silicon substrates are systematically investigated by angle-resolved photoelectron spectroscopy and scanning tunneling microscopy. It was reveled that the internal atomic structure of the film below 8 atomic layers is BP-like. The films are hole-doped by charge transfer from the substrate. The two-step growth in which the Bi atoms are deposited at 100 K followed by annealing to room temperature resulted in the films with unique height in a wide area.

Academic Significance and Societal Importance of the Research Achievements

黒リン構造のBi(110)超薄膜は、基板との相互作用や電荷移動によるトポロジカル絶縁体転移が予想されており、その電子状態が大変興味深いにもかかわらず、研究例は少ない状態であった。本研究により、デバイス整合性のよい半導体基板を用いて将来的に半導体技術で電荷量を制御する可能性を担保したうえで、Bi(110超薄膜の成長過程と電子状態についての系統的な知見を得ることができたことは、学術的にも社会的にも大変意義深いことと考えている。

Report

(6 results)
  • 2021 Annual Research Report   Final Research Report ( PDF )
  • 2020 Research-status Report
  • 2019 Research-status Report
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (19 results)

All 2020 2019 2018 2017 Other

All Journal Article (2 results) (of which Peer Reviewed: 2 results) Presentation (16 results) (of which Int'l Joint Research: 5 results) Remarks (1 results)

  • [Journal Article] Growth of extremely flat Bi(110) films on a Si(111)√3 × √3-B substrate2020

    • Author(s)
      Nagase Kentaro、Ushioda Ryota、Nakatsuji Kan、Shirasawa Tetsuroh、Hirayama Hiroyuki
    • Journal Title

      Applied Physics Express

      Volume: 13 Issue: 8 Pages: 085506-085506

    • DOI

      10.35848/1882-0786/aba0df

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] Structure and growth of Bi(110) islands on Si(111)√3×√3-B substrates2018

    • Author(s)
      Nagase Kentaro、Kokubo Ikuya、Yamazaki Shiro、Nakatsuji Kan、Hirayama Hiroyuki
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 19 Pages: 195418-195418

    • DOI

      10.1103/physrevb.97.195418

    • Related Report
      2018 Research-status Report
    • Peer Reviewed
  • [Presentation] Si(110)3x2-Bi表面の電子状態2020

    • Author(s)
      金野達、勝俣錬、木村彰博、中村玲雄、諸貫亮太、山崎詩郎、小澤健一、間瀬一彦、飯盛拓嗣、小森文夫、平山博之、中辻寬
    • Organizer
      2020年日本表面真空学会学術講演会
    • Related Report
      2020 Research-status Report
  • [Presentation] Si(111)√3×√3-(Bi,In)表面の電子状態2020

    • Author(s)
      勝俣錬, 中村玲雄, 金野達, 木村彰博, 大内拓実, 永友慶, 田中和也, 下川裕理, 小澤健一, 間瀬一彦, 小森文夫, 飯盛拓嗣, 平山博之, 中辻寬
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Research-status Report
  • [Presentation] Si(110)3×2-Bi表面の構造解析2020

    • Author(s)
      諸貫亮太, 大内拓実, 永友慶, 森井七生, 金野達, 白澤徹郎, 平山博之, 中辻寬
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Research-status Report
  • [Presentation] Si(111)7×7 基板上における奇数層高さBi(110)島の出現2020

    • Author(s)
      潮田亮太、長瀬謙太郎、荻野嵩大、車尾ヴァレンティン基、中辻 寛、白澤 徹郎、平山 博之
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Research-status Report
  • [Presentation] Si(110)3x2-Bi表面の電子状態2020

    • Author(s)
      金野達、勝俣錬、木村彰博、中村玲雄、山崎詩郎、小澤健一、 間瀬一彦、飯盛拓嗣、小森文夫、平山博之、中辻寛
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Research-status Report
  • [Presentation] Electronic structure of Bi(110) ultra-thin films grown on a Si(111)√3×√3-B substrate2019

    • Author(s)
      K. Nakatsuji, Y. Shimokawa, T. Fujiwara, K. Nagase, S. Yamazaki, Y. Watanabe, K. Mase, K. Takahashi and H. Hirayama
    • Organizer
      21th International Vacuum Congress (IVC-21)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Si(111)√3×√3-B基板上に低温蒸着したビスマス超薄膜の室温アニールによる構造変化2019

    • Author(s)
      長瀬謙太郎、山崎詩郎、中辻寛、平山博之
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Research-status Report
  • [Presentation] Structural change of Bi ultrathin films in the two-step growth on Si(111)√3 x √3-B substrates2019

    • Author(s)
      K. Nagase, S. Yamazaki, K. Nakatsuji and H. Hirayama
    • Organizer
      12th International Symposium on Atomic Level Characterizations for New Materials and Devices (ALC-19)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Si(111)√3x√3-B基板上に低温吸着したビスマス超薄膜のアニールによる構造変化2018

    • Author(s)
      長瀬謙太郎、山崎詩郎、中辻寛、平山博之
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Research-status Report
  • [Presentation] Atomic Structure and Growth of Bi(110) Islands on Si(111)√3×√3-B Substrates2018

    • Author(s)
      K. Nagase, I. Kokubo, S. Yamazaki, K. Nakatsuji and H. Hirayama
    • Organizer
      14th International Conference on Atomically Controlled Surfaces, Interfaces and Nanostructures (ACSIN-14)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Electronic Structure of Bi(110) Islands Grown on a Si(111)√3×√3-B Substrate2018

    • Author(s)
      K. Nakatsuji, Y. Shimokawa, T. Fujiwara, K. Nagase, S. Yamazaki, Y. Watanabe, K. Mase, K. Takahashi and H. Hirayama
    • Organizer
      14th International Conference on Atomically Controlled Surfaces, Interfaces and Nanostructures (ACSIN-14)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Si(111)基板上におけるBi-In表面合金の構造と電子状態2018

    • Author(s)
      田中和也、金野達、下川裕理、佐藤圭介、山崎詩郎、飯盛拓嗣、小森文夫、間瀬一彦、平山博之、中辻寛
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Research-status Report
  • [Presentation] Bi/Si(111)4×1-In表面の構造と電子状態2018

    • Author(s)
      下川裕理、田中和也、佐藤圭介、渡邊瞳、山崎詩郎、飯盛拓嗣、小森文夫、間瀬一彦、平山博之、中辻寛
    • Organizer
      日本物理学会第73回年次大会
    • Related Report
      2017 Research-status Report
  • [Presentation] Si(111)√3x√3-B表面上に成長した数層Bi(110)薄膜の電子状態2017

    • Author(s)
      下川裕理、藤原翼、長瀬謙太郎、山崎詩郎、渡辺義夫、仲武昌史、間瀬一彦、高橋和敏、中辻寛、平山博之
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Research-status Report
  • [Presentation] 低温蒸着によるBi超薄膜の構造と電子状態2017

    • Author(s)
      長瀬謙太郎、山崎詩郎、中辻寛、平山博之
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Research-status Report
  • [Presentation] Electronic structure of Bi(110) ultra-thin films grown on Si(111)√3×√3-B surfaces2017

    • Author(s)
      Y. Shimokawa, T. Fujiwara, K. Nagase, S. Yamazaki, Y. Watanabe, M. Nakatake, K. Mase, K. Takahashi, K. Nakatsuji, H. Hirayama
    • Organizer
      The 8th International Symposium on Surface Science (ISSS-8)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Remarks]

    • URL

      http://www.materia.titech.ac.jp/~hirayama/2009hirayamalabHP/

    • Related Report
      2017 Research-status Report

URL: 

Published: 2017-04-28   Modified: 2023-01-30  

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