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Angular dependence of ionization probabilities on the angle between molecular axis and laser polarization direction

Research Project

Project/Area Number 17K05593
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Atomic/Molecular/Quantum electronics
Research InstitutionThe University of Tokyo

Principal Investigator

Hasegawa Hirokazu  東京大学, 大学院総合文化研究科, 准教授 (20373350)

Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2019: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2018: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2017: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Keywords高強度光 / 分子配列 / イオン化 / 角度依存性 / イオン化確率の角度依存性 / 回転波束 / イオン化確率 / 原子・分子物理
Outline of Final Research Achievements

In this study, a new method to determine the dependence of the ionization probabilities on the angle between a laser polarization direction and a molecular axis was developed. We showed that the angular dependence of the ionization probabilities can be determined by using the developed method. Two intense laser pulses were used in this method. The first pulse made a rotational wave packet. After the irradiation of the first pulse, molecules were ionized by the second pulse. We can determine the angular dependence of the ionization probabilities by measuring the dependence of the ion yields on the delay. We applied this method to NO molecule and showed that this method is available for the determination of the angular dependence of the ionization probabilities.In addition, we developed a new apparatus to measure molecular axis distribution by observing third-order harmonics induced by a probe pulse.

Academic Significance and Societal Importance of the Research Achievements

本研究では,高強度レーザー光による分子のイオン化確率の角度依存性の計測法開発を行い,この手法に基づいた高強度レーザー光の電場と分子軸のなす角度に依存したイオン化確率の決定を行った。この方法を用いることにより,分子の向きによりイオン化の確率の変化を明瞭に観測することができる。この成果は,強い光と物質の相互作用の起源を深く理解し,極限的な環境下での分子の振る舞いを明らかしたものである。

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (9 results)

All 2020 2018 2017

All Journal Article (3 results) (of which Peer Reviewed: 3 results) Presentation (6 results) (of which Int'l Joint Research: 2 results,  Invited: 2 results)

  • [Journal Article] Bromine-isotope Selective Ionization Using Field-free Alignment of IBr Isotopologues with a Switched Nanosecond Laser Pulse2020

    • Author(s)
      Akagi Hiroshi、Kumada Takayuki、Otobe Tomohito、Itakura Ryuji、Hasegawa Hirokazu、Ohshima Yasuhiro
    • Journal Title

      Chemistry Letters

      Volume: 49 Issue: 4 Pages: 416-418

    • DOI

      10.1246/cl.200024

    • NAID

      130007828845

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Field-free molecular orientation of nonadiabatically aligned OCS2018

    • Author(s)
      K.Sonoda, A.Iwasaki, K.Yamanouchi, and H.Hasegawa
    • Journal Title

      Chemical Physics Letters

      Volume: 693 Pages: 114-120

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Enhancement of field-free molecular orientation of OCS by intense laser fields2017

    • Author(s)
      K.Sonoda, A.Iwasaki, K.Yamanouchi, and H.Hasegawa
    • Journal Title

      AIP Conference Proceedings

      Volume: 1906 Pages: 030026-030026

    • DOI

      10.1063/1.5012306

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Presentation] 非共鳴 2 色高強度ピコ秒パルス光による NO のラムダ型二重項 間における波束生成2020

    • Author(s)
      中村健汰,深堀信一,長谷川宗良
    • Organizer
      日本化学会春季年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Single and double ionization of aligned NO in intense laser fields2020

    • Author(s)
      FUKAHORI Shinichi, IWASAKI Atsushi, YAMANOUCHI, Kaoru, HASEGAWA, Hirokazu
    • Organizer
      日本化学会春季年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 波形整形ナノ秒パルスによる分子整列制御を用いた IBr同位体選択的イオン化2018

    • Author(s)
      赤木浩,熊田高之,乙部智仁,板倉隆二,長谷川宗良,大島康裕
    • Organizer
      第12回分子科学討論会
    • Related Report
      2018 Research-status Report
  • [Presentation] ベンゼンクラスターにおける分子間振動ダイナミクスの時間領域観測2018

    • Author(s)
      村井友海,水瀬賢太,長谷川宗良,大島康裕
    • Organizer
      第12回分子科学討論会
    • Related Report
      2018 Research-status Report
  • [Presentation] Orientation Enhancement Of Aligned OCS In Field-Free Space2018

    • Author(s)
      Hirokazu Hasegawa
    • Organizer
      The 10th Asian Symposium on Intense Laser Science
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Enhancement of field-free molecular orientation of OCS by intense laser fields2017

    • Author(s)
      Hirokazu Hasegawa
    • Organizer
      3rd Computational Chemistry Symposium of International Conference of Computational Methods in Science and Engineering
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research / Invited

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Published: 2017-04-28   Modified: 2021-02-19  

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