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Development of hydrogen permeable catalytic membrane electrode for the synthesis of hydrogen carrier

Research Project

Project/Area Number 17K06902
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Reaction engineering/Process system
Research InstitutionUtsunomiya University

Principal Investigator

Sato Takafumi  宇都宮大学, 工学部, 准教授 (60375524)

Co-Investigator(Kenkyū-buntansha) 伊藤 直次  宇都宮大学, 工学部, 教授 (90356478)
Project Period (FY) 2017-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2019: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2018: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Fiscal Year 2017: ¥1,950,000 (Direct Cost: ¥1,500,000、Indirect Cost: ¥450,000)
Keywords水素透過膜 / 水電解 / 水素化 / ケミカルハイドライド / パラジウム膜 / 水素製造 / 水素分離膜 / 電解
Outline of Final Research Achievements

The system that enables electrolysis of water and hydrogenation for producing hydrogen carrier with hydrogen permeated through the membrane by using hydrogen permeable palladium membrane were developed. The platinum/alumina catalyst supported on stainless mesh promoted the hydrogenation of toluene to produce methylcyclohexane. Further, the modified electrolysis cell whose membrane area was larger and distance between electrodes was shorter was developed and the flow rate of hydrogen permeated through the membrane increased with increasing temperature.

Academic Significance and Societal Importance of the Research Achievements

再生可能エネルギー由来の電力の有効利用のためには、電力を用いて水を電気分解して水素を製造するシステムの構築が必要である。本研究で開発したシステムは、水電解に加えて生成した水素を水や酸素から分離することが可能となる利点を有する。また、そこで生成した水素を用いて有機化合物の水素化を行うと水素を液体として貯蔵・輸送することが可能となり、本研究の結果は、その一助となりうるものである。

Report

(5 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Research-status Report
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (8 results)

All 2020 2019 2018 2017

All Journal Article (2 results) (of which Peer Reviewed: 2 results) Presentation (6 results) (of which Int'l Joint Research: 3 results)

  • [Journal Article] Extraction of strawberry leaves with supercritical carbon dioxide and entrainers: Antioxidant capacity, total phenolic content, and inhibitory effect on uric acid production of the extract2019

    • Author(s)
      Sato Takafumi、Ikeya Yoshiro、Adachi Shin-ichi、Yagasaki Kazumi、Nihei Ken-ichi、Itoh Naotsugu
    • Journal Title

      Food and Bioproducts Processing

      Volume: 117 Pages: 160-169

    • DOI

      10.1016/j.fbp.2019.07.003

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Hydrothermal extraction of antioxidant compounds from green coffee beans and decomposition kinetics of 3-o-caffeoylquinic acid2018

    • Author(s)
      Takafumi Sato, Takuya Takahata, Tetsuo Honma, Masaru Watanabe, Masayoshi Wagatsuma, Shiho Matsuda, Richard Lee Smith, Jr., Naotsugu Itoh
    • Journal Title

      Ind. Eng. Chem. Res.

      Volume: 57 Issue: 22 Pages: 7624-7652

    • DOI

      10.1021/acs.iecr.8b00821

    • Related Report
      2018 Research-status Report
    • Peer Reviewed
  • [Presentation] 水素透過Pd-Ag膜セルを用いた水電解における水素生成速度の評価2020

    • Author(s)
      島村雛季,佐藤剛史,伊藤直次
    • Organizer
      化学工学会第51回秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 水素透過パラジウム膜を用いた水電解におけるセル特性評価2020

    • Author(s)
      島村雛季、佐藤剛史、伊藤直次
    • Organizer
      化学工学会第85年会
    • Related Report
      2019 Research-status Report
  • [Presentation] Hydrogenation of toluene by electrolysis of water with hydrogen permeable palladium membrane electrode and structured catalyst2019

    • Author(s)
      Takafumi Sato, Hinaki Shimamura, Naotsugu Itoh
    • Organizer
      14th International Conference on Catalysis in Membrane Reactors
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Chemical hydride synthesis with hydrogen permeable Pd-Ag membrane electrode and structured Pt/Al2O3 catalyst2019

    • Author(s)
      Hinaki Shimamura, Takafumi Sato, Naotsugu Itoh
    • Organizer
      The 18th Asian Pacific Confederation of Chemical Engineering Congress (APCChE 2019)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] 水素透過膜電極と構造体触媒を用いた水電解によるケミカルハイドライド製造2018

    • Author(s)
      島村 雛季, 佐藤 剛史, 伊藤 直次
    • Organizer
      第21回化学工学会学生発表会(東京大会)
    • Related Report
      2018 Research-status Report
  • [Presentation] Methane steam reforming using wall-tube reactor combined with palladium membrane as hydrogen extractor2017

    • Author(s)
      N. Itoh, M. Vasquez, T. Sato
    • Organizer
      APCChE 2017
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research

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Published: 2017-04-28   Modified: 2022-01-27  

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