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Study on hydrogen isotope behavior in fusion test device using tracer tritium by D-D reaction

Research Project

Project/Area Number 17K06998
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Research Field Nuclear fusion studies
Research InstitutionNational Institute for Fusion Science

Principal Investigator

Tanaka Masahiro  核融合科学研究所, ヘリカル研究部, 准教授 (00435520)

Project Period (FY) 2017-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2020: ¥390,000 (Direct Cost: ¥300,000、Indirect Cost: ¥90,000)
Fiscal Year 2019: ¥390,000 (Direct Cost: ¥300,000、Indirect Cost: ¥90,000)
Fiscal Year 2018: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2017: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywordsトリチウム挙動 / 物質収支 / 化学形態 / プラズマ対向壁材 / 赤外吸収分光計測 / 排気ガス組成 / トリチウム / トリチウム化学形態 / 分光計測 / プラズマ対向壁材料 / 排気ガス組成分析 / 放電洗浄
Outline of Final Research Achievements

The hydrogen isotope behavior in a large fusion test facility was evaluated for four years using tritium produced by D-D reaction as a tracer. As the results, it was found that: 1. 56% of the produced tritium remained in the vacuum vessel at the end of the fourth year of the deuterium plasma experiment; 2. the tritium release from the vacuum vessel was rate-limiting due to the isotope exchange reaction and tritium diffusion in the material; 3. the chemical form of the released tritium was molecular (Q2) >> hydrocarbon (CxQy) > water vapor (Q2O); 4. The exhaust gas composition was analyzed by infrared absorption spectroscopy, and deuterated hydrocarbons (CxHyDz), carbon monoxide, and ammonia were observed. The present study clarified the tritium balance in the fusion system and the complex behavior of the exhaust gas.

Academic Significance and Societal Importance of the Research Achievements

大型核融合試験装置の重水素実験で生成される極僅かのトリチウムをトレーサー(追跡子)として利用することで、核融合装置内外の水素同位体挙動を明らかにすることができました。さらに、核融合装置内から排出されるトリチウムは、さまざまな化学形態として存在すること、水素同位体交換反応と材料内での拡散速度に律速されていることを明らかにしました。この研究成果は、将来の核融合炉で燃料として使用されるトリチウムの安全取り扱いや、燃料を処理し再利用する循環システムに関する重要な知見となります。

Report

(5 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Research-status Report
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (24 results)

All 2021 2020 2019 2018 2017

All Journal Article (10 results) (of which Peer Reviewed: 10 results,  Open Access: 3 results) Presentation (14 results) (of which Int'l Joint Research: 7 results,  Invited: 2 results)

  • [Journal Article] Detection of Ammonia and Deuterated Hydrocarbons in Exhaust Gas by Infrared Absorption Spectroscopy during Wall Conditioning2021

    • Author(s)
      Tanaka Masahiro、Kato Hiromi、Suzuki Naoyuki、Chimura Hiroki
    • Journal Title

      Plasma and Fusion Research

      Volume: 16 Issue: 0 Pages: 2405062-2405062

    • DOI

      10.1585/pfr.16.2405062

    • NAID

      130008037256

    • ISSN
      1880-6821
    • Year and Date
      2021-04-21
    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Performance of exhaust detritiation system for a fusion test device in the initial phase of the operation2021

    • Author(s)
      Tanaka Masahiro、Suzuki Naoyuki、Kato Hiromi、Chimura Hiroki
    • Journal Title

      Fusion Engineering and Design

      Volume: 164 Pages: 112172-112172

    • DOI

      10.1016/j.fusengdes.2020.112172

    • NAID

      120007126864

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Tritium Balance in Large Helical Device during and after the First Deuterium Plasma Experiment Campaign2020

    • Author(s)
      TANAKA Masahiro、KATO Hiromi、SUZUKI Naoyuki、MASUZAKI Suguru、YAJIMA Miyuki、NAKADA Miki、IWATA Chie
    • Journal Title

      Plasma and Fusion Research

      Volume: 15 Issue: 0 Pages: 1405062-1405062

    • DOI

      10.1585/pfr.15.1405062

    • NAID

      130007896414

    • ISSN
      1880-6821
    • Year and Date
      2020-08-19
    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Analysis of Hydrocarbons in the Exhaust Gas of a Fusion Test Device Using Infrared Absorption Spectroscopy2020

    • Author(s)
      Masahiro TANAKA, Hiromi KATO and Naoyuki SUZUKI
    • Journal Title

      Plasma and Fusion Research

      Volume: 15 Issue: 0 Pages: 2405008-2405008

    • DOI

      10.1585/pfr.15.2405008

    • NAID

      130007840503

    • ISSN
      1880-6821
    • Year and Date
      2020-04-14
    • Related Report
      2019 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Initial operation results of exhaust detritiation system using a polymer membrane2020

    • Author(s)
      Tanaka Masahiro、Suzuki Naoyuki、Kato Hiromi、Yokosawa Minoru
    • Journal Title

      Fusion Engineering and Design

      Volume: 160 Pages: 111980-111980

    • DOI

      10.1016/j.fusengdes.2020.111980

    • NAID

      120007126865

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Exhaust behavior of tritium from the large helical device in the first deuterium plasma experiment2020

    • Author(s)
      Tanaka Masahiro、Suzuki Naoyuki、Kato Hiromi
    • Journal Title

      Journal of Nuclear Science and Technology

      Volume: 57 Issue: 12 Pages: 1297-1306

    • DOI

      10.1080/00223131.2020.1782282

    • NAID

      120007089661

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Monitoring and Recovery of Tritium in Fusion Test Facility2020

    • Author(s)
      M. Tanaka, N. Suzuki, H. Kato, C. Iwata, N. Akata, H. Hayashi, and H. Miyake
    • Journal Title

      Fusion Science and Technology

      Volume: - Issue: 4 Pages: 475-480

    • DOI

      10.1080/15361055.2020.1718840

    • NAID

      120007126861

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Determination of tritium activity and chemical forms in the exhaust gas from a large fusion test device2018

    • Author(s)
      Tanaka Masahiro、Kato Hiromi、Suzuki Naoyuki、Iwata Chie、Akata Naofumi
    • Journal Title

      Journal of Radioanalytical and Nuclear Chemistry

      Volume: 318 Issue: 2 Pages: 877-885

    • DOI

      10.1007/s10967-018-6075-y

    • NAID

      120007089670

    • Related Report
      2018 Research-status Report
    • Peer Reviewed
  • [Journal Article] Control of dehumidification using polymer permeable membrane and its application to tritium removal system design2018

    • Author(s)
      Tanaka Masahiro
    • Journal Title

      Fusion Engineering and Design

      Volume: 136 Pages: 141-145

    • DOI

      10.1016/j.fusengdes.2018.01.031

    • NAID

      120007089669

    • Related Report
      2018 Research-status Report 2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Design and commissioning of the exhaust detritiation system for the Large Helical Device2018

    • Author(s)
      Tanaka Masahiro、Suzuki Naoyuki、Kato Hiromi、Kondo Tomoki、Yokosawa Minoru、Kawamata Tomonori、Ikeda Mitsuru、Meguro Tsuyoshi、Tanaka Tomonari、Sonoi Kazuro
    • Journal Title

      Fusion Engineering and Design

      Volume: 127 Pages: 275-283

    • DOI

      10.1016/j.fusengdes.2017.12.034

    • NAID

      120007126866

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Presentation] Performance of exhaust detritiation system for a fusion test device in the initial phase of the deuterium plasma experiment2020

    • Author(s)
      Masahiro Tanaka, Naoyuki Suzuki, Hiromi Kato, Hiroki Chimura
    • Organizer
      31st Symposium on Fusion Technology
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Estimation of tritium inventory in exhaust detritiation system for fusion test device in the initial tritium recovery operation2020

    • Author(s)
      Masahiro Tanaka, Naoyuki Suzuki, Hiromi Kato, Hiroki Chimura
    • Organizer
      3rd Asia Pacific Symposium on Tritium Science
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Detection of ammonia and deuterated hydrocarbons in the exhaust gas during wall conditioning operation by infrared absorption spectroscopy2020

    • Author(s)
      Masahiro Tanaka, Hiromi Kato, Naoyuki Suzuki, Hiroki Chimura
    • Organizer
      The 29th International Toki Conference on Plasma and Fusion Research
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 赤外吸収分光法による核融合試験装置の排気ガス組成分析の試み2019

    • Author(s)
      田中 将裕,加藤 ひろみ,鈴木 直之
    • Organizer
      日本原子力学会 秋の大会
    • Related Report
      2019 Research-status Report
  • [Presentation] LHD重水素実験における水素同位体挙動と物質収支2019

    • Author(s)
      田中将裕、加藤ひろみ、鈴木直之、増﨑 貴、矢嶋美幸、中田実希、岩田智恵
    • Organizer
      プラズマ・核融合学会 年会
    • Related Report
      2019 Research-status Report
    • Invited
  • [Presentation] Monitoring and Recovery of Tritium in Fusion Test Facility2019

    • Author(s)
      M. Tanaka, N. Suzuki, H. Kato, C. Iwata, N. Akata, H. Hayashi, and H. Miyake
    • Organizer
      12th International Conference on Tritium Science and Technology
    • Related Report
      2019 Research-status Report
  • [Presentation] Initial operation results of exhaust detritiation system using a polymer membrane2019

    • Author(s)
      M. Tanaka, N. Suzuki, H. Kato, M. Yokosawa
    • Organizer
      14th International Symposium on Fusion Nuclear Technology
    • Related Report
      2019 Research-status Report
  • [Presentation] Analysis of hydrocarbons in the exhaust gas of a fusion test device using infrared absorption spectroscopy2019

    • Author(s)
      M. Tanaka, H. Kato, N. Suzuki,
    • Organizer
      28th International Toki Conference
    • Related Report
      2019 Research-status Report
  • [Presentation] 大型核融合試験装置用排気ガス分析システムの構築と運用2018

    • Author(s)
      田中将裕 加藤ひろみ 鈴木直之
    • Organizer
      第12回核融合エネルギー連合講演会
    • Related Report
      2018 Research-status Report
  • [Presentation] 大型核融合試験施設におけるトリチウム管理機器の整備2018

    • Author(s)
      田中将裕
    • Organizer
      日本放射線安全管理学会 第17回 学術大会
    • Related Report
      2018 Research-status Report
  • [Presentation] Exhaust behavior and mass balance of tritium in Large Helical Device2018

    • Author(s)
      Masahiro Tanaka, Naoyuki Suzuki, Hiromi Kato
    • Organizer
      27th IAEA Fusion Energy Conference (FEC 2018)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Behavior and mass balance of tritium in the exhaust gas from LHD2018

    • Author(s)
      Masahiro Tanaka, Naoyuki Suzuki, Hiromi Kato
    • Organizer
      2nd LHD Deuterium Workshop
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Preliminary operation results of exhaust detritiation system for large fusion test device2017

    • Author(s)
      Masahiro Tanaka, Naoyuki Suzuki, Hiromi Kato
    • Organizer
      2nd Asia-Pacific Symposium on Tritium Science
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Control of dehumidification by the polymer permeable membrane and its application to a tritium removal system2017

    • Author(s)
      Masahiro Tanaka
    • Organizer
      13th International Symposium on Fusion Nuclear Technology
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research

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Published: 2017-04-28   Modified: 2022-01-27  

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