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Observation of quantum spin-nematic phase in a one-dimensional quantum antiferromagnet

Research Project

Project/Area Number 17K14344
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Condensed matter physics II
Research InstitutionTokyo University of Science

Principal Investigator

Fujihara Masayoshi  東京理科大学, 理学部第一部物理学科, 講師 (60722840)

Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥3,510,000 (Direct Cost: ¥2,700,000、Indirect Cost: ¥810,000)
Fiscal Year 2019: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2018: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2017: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Keywords量子スピン / スピン液体 / 低次元磁性体 / フラストレーション / 低温合成 / 量子磁性 / スピンネマティック / 中性子散乱 / μSR / 一次元量子スピン系 / DM相互作用 / 巨大単結晶 / 量子スピン液体 / 物性実験
Outline of Final Research Achievements

We study the spin dynamics in the one-dimensional quantum antiferromagnets, in order to observe a new type of spin liquid, so-called spin nematic state.
Several new low-dimensional quantum antiferromagnets were successfully synthesized: a model compound for investigation of DM-induced frustration effects in a 1D quantum spin system Na2CuSO4Cl2, edge-shared tetrahedral spin-cluster chain system K2Cu3O(SO4)3, and first compound of a square-kagome quantum antiferromagnet KCu6AlBiO4(SO4)5Cl.
Comprehensive experimental studies by magnetic susceptibility, magnetization, heat capacity, inelastic neutron scattering measurements and rigorous theoretical studies revealed the presence of an quantum spin state in these compound.

Academic Significance and Societal Importance of the Research Achievements

モデル物質の探索領域をある地域で産出された鉱物群に絞った結果、新規低次元磁性体を複数見出すことに成功した。その結果、低次元磁性体の効率的な探索の指針確立にまで至った。今後のこの系の研究の発展に大きく寄与しているといえる。

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (12 results)

All 2020 2019 2018 2017 Other

All Int'l Joint Research (2 results) Journal Article (2 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 2 results) Presentation (6 results) Remarks (2 results)

  • [Int'l Joint Research] ANSTO(オーストラリア)

    • Related Report
      2018 Research-status Report
  • [Int'l Joint Research] ANSTO(オーストラリア)

    • Related Report
      2017 Research-status Report
  • [Journal Article] Spin dynamics and magnetic ordering in the quasi-one-dimensional S= 1/2 antiferromagnet Na2CuSO4Cl22020

    • Author(s)
      M. Fujihala, S. Mitsuda, R. A. Mole, D. H. Yu, I. Watanabe, S. Yano, T. Kuwai, H. Sagayam a, T. Kouchi, H. Kamebuchi, M. Tadokoro
    • Journal Title

      Physical Review B

      Volume: 101 Issue: 2 Pages: 024410-024410

    • DOI

      10.1103/physrevb.101.024410

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Cluster-Based Haldane State in an Edge-Shared Tetrahedral Spin-Cluster Chain: Fedotovite K2Cu3O(SO4)32018

    • Author(s)
      Fujihala M.、Sugimoto T.、Tohyama T.、Mitsuda S.、Mole R.?A.、Yu D.?H.、Yano S.、Inagaki Y.、Morodomi H.、Kawae T.、Sagayama H.、Kumai R.、Murakami Y.、Tomiyasu K.、Matsuo A.、Kindo K.
    • Journal Title

      Physical Review Letters

      Volume: 120 Issue: 7 Pages: 77201-77201

    • DOI

      10.1103/physrevlett.120.077201

    • Related Report
      2018 Research-status Report 2017 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] 擬一次元反強磁性体Na2CuSO4Cl2の磁気構造と誘電特性2019

    • Author(s)
      佐久間 裕太, 藤原 理賀, 満田 節生, 佐藤 拓実, 中尾 朗子, 宗像 孝司,矢野 真一郎, R. Mole, 玉造 博夢, 佐賀山 基, 渡邊 功雄
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 一次元量子磁性体Na2CuSO4Cl2の構造・磁気相転移2019

    • Author(s)
      藤原理賀, 佐久間裕太, 満田節生, 矢野真一郎, R. Mole, 渡邊功雄
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2019 Annual Research Report 2018 Research-status Report
  • [Presentation] 正方カゴメ格子反強磁性体Cu6AlBiO4(SO4)5・KClの27Al-NMR2019

    • Author(s)
      後藤貴行, 藤原理賀, 植野航, 満田節生
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2019 Annual Research Report 2018 Research-status Report
  • [Presentation] 正方カゴメ格子反強磁性体Cu6AlBiO4(SO4)5・KCl におけるスピン液体の可能2018

    • Author(s)
      藤原理賀, 森田克洋, 満田節生, 遠山貴巳, 桑井智彦, 岡部博孝, 幸田章宏, R. Mole, 矢野真一郎
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Research-status Report
  • [Presentation] 正方カゴメ格子反強磁性体Cu6AlBiO4(SO4)5・KClの磁気解析2018

    • Author(s)
      森田克洋, 藤原理賀, 満田節生, 松尾晶, 金道浩一, 曽田繁利, 遠山貴巳
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Research-status Report
  • [Presentation] J1-J2-J3正方カゴメ量子スピン磁性体の合成、構造、磁性2017

    • Author(s)
      藤原理賀, 森田克洋, 満田節生, 遠山貴巳, 桑井智彦
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Research-status Report
  • [Remarks] 量子コンピュータの新たな設計指針 ~カムチャッカ半島産の鉱物の中に量子ビットを発見~

    • URL

      http://www.tus.ac.jp/today/20180214100.pdf

    • Related Report
      2017 Research-status Report
  • [Remarks] ANSTO News

    • URL

      http://www.ansto.gov.au/AboutANSTO/MediaCentre/News/ACS177353

    • Related Report
      2017 Research-status Report

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Published: 2017-04-28   Modified: 2021-02-19  

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