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Study of development process of vacancy-type defects in rare-gas-plasma-induced metal-nanostructure formation process

Research Project

Project/Area Number 17K14896
Research Category

Grant-in-Aid for Young Scientists (B)

Allocation TypeMulti-year Fund
Research Field Nuclear fusion studies
Research InstitutionKyoto University

Principal Investigator

YABUUCHI ATSUSHI  京都大学, 複合原子力科学研究所, 助教 (90551367)

Project Period (FY) 2017-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2019: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2018: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2017: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Keywordsタングステン / 原子空孔 / 空孔-不純物複合体 / 照射損傷 / 陽電子消滅 / 第一原理計算 / 陽電子消滅分光法 / 陽電子寿命 / 結合エネルギー / 陽電子消滅ガンマ線ドップラー広がり / 格子欠陥 / 照射誘起欠陥 / 核融合 / プラズマ・壁相互作用 / 金属物性 / ナノ構造金属 / 希ガスプラズマ
Outline of Final Research Achievements

Vacancy-type defects formed by electron- or rare-gas-ion-irradiation and the differences in their development behaviors during the post-irradiation annealing process were investigated using positron annihilation spectroscopy. A comparison between helium- and neon-ion irradiated tungsten implied that the defect species are the same in both as-irradiated samples. However, in the case of neon-irradiated tungsten, in contrast to helium-ion irradiated one, the aggregation of vacancies and the formation of vacancy clusters were observed. Vacancy-hydrogen complexes were observed in tungsten irradiated with electrons in water, and the complexes began to dissociate from 623 K and formed vacancy clusters. In addition, when the sample purity was low, the formation of vacancy clusters was suppressed during the annealing process compared to the high-purity sample.

Academic Significance and Societal Importance of the Research Achievements

核融合炉ではプラズマ冷却ガスとしてNeガスの導入が検討されているが,このようなHやHeよりも重いイオンの導入はプラズマ対向壁であるタングステンに,より重大な損傷を与える可能性が示された.一方で,原子空孔と大きな結合エネルギー持つ元素を意図的に添加することで,空孔集合体の形成を抑制し得る可能性も示された.

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (47 results)

All 2020 2019 2018 2017

All Journal Article (8 results) (of which Peer Reviewed: 8 results,  Open Access: 8 results) Presentation (39 results) (of which Int'l Joint Research: 16 results,  Invited: 3 results)

  • [Journal Article] Contribution of cadmium to the total amount of positron creation in a reactor-based slow positron beamline2020

    • Author(s)
      Yabuuchi A.、Yoshiie T.、Kinomura A.
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

      Volume: 463 Pages: 40-49

    • DOI

      10.1016/j.nimb.2019.11.028

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Significant growth of vacancy-type defects by post-irradiation annealing in neon ion-irradiated tungsten probed by a slow positron beam2020

    • Author(s)
      Yabuuchi A.、Tanaka M.、Kinomura A.
    • Journal Title

      Journal of Nuclear Materials

      Volume: 531 Pages: 152018-152018

    • DOI

      10.1016/j.jnucmat.2020.152018

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Measurement of Defect-induced Electrical Resistivity Change of Tungsten Wire at Cryogenic Temperature Using High-energy Proton Irradiation2020

    • Author(s)
      Iwamoto Yosuke、Yoshida Makoto、Matsuda Hiroki、Meigo Shin-ichiro、Satoh Daiki、Yashima Hiroshi、Yabuuchi Atsushi、Kinomura Atsushi、Shima Tatsushi
    • Journal Title

      JPS Conf. Proc.

      Volume: 28 Pages: 1-5

    • DOI

      10.7566/jpscp.28.061003

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Slow-positron beamline temperature rise reduction at Kyoto University Research Reactor2019

    • Author(s)
      Yabuuchi A.、Naka R.、Sato K.、Xu Q.、Kinomura A.
    • Journal Title

      Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

      Volume: 461 Pages: 137-141

    • DOI

      10.1016/j.nimb.2019.09.036

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Magnetic Doppler broadening measurement on Gadolinium-doped GaN2019

    • Author(s)
      Maekawa M.、Sakai S.、Hagiwara S.、Miyashita A.、Wada K.、Kawasuso A.、Yabuuchi A.、Hasegawa S.
    • Journal Title

      AIP Conference Proceedings

      Volume: 2182 Pages: 050007-050007

    • DOI

      10.1063/1.5135850

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Irradiation-induced vacancy defects and its recovery behavior in 5N-purity tungsten and 3N-purity tantalum2019

    • Author(s)
      Tanaka M.、Yabuuchi A.、Kinomura A.
    • Journal Title

      AIP Conf. Proc.

      Volume: 2182 Pages: 1-4

    • DOI

      10.1063/1.5135857

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] High-temperature in-situ measurements of thermal vacancies in a TiAl intermetallic compound using a desktop positron beam2018

    • Author(s)
      A. Yabuuchi, S. Sakai, M. Mizuno, H. Araki, Y. Shirai
    • Journal Title

      JJAP Conf. Proc.

      Volume: 7 Pages: 011102-011102

    • DOI

      10.7567/jjapcp.7.011102

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Design of an Acceleration Gap for Brightness Enhancement in a Reactor-Based Slow Positron Beamline2017

    • Author(s)
      Y. Kuzuya, N. Oshima, A. Kinomura, and A. Yabuuchi
    • Journal Title

      Acta Phys. Pol. A

      Volume: 132 Pages: 1620-1623

    • Related Report
      2017 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] 電子線照射でタングステンに形成される欠陥の陽電子寿命法による評価2019

    • Author(s)
      薮内敦,田中美穂,木野村淳
    • Organizer
      第56回アイソトープ・放射線研究発表会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 陽電子寿命分光法による電子線照射タングステンの空孔回復挙動の評価2019

    • Author(s)
      薮内敦,田中美穂,木野村淳
    • Organizer
      日本金属学会2019年秋期(第165回)講演大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Estimation of the effect of positron production amount by installing Cd-cap in the KUR slow positron beamline2019

    • Author(s)
      A. Yabuuchi, T. Yoshiie, and A. Kinomura
    • Organizer
      15th International Workshop on Slow Positron Beam Techniques & Applications (SLOPOS-15)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Monte Carlo simulation of positron creation and heat generation at the KUR reactor-based slow positron beamline2019

    • Author(s)
      A. Yabuuchi, T. Yoshiie, and A. Kinomura
    • Organizer
      4th Japan-China Joint Workshop on Positron Science (JWPS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] KUR低速陽電子ビームラインにおける陽電子生成シミュレーション2019

    • Author(s)
      薮内敦,義家敏正,木野村淳
    • Organizer
      令和元年度京都大学複合原子力科学研究所専門研究会「陽電子科学とその理工学への応用」
    • Related Report
      2019 Annual Research Report
  • [Presentation] イオンビーム合成β-FeSi2におけるAlドープがもたらすFe空孔形成2019

    • Author(s)
      薮内敦,唐津拓弥,木野村淳,前川雅樹,河裾厚男
    • Organizer
      QST高崎サイエンスフェスタ2019
    • Related Report
      2019 Annual Research Report
  • [Presentation] 陽電子消滅寿命法による光照射した化合物半導体ZnOの欠陥状態変化観測2019

    • Author(s)
      中島諒,木野村淳,薮内敦,栗山一男
    • Organizer
      第56回アイソトープ・放射線研究発表会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Improvement of positron lifetime measurement systems for the KUR slow positron beamline2019

    • Author(s)
      M. Nakajima, R. Taguchi, Y. Kuzuya, A. Yabuuchi and A. Kinomura
    • Organizer
      15th International Workshop on Slow Positron Beam Techniques & Applications (SLOPOS-15)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Ge(110)表面への低エネルギーArイオン照射効果と陽電子消滅を用いた表面構造の研究2019

    • Author(s)
      塚元隆太,一宮正義,薮内敦,高宮幸一,木野村淳,柳沢淳一
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Progress of the slow-positron beamline development at the Kyoto University research reactor2019

    • Author(s)
      A. Kinomura, A. Yabuuchi, K. Sato, and Q. Xu
    • Organizer
      4th Japan-China Joint Workshop on Positron Science (JWPS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Investigation of defect states in light-irradiated single crystal ZnO by low-temperature positron annihilation lifetime spectroscopy2019

    • Author(s)
      M. Nakajima, A. Kinomura, A. Yabuuchi, and K. Kuriyama
    • Organizer
      4th Japan-China Joint Workshop on Positron Science (JWPS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Annealing behavior of vacancy-type defects I rare-earth implanted GaN studied by a slow positron beam2019

    • Author(s)
      T. Karatsu, A. Yabuuchi, and A. Yabuuchi
    • Organizer
      4th Japan-China Joint Workshop on Positron Science (JWPS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Characterization of Diamond-Like Carbon Films by Slow-Positron and MeV Ion Beams to Investigate the Origin of Water Wettability2019

    • Author(s)
      A. Kinomura, S. Nakao, K. Suzuki, T. Sonoda, Y. Kuzuya, M. Nakajima, K. Ikeda, A. Yabuuchi, and K. Yasuda
    • Organizer
      23rd International Workshop on Inelastic Ion-Surface Collisions (IISC-23)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 高エントロピー合金CoCrFeMnNi中の原子空孔挙動2019

    • Author(s)
      松岡直希,小川竜生,杉田一樹,水野正隆,薮内敦,木野村淳,荒木秀樹
    • Organizer
      令和元年度京都大学複合原子力科学研究所専門研究会「陽電子科学とその理工学への応用」
    • Related Report
      2019 Annual Research Report
  • [Presentation] イオンビーム合成法で作製したβ-FeSi2 膜中の空孔型欠陥評価2019

    • Author(s)
      薮内敦,唐津拓弥,木野村淳,前川雅樹,河裾厚男
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Research-status Report
  • [Presentation] Vacancy-type defects study in metals by using a positron beam2018

    • Author(s)
      A. Yabuuchi
    • Organizer
      3rd Kyoto Workshop on Positron Sciences (KWPS2018)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Development Status of the KUR Reactor-Based Slow Positron Beamline: Evaluation of Positron Source Temperature and Beam Intensity2018

    • Author(s)
      A. Yabuuchi, R. Naka, T. Yoshiie, Y. Kuzuya, R. Taguchi, A. Kinomura
    • Organizer
      18th International Conference on Positron Annihilation (ICPA-18)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Irradiation-Induced Vacancy Defects and Its Recovery Behavior in High-Purity Tungsten2018

    • Author(s)
      M. Tanaka, A. Yabuuchi, A. Kinomura
    • Organizer
      18th International Conference on Positron Annihilation (ICPA-18)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Current status and prospect of the reactor-based slow positron beamline at Kyoto University2018

    • Author(s)
      A. Kinomura, A. Yabuuchi, K. Sato, Q. Xu
    • Organizer
      18th International Conference on Positron Annihilation (ICPA-18)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Performance of brightness enhancement system for the KUR slow positron beamline2018

    • Author(s)
      Y. Kuzuya, N. Oshima, A. Kinomura, A. Yabuuchi
    • Organizer
      18th International Conference on Positron Annihilation (ICPA-18)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Magnetic Doppler Broadening Measurement on Gadolinium-doped GaN2018

    • Author(s)
      M. Maekawa, S. Sakai, K. Wada, A. Miyashita, S. Hagiwara, A. Kawasuso, A. Yabuuchi, S. Hasegawa
    • Organizer
      18th International Conference on Positron Annihilation (ICPA-18)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] KUR低速陽電子ビームラインの開発状況:線源部温度とビーム強度に関する考察2018

    • Author(s)
      薮内敦,仲竜太朗,義家敏正,葛谷佳広,田口遼,木野村淳
    • Organizer
      第55回アイソトープ・放射線研究発表会
    • Related Report
      2018 Research-status Report
  • [Presentation] スピン偏極陽電子ビームを用いたガドリニウム添加窒化ガリウム薄膜の空孔誘起磁性検出2018

    • Author(s)
      前川雅樹,境誠司,萩原聡,和田健,宮下敦己,河裾厚男,薮内敦,長谷川繁彦
    • Organizer
      日本物理学会第73回秋季大会
    • Related Report
      2018 Research-status Report
  • [Presentation] KUR低速陽電子ビームライン測定系のパラメータ最適化2018

    • Author(s)
      田口遼,葛谷佳広,中島諒,薮内敦,木野村淳
    • Organizer
      日本物理学会第73回秋季大会
    • Related Report
      2018 Research-status Report
  • [Presentation] イオンビームを用いたβ-FeSi2薄膜の合成とその空孔型欠陥評価2018

    • Author(s)
      薮内敦,木野村淳,前川雅樹,河裾厚男
    • Organizer
      QST 高崎サイエンスフェスタ2018
    • Related Report
      2018 Research-status Report
  • [Presentation] 高純度タングステンにおける電子線照射誘起空孔の回復挙動2018

    • Author(s)
      田中美穂,薮内敦,木野村淳
    • Organizer
      平成30年度京都大学複合原子力科学研究所専門研究会「陽電子科学とその理工学への応用」
    • Related Report
      2018 Research-status Report
  • [Presentation] KUR低速陽電子ビームラインのパルス化電極に関する考察2018

    • Author(s)
      田口遼,葛谷佳広,中島諒,薮内敦,木野村淳
    • Organizer
      平成30年度京都大学複合原子力科学研究所専門研究会「陽電子科学とその理工学への応用」
    • Related Report
      2018 Research-status Report
  • [Presentation] 電子線照射したSUS430ステンレス鋼の水素トラップ挙動2018

    • Author(s)
      来山雄太,杉田一樹,水野正隆,荒木秀樹,薮内敦,木野村淳
    • Organizer
      平成30年度京都大学複合原子力科学研究所専門研究会「陽電子科学とその理工学への応用」
    • Related Report
      2018 Research-status Report
  • [Presentation] KUR陽電子ビームラインのビーム強度に対する線源部の影響評価2018

    • Author(s)
      薮内敦,仲竜太朗,義家敏正,葛谷佳広,田口遼,木野村淳
    • Organizer
      日本物理学会第73回年次大会
    • Related Report
      2017 Research-status Report
  • [Presentation] イオンビーム合成法で作製したβ-FeSi2膜の低速陽電子ビームによる評価2018

    • Author(s)
      薮内敦,木野村淳,前川雅樹,河裾厚男
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2017 Research-status Report
  • [Presentation] 京大原子炉低速陽電子ビームライン輝度増強システムの開発の現状報告(3)2018

    • Author(s)
      葛谷佳広,大島永康,木野村淳,薮内敦
    • Organizer
      日本物理学会第73回年次大会
    • Related Report
      2017 Research-status Report
  • [Presentation] High-temperature in-situ measurements of thermal vacancies in a TiAl intermetallic compound using a desktop positron beam2017

    • Author(s)
      A. Yabuuchi, S. Sakai, M. Mizuno, H. Araki, and Y. Shirai
    • Organizer
      3rd China-Japan Joint Workshop on Positron Science (JWPS2017)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] The estimation of positron production and heat generation in KUR beam line by PHITS2017

    • Author(s)
      A. Yabuuchi, T. Yoshiie, Y. Kuzuya, Y. Iwamoto, T. Sano, and A. Kinomura
    • Organizer
      International Workshop on Positron Studies of Defects 2017 (PSD-17)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] KUR低速陽電子ビームラインパルス化装置の特性解析2017

    • Author(s)
      薮内敦,木野村淳,B.E. O'Rourke
    • Organizer
      第54回アイソトープ・放射線研究発表会
    • Related Report
      2017 Research-status Report
  • [Presentation] 高融点金属中の格子欠陥除去の陽電子寿命法による評価2017

    • Author(s)
      薮内敦,木野村淳
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Research-status Report
  • [Presentation] Study of Ion-Beam-Synthesized β-FeSi2 Films Probed by a Slow Positron Beam2017

    • Author(s)
      A. Yabuuchi, A. Kinomura, M. Maekawa, and A. Kawasuso
    • Organizer
      International Workshop on Positron Studies of Defects 2017 (PSD-17)
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] 京大原子炉低速陽電子ビームラインの輝度増強システムの開発の現状報告(Ⅱ)2017

    • Author(s)
      葛谷佳広,大島永康,木野村淳,薮内敦,鈴木良一,松本哲郎
    • Organizer
      日本物理学会2017年秋季大会
    • Related Report
      2017 Research-status Report
  • [Presentation] KUR陽電子ビームラインの線源部温度とビーム強度の評価2017

    • Author(s)
      仲竜太朗,木野村淳,薮内敦
    • Organizer
      平成29年度京都大学原子炉実験所専門研究会
    • Related Report
      2017 Research-status Report
  • [Presentation] KUR低速陽電子ビームライン高輝度化装置の開発状況とリモデレータ処理2017

    • Author(s)
      葛谷佳広,大島永康,木野村淳,薮内敦
    • Organizer
      第54回アイソトープ・放射線研究発表会
    • Related Report
      2017 Research-status Report

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Published: 2017-04-28   Modified: 2021-02-19  

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