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In situ viscosity measurement of silicate melts under high pressure by X-ray photon correlation spectroscopy

Research Project

Project/Area Number 17K18813
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Research Field Earth and planetary science and related fields
Research InstitutionHigh Energy Accelerator Research Organization

Principal Investigator

FUNAMORI NOBUMASA  大学共同利用機関法人高エネルギー加速器研究機構, 物質構造科学研究所, 教授 (70306851)

Project Period (FY) 2017-06-30 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥6,370,000 (Direct Cost: ¥4,900,000、Indirect Cost: ¥1,470,000)
Fiscal Year 2019: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Fiscal Year 2018: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2017: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
KeywordsSiO2ガラス / 水ガラス / 非晶質 / 相転移カイネティクス / 静的圧縮 / 動的圧縮 / 相転移カイネティクスモデル / 粘性測定 / 小角X線散乱測定 / X線光子相関分光法 / 含水SiO2ガラス / 相転移ダイナミクスモデル / ケイ酸塩メルト / 小角X線散乱 / コヒーレントX線 / 超高圧 / マグマ / 粘性
Outline of Final Research Achievements

In this study, we obtained the following results on the dynamics of the water-silicate system.
For water glasses (Na2O-SiO2-H2O system), the origin of the characteristic low-Q diffraction peak, which is the key to understanding their structure, is the Na-Na correlation in Na2O-rich clusters. Upon pressurization up to several tens of thousands of atmospheres, the structure of water glasses becomes homogeneous and the peak disappears. A model is proposed for the phase transition kinetics of amorphous materials, formulated in terms of energy levels and activation energy ranges, which successfully reproduces various experimental data on the phenomenon of permanent densification of SiO2 glass.

Academic Significance and Societal Importance of the Research Achievements

マグマの振る舞いを理解する上で、水-ケイ酸塩系の混和-不混和の相転移は重要である。水ガラスに関する研究成果は、この相転移の際の構造変化に関する直接的な情報を与えるものである。また、マグマの振る舞いを理解する上で、液体の相転移ダイナミクスは重要である。非晶質の相転移カイネティクスに関する研究成果は、ガラスを対象としており、液体の相転移カイネティクスのモデルの検討に繋がるものである。

Report

(6 results)
  • 2021 Annual Research Report   Final Research Report ( PDF )
  • 2020 Research-status Report
  • 2019 Research-status Report
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (47 results)

All 2022 2021 2020 2019 2018 2017

All Journal Article (16 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 13 results,  Open Access: 5 results) Presentation (31 results) (of which Int'l Joint Research: 3 results,  Invited: 3 results)

  • [Journal Article] Conceptual design of the Hybrid Ring with superconducting linac2022

    • Author(s)
      Harada Kentaro、Funamori Nobumasa、Yamamoto Naoto、Shimosaki Yoshito、Shimada Miho、Miyajima Tsukasa、Umemori Kensei、Sakai Hiroshi、Nakamura Norio、Sakanaka Shogo、Kobayashi Yukinori、Honda Tohru、Nozawa Shunsuke、Nakao Hironori、Niwa Yasuhiro、Wakabayashi Daisuke、Amemiya Kenta、Igarashi Noriyuki
    • Journal Title

      Journal of Synchrotron Radiation

      Volume: 29 Issue: 1 Pages: 118-124

    • DOI

      10.1107/s1600577521012753

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Structure of sodium silicate water glass: X-ray scattering experiments and force-field molecular dynamics simulations2022

    • Author(s)
      Noritake Fumiya、Sato Tomoko、Yamamoto Akane、Wakabayashi Daisuke、Urakawa Satoru、Funamori Nobumasa
    • Journal Title

      Journal of Non-Crystalline Solids

      Volume: 579 Pages: 121370-121370

    • DOI

      10.1016/j.jnoncrysol.2021.121370

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] X-ray zooming microscopy with two Fresnel zone plates2022

    • Author(s)
      Wakabayashi Daisuke、Suzuki Yoshio、Shibazaki Yuki、Sugiyama Hiroshi、Hirano Keiichi、Nishimura Ryutaro、Hyodo Kazuyuki、Igarashi Noriyuki、Funamori Nobumasa
    • Journal Title

      Review of Scientific Instruments

      Volume: 93 Issue: 3 Pages: 033701-033701

    • DOI

      10.1063/5.0070720

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] X-ray zooming optics for analyzer-based multi-contrast computed tomography2022

    • Author(s)
      Hirano Keiichi、Sugiyama Hiroshi、Nishimura Ryutaro、Wakabayashi Daisuke、Suzuki Yoshio、Igarashi Noriyuki、Funamori Nobumasa
    • Journal Title

      Journal of Synchrotron Radiation

      Volume: 29 Issue: 3 Pages: 787-793

    • DOI

      10.1107/s1600577522001412

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Kinetic model for phase transformation of noncrystalline solids: Application to permanent densification of SiO2 glass2021

    • Author(s)
      Wakabayashi Daisuke、Funamori Nobumasa、Sato Tomoko
    • Journal Title

      Physical Review B

      Volume: 103 Issue: 14 Pages: 144104-144104

    • DOI

      10.1103/physrevb.103.144104

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] Effect of sulfur on sound velocity of liquid iron under Martian core conditions2020

    • Author(s)
      Nishida, K., Shibazaki, Y., Terasaki, H., Higo, Y., Suzuki, A., Funamori, N., and Hirose, H.
    • Journal Title

      Nature Communications

      Volume: 11 Issue: 1 Pages: 1954-1954

    • DOI

      10.1038/s41467-020-15755-2

    • Related Report
      2020 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] In situ observation of the phase transition behavior of shocked baddeleyite.2020

    • Author(s)
      Sota Takagi, Atsushi Kyono, Shunsuke Nozawa, Nobuaki Kawai, Koji Inukai, Ryo Fukaya, Nobumasa Funamori, Shin‐ichi Adachi, Kouhei Ichiyanagi
    • Journal Title

      Geophysical Research Letters

      Volume: 47 Issue: 17 Pages: 1-8

    • DOI

      10.1029/2020gl089592

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] X-ray and Neutron Study on the Structure of Hydrous SiO2 Glass up to 10 GPa2020

    • Author(s)
      Urakawa Satoru、Inoue Toru、Hattori Takanori、Sano-Furukawa Asami、Kohara Shinji、Wakabayashi Daisuke、Sato Tomoko、Funamori Nobumasa、Funakoshi Ken-ichi
    • Journal Title

      Minerals

      Volume: 10 Issue: 1 Pages: 84-84

    • DOI

      10.3390/min10010084

    • NAID

      120006839438

    • Related Report
      2019 Research-status Report
    • Peer Reviewed / Open Access
  • [Journal Article] Development of shock-dynamics study with synchrotron-based time-resolved X-ray diffraction using an Nd:glass laser system2020

    • Author(s)
      Takagi Sota、Ichiyanagi Kouhei、Kyono Atsushi、Nozawa Shunsuke、Kawai Nobuaki、Fukaya Ryo、Funamori Nobumasa、Adachi Shin-ichi
    • Journal Title

      Journal of Synchrotron Radiation

      Volume: 27 Issue: 2 Pages: 371-377

    • DOI

      10.1107/s1600577519016084

    • Related Report
      2019 Research-status Report
    • Peer Reviewed
  • [Journal Article] Coexistence of two states in optically homogeneous silica glass during the transformation in short-range order2018

    • Author(s)
      Sato Tomoko、Funamori Nobumasa、Wakabayashi Daisuke、Nishida Keisuke、Kikegawa Takumi
    • Journal Title

      Physical Review B

      Volume: 98 Issue: 14

    • DOI

      10.1103/physrevb.98.144111

    • Related Report
      2018 Research-status Report
    • Peer Reviewed
  • [Journal Article] High-pressure in-situ XAFS-XRD measurements of liquid iodine with MAX802018

    • Author(s)
      D. Wakabayashi, N. Funamori, T. Kikegawa, K. Watanabe, S. Kohara, H. Nitani, Y. Niwa, Y. Takeichi, H. Abe, and M. Kimura
    • Journal Title

      Photon Factory Highlights 2017

      Volume: N/A Pages: 22-23

    • Related Report
      2018 Research-status Report
    • Open Access
  • [Journal Article] High-pressure glass formation of a series of 1-alkyl-3-methylimidazolium bis(trifluoromethanesulfonyl)imide homologues2018

    • Author(s)
      Yoshimura Yukihiro、Takekiyo Takahiro、Koyama Yoshihiro、Takaku Mayumi、Yamamura Misaho、Kikuchi Natsumi、Wakabayashi Daisuke、Funamori Nobumasa、Matsuishi Kiyoto、Abe Hiroshi、Hamaya Nozomu
    • Journal Title

      Physical Chemistry Chemical Physics

      Volume: 20 Issue: 1 Pages: 199-205

    • DOI

      10.1039/c7cp06594a

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Long Periodic Structure of a Room-Temperature Ionic Liquid by High-Pressure Small-Angle X-Ray Scattering and Wide-Angle X-Ray Scattering: 1-Decyl-3-Methylimidazolium Chloride2018

    • Author(s)
      Abe Hiroshi、Hamaya Nozomu、Koyama Yoshihiro、Kishimura Hiroaki、Takekiyo Takahiro、Yoshimura Yukihiro、Wakabayashi Daisuke、Funamori Nobumasa、Matsuishi Kiyoto
    • Journal Title

      ChemPhysChem

      Volume: in press Issue: 12 Pages: 1441-1447

    • DOI

      10.1002/cphc.201701273

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] Nature of the transformation in liquid iodine at 4 GPa2017

    • Author(s)
      Wakabayashi Daisuke、Funamori Nobumasa、Kikegawa Takumi、Watanabe Kazuki、Kohara Shinji、Nitani Hiroaki、Niwa Yasuhiro、Takeichi Yasuo、Abe Hitoshi、Kimura Masao
    • Journal Title

      Physical Review B

      Volume: 96 Issue: 2

    • DOI

      10.1103/physrevb.96.024105

    • Related Report
      2017 Research-status Report
    • Peer Reviewed
  • [Journal Article] 放射光によるSiO2 ガラスの構造と物性の高圧下その場観察2017

    • Author(s)
      佐藤友子、船守展正
    • Journal Title

      セラミックス

      Volume: 52 Pages: 352-356

    • Related Report
      2017 Research-status Report
  • [Journal Article] Highly Accurate Sound Velocity Measurement in Liquid Fe-S System under High Pressure2017

    • Author(s)
      Keisuke Nishida、Akio Suzuki、Yuki Shibazaki、Daisuke Wakabayashi、Nobumasa Funamori
    • Journal Title

      High Pressure, Photon Factory Activity Report 2016 (Part A: Highlight and Facility Report #34)

      Volume: 34 Pages: 40-41

    • Related Report
      2017 Research-status Report
  • [Presentation] KEK-PFにおけるリモート実験2022

    • Author(s)
      船守展正、山田悠介
    • Organizer
      第35回日本放射光学会年会
    • Related Report
      2021 Annual Research Report
  • [Presentation] BL-20BにおけるChannel-cut型X線コンデンサ2022

    • Author(s)
      杉山弘、平野馨一、若林大佑、鈴木芳生、五十嵐教之、船守展正
    • Organizer
      第35回日本放射光学会年会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 2つのFZPを用いた結像型X線ズーミング顕微鏡2022

    • Author(s)
      若林大佑、鈴木芳生、柴崎裕樹、杉山弘、平野馨一、西村龍太郎、兵藤一行、五十嵐教之、船守展正
    • Organizer
      第35回日本放射光学会年会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 偏光特性を活用した核共鳴前方散乱法によるFe型化合物の軌道秩序とその揺らぎの観測2022

    • Author(s)
      小林寿夫、池田修吾、神田智弘、河智史朗、柴崎裕樹、岸本俊二、船守展正
    • Organizer
      2021年度量子ビームサイエンスフェスタ
    • Related Report
      2021 Annual Research Report
  • [Presentation] 3次元X線ズーミング顕微鏡の開発2022

    • Author(s)
      平野馨一、若林大佑、杉山弘、柴崎裕樹、西村龍太郎、鈴木芳生、五十嵐教之、船守展正
    • Organizer
      2021年度量子ビームサイエンスフェスタ
    • Related Report
      2021 Annual Research Report
  • [Presentation] Simplified x-ray zooming optics for analyzer-based multi-contrast imaging2022

    • Author(s)
      Keiichi Hirano, Hiroshi Sugiyama, Ryutaro Nishimura, Daisuke Wakabayashi, Yoshio Suzuki, Noriyuki Igarashi, Nobumasa Funamori
    • Organizer
      SRI2021
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] CuInS2ナノ粒子の粒子間隔と光学特性II2021

    • Author(s)
      丹羽正貴、大野圭太、林純一、葛谷俊博、関根ちひろ、武田圭生、濱中泰、若林大佑、佐藤友子、船守展正
    • Organizer
      第62回高圧討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 高空間分解能イメージングシステムの導入とPF AR-NE1Aの将来運用2021

    • Author(s)
      柴崎裕樹、船守展正
    • Organizer
      第62回高圧討論会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 地球内部における水ケイ酸塩流体の構造に関する研究 22020

    • Author(s)
      山本あかね、佐藤友子、船守展正、若林大佑、浦川啓、服部高典
    • Organizer
      第61回高圧討論会
    • Related Report
      2020 Research-status Report
  • [Presentation] 時分割 X 線回折による SiO2 ガラスの高密度化観察2020

    • Author(s)
      佐藤友子、船守展正、柴崎裕樹
    • Organizer
      第61回高圧討論会
    • Related Report
      2020 Research-status Report
  • [Presentation] 地球内部における水ケイ酸塩流体の構造に関する研究2019

    • Author(s)
      山本あかね、佐藤友子、船守展正、若林大佑、浦川啓
    • Organizer
      第60回高圧討論会
    • Related Report
      2019 Research-status Report
  • [Presentation] AgInS2ナノ粒子の高圧下発光特性と構造2019

    • Author(s)
      大野圭太、仲条一輝、林純一、葛谷俊博、関根ちひろ、武田圭生、濱中泰、若林大佑、佐藤友子、船守展正
    • Organizer
      第60回高圧討論会
    • Related Report
      2019 Research-status Report
  • [Presentation] CuInS2ナノ粒子の高圧下発光特性と構造2019

    • Author(s)
      仲条一輝、大野圭太、林純一、葛谷俊博、関根ちひろ、武田圭生、濱中泰、若林大佑、佐藤友子、船守展正
    • Organizer
      第60回高圧討論会
    • Related Report
      2019 Research-status Report
  • [Presentation] 3YTZPの静的・動的圧縮下での挙動のその場観察2019

    • Author(s)
      髙木壮大、一柳光平、川合伸明、深谷亮、野澤俊介、興野純、船守展正、足立伸一
    • Organizer
      第32回日本放射光学会年会・放射光科学合同シンポジウム
    • Related Report
      2018 Research-status Report
  • [Presentation] ナノ秒時間分解XRDを用いた衝撃下における正方晶安定化ジルコニアの変態強化過程のその場観察2019

    • Author(s)
      髙木壮大、一柳光平、川合伸明、深谷亮、野澤俊介、興野純、船守展正、足立伸一
    • Organizer
      2018年度量子ビームサイエンスフェスタ
    • Related Report
      2018 Research-status Report
  • [Presentation] 高圧下におけるシリカガラス2018

    • Author(s)
      佐藤友子、若林大佑、船守展正
    • Organizer
      第79回応用物理学会秋季学術講演会
    • Related Report
      2018 Research-status Report
    • Invited
  • [Presentation] High-pressure in-situ XAFS-XRD measurements with MAX80 at PF-AR NE5C2018

    • Author(s)
      D. Wakabayashi, N. Funamori, T. Kikegawa, K. Watanabe, S. Kohara, H. Nitani, Y. Niwa, Y. Takeichi, H. Abe, M. Kimura
    • Organizer
      SRI 2018
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Seamless structural transformations of SiO2 glass under high pressure2018

    • Author(s)
      D. Wakabayashi, T. Sato, and N. Funamori
    • Organizer
      ICG Annual Meeting 2018
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] イットリア添加正方晶ジルコニアの静的・動的圧縮下での挙動2018

    • Author(s)
      髙木壮大、一柳光平、川合伸明、野澤俊介、深谷亮、興野純、船守展正、足立伸一
    • Organizer
      第58回高圧討論会
    • Related Report
      2018 Research-status Report
  • [Presentation] PFにおける高圧下その場XAFS測定システムの開発2018

    • Author(s)
      若林大佑、渡邉一樹、亀卦川卓美、船守展正
    • Organizer
      第58回高圧討論会
    • Related Report
      2018 Research-status Report
  • [Presentation] 高圧下におけるSiO2ガラスの相転移カイネティクス2018

    • Author(s)
      若林大佑、船守展正、佐藤友子
    • Organizer
      第58回高圧討論会
    • Related Report
      2018 Research-status Report
  • [Presentation] 圧下における半導体ナノ粒子MInS2(M=Cu,Ag)の発光と構造2018

    • Author(s)
      武田圭生、澤口健文、仲条一輝、林純一、葛谷俊博、関根ちひろ、濱中泰、若林大佑、佐藤友子、船守展正
    • Organizer
      第58回高圧討論会
    • Related Report
      2018 Research-status Report
  • [Presentation] ルビジウムジャーマネートガラスの圧力誘起局所構造変化2018

    • Author(s)
      吉田桃太朗、大西佑輝、有馬寛、若林大佑、舟越賢一、船守展正、大高理
    • Organizer
      第58回高圧討論会
    • Related Report
      2018 Research-status Report
  • [Presentation] 衝撃実験から迫るAlCuFe準結晶鉱物の形成起源2018

    • Author(s)
      髙木壮大、一柳光平、深谷亮、野澤俊介、川合伸明、興野純、船守展正、足立伸一
    • Organizer
      2017年度量子ビームサイエンスフェスタ
    • Related Report
      2017 Research-status Report
  • [Presentation] 高強度レーザー誘起衝撃圧縮下における構造・反応ダイナミクス2018

    • Author(s)
      一柳光平、髙木壮大、川合伸明、野澤俊介、深谷亮、福本恵紀、若林大佑、興野純、中村一隆、船守展正、足立伸一
    • Organizer
      2017年度量子ビームサイエンスフェスタ
    • Related Report
      2017 Research-status Report
  • [Presentation] フォトンファクトリーにおける鉱物科学の将来展望2017

    • Author(s)
      若林大佑、亀卦川卓美、船守展正
    • Organizer
      日本鉱物科学会2017年会
    • Related Report
      2017 Research-status Report
    • Invited
  • [Presentation] SiO2ガラスの圧力誘起相転移の大規模分子動力学シミュレーション2017

    • Author(s)
      若林大佑、船守展正、下條冬樹
    • Organizer
      第58回高圧討論会
    • Related Report
      2017 Research-status Report
  • [Presentation] イミダゾリウム系イオン液体のlow-Qピークの圧力応答2017

    • Author(s)
      菊地なつみ、高久真由美、山村実早保、浜谷望、岸村浩明、阿部洋、若林大佑、船守展正、竹清貴浩、吉村幸浩
    • Organizer
      第58回高圧討論会
    • Related Report
      2017 Research-status Report
  • [Presentation] イオン液体の高圧誘起ハイブリッド層構造2017

    • Author(s)
      阿部洋、浜谷望、小山良尋、岸村浩明、竹清貴浩、吉村幸浩、若林大佑、船守展正、松石清人
    • Organizer
      第58回高圧討論会
    • Related Report
      2017 Research-status Report
  • [Presentation] 液体ヨウ素の圧力誘起構造変化:XAFS-XRDデータのRMC解析2017

    • Author(s)
      若林大佑、亀卦川卓美、渡邉一樹、小原真司、仁谷浩明、丹羽尉博、武市泰男、阿部仁、木村正雄、船守展正
    • Organizer
      第58回高圧討論会
    • Related Report
      2017 Research-status Report
  • [Presentation] 20GPaまでのFe-S系メルトの音速測定 II2017

    • Author(s)
      西田圭佑、柴崎裕樹、戸邉宙、寺崎英紀、肥後祐司、若林大佑、船守展正、鈴木昭夫
    • Organizer
      第58回高圧討論会
    • Related Report
      2017 Research-status Report

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Published: 2017-07-21   Modified: 2023-01-30  

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