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Challenging research on Earth and Planetary surface environment by in-situ high precision isotope analyses of fine-grained carbonate minerals

Research Project

Project/Area Number 17K18814
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Research Field Earth and planetary science and related fields
Research InstitutionJapan Agency for Marine-Earth Science and Technology

Principal Investigator

USHIKUBO Takayuki  国立研究開発法人海洋研究開発機構, 超先鋭研究開発部門(高知コア研究所), 技術研究員 (10722837)

Co-Investigator(Kenkyū-buntansha) 藤谷 渉  茨城大学, 理工学研究科(理学野), 助教 (20755615)
池原 実  高知大学, 教育研究部自然科学系理工学部門, 教授 (90335919)
Project Period (FY) 2017-06-30 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥5,980,000 (Direct Cost: ¥4,600,000、Indirect Cost: ¥1,380,000)
Fiscal Year 2018: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Fiscal Year 2017: ¥2,730,000 (Direct Cost: ¥2,100,000、Indirect Cost: ¥630,000)
Keywords二次イオン質量分析計 / SIMS / 炭酸塩 / 隕石 / 耳石 / クロマグロ / 有孔虫 / 同位体 / 酸素同位体 / 探査念
Outline of Final Research Achievements

We have established analytical techniques for in-situ carbon, oxygen, and sulfur isotopes with the ion microprobe, IMS 1280-HR of Kochi Institute, JAMSTEC. We applied these techniques for various geologic and meteoritic studies. We found that carbonates in Tagish Lake meteorite have extremely high d13C value in contrast with those of most carbonates in CM chondrites, indicating of accretion of CO2 ice into its parent body. By analyzing bluefin tuna otoliths, we could distinguish difference of seawater temperatures of spawning ocean areas. We also found that sulfur isotope ratios of pyrites in the seafloor hydrothermal deposit significantly changed by more than 20 permil according to growth of the deposit, indicating of change of supply sources of sulfur and growth mechanisms.

Academic Significance and Societal Importance of the Research Achievements

柔らかい炭酸塩や硫化鉱物を平滑に研磨できるようになり、微小試料の精密な元素・同位体比分析が可能となった。炭酸塩は耳石やプランクトン炭酸塩殻の様に生態や環境変動の記録を調べたり、熱水活動などの無機的な化学反応の変動を調べたりするなど、多様な研究に於いて有効な鉱物である。局所同位体比分析手法を確立し、かつクロマグロ耳石試料や隕石試料研究で成果を上げた事で、同手法が研究手法として実用的である事を証明した。

Report

(4 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Research-status Report
  • 2017 Research-status Report
  • Research Products

    (24 results)

All 2020 2019 2018 2017 Other

All Int'l Joint Research (5 results) Journal Article (3 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 3 results,  Open Access: 1 results) Presentation (16 results) (of which Int'l Joint Research: 9 results,  Invited: 1 results)

  • [Int'l Joint Research] Max Planck Institute for Chemistry(ドイツ)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Lund University(スウェーデン)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] University of Wisconsin-Madison(米国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] University of Glasgow(英国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] University of Wisconsin-Madison/University of Hawaii at Manoa(米国)

    • Related Report
      2018 Research-status Report
  • [Journal Article] Carbon isotopic evolution of aqueous fluids in CM chondrites: Clues from in-situ isotope analyses within calcite grains in Yamato-7911982020

    • Author(s)
      Fujiya Wataru、Aoki Yuto、Ushikubo Takayuki、Hashizume Ko、Yamaguchi Akira
    • Journal Title

      Geochimica et Cosmochimica Acta

      Volume: 274 Pages: 246-260

    • DOI

      10.1016/j.gca.2020.02.003

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Migration of D-type asteroids from the outer solar system inferred from carbonate in meteorites.2019

    • Author(s)
      Fujiya, W., Hoppe, P., Ushikubo, T., Fukuda, K., Lindgren, P., Lee, M. R., Koike, M., Shirai, K., and Sano, Y.
    • Journal Title

      Nature Astronomy

      Volume: 3 Issue: 10 Pages: 910-915

    • DOI

      10.1038/s41550-019-0801-4

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Beryllium-boron relative sensitivity factors for melilitic glasses measured with a NanoSIMS ion microprobe2018

    • Author(s)
      Fukuda Kohei、Fujiya Wataru、Hiyagon Hajime、Makino Yoshiki、Sugiura Naoji、Takahata Naoto、Hirata Takafumi、Sano Yuji
    • Journal Title

      GEOCHEMICAL JOURNAL

      Volume: 52 Issue: 3 Pages: 255-262

    • DOI

      10.2343/geochemj.2.0510

    • NAID

      130007379061

    • ISSN
      0016-7002, 1880-5973
    • Year and Date
      2018-05-30
    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Development for in-situ volatile element abundances, and hydrogen and sulfur 2-isotope analyses of silicate glasses by SIMS2019

    • Author(s)
      Takayuki Ushikubo, Kenji Shimizu
    • Organizer
      82nd Annual Meeting of the Meteoritical Society
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 無水鉱物の酸素同位体比から水の存在を探る2019

    • Author(s)
      牛久保 孝行
    • Organizer
      水惑星学全体会議
    • Related Report
      2019 Annual Research Report
  • [Presentation] 耳石酸素安定同位体比分析によるクロマグロの仔魚経験水温の推定2019

    • Author(s)
      木村 伸吾、羽根 由里奈、横山 裕典、牛久保 孝行、石村 豊穂、宮入 陽介、小川 展弘
    • Organizer
      2019年水産海洋学会研究発表大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] GEMSを産する微隕石と惑星間塵に含まれるコンドルールと何揮発性包有物について2019

    • Author(s)
      野口 高明、大橋 憲昭、ブラッドレー ジョン、中嶋 大輔、中村 智樹、木村 眞、牛久保 孝行、木多 紀子、今栄 直也
    • Organizer
      日本地球惑星科学連合2019年大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Yamato 791198 CMコンドライト中の 炭酸塩鉱物粒子内における酸素・炭素同位体比の不均一性と水質変成過程での同位体比の変化2019

    • Author(s)
      藤谷 渉、青木 佑斗、牛久保 孝行、橋爪 光
    • Organizer
      日本地球惑星科学連合2019年大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] タギッシュレイク隕石のコンドルールとアイソレートオリビン粒子の酸素同位体比分布2019

    • Author(s)
      牛久保 孝行、木村 眞
    • Organizer
      日本地球惑星科学連合2019年大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 小惑星の揮発性物質存在量2019

    • Author(s)
      藤谷 渉
    • Organizer
      2019年日本地球化学会年会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Oxygen isotope systematics of chondrules and isolated olivine grains from the Tagish Lake C2 chondrite.2019

    • Author(s)
      Ushikubo T., Kimura M.
    • Organizer
      50th Lunar and Planetary Science Conference
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Chondrule-like objects and a refractory inclusion in GEMS-bearing antarctic micrometeorites and Interplanetary dust particles.2019

    • Author(s)
      Noguchi T., Ohashi N., Bradley J. P., Nakashima D., Nakamura T., Kimura M., Ushikubo T., Kita N. T., Imae N.
    • Organizer
      50th Lunar and Planetary Science Conference
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Evolution of fluid composition inferred from calcite in the Yamato 791198 CM chondrite.2019

    • Author(s)
      Fujiya W., Aoki Y., Ushikubo T., Hashizume K.
    • Organizer
      50th Lunar and Planetary Science Conference
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] The application of SIMS d18O analysis for estimating spawning temperature of Pacific bluefin tuna using otolith.2018

    • Author(s)
      Hane Y., Kimura S., Yokoyama Y., Miyairi Y., Ushikubo T., Ogawa N.
    • Organizer
      6th International Otolith Symposium 2018
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Identifying natal origin of Pacific bluefin tuna using otolith oxygen isotopes measured by SIMS.2018

    • Author(s)
      Hane Y., Kimura S., Yokoyama Y., Miyairi Y., Ushikubo T., Ogawa N.
    • Organizer
      4th CLIOTOP symposium
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Effects of global warming on spawning behavior of the Pacific bluefin tuna based on otolith oxygen stable isotope analysis.2018

    • Author(s)
      Kimura S., Hane Y., Yokoyama Y., Miyairi Y., Ushikubo T., Ogawa N.
    • Organizer
      PICES-2018 Annual Meeting
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] In situ oxygen three-isotope analysis of carbonates with 15um and 3um beam: Preliminary results.2018

    • Author(s)
      Ushikubo T., Fujiya W.
    • Organizer
      Hayabusa 2018
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] SIMSによる局所同位体比分析の地球科学への応用2018

    • Author(s)
      牛久保 孝行
    • Organizer
      北陸古海洋勉強会
    • Related Report
      2017 Research-status Report
  • [Presentation] Development of methodology for analyses of larval ambient water temperature of Pacific bluefin tuna using SIMS2017

    • Author(s)
      Yulina Hane
    • Organizer
      PICES-2017 Annual Meeting
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research

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Published: 2017-07-21   Modified: 2021-02-19  

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