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Topological control of oxygen vacancy distribution in memristive materials for hypercomplex synaptic devices

Research Project

Project/Area Number 17K18881
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Research Field Electrical and electronic engineering and related fields
Research InstitutionOsaka University

Principal Investigator

Sakai Akira  大阪大学, 基礎工学研究科, 教授 (20314031)

Project Period (FY) 2017-06-30 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥6,500,000 (Direct Cost: ¥5,000,000、Indirect Cost: ¥1,500,000)
Fiscal Year 2018: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2017: ¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Keywordsシナプス素子 / メモリスタ / 酸素空孔分布 / トポロジー / 抵抗変化 / 電気着色現象 / 増強/抑圧特性 / ゲート効果 / 酸素空孔 / シナプス / ドリフト・拡散 / 有限要素法シミュレーション / 不可逆領域 / 走査透過電子顕微鏡 / 結晶場分裂 / 先端機能デバイス
Outline of Final Research Achievements

Resistive switching (RS) was demonstrated in four-terminal planar memristive devices fabricated on reduced TiO2 single crystal substrates. In the device, a pair of diagonally opposing electrode terminals (PADOET) is used to modify the topology of oxygen vacancy distribution in the region between another PADOET. The surface orientation of the substrate has a strong influence on the reversible RS phenomenon. Mechanisms behind the voltage-driven resistance change are elaborated for both crystalline and electronic structures in the electrically active zone of the device. Suppression of the irreversible conductive structure formation caused by accumulated oxygen vacancies is a key to establishing reversible RS in the device. Tuning protocols for the write and the gate voltage applications enables high precision control of resistance, or synaptic plasticity, paving the way for the manipulation of learning efficiency through neuromorphic devices.

Academic Significance and Societal Importance of the Research Achievements

メモリスタ結晶における酸素空孔分布トポロジーをダイナミックに制御し,素子のバルク的電気抵抗に結晶学的異方性を持たせることは,物性改質の根源的理解にも通じ,その原子・電子構造と素子特性の相関に関わる物理学的知見を獲得することに学術的意義がある.また,本研究で開発する多元シナプス素子を用いれば,深層学習に関わる従来のソフトウェア的機械学習をハードウェア的に高密度に実装できる.加えて,一素子への連合的多入力によって,一シナプスの重みを他のシナプスとの相関性をもって遷移させる高次脳機能が発現されるため,学習や連想機能を模倣する次世代脳型コンピュータの発展に繋がり,社会的にも意義深い.

Report

(3 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • Research Products

    (11 results)

All 2019 2018 2017

All Journal Article (2 results) (of which Peer Reviewed: 2 results,  Open Access: 1 results) Presentation (9 results) (of which Int'l Joint Research: 3 results)

  • [Journal Article] Demonstrative operation of four-terminal memristive devices fabricated on reduced TiO2 single crystals2019

    • Author(s)
      Takeuchi Shotaro、Shimizu Takuma、Isaka Tsuyoshi、Tohei Tetsuya、Ikarashi Nobuyuki、Sakai Akira
    • Journal Title

      Scientific Reports

      Volume: 9 Issue: 1

    • DOI

      10.1038/s41598-018-38347-z

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Analysis of Ti valence states in resistive switching regions of a rutile TiO2-x four-terminal memristive device2018

    • Author(s)
      Yamaguchi Kengo、Takeuchi Shotaro、Tohei Tetsuya、Ikarashi Nobuyuki、Sakai Akira
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 57 Issue: 6S3 Pages: 06KB02-06KB02

    • DOI

      10.7567/jjap.57.06kb02

    • NAID

      210000149225

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] ドナー密度分布制御型メモリスタ素子における抵抗変化機構の有限要素法シミュレーション2019

    • Author(s)
      永田善也,藤平哲也,酒井朗
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] TiO2-xエピタキシャル薄膜を用いた4端子メモリスタ素子の抵抗変化特性2019

    • Author(s)
      三宅亮太郎,藤平哲也,酒井朗
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Sakai A, Shimizu T, Shimotani M, Takeuchi S, Tohei T Demonstrative operation of four-terminal memristive devices by controlling oxygen vacancy distribution in TiO2-x single crystals2018

    • Author(s)
      Sakai A, Shimizu T, Shimotani M, Takeuchi S, Tohei T
    • Organizer
      2018 MRS Spring Meeting
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Gate-Tuning of Synaptic Function Based on the Oxygen Vacancy Distribution Control in Four-Terminal TiO2-x Memristive Devices2018

    • Author(s)
      Nagata Z, Shimizu T, Isaka T, Tohei T, Sakai A
    • Organizer
      International Conference on Solid State Devices and Materials 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] ゲート制御型4端子TiO2-xメモリスタによる可変シナプス機能の実装2018

    • Author(s)
      永田善也,清水琢磨,井坂健,藤平哲也,酒井朗
    • Organizer
      平成30年度応用物理学会第2回関西支部講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 酸素空孔分布制御型4 端子メモリスタ素子の抵抗変化特性精密制御2018

    • Author(s)
      清水拓磨,永田善也,竹内正太郎,藤平哲也,酒井朗
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2017 Research-status Report
  • [Presentation] 酸素空孔分布制御型4端子メモリスタ素子における抵抗変化機構の有限要素法シミュレーション2018

    • Author(s)
      永田善也,清水拓磨,竹内正太郎,藤平哲也,酒井朗
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2017 Research-status Report
  • [Presentation] Resistive switching characteristics of four-terminal TiO2-x single crystal memristive devices2017

    • Author(s)
      Shimizu Takuma, Takeuchi Shotaro, Tohei Tetsuya, Sakai Akira
    • Organizer
      2017 International Workshop on DIELECTRIC THIN FILMS FOR FUTURE ELECTRON DEVICES -SCIENCE AND TECHNOLOGY-
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] 4端子TiO2単結晶メモリスタの抵抗変化特性2017

    • Author(s)
      清水拓磨,竹内正太郎,藤平哲也,酒井朗
    • Organizer
      第78回応用物理学会秋季学術講演会
    • Related Report
      2017 Research-status Report

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Published: 2017-07-21   Modified: 2020-03-30  

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