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Challenge to analysis of biogenic volatile organic compounds based on measurement of ozone reactivity in forest air

Research Project

Project/Area Number 17K20048
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Research Field Environmental analyses and evaluation and related fields
Research InstitutionWaseda University

Principal Investigator

Matsumoto Jun  早稲田大学, 人間科学学術院, 教授 (70402394)

Co-Investigator(Kenkyū-buntansha) 加藤 俊吾  首都大学東京, 都市環境科学研究科, 准教授 (20381452)
Research Collaborator SOMMARIVA roberto  
PRAPLAN arnaud  
HONG zhengyi  
Project Period (FY) 2017-06-30 – 2019-03-31
Project Status Completed (Fiscal Year 2018)
Budget Amount *help
¥6,370,000 (Direct Cost: ¥4,900,000、Indirect Cost: ¥1,470,000)
Fiscal Year 2018: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Fiscal Year 2017: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Keywords大気化学反応 / 揮発性有機化合物 / 森林大気 / 反応性 / 温度依存 / オゾン / 光化学オキシダント / 包括計測 / 環境分析 / 大気汚染防止・浄化 / 自然現象観測・予測
Outline of Final Research Achievements

In this study, the original analyzer for measuring ozone reactivity, RO3, was improved and applied to field observations and analyses of RO3 of ambient air in a forest were conducted. It was found experimentally that the contribution of individually unmeasured VOCs like sesquiterpenes to RO3 was significant, especially in the summer daytime. It was also indicated that dependence analyses of RO3 on ambient temperature and light intensity could be useful for discussion on the situation of surrounding forests like tree species and BVOCs emission. Consequently, BVOCs analyses by RO3 measurements in ambient forest air were carried out successfully for the first time in the world. RO3 analyzer is a promising tool for studying BVOCs' behavior in the forest.

Academic Significance and Societal Importance of the Research Achievements

PM2.5や対流圏オゾンO3などの大気汚染問題において、人為発生源の効果的な対策には、自然発生源の把握が前提となる。揮発性有機化合物VOCsに関しては、樹木から放出される生物起源VOCs(BVOCs)が注目されるが、多様なVOCsの濃度と反応特性を個別成分分析により網羅するのは困難である。代表者はBVOCsがO3と反応しやすい点に注目し、オゾン反応性RO3としてBVOCsを包括測定する装置を構築してきた。本研究にてRO3計による森林大気観測とBVOCs挙動把握の試みに成功したことは、大気化学において学術的に有意義であるうえ、効果的な対策につながる第一歩として社会的にも期待される。

Report

(3 results)
  • 2018 Annual Research Report   Final Research Report ( PDF )
  • 2017 Research-status Report
  • Research Products

    (19 results)

All 2019 2018 2017 Other

All Int'l Joint Research (3 results) Journal Article (3 results) (of which Peer Reviewed: 3 results,  Open Access: 1 results) Presentation (11 results) (of which Int'l Joint Research: 4 results) Remarks (2 results)

  • [Int'l Joint Research] バーミンガム大学(英国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Finnish Meteorological Institute(フィンランド)

    • Related Report
      2017 Research-status Report
  • [Int'l Joint Research] University of Birmingham(英国)

    • Related Report
      2017 Research-status Report
  • [Journal Article] Ground-based observation of lightning-induced nitrogen oxides at a mountaintop in free troposphere2019

    • Author(s)
      WADA Ryuichi、SADANAGA Yasuhiro、KATO Shungo、KATSUMI Naoya、OKOCHI Hiroshi、IWAMOTO Yoko、MIURA Kazuhiko、KOBAYASHI Hiroshi、KAMOGAWA Masashi、MATSUMOTO Jun、YONEMURA Seiichiro、MATSUMI Yutaka、KAJINO Mizuo、HATAKEYAMA Shiro
    • Journal Title

      Journal of Atmospheric Chemistry

      Volume: in press

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Development of an Analytical Method for the Detection of NO<sub>z</sub> and Its Application to the Atmospheric Analysis at a Mountain Site2018

    • Author(s)
      和田龍一, 定永靖宗, 加藤俊吾, 勝見尚也, 大河内博, 岩本洋子, 三浦和彦, 小林拓, 鴨川仁, 松本淳, 米村正一郎, 松見豊, 梶野瑞王, 畠山史郎
    • Journal Title

      BUNSEKI KAGAKU

      Volume: 67 Issue: 6 Pages: 333-340

    • DOI

      10.2116/bunsekikagaku.67.333

    • NAID

      130007393929

    • ISSN
      0525-1931
    • Year and Date
      2018-06-05
    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Measurement of atmospheric total organic nitrates at a suburban site in Tokorozawa, Saitama, in summer2018

    • Author(s)
      松本 淳
    • Journal Title

      Journal of Japan Society for Atmospheric Environment / Taiki Kankyo Gakkaishi

      Volume: 53 Issue: 1 Pages: 1-12

    • DOI

      10.11298/taiki.53.1

    • NAID

      130006483369

    • ISSN
      1341-4178, 2185-4335
    • Related Report
      2018 Annual Research Report 2017 Research-status Report
    • Peer Reviewed
  • [Presentation] Applications of total ozone reactivity analyzer to a trial observation in the ambient air and to a further experiment on kinetics of terpene-ozone reactions2018

    • Author(s)
      J.Matsumoto and S.Kato
    • Organizer
      the 2018 joint 14th iCACGP Quadrennial Symposium and 15th IGAC Science Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Long term measurements of CO, O3, and VOCs at Moshiri, Hokkaido in northern Japan2018

    • Author(s)
      Shungo Kato, Hong Lam Hong Sandra, Yoshizumi Kajii, Masayuki Sera, Yutaka Matsumi
    • Organizer
      the 2018 joint 14th iCACGP Quadrennial Symposium and 15th IGAC Science Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 能登半島珠洲における粒子状有機硝酸エステル濃度の連続観測2018

    • Author(s)
      松本 淳, 定永 靖宗, 松木 篤
    • Organizer
      第59回大気環境学会年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 都市郊外にて観測されたオゾン反応性の温度依存性2018

    • Author(s)
      松本 淳
    • Organizer
      日本地球惑星科学連合2018年大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 都市郊外にて観測されたオゾン反応性の温度依存性2018

    • Author(s)
      松本淳
    • Organizer
      日本地球惑星科学連合2018年大会
    • Related Report
      2017 Research-status Report
  • [Presentation] Applications of total ozone reactivity analyzer to a trial observation in the ambient air and to a further experiment on kinetics of terpene-ozone reactions2018

    • Author(s)
      Jun Matsumoto, Shungo Kato
    • Organizer
      the 2018 joint 14th iCACGP Quadrennial Symposium and 15th IGAC Science Conference
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] Response of total ozone reactivity analyzer to mixture of gaseous isoprene and NO2017

    • Author(s)
      Jun Matsumoto, Roberto Sommariva
    • Organizer
      JpGU-AGU Joint Meeting 2017
    • Related Report
      2017 Research-status Report
    • Int'l Joint Research
  • [Presentation] 発生源排気 NO2/NOx 比の直接測定に基づく正確なポテンシャルオゾン評価の提案2017

    • Author(s)
      松本淳
    • Organizer
      第58回大気環境学会
    • Related Report
      2017 Research-status Report
  • [Presentation] 埼玉県所沢市における都市郊外大気の有機硝酸全量の連続観測2017

    • Author(s)
      松本淳、洪征翌
    • Organizer
      第58回大気環境学会
    • Related Report
      2017 Research-status Report
  • [Presentation] 所沢におけるPANsと有機硝酸の連続観測2017

    • Author(s)
      洪征翌、松本淳
    • Organizer
      第23回大気化学討論会
    • Related Report
      2017 Research-status Report
  • [Presentation] 所沢における実大気試料のオゾン反応性観測の試み2017

    • Author(s)
      松本淳
    • Organizer
      第23回大気化学討論会
    • Related Report
      2017 Research-status Report
  • [Remarks] 早稲田大学人間科学学術院 松本淳研究室

    • URL

      http://www.f.waseda.jp/jmatsumoto/index-j.html

    • Related Report
      2018 Annual Research Report
  • [Remarks] 早稲田大学人間科学学術院松本研究室

    • URL

      http://www.f.waseda.jp/jmatsumoto/index-j.html

    • Related Report
      2017 Research-status Report

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Published: 2017-07-21   Modified: 2020-03-30  

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