| Budget Amount *help |
¥16,600,000 (Direct Cost: ¥16,600,000)
Fiscal Year 2009: ¥3,200,000 (Direct Cost: ¥3,200,000)
Fiscal Year 2008: ¥3,400,000 (Direct Cost: ¥3,400,000)
Fiscal Year 2007: ¥7,500,000 (Direct Cost: ¥7,500,000)
Fiscal Year 2006: ¥2,500,000 (Direct Cost: ¥2,500,000)
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| Research Abstract |
We investigated the dynamics of molecules interacting with near-infrared intense laser pulses by using the time-dependent adiabatic state approach developed. The results for C60 indicate that the mode selectivity of vibrational excitation can be achieved by a pulse train, i.e., by changing the intervals between pulses. Time-dependent multiconfiguration theory is also developed to investigate the multielectron (ionization) dynamics of molecules. We have demonstrated that nuclear vibration is nonadiabatically coupled to the ring current of π electrons.
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