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Studies on Size Distribution and Mixing State of Black Carbon Aerosols in China

Research Project

Project/Area Number 18310007
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental dynamic analysis
Research InstitutionThe University of Tokyo

Principal Investigator

KOIKE Makoto  The University of Tokyo, Graduate School of Science, Associate Professor (00225343)

Co-Investigator(Kenkyū-buntansha) TAKEGAWA Nobuyki  The University of Tokyo, Research Center for Advanced Science and Technology, Associate Professor (00324369)
MIYAZAKI Yuzo  The University of Tokyo, Research Center for Advanced Science and Technology, Research Associate (60376655)
KITA Kazuyuki  Ibaraki University, Faculty of Science, Associate Professor (30221914)
Project Period (FY) 2006 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥16,880,000 (Direct Cost: ¥15,500,000、Indirect Cost: ¥1,380,000)
Fiscal Year 2007: ¥5,980,000 (Direct Cost: ¥4,600,000、Indirect Cost: ¥1,380,000)
Fiscal Year 2006: ¥10,900,000 (Direct Cost: ¥10,900,000)
Keywordsaerosol / black carbon / soot / China / Beijing / PRD / radiative forcing / climate change / 気候変動 / 気候影響
Research Abstract

Recent rapid growth of industrial activities in East Asia has been causing large increase in aerosols in this area. Atmospheric aerosols modify the radiation budget through scattering and absorption. Because black carbon (BC) aerosols (e.g., soot) efficiently absorb the solar radiation, they have been recognized one of the most important aerosol compounds the solar radiation, they have been recognized one of the mot important aerosol compounds for climate change.
In the physical year of 2006, measurements of BC mass concentrations, size distribution, and mixing sate were in the Beijing region and Peal River Delta (PRD) region in China with Peking University Research Groups and some other international research groups. Aerosol chemical composition and some other parameters were also simultaneously measured.
In the physical year of 2007, these data were precisely analyzed and interpreted from the viewpoint of emission sources, chemical production, transport processes, and removal processes using three-dimensional chemistry transport model. Observations show that BC concentrations in Beijing have a clear diurnal variation with a maximum during night. This feature was well reproduced by model calculations through diurnal variations, such as that in the boundary layer height. Although large day-to-day variations were found for secondary aerosols, such as inorganic aerosols, they were small for BC. Model calculations showed that BC concentrations were generally controlled by BC emissions within 100 km around Beijing within previous 24 hours. On the centrally, emissions as far as 500 km within previous 3 days were found to affect concentrations of secondary aerosols, such as sulfate through accumulations under stable synoptic-scale meteorological conditions.

Report

(3 results)
  • 2007 Annual Research Report   Final Research Report Summary
  • 2006 Annual Research Report
  • Research Products

    (35 results)

All 2007 2006

All Journal Article (25 results) (of which Peer Reviewed: 14 results) Presentation (10 results)

  • [Journal Article] Measurements of Reactive Nitrogen Produced by Tropical Thunderstorms during BIBLE-C2007

    • Author(s)
      M.Koike, 他
    • Journal Title

      J. Geophys. Res. 112

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Urban photochemistry in central Tokyo: 1. Observed and modeled OH and HO2 radical concentrations during the winter and summer of 20042007

    • Author(s)
      Y. Kanaya, M. Koike, 他
    • Journal Title

      J. Geophys. Res. 112

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Seasonal variation of atmospheric C2-C7 nonmethane hydrocarbons in Tokyo2007

    • Author(s)
      T. Shirai, M. Koike, 他
    • Journal Title

      J. Geophys. Res. 112

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Evolution of mixing state of black carbon particles: Aircraft measurements over the western Pacific in March 20042007

    • Author(s)
      N. Moteki, M. Koike, 他
    • Journal Title

      Geophys. Res. Lett 34

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Nitric acid condensation on ice: 2. Kinetic limitations, a possible 'cloud clock' for determining cloud parcel lifetime2007

    • Author(s)
      B. Gamblin, M. Koike, 他
    • Journal Title

      J. Geophys. Res 112

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Urban photochemistry in central Tokyo : 1. Observed and modeled OH and H02 radical concentrations during the winter and summer of 20042007

    • Author(s)
      Kanaya, Y., R. Cao, H. Akimoto, M. Fukuda, Y. Komazaki, Y. Yokouchi, M. Koike, H. Tanimoto, N. Takegawa, Y. Kondo
    • Journal Title

      J. Geophys. Res doi : 10. 1029/2007JD008670 112

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Seasonal variation of atmospheric C2-C7 nonmethane hydrocarbons in Tokyo2007

    • Author(s)
      Shirai, T., Y. Yokouchi, D. R. Blake, K. Kita, K. Izumi, M. Koike, Y. Komazaki, Y. Miyazaki, M. Fukuda, Y. Kondo
    • Journal Title

      I Geophys. Res doi : 10.1029/2006JD008163 112

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Measurements of Reactive Nitrogen Produced by Tropical Thunderstorms during BIBLE-C2007

    • Author(s)
      Koike, M., Y. Kondo, K. Kita, N. Takegawa, N. Nishi, B. Liley, T. Kashihara, S. Kudoh, S. Kawakami, D. Blake, T. Shirai, M. Ko, Y. Miyazaki, Z. Kawasaki, T. Ogawa
    • Journal Title

      I Geophys. Res. doi : 10.1029/2006JD008193 112

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Evolution of mixing state of black carbon particles : Aircraft asurements over the western Pacific in March 20042007

    • Author(s)
      Moteki, N., Y. Kondo, Y. Miyazaki, N. Takegawa, T. Miyakawa, Y. Komazaki, G. Kurata, T. Shirai, D. R. Blake, M. Koik
    • Journal Title

      Geophys. Res. Lett. 10.1029/2006GL028943 34

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Nitric acid condensation on ice : 2. Kinetic limitations, a possible "cloud clock" for determining cloud parcel lifetime2007

    • Author(s)
      Gamblin, B., O. B. Toon, M.A. Tolbert, Y. Kondo, N. Takegawa, H. Irie, M. Koike, P. K. Hudson, J.0. Ballenthin, D. E. Hunton, T. M. Miller, A.A. Viggiano, B. E. Anderson, M. Avery, G. W. Sachse, K. Guenther, C. Sorenson, M. J. Mahoney
    • Journal Title

      J. Geophys. Res. doi : 10.1029/2005JD006049 112

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Measurements of Reactive Nitrogen Produced by Tropical Thunderstorms during BIBLE-C2007

    • Author(s)
      M.Koike, 他
    • Journal Title

      J.Geophys.Res 112

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Urban photochemistly in central Tokyo:1.Observed and modeled OH and HO2 radical concentrations during the winter and summer of 20042007

    • Author(s)
      Y.Kanaya, M.Koike, 他
    • Journal Title

      J.Geophys.Res 112

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Seasonal variation of atmospheric C2-C7 nonmethane hydrocarbons in Tokyo2007

    • Author(s)
      T.Shirai, M.Koike, 他
    • Journal Title

      J.Geophys.Res 112

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Evolution of mixing state of black carbon particles:Aircraft measurements over the westem Pacific in March 20042007

    • Author(s)
      N.Moteki, M.Koike, 他
    • Journal Title

      Geophys.Res.Lett 34

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nitric acid condensation on ice:2.Kinetic limitations, a possible‘cloud clock'for determining cloud parcel lifetime2007

    • Author(s)
      B.Gamblin, M.Koike, 他
    • Journal Title

      J.Geophys.Res 112

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Seasonal Variation of Carbon Monoxide in Northern Japan: FTIR Measurements and Source-labeled Model Calculations2006

    • Author(s)
      M. Koike, 他
    • Journal Title

      J. Geophys. Res. 111

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Temporal variations of elemental carbon in Tokyo2006

    • Author(s)
      Y. Kondo, M. Koike, 他
    • Journal Title

      J. Geophys. Res. 111

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Evolution of submicron organic aerosol in polluted air exported from Tokyo2006

    • Author(s)
      N.. Takegawa, M. Koike, 他
    • Journal Title

      Geophys. Res. Lett. 33

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Nitric acid condensation on ice: 1. Non-HNO3 constituent of NOY condensing cirrus particles on upper tropospheric2006

    • Author(s)
      B. Gamblin, M. Koike, 他
    • Journal Title

      J. Geophys. Res. 111

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Seasonal Variation of Carbon Monoxide in Northern Japan : FTIR Measurements and Source-labeled Model Calculations2006

    • Author(s)
      Koike, M., N. B. Jones, P. I. Palmer, H. Matsui, Y. Zhao, Y. Kondo, Y. Matsumi, H. Tanimoto
    • Journal Title

      J. Geophys. Res. dio : 10.1029/2005JD006643 111

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Nitric acid condensation on ice : 1. Non-HN03 constituent of NOY condensing cirrus particles on upper tropospheric2006

    • Author(s)
      Gamblin, B., O. B. Toon, M.A. Tolbert, Y. Kondo, N. Takegawa, H. Irie, M. Koike, J. O. Ballenthin, D. E. Hunton, T. M. Miller, A.A. Viggiano, B. E. Anderson, M. Avery, G. W. Sachse, J. R. Podolske, K. Guenther, C. Sorenson, M. J. Mahoney
    • Journal Title

      I Geophys. Res. doi : 10.1029/2005JD006048 111

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Temporal variations of elemental carbon in Tokyo2006

    • Author(s)
      Kondo, Y., Y. Komazaki, Y. Miyazaki, N. Moteki, N. Takegawa, M. Nogami, S. Deguchi, M. Fukuda, T. Miyakawa, Y. Morino, D. Kodama, M. Koike
    • Journal Title

      J. Geophys. Res. doi : 10.1029/2005JD006257 111

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Evolution of submicron organic aerosol in polluted air exported from Tokyo2006

    • Author(s)
      Takegawa, N., T. Miyakawa, Y. Kondo, D. R. Blake, Y. Kanaya, M. Koike, M. Fukuda, Y. Komazaki, Y. Miyazaki, A. Shimono, T. Takeuchi
    • Journal Title

      Geophys. Res. Lett. doi : 10.1029/2006GL025815 33

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Seasonal Variation of Carbon Monoxide in Northern Japan : FTIR Measurements and Source-labeled Model Calculations2006

    • Author(s)
      Koike, M., N.B.Jones, P.I.Palmer, H.Matsui, Y.Zhao, Y.Kondo, Y.Matsumi, H.Tanimoto
    • Journal Title

      Journal of Geophysical Research 111

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Temporal variations of elemental carbon in Tokyo2006

    • Author(s)
      Kondo, Y., Y.Komazaki, Y.Miyazaki, N.Moteki, N.Takegawa, M.Nogami, S.Deguchi, M.Fukuda, T.Miyakawa, Y.Morino, D.Kodama, M.Koike
    • Journal Title

      Journal of Geophysical Research 111

    • Related Report
      2006 Annual Research Report
  • [Presentation] ブラックカーボンの物理化学的変容過程と混合状態を表現したモデルの開発2007

    • Author(s)
      大島、小池, 他
    • Organizer
      日本地球惑星科学連合2007年大会
    • Place of Presentation
      幕張メッセ国際会議場
    • Year and Date
      2007-05-21
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 3次元モデルを用いた関東域における2次有機エアロゾルの変動過程について2007

    • Author(s)
      松井、小池, 他
    • Organizer
      日本地球惑星科学連合2007年大会
    • Place of Presentation
      幕張メッセ国際会議場
    • Year and Date
      2007-05-21
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Development of new aerosol model to study volution of size dependent BC mixing state2007

    • Author(s)
      Oshima, Koike, et. al.
    • Organizer
      Japan Geoscience Union Meeting 2007
    • Place of Presentation
      Makuhari Messe, International Convention Complex
    • Year and Date
      2007-05-21
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Studies on secondary organic aerosol formation over the Kanto area2007

    • Author(s)
      Matsui, Koike, et. al.
    • Organizer
      Japan Geoscience Union Meeting 2007
    • Place of Presentation
      Makuhari Messe, International Convention Complex
    • Year and Date
      2007-05-21
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 人為起源ブラックカーボンの混合状態の時間的変化とその要因:エアロゾルの粒径分布と混合状態を表現した新しいモデルの開発2007

    • Author(s)
      大島長、小池真, 他
    • Organizer
      日本気象学会
    • Place of Presentation
      東京・国立オリンピック記念青少年総合センター
    • Year and Date
      2007-05-13
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
  • [Presentation] 都市域から輸送される汚染空気塊における有機エアロゾル生成率2006

    • Author(s)
      竹川、小池, 他
    • Organizer
      日本地球惑星科学連合2006年大会
    • Place of Presentation
      幕張メッセ国際会議場
    • Year and Date
      2006-05-16
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 3次元化学輸送モデルによる都市大気中の二次有機エアロゾル濃度の再現2006

    • Author(s)
      松井、小池, 他
    • Organizer
      日本地球惑星科学連合2006年大会
    • Place of Presentation
      幕張メッセ国際会議場
    • Year and Date
      2006-05-16
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Secondary organic aerosol formation efficiency within urban plume2006

    • Author(s)
      Takegawa, Koike, et. al.
    • Organizer
      Japan Geoscience Union Meeting 2006
    • Place of Presentation
      Makuhari Messe, International Convention Complex
    • Year and Date
      2006-05-16
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Three-dimensional model calculations on secondary organic aerosol in urban air2006

    • Author(s)
      Matsui, Koike, et. al.
    • Organizer
      Japan Geoscience Union Meeting 2006
    • Place of Presentation
      Makuhari Messe, International Convention Complex
    • Year and Date
      2006-05-16
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Evolution and processes of BC mixing state in air : Development of size resolved mixing state aerosol model2006

    • Author(s)
      Oshima, Koike, et. al.
    • Organizer
      Japan Meteorological Society annual meeting in 2008
    • Place of Presentation
      Tokyo national Olympic center
    • Year and Date
      2006-05-13
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary

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Published: 2006-04-01   Modified: 2016-04-21  

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