Theory of single adsorbate dynamics induced by electronic and vibrational excitation

• Project/Area Number: 18340085
• Research Category: Grant-in-Aid for Scientific Research (B)
• Allocation Type: Single-year Grants
• Section: 一般
• Research Field: Condensed matter physics I
• Research Institution: University of Toyama
• Principal Investigator: UEBA Hiromu University of Toyama, 大学院・理工学研究部(工学), 教授 (70019214)
• Project Period (FY): 2006 – 2008
• Project Status: Completed (Fiscal Year 2008)
• Budget Amount: ¥7,130,000 (Direct Cost: ¥5,900,000、Indirect Cost: ¥1,230,000); Fiscal Year 2008: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000); Fiscal Year 2007: ¥3,640,000 (Direct Cost: ¥2,800,000、Indirect Cost: ¥840,000); Fiscal Year 2006: ¥1,800,000 (Direct Cost: ¥1,800,000)
• Keywords: 走査トンネル顕微鏡 / 振動励起 / 電子励起 / 吸着 / フェムト秒 / 表面反応 / 表面光化学反応 / トンネル効果 / エネルギー移動 / 熱移動

Research Abstract

トンネル電子やフェムト秒レーザパルスによって直接あるいは間接的に励起された振動数モード(分子を構成する原子間の伸縮モード、基板-分子伸縮、束縛並進、束縛回転などの低振動数モード)との非調和相互作用による反応座標モードの振動加熱の理論構築を行い、これらの分野での先駆的な実験結果を説明することで、電子・振動励起による一酸化炭素などの吸着分子ダイナミックスの理論で世界をリードする研究成果を挙げることができた。

Research Products

• [Journal Article] Unified Description of Inelastic Propensity Rules for Electron Tr ansport through Nanoscale Junctions (2008)
  • Author(s): M. Paulsson, T. Frederiksen, H, eba, N. Lorente, M.
  • Journal Title: Brandbyge, Physical Review Letters 100226604 Pages: 4-4
• [Journal Article] Heat transfer between adsorbate and laser-heated hot electrons (2008)
  • Author(s): H. Ueba, B.N.J. Persson
  • Journal Title: Journal of Physics Condensed Matter 20 Pages: 224016-11
• [Journal Article] Heating of adsorbates by vibrational mode coupling (2008)
  • Author(s): H. Ueba, B.N.J. Persson
  • Journal Title: Physical Review 77 Pages: 035413-5
• [Journal Article] Adsorbate hopping via vibrational mode coupling induced by femtosecond laser pulses (2008)
  • Author(s): H. Ueba, M. Hayashi, M. Paulsson, B.N.J. Persson
  • Journal Title: Physical Review B B78 Pages: 113408-4
• [Journal Article] Unified Description of Inelastic Propensity Rules for Electron Transport through Nanoscale Junctions (2008)
  • Author(s): M. Paulsson, T. Frederiksen, H, Ueba, N. Lorente, M. Brandbyge
  • Journal Title: Review Letters 100(226604) Pages: 4-4
• [Journal Article] Heat transfer between adsorbate and laser-heated hot electrons (2008)
  • Author(s): H. Ueba and B.N.J. Persson
  • Journal Title: Journal of Physics : Condensed Matter 20(224016) Pages: 11-11
• [Journal Article] Heating of adsorbates by vibrational mode coupling (2008)
  • Author(s): H. Ueba and B.N.J. Persson
  • Journal Title: Physical Review B 77(035413) Pages: 5-5
• [Journal Article] Adsorbate hopping via vibrational mode coupling induced by femtosecond laser pulses (2008)
  • Author(s): H. Ueba, M. Hayashi, M. Paulsson and B.N. J. Persson
  • Journal Title: Physical Review B 78(113408) Pages: 4-4
• [Journal Article] Unified Description of Inelastic Propensity Rules for Electron Transport through Nanoscale Junctions (2008)
  • Author(s): M. Paulsson, H. Ueba ら
  • Journal Title: Physical Review Letters 100
  • Peer Reviewed
• [Journal Article] Heat transfer between adsorbate and laser-heated hot electrons (2008)
  • Author(s): H. Ueba, B. N. J. Persson
  • Journal Title: Journal of Physics : Condensed Matter 20
  • Peer Reviewed
• [Journal Article] Heating of adsorbates by vibrational mode coupling (2008)
  • Author(s): H. Ueba, B. N. T. Persson
  • Journal Title: Physical Review B 77
  • Peer Reviewed
• [Journal Article] Heating of adsoubate by vibrational mode coupling (2008)
  • Author(s): H. Ueba, B. N. J. Persson
  • Journal Title: Physical Review B 77
  • Peer Reviewed
• [Journal Article] Theory of inelastic tunneling spectroscopy of a single molecule-Competition between elastic and inelastic current- (2007)
  • Author(s): H. Ueba, T. Mii, S.G. Tikhodeev
  • Journal Title: Surface Science 601 Pages: 5220-5225
• [Journal Article] Adsorbate motions induced by vibrational mode coupling (2007)
  • Author(s): H. Ueba
  • Journal Title: Surface Science 601 Pages: 5212-5219
• [Journal Article] Action spectroscopy for single-molecule motion induced by vibrational excitation with a scanning tunneling microscope (2007)
  • Author(s): H. Ueba, B.N.J.
  • Journal Title: Physical Review B B75 Pages: 041403-4
• [Journal Article] Heat transfer at surfaces exposed to short-pulsed laser fields (2007)
  • Author(s): B.N. Persson, H. Ueba
  • Journal Title: Physical Review B75 Pages: 125401-4
• [Journal Article] Theory of inelastic tunneling spectroscopy of a single molecule-Competition between elastic and inelastic current (2007)
  • Author(s): H. Ueba, T. Mii and S.G. Tikhodeev
  • Journal Title: Surface Science 601 Pages: 5220-5225
• [Journal Article] Action spectroscopy for single-molecule motion induced by vibrational excitation with a scanning tunneling microscope (2007)
  • Author(s): H. Ueba and B.N.J. Persson
  • Journal Title: Physical Review B75, 041403R Pages: 4-4
• [Journal Article] Heat transfer at surfaces exposed to short-pulsed laser fields (2007)
  • Author(s): B. N. Persson and H. Ueba
  • Journal Title: Physical Review B76, 125401 Pages: 4-4
• [Journal Article] Vibrational heating of molecules adsorbed an insulating surfaces using localized photon tunneling (2007)
  • Author(s): B.N.J. Persson, T. Kato H. Ueba
  • Journal Title: Physical Review B 75
  • Peer Reviewed
• [Journal Article] Theory of inelastic tunneling spectroscopy of a single molecule (2007)
  • Author(s): H. Ueba, T. Mii, S. G. Tikhoddev
  • Journal Title: Surface Science 601 Pages: 5220-5225
  • Peer Reviewed
• [Journal Article] Adsorbate moions induced by vibrational mode coupling (2007)
  • Author(s): H. Ueba
  • Journal Title: Surface Science 601 Pages: 5212-5219
  • Peer Reviewed
• [Journal Article] Heat transfer at surfaces exposed to shout-pulsed laser fields (2007)
  • Author(s): B. N. J. Persson, H. Ueba
  • Journal Title: Physical Review B 76
  • Peer Reviewed
• [Journal Article] 非弾性トンネリングと単一吸着子の運動 (2007)
  • Author(s): 上羽 弘
  • Journal Title: 固体物理 42 Pages: 161-174
  • Peer Reviewed
• [Journal Article] Action spectroscopy for single-molecule motion induced by vibrational excitation with a scanning tunneling microscope (2007)
  • Author(s): H.Ueba, B.N.J.Perssion
  • Journal Title: Physical Review B 75
• [Journal Article] Adsorbate motions induced by vibrational mode coupling (2007)
  • Author(s): H.Ueba
  • Journal Title: Surface Science (掲載決定)
• [Journal Article] Theory of inelastic tunneling spectroscopy of a single molecule (2007)
  • Author(s): H.Ueba, T.Mii, S.Tikhodeev
  • Journal Title: Surface Science (掲載決定)
• [Journal Article] Enhancement of noncontactt friction between closely spaced bodies by two-dimensional systems (2006)
  • Author(s): A.I.Volokitin, B.N.J.Perssion, H.Ueba
  • Journal Title: Physical Review B 73
• [Presentation] Action spectroscopy of single molecule motion (2007)
  • Author(s): H. Ueba
  • Organizer: 54^<th> American Vacuum Society International Symposiu(招待講演)
  • Place of Presentation: シアトル,アメリカ
  • Year and Date: 2007-10-15
• [Presentation] Action spectroscopy of single molecule motion (招待講演) (2007)
  • Author(s): H. Ueba
  • Organizer: 54th American Vacuum Society International Symposium
  • Place of Presentation: シアトル(アメリカ)
  • Year and Date: 2007-10-15
• [Presentation] Action spectroscopy of single molecule motion (2007)
  • Author(s): H. Ueba
  • Organizer: 54th American Vacuum Society International Symposium
  • Place of Presentation: シア卜ル, アメリカ
  • Year and Date: 2007-07-24
• [Presentation] Heat transfer at surfaces (2007)
  • Author(s): H. Ueba
  • Organizer: 12th International Conference on Vibrations at Surface
  • Place of Presentation: エリーチエ, イタリア
  • Year and Date: 2007-07-24
• [Presentation] Heat transfer at surfaces (2007)
  • Author(s): H. Ueba
  • Organizer: 12^<th> International Conference on Vibrations at Surfaces
  • Place of Presentation: エリーチェ、イタリア
  • Year and Date: 2007-07-24
• [Presentation] Heat transter at surfaces (2007)
  • Author(s): H. Ueba
  • Organizer: 12th International Conference on Vibrations at Surfaces
  • Place of Presentation: エリーチェ、シシリー(イタリア)
  • Year and Date: 2007-07-24
• [Presentation] Action spectroscopy for single molecule motion (2007)
  • Author(s): H. Ueba
  • Organizer: 12th International Conference on Vibrations at Surfaces
  • Place of Presentation: エリーチェ、シシリー(イタリア)
  • Year and Date: 2007-07-23
• [Presentation] Theory of single molecule motions induced by vibrational STM (2006)
  • Author(s): H. Ueba
  • Organizer: 232th American Chemical Society National Meeting
  • Place of Presentation: San Francisco
• [Presentation] Theory of single molecule motion induced by vibrational excitation (2006)
  • Author(s): H. Ueba
  • Organizer: CREST Workshop on Physics of a single molecules
  • Place of Presentation: Kanagawa, Japan
• [Presentation] Theory of single molecule motions induced by vibrational excitation with STM (2006)
  • Author(s): H. Ueba
  • Organizer: 232^<th> American Chemical Society National Meeting(招待講演)
  • Place of Presentation: SanFrancisco
• [Presentation] Theory of single molecule motion induced by vibrational excitation (2006)
  • Author(s): H. Ueba
  • Organizer: CREST Workshop on Physics of a single molecules(招待講演)
  • Place of Presentation: Kanagawa, Japan
• [Book] Inelastic Tunneling Current-Motions of Single Adsorbates (2009)
  • Author(s): H. Ueba, S. G. Tikhodeev, B. N. J
  • Publisher: Pan Stanford Publishing
• [Book] Dynamics at solid state surfaces and interfaces (2009)
  • Author(s): processes, J. Guedde, M. Bonn, H. Ueba, U. Hoefer
  • Publisher: Wiley Publishing
• [Book] Current-Driven Phenomena in Nanoelectronics(T. Seideman)(Inelastic Tunneling Current-Driven Motions of Single Adsorbates) (2009)
  • Author(s): H. Ueba, S.G. Tikhodeev and B.N.J. Persson
  • Publisher: Pan Stanford Publishing
• [Book] Problems of Condensed Matter Physics (2008)
  • Author(s): H. Ueba
  • Publisher: Oxford Science Publications
• [Book] Problems of Condensed Matter Physics(Inelastic tunneling spectroscopy of single surface adsorbed molecules) (2008)
  • Author(s): S.G. Tikhodeev, H. Ueba
  • Publisher: Oxford Science Publications
• [Book] International Series of Monographs on Physics“Problems of Condensed Matter Physics" (2008)
  • Author(s): S. G. Tikhodeev, H. Ueba
  • Total Pages: 24
  • Publisher: Oxford Science Publications