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Study on the origin of induced magnetic anisotropy of metal-insulator nano-granular soft-magnetic film by small-angle X-ray and neutron scattering

Research Project

Project/Area Number 18360340
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Structural/Functional materials
Research InstitutionNational Institute for Materials Science

Principal Investigator

MASATO Ohnuma  National Institute for Materials Science, Quantum beam center, senior researcher (90354208)

Co-Investigator(Kenkyū-buntansha) OHNUMA Shigehiro  Research Institute for Electric and Magnetic Materials, magnetic thin films group, Senior researcher (50142633)
SUZUKI Jun-ichi  Japan Atomic Energy Agency, J-PARC center, Senior researcher (40354899)
Project Period (FY) 2006 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥10,620,000 (Direct Cost: ¥9,300,000、Indirect Cost: ¥1,320,000)
Fiscal Year 2007: ¥5,720,000 (Direct Cost: ¥4,400,000、Indirect Cost: ¥1,320,000)
Fiscal Year 2006: ¥4,900,000 (Direct Cost: ¥4,900,000)
Keywordssoft-magnetic materials / induced magnetic anisotropy / small-angle scattering / neutron scattering / quantum beam / 磁性 / 複合材料・物性
Research Abstract

For achieving high density and fast electronic devices, soft magnetic materials with high-magnetic permeability at the GHz frequency regions are required. Nano-granular soft-magnetic films are one of the promising candidates because of their high saturation magnetization, large resistivity and large induced magnetic anisotropy field, Hk, that sometimes exceed 200 Oe. Except large Hk, the origin of the properties is attribute to the microstructure which consists of almost pure Co and Si-O base amorphous matrix. Elk also shows weak dependence of the average particle size, however, no microstructural anisotropy has been found yet. For full understanding of the origin of anisotropy, it is needed to know the magnetization process in the field smaller than Hk. For this purpose, we use small-angle neutron scattering (SANS). Our findings are follows;
1. Intensity maximum in SANS appears parallel to the major axis of magnetization. This indicates the existence of minor contribution of magnetizat … More ion which lies perpendicular direction to the major magnetization axis.
2. By applying magnetic field perpendicular to easy axis, the intensity maximum rotate continuously to the external field, indicating the minor contribution also rotate together with major component of magnetization.
3. The size of the magnetic domain of minor component is changed by the external field. Larger in the small field and smaller in the field close to the Bk. Latter ease, it is about 10 nm which is still larger than the particle size (〜3nm). Magnetic domain size of the major component is larger than a few thousand nm that is the maximum size of our SANS measurements. Therefore, it indicates the existence of hierarchical structure in the magnetic domain.
Such of hierarchical structure in the magnetic domain has never reported in the soft-magnetic materials. Hence it can be a key factor for showing large Bk. For confirming it, we are now conducting further experiments using stronger neutron source which starts from Dec. 2008. Less

Report

(3 results)
  • 2007 Annual Research Report   Final Research Report Summary
  • 2006 Annual Research Report
  • Research Products

    (48 results)

All 2008 2007 2006

All Journal Article (32 results) (of which Peer Reviewed: 17 results) Presentation (16 results)

  • [Journal Article] Observation of an extended magnetic field penetration in amorphous superconducting MoGe films2008

    • Author(s)
      T.Nishio,S.Okayasu,J.Suzuki,N.Kokubo,K.Kadowaki
    • Journal Title

      PHYSICAL REVIEW B 77

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Thermal embrittlement of Fe-based amorphous ribbons2008

    • Author(s)
      G.Kumar,M.Ohnuma,T.Furubayashi,T.Ohkubo,K.Hono,
    • Journal Title

      JOURNAL OF NON-CRYSTALLINE SOLIDS 354

      Pages: 882-888

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Direct observation of hydrogen trapped by NbC in steel using small-angle neutron scattering2008

    • Author(s)
      M.Ohnuma,J.Suzuki,F.G.Wei,K.Tsuzaki
    • Journal Title

      SCRIPTA MATERIALIA 58

      Pages: 142-145

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Observation of an extended magnetic field penetration in amorphous superconduction MoGe films2008

    • Author(s)
      T. Nishio, S. Okayasu, J. Suzuki, N. Nokubo, K.Kadowaki
    • Journal Title

      PHYSICAL REVIEW B 77

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Thermal embrittlement of Fe-based amorphous ribbons2008

    • Author(s)
      G. Kumar, M. Ohnuma, T. Furubayashi, T. Ohkubo, K. Hono
    • Journal Title

      JOURNAL OF NON-CRYSTALLINE SOLIDS 354

      Pages: 882-888

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
  • [Journal Article] Direct observation of hydrogen trapped by NbC in steel using small-angle neutron scattering2008

    • Author(s)
      M. Ohnuma, J. Suzuki, F. G. Wei, K. Tsuzaki
    • Journal Title

      SCRIPTA MATERIALIA 58

      Pages: 142-145

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Observation of an extended magnetic field penetration in amorphous superconducting Mote films2008

    • Author(s)
      T. Nishio, S. Okayasu, J. Suzuki, N. Kokubo, K. Kadowaki
    • Journal Title

      PHYSICAL REVIEW B 77

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Direct observation of hydrogen trapped by NbC in steel using small-angle neutron scatterin2008

    • Author(s)
      M. Ohnuma, J. Suzuki, F. G. Wei, K. Tsuzaki
    • Journal Title

      SCRIPTA MATERIALIA 58

      Pages: 142-145

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Microstructure of Ge: Ta205 granular thin films: an application of TEM-tomography2007

    • Author(s)
      H.Gao,S.Toh.S.Matsumura,S.Abe S.Ohnuma
    • Journal Title

      MATERIALS TRANSACTIONS 48

      Pages: 2567-2571

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Metal-insulator type nano-granular soft magnetic thin. Ims investigations on mechanism and applications2007

    • Author(s)
      S.Ohnuma,M.Ohnuma,H.Fujimori,T.Masumoto
    • Journal Title

      JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 310

      Pages: 2503-2509

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Brillouin light scattering from TM-AI-O granular films (TM=Co,Fe)2007

    • Author(s)
      A.Yoshihara,S.Ohnuma,H.Fujimori
    • Journal Title

      JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 310

      Pages: 2513-2515

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Comparison of field-cooled,zero-field-cooled, and thermoremanent magnetization in nanomagnet, random magnet, and bulk ferromagnet2007

    • Author(s)
      H.Mamiya,S.Nimori,,M.Ohnuma,I.Nakatani,M.Demura,T.Furubayashi
    • Journal Title

      JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 316

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Microstructure of Ge : Ta_2O_5 granular thin films : an appilcation fo TEM-tomography2007

    • Author(s)
      H. Gao, S. Toh. S. Matsumura, S. Abe S.Ohnuma
    • Journal Title

      Materials Trans. 48

      Pages: 2567-2571

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Metal insulator type nano-granular soft magnetic thin. Lms investigations on mechanism and applications2007

    • Author(s)
      S. Ohnuma, M. Ohnuma, H. Fujimori, T. Masumoto
    • Journal Title

      J. Magn. Magn. Mat. 310

      Pages: 2503-2509

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Brillouin light scattering from TM-AI-O granular films(TM=Co, Fe)2007

    • Author(s)
      A. Yoshihara, S. Ohnuma, H. Fujimori
    • Journal Title

      J. Magn. Magn. Mat. 310

      Pages: 2513-2515

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Comparison of field-cooled, zero-field-cooled, and thermoremanent magnetization in nanomagnet, random magnet, and bulk ferromagnet2007

    • Author(s)
      H. Mamiya, S. Nimori, M. Ohnuma, I. Nakatani, M.Demura, T. Furubayashi
    • Journal Title

      J. Magn. Magn. Mat. 316

      Pages: 535-537

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Microstructure of Ge:Ta205 granular thin films:an application of TEM-tomography2007

    • Author(s)
      H. Gao, S. Toh. S. Matsumura, S. Abe S. Ohnuma
    • Journal Title

      MATERIALS TRANSACTIONS 48

      Pages: 2567-2571

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Metal-insulator type nano-granular soft magnetic thin.Ims investigations on mechanism and applications2007

    • Author(s)
      S. Ohnuma, M. Ohnuma, H. Fujimori, T. Masumoto
    • Journal Title

      JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 310

      Pages: 2503-2509

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Brillouin light scattering from TM-AI-O granular films (TM =Co,Fe)2007

    • Author(s)
      A. Yoshihara, S. Ohnuma, H. Fujimori
    • Journal Title

      JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 310

      Pages: 2513-2515

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Comparison of field-cooled, zero-field-coaIed,and thermoremanent magnetization in nanomagnet,random magnet,and bulk ferromagnet2007

    • Author(s)
      H. Mamiya, S. Nimori, M. Ohnuma, I. Nakatani, M. Demura, T. Furubayashi
    • Journal Title

      JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS 316

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] X線および中性子小角散乱による先端金属材料の微細組織解析2006

    • Author(s)
      大沼正人、鈴木淳市
    • Journal Title

      分析化学 55・6

      Pages: 381-390

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] 中性子およびX線小角散乱によるミクロ組織定量評価2006

    • Author(s)
      大沼正人、鈴木淳市
    • Journal Title

      ふぇらむ 11・10

      Pages: 631-640

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Noise suppression effect of soft magnetic Co-Pd-B-O films with large p and Bs2006

    • Author(s)
      S.Ohnuma,T.Iwasa,H.Fujimori,T.Masumoto
    • Journal Title

      IEEE TRANSACTIONS ON MAGNETICS 42

      Pages: 2769-2771

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Spintronics in metal-insulator nanogranular magnetic thin films2006

    • Author(s)
      H.Fujimori,S.Ohnuma,N.Kobayashi,T.Masumoto
    • Journal Title

      J.Magn.Magn.Mat. 304

      Pages: 32-35

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
    • Peer Reviewed
  • [Journal Article] Study on microstructuers of advanced metallic materials by small-angle X-ray and Neutron Scattering2006

    • Author(s)
      Masato Ohnuma, Jun-ichi Suzuki
    • Journal Title

      Bunseki Kagaku 55

      Pages: 381-390

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Quantitative Analysis of Microstruture by Small-angle Neutron and X-ray Sattering(overview paper)2006

    • Author(s)
      Masato Ohnuma, Jun-ichi Suzuki
    • Journal Title

      Bulletin of the Iron and Steel Institute of of Japan 11

      Pages: 631-640

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Noise suppression effect of soft magnetic Co-Pd-B-O films with large p and Bs2006

    • Author(s)
      S. Ohnuma, T. Iwasa, H. Fujimori, T. Masumoto
    • Journal Title

      IEEE TRANSACTIONS ON MAGNETICS 42

      Pages: 2769-2771

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Spintronics in metal-insulator nanogranular magnetic thin films2006

    • Author(s)
      H. Fujimori, S. Ohnuma, N. Kobayashi, T. Masumoto
    • Journal Title

      J. Magn. Magn. Mat. 304

      Pages: 32-35

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] X線および中性子小角散乱による先端金属材料の微細組織解析2006

    • Author(s)
      大沼正人, 鈴木淳市
    • Journal Title

      分析化学 55・6

      Pages: 381-390

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 中性子およびX線小角散乱によるミクロ組織定量評価2006

    • Author(s)
      大沼正人, 鈴木淳市
    • Journal Title

      ふぇらむ 11・10

      Pages: 631-640

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Noise suppression effect of soft magnetic Co-Pd-B-O films with large p and Bs2006

    • Author(s)
      S.Ohnuma, T.Iwasa, H.Fujimori, T.Masumoto
    • Journal Title

      IEEE TRANSACTIONS ON MAGNETICS 42・10

      Pages: 2769-2771

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Spintronics in metal-insulator nanogranular magnetic thin films2006

    • Author(s)
      H.Fujimori, S.Ohnuma, N.Kobayashi, T.Masumoto
    • Journal Title

      J. Magn. Magn. Mat. 304・1

      Pages: 32-35

    • Related Report
      2006 Annual Research Report
  • [Presentation] 偏極中性子小角散乱法によるナノ結晶軟磁性材料の磁化過程の検討2008

    • Author(s)
      篠原武尚、鈴木淳市、大沼正人、奥隆之、大沼繁弘
    • Organizer
      日本物理学会
    • Place of Presentation
      近畿大学
    • Year and Date
      2008-03-23
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
  • [Presentation] Magnetization process of nano-crystalline magnetic materials2008

    • Author(s)
      T. Shinohara, J. Suzuki, M. Ohnuma, T. Oku, S. Ohnuma
    • Organizer
      Spring meeting of Physiscal Society of Japan
    • Place of Presentation
      Oosaka
    • Year and Date
      2008-03-23
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] ナノグラニュラ軟磁性膜の熱的安定性2007

    • Author(s)
      大沼繁弘、大沼正人、藤森啓安、増本建
    • Organizer
      日本金属学会
    • Place of Presentation
      岐阜大学
    • Year and Date
      2007-09-20
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
  • [Presentation] X線小角散乱による半導体名の粒子膜の微細構造2007

    • Author(s)
      大沼正人、平徳海、大沼繁弘、阿部世嗣
    • Organizer
      日本金属学会
    • Place of Presentation
      岐阜大学
    • Year and Date
      2007-09-20
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Annual Research Report 2007 Final Research Report Summary
  • [Presentation] Thermal stability of nano-granular soft magnetic films2007

    • Author(s)
      S. Ohnuma, M, Ohnuma, H. Fujimori, T. Masumoto
    • Organizer
      Fall meeting of Japan Insitute of Metals
    • Place of Presentation
      Gifu
    • Year and Date
      2007-09-20
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Microstructure of nano-granular semi-conductor2007

    • Author(s)
      M. Ohnuma, D. H. Ping, S. Ohnuma, S. Abe
    • Organizer
      Fall meeting of Japan Insitute of Metals
    • Place of Presentation
      Gifu
    • Year and Date
      2007-09-20
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 中性子小角散乱法による大きな異方性を有するナノグラニュラ軟磁性膜の研究(依頼講演)2006

    • Author(s)
      大沼正人
    • Organizer
      茨城県中性子利用促進研究会ナノ磁性材料研究会
    • Place of Presentation
      東京
    • Year and Date
      2006-11-21
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Small-angle neutron scattting study on nano-granulat soft-magnetic films(invited) nano-magnetic materials2006

    • Author(s)
      M. Ohnuma
    • Organizer
      Ibaraki prefecture Program for promoting use of neutron
    • Place of Presentation
      Tokyo
    • Year and Date
      2006-11-21
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Microstructure and Magnetic domain structure of metal-nonmetal softmagneti granular film"2006

    • Author(s)
      M.Ohnuma,J.Suzuki,S.Ohnuma,H.Fujimori
    • Organizer
      13th conference on Small-Angle Scattering
    • Place of Presentation
      Kyoto
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] コバルト基ナノグラニュラソフト磁性膜の磁性2006

    • Author(s)
      間宮宏明、大沼繁弘、大沼正人、古林孝夫、藤森啓安
    • Organizer
      17th Internatinal Conference on Magnetism
    • Place of Presentation
      京都
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Origin of stress-induced magnetic anisotropy in Fe-Si-B-Nb-Cu nanocrystalline alloy2006

    • Author(s)
      M.Ohnuma,T.Yanai,M.Nakano,H.Fukunaga
    • Organizer
      European conference on Residual stresses
    • Place of Presentation
      Berlin
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] ナノグラニュラ磁性薄膜における熱アシスト型軟磁性2006

    • Author(s)
      間宮宏明、大沼繁弘、大沼正人、古林孝夫、藤森啓安
    • Organizer
      日本物理学会
    • Place of Presentation
      千葉
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Microstructure and Magnetic domain structure of metal-nonmetal softmagneti granular film2006

    • Author(s)
      M. Ohnuma, J. Suzuki, S.Ohnuma, H.Fujimori
    • Organizer
      13th conference on Small-Angle Scattering
    • Place of Presentation
      Kyoto
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Magnetic properties of Cobalt based nano-ganular soft magnetic fims2006

    • Author(s)
      H. Mamiya, S. Ohnuma, M. Ohnuma, T. Furubayashi, H. Fujimori
    • Organizer
      17th Internatinal Conference on Magnetism
    • Place of Presentation
      Kyoto
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Origin of stress-inducedmagnetic anisotropy in Fe-Si-B-Nb-Cu nanocrystalline alloy2006

    • Author(s)
      M. Ohnuma, T.Yanai, M.Nakano, H.Fukunaga
    • Organizer
      European confference on Residual stresses
    • Place of Presentation
      Berlin
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Thermally assisted soft-magnetism in nano- granular films2006

    • Author(s)
      H. Mamiya, S. Ohnuma, M. Ohnuma, T. Furubayashi, H. Fujimori
    • Organizer
      Fall meeting of Physiscal Society of Japan
    • Place of Presentation
      Chiba
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary

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Published: 2006-04-01   Modified: 2016-04-21  

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