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Generation of plasmas in liquid media and its application to light emitting devices

Research Project

Project/Area Number 18540493
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Plasma science
Research InstitutionKyoto University

Principal Investigator

SHIRAFUJI Tatsuru  Kyoto University, Innovative Collaboration Center, Associate Professor (10235757)

Project Period (FY) 2006 – 2007
Project Status Completed (Fiscal Year 2007)
Budget Amount *help
¥3,900,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥300,000)
Fiscal Year 2007: ¥1,300,000 (Direct Cost: ¥1,000,000、Indirect Cost: ¥300,000)
Fiscal Year 2006: ¥2,600,000 (Direct Cost: ¥2,600,000)
KeywordsLiquid / Plasma / Pulse Power / Optical Emission / Environment / Micro Bubbles / Water / Discharge / 水面上放電 / 水中気泡放電 / エタノール中放電 / 液体プラズマ処理 / 発光デバイス / 液中元素分析 / 水質浄化
Research Abstract

We have investigated characteristics of the electrical discharge and optical emission of the plasmas in/on/with liquid media such as pure water, several aqueous solution and hydrocarbons. In order to perform these investigations, we have constructed following electrical discharge devices ; dielectric barrier discharge systems with liquid electrodes, mangrove-type barrier discharge systems, single-bubble discharge systems, water-electrolysis-bubble discharge systems and porous-dielectric-covered metal electrode systems. On the basis of the characteristics obtained, we have discussed possibility of these plasmas as light emitting devices. In electrical discharge on the water surface, sufficient visible luminescence has been obtained when we employ argon or helium for discharge gases in addition to the air. We have also found that the intense discharge on the water can decompose organic compounds in the water, and that OH radicals seem to be responsible for the decomposition. In case of t … More he discharge in the single bubble floating in a water-filled tube, we have obtained electrical discharge in the bubble only when we employ the water which includes metal particles. Ignition of discharge in the bubble has become easier when the bubbles are on metal surface. We have employed an electrolysis technique for generating and fixing the bubbles on metal surface without feeding gases into the water, and have successfully obtained discharge in hydrogen or oxygen bubbles on the electrolysis electrode although its optical emission is not high enough at present. In order to obtain gas bubbles without feeding gases into a liquid medium, we have also utilized a metal electrode covered with a porous dielectric film on which high voltage is applied in the ethanol. The bubbles in the ethanol have been generated by Joule heating in this case. Although we cannot observe any optical emission from the bubbles floating in the ethanol, we have obtained discharge and its optical emission in the bubbles between the dielectric film and the metal electrode. In summary, we have demonstrated several possible types of electrical discharge with, on or in liquid media, although, at this moment, intensity of the optical emission obtained in this work is not high enough to apply this technique to light emitting devices. Less

Report

(3 results)
  • 2007 Annual Research Report   Final Research Report Summary
  • 2006 Annual Research Report
  • Research Products

    (31 results)

All 2008 2007 2006

All Journal Article (14 results) Presentation (17 results)

  • [Journal Article] Generation of micro bubbles in a liquid medium and observation of their discharges2007

    • Author(s)
      T. Shirafuji, M. Kimura, O. sakai, K. Tachibana
    • Journal Title

      Proc.18th International Symp. Plasma Chem. 18

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Discharge characteristics of the plasma on liquid media2007

    • Author(s)
      M. Kimura, T. Shirafuji, O. Sakai, K. Tachibana
    • Journal Title

      Proc.18th International Symp. Plasma Chem. 18

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Atmospheric-pressure discharge ignited on flexible electrodes of fabric structure2007

    • Author(s)
      O. Sakai, T. Shirafuji, K. Tachibana
    • Journal Title

      Proc.18th International Symp. Plasma Chem. 18

    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Discharge characteristics of the plasma on liquid media2007

    • Author(s)
      M., Kimura, T., Shirafuji, O., Sakai, K., Tachibana
    • Journal Title

      Proc. 18th International Symp. Plasma Chem 18, 28

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Atmospheric-pressure discharge ignited on flexible electrodes of fabric structure2007

    • Author(s)
      O., Sakai, T., Shirafuji, K., Tachibana
    • Journal Title

      Proc. 18th International Symp. Plasma Chem 18, 27

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Observation of plasma on ePTFE-covered metal rod in ethanol2007

    • Author(s)
      T., Shirafuji, M., Kimura, O., Sakai, K., Tachibana
    • Journal Title

      Proc. 18th International Symp. Plasma Chem 18, 27

    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Journal Article] Generation of micro bubbles in a liquid medium and observation of their discharges2007

    • Author(s)
      T. Shirafuji, M. Kimura, O. Sakai, K. Tachibana
    • Journal Title

      Proc. 18th International Symp. Plasma Chem. 18

    • Related Report
      2007 Annual Research Report
  • [Journal Article] Discharge characteristics of the plasma on liquid media2007

    • Author(s)
      M. Kimura, T. Shirafuji, O. Sakai, K. Tachibana
    • Journal Title

      Proc. 18th International Symp. Plasma Chem. 18

    • Related Report
      2007 Annual Research Report
  • [Journal Article] Microdischarges on metal surface in a liquid medium2007

    • Author(s)
      M. Kimura, O. Sakai, T. Shirafuji, K. Tachibana
    • Journal Title

      Proc. 4th International Workshop on Microplasmas 4

      Pages: 63-63

    • Related Report
      2007 Annual Research Report
  • [Journal Article] Plasma-liquid interaction in liquid-electrode embedded dielectric barrier discharge2006

    • Author(s)
      T.Shirafuji, M.Kimura, K.Tachibana
    • Journal Title

      8th Asia-Pasific Conference on Plasma Science and Technology 8

      Pages: 253-253

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 水及び誘電体壁で囲まれた単一気泡内における放電の観測2006

    • Author(s)
      白藤立, 木村優, 橘邦英
    • Journal Title

      第67回応用物理学会学術講演会 67・1

      Pages: 178-178

    • Related Report
      2006 Annual Research Report
  • [Journal Article] 水電極誘電体バリア放電の生成と評価2006

    • Author(s)
      木村優, 白藤立, 橘邦英
    • Journal Title

      第47回真空に関する連合講演会 47

      Pages: 152-152

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Generation of micro bubbles in a liquid medium and observation of their discharges2006

    • Author(s)
      T.Shirafuji, M.Kimura, K.Tachibana
    • Journal Title

      The 24th Symposium on Plasma Processing 24

      Pages: 179-180

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Discharge characteristics of the plasma on liquid media2006

    • Author(s)
      M.Kimura, T.Shirafuji, K.Tachibana
    • Journal Title

      The 24th Symposium on Plasma Processing 24

      Pages: 207-208

    • Related Report
      2006 Annual Research Report
  • [Presentation] マングローブ型電極を用いた気液界面放電とその液体への効果2008

    • Author(s)
      森田直祐, 木村優, 久保寔, 酒井道, 白藤立, 橘邦英
    • Organizer
      第55回応用物理学関係連合講演会
    • Place of Presentation
      東京
    • Year and Date
      2008-03-28
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Electrical discharge at gas/liquid interface using mangrove-shaped electrodes and its effects on the liquid properties2008

    • Author(s)
      T., Morita, M., Kimura, M., Kubo, O., Sakai, T., Shirafuji, K., Tachibana
    • Organizer
      The 55th Spring Meeting of The Japan Society of Applied Physics
    • Place of Presentation
      Tokyo, Japan
    • Year and Date
      2008-03-28
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 液体が関与する放電とその応用について2008

    • Author(s)
      白藤 立, 酒井 道, 橘 邦英
    • Organizer
      仙台プラズマフォーラム
    • Place of Presentation
      東北大学
    • Year and Date
      2008-02-22
    • Related Report
      2007 Annual Research Report
  • [Presentation] 液体が関与する放電とその応用について2008

    • Author(s)
      白藤立, 酒井道, 橘邦英
    • Organizer
      平成19 年度東北大学電気通信研究所共同プロジェクト研究会
    • Place of Presentation
      仙台
    • Year and Date
      2008-02-21
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] On the discharges involving liquids and their applications2008

    • Author(s)
      T., Shirafuji, O., Sakai, K., Tachibana
    • Organizer
      Annual Meeting for The Collaborative Projects in The Research Institute of Electrical Communication
    • Place of Presentation
      Sendai, Japan
    • Year and Date
      2008-02-21
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Microdischarges on metal surface in a liquid medium2007

    • Author(s)
      M. Kimura, O. Sakai and T. Shirafuji, K. Tachibana:
    • Organizer
      The 4th International Workshop on Microplasmas
    • Place of Presentation
      Tainan, Taiwan
    • Year and Date
      2007-10-29
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 多孔質テフロンで被覆された金属電極近傍におけるエタノール中放電の観測2007

    • Author(s)
      白藤立, 木村優, 酒井道, 橘邦英
    • Organizer
      第54回応用物理学関係連合講演会
    • Place of Presentation
      東京
    • Year and Date
      2007-03-29
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Observation of discharge on the metal rod covered with porous Teflon tube in ethanol2007

    • Author(s)
      T., Shirafuji, M., Kimura, O., Sakai, K., Tachibana
    • Organizer
      The 54th Spring Meeting of The Japan Society of Applied Physics
    • Place of Presentation
      Tokyo, Japan
    • Year and Date
      2007-03-29
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Generation of micro bubbles in a liquid medium and observation of their discharges2007

    • Author(s)
      T. Shirafuji, M. Kimura and K. Tachibana
    • Organizer
      The 24th Symposium on Plasma Processing
    • Place of Presentation
      大阪
    • Year and Date
      2007-01-30
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Discharge characteristics of the plasma on liquid media2007

    • Author(s)
      M. Kimura, T. Shirafuji and K. Tachibana
    • Organizer
      The 24th Symposium on Plasma Processing
    • Place of Presentation
      大阪
    • Year and Date
      2007-01-30
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Generation of micro bubbles in a liquid medium and observation of their discharges2007

    • Author(s)
      T., Shirafuji, M., Kimura, K., Tachibana
    • Organizer
      The 24th Symposium on Plasma Processing
    • Place of Presentation
      Osaka, Japan
    • Year and Date
      2007-01-30
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Discharge characteristics of the plasma on liquid media2007

    • Author(s)
      M., Kimura, T., Shirafuji, K., Tachibana
    • Organizer
      The 24th Symposium on Plasma Processing
    • Place of Presentation
      Osaka, Japan
    • Year and Date
      2007-01-30
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 水電極誘電体バリア放電の生成と評価2006

    • Author(s)
      木村優, 白藤立, 橘邦英
    • Organizer
      第47回真空に関する連合講演会
    • Place of Presentation
      大阪
    • Year and Date
      2006-11-08
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Dielectric barrier discharge using water electrodes and its characteristics2006

    • Author(s)
      M., Kimura, T., Shirafuji, K., Tachibana
    • Organizer
      The 47th Meeting of The Vacuum Society Japan
    • Place of Presentation
      Osaka, Japan
    • Year and Date
      2006-11-08
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] 水及び誘電体壁で囲まれた単一気泡内における放電の観測2006

    • Author(s)
      木村優, 白藤立, 橘邦英
    • Organizer
      第67回応用物理学会学術講演会
    • Place of Presentation
      草津
    • Year and Date
      2006-09-01
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Observation of discharge in a bubble surrounded by water and dielectric wall2006

    • Author(s)
      M., Kimura, T., Shirafuji, K., Tachibana
    • Organizer
      The 67th Autumn Meeting of The Japan Society of Applied Physics
    • Place of Presentation
      Kusatsu, Japan
    • Year and Date
      2006-09-01
    • Description
      「研究成果報告書概要(欧文)」より
    • Related Report
      2007 Final Research Report Summary
  • [Presentation] Plasma-liquid interaction in liquid-electrode-embedded dielectric barrier discharge2006

    • Author(s)
      M. Kimura, T. Shirafuji, K. Tachibana
    • Organizer
      The 8th Asia Pacific Conference on Plasma Science and Technology
    • Place of Presentation
      Cairns, Australia
    • Year and Date
      2006-07-03
    • Description
      「研究成果報告書概要(和文)」より
    • Related Report
      2007 Final Research Report Summary

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Published: 2006-04-01   Modified: 2016-04-21  

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