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Catalytic and Electrochemical Properties of Ceria doped YSZ Anode Catalysts for Solid Oxide Fuel Cells

Research Project

Project/Area Number 18560738
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Catalyst/Resource chemical process
Research InstitutionHokkaido University

Principal Investigator

TATSUYA Takeguchi  Hokkaido University, 触媒化学研究センター, 准教授 (30227011)

Project Period (FY) 2006 – 2008
Project Status Completed (Fiscal Year 2008)
Budget Amount *help
¥3,910,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥510,000)
Fiscal Year 2008: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2007: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2006: ¥1,700,000 (Direct Cost: ¥1,700,000)
Keywordsエネルギー変換プロセス / SOFC / CeO_2-Y_2O_3-ZrO_2固溶体 / 炭素析出 / Niサーメット / メタン / 内部改質 / CeO_2-Y_2O3-ZrO_2固溶体
Research Abstract

ペロブスカイト酸化物の還元処理を行いNi-Co合金アノード触媒を合成した。次に、グリコサーマル法を用いて表面水酸基を多く持ったYSZ を合成しNi を担持したNi/YSZを合成した。これらの知見を生かして、固体酸化物形燃料電池用Ni-セリア固溶YZS アノードの触媒および電気化学特性の検討を行なった。内部改質型SOFCの課題である炭素析出は、YSZアノードへセリアの固溶により大幅に抑制され、電気化学特性も向上した。

Report

(4 results)
  • 2008 Annual Research Report   Final Research Report ( PDF )
  • 2007 Annual Research Report
  • 2006 Annual Research Report
  • Research Products

    (13 results)

All 2008 2007 2006

All Journal Article (9 results) (of which Peer Reviewed: 7 results) Presentation (4 results)

  • [Journal Article] Synthesis of Biogasoline from Ethanol over Hydroxyapatite Catalyst2008

    • Author(s)
      Takashi Tsuchida, Tetsuya, Yoshioka, Shuji Sakuma, Tatsuya Takeguchi and Wataru Ueda
    • Journal Title

      Ind. Eng. Chem. Res 47, No.5

      Pages: 1443-1452

    • Related Report
      2008 Final Research Report
    • Peer Reviewed
  • [Journal Article] Synthesis of Biogasoline from Ethanol over Hydroxyapatite Catalyst2008

    • Author(s)
      Takashi Tsuchida
    • Journal Title

      Ind. Eng. Chem. Res 47

      Pages: 1443-1452

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] The Effect of Modification of PtRu Anode Catalyst with SnO2 on CO Tolerance2008

    • Author(s)
      Tatsuya Takeguchi
    • Journal Title

      ECS Transactions 16(2)

      Pages: 713-716

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Adsorbed Species on CO Preferential Oxidation in the Presence of H_2S over Ru/Al_2O_3 Catalyst2007

    • Author(s)
      Hidenobu Wakita, TatsuyaTakeguchi, and Wataru Ueda
    • Journal Title

      Stud. Surf. Sci. Catal 172

      Pages: 587-588

    • Related Report
      2008 Final Research Report
    • Peer Reviewed
  • [Journal Article] Mechanistic Investigation of Deactivationof Ru/Al_2O_3 Catalyst for Preferential COOxidation in the Presence of NH_32007

    • Author(s)
      Hidenobu Wakita, Kunihiro Ukai, Tatsuya Takeguchi, and Wataru Ueda
    • Journal Title

      J. Phys. Chem. C 111, No.5

      Pages: 2205-2211

    • Related Report
      2008 Final Research Report
    • Peer Reviewed
  • [Journal Article] Preparation and Characterization of CO-Tolerant Pt and Pd Anodes Modified with SnO_2 Nanoparticles for PEFC2007

    • Author(s)
      Tatsuya Takeguchi,
    • Journal Title

      J. Electrochem. Soc. 154

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Adsorbed Species on CO Preferential Oxidation in the Presence of H2Sover Ru/Al_2O_3 Catalyst2007

    • Author(s)
      Hidenobu Wakita
    • Journal Title

      Stud. Surf. Sci. Catal. 172

      Pages: 587-588

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Mechanistic Investigation of Deactivation of Ru/Al_2O_3 Catalyst for Preferential CO Oxidation in the Presence of NH_32007

    • Author(s)
      Hidenobu Wakita
    • Journal Title

      J. Phys. Chem. C 111

      Pages: 2205-2211

    • Related Report
      2006 Annual Research Report
  • [Journal Article] Synthesis of γ-Ga_2O_3-Al_2O_3 Solid Solutions by the Glycothermal Method2006

    • Author(s)
      Masaru Takahashi
    • Journal Title

      J. Am. Ceram. Soc. 89巻

      Pages: 2158-2166

    • Related Report
      2006 Annual Research Report
  • [Presentation] LaNi_xCo_<1-x>O_3ペロブスカイトの還元によるNi-Co合金の析出2007

    • Author(s)
      高橋弘樹、竹口竜弥、上田渉
    • Organizer
      SOFC研究会
    • Place of Presentation
      科学技術館
    • Year and Date
      2007-12-20
    • Related Report
      2008 Final Research Report
  • [Presentation] LaNi_xCo_<1-x>O_3ペロブスカイトの還元によるNi-Co合金の析出2007

    • Author(s)
      高橋弘樹
    • Organizer
      SOFC研究会
    • Place of Presentation
      科学技術館(東京)
    • Year and Date
      2007-12-20
    • Related Report
      2007 Annual Research Report
  • [Presentation] Reforming of Methane on the Ni/Sr (La) TiO_3 Cermet Catalyst and Reduction Behavior of the Catalyst2007

    • Author(s)
      Tatsuya Takeguchi, Norikazu, Yamamoto, and Wataru Ueda Steam
    • Organizer
      20th CRC International Symposium on In-situe Characterization of Catalyst-Presence and Future Aspects
    • Place of Presentation
      Research Center, Hokkaido University
    • Related Report
      2008 Final Research Report
  • [Presentation] Internal Reforming SOFC with the Ni Cermet Anode Prepared from Nanoparticle YSZ2007

    • Author(s)
      Tatsuya Takeguchi, Norikazu, Yamamoto, Wataru Ueda
    • Organizer
      Joint Symposium on Fundamental Aspects of Nanostructured Materials and Electrocatalysis
    • Place of Presentation
      Catalysis Research Center and Graduate School of Science, Hokkaido University
    • Related Report
      2008 Final Research Report

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Published: 2006-04-01   Modified: 2016-04-21  

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