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Development of apparatus for measuring field-angle-resolved entropy and its application to frustrated magnetic materials

Research Project

Project/Area Number 18H01161
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
Research InstitutionChuo University (2020)
The University of Tokyo (2018-2019)

Principal Investigator

Kittaka Shunichiro  中央大学, 理工学部, 准教授 (80579805)

Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥18,200,000 (Direct Cost: ¥14,000,000、Indirect Cost: ¥4,200,000)
Fiscal Year 2020: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2019: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2018: ¥15,340,000 (Direct Cost: ¥11,800,000、Indirect Cost: ¥3,540,000)
Keywordsエントロピー / 比熱 / 磁気熱量効果 / 磁場回転 / フラストレート磁性体 / スピンアイス / 磁場角度依存性
Outline of Final Research Achievements

We have developed an innovative experimental method to measure the field-angle dependence of the entropy by taking advantage of the field-rotational magnetocaloric effect. By using this technique, we made the field-angle-resolved entropy landscape and succeeded in detecting the well-known spin-flip transition in the spin-ice compound Dy2Ti2O7 under a rotating magnetic field within the (1-10) plane. We also studied the quasi-kagome Kondo lattice CeRhSn and revealed that the high-entropy state survives up to a relatively high magnetic field when the field is applied precisely along the quasi-kagome plane. Thus, we have established a new experimental technique which is useful to investigate various phenomena in anisotropic systems.

Academic Significance and Societal Importance of the Research Achievements

エントロピーは系の縮重度を反映する基礎的な熱力学量である。本研究では、準断熱環境下で磁場回転に伴う試料の温度変化を精密に測定できる装置を開発し、従来の手法に比べて高速かつ精密にエントロピーの磁場角度変化を調べることを可能にした。これにより、異方性の大きな系で発現する新奇物性機構に迫る新たな実験手法を確立することができた。本装置を用いればエントロピーの温度-磁場-磁場角度マップを作成することができ、特定の磁場方位で観測される新奇現象の探究と解明に取り組むことが可能である。実際に、フラストレート磁性体や多極子伝導系の研究に応用し、物性機構の解明に貢献した。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (45 results)

All 2021 2020 2019 2018 Other

All Int'l Joint Research (5 results) Journal Article (21 results) (of which Int'l Joint Research: 9 results,  Peer Reviewed: 21 results,  Open Access: 4 results) Presentation (16 results) (of which Int'l Joint Research: 8 results,  Invited: 6 results) Remarks (3 results)

  • [Int'l Joint Research] Southeast University/Zhejiang University of Technology(中国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] Max Planck Institute(ドイツ)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Max Planck Institute(ドイツ)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] University of Oxford/Durham University/University of Warwick(英国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Los Alamos National Laboratory/Florida State University/Eastern Washington University(米国)

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Field-angle-resolved Landscape of Non-Fermi-liquid Behavior in the Quasi-kagome Kondo Lattice CeRhSn2021

    • Author(s)
      Shunichiro Kittaka, Yohei Kono, Suguru Tsuda, Toshiro Takabatake, and Toshiro Sakakibara
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 90 Issue: 6 Pages: 064703-064703

    • DOI

      10.7566/jpsj.90.064703

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Orientation of point nodes and nonunitary triplet pairing tuned by the easy-axis magnetization in UTe22020

    • Author(s)
      Kittaka Shunichiro、Shimizu Yusei、Sakakibara Toshiro、Nakamura Ai、Li Dexin、Homma Yoshiya、Honda Fuminori、Aoki Dai、Machida Kazushige
    • Journal Title

      Physical Review Research

      Volume: 2 Issue: 3 Pages: 032014-032014

    • DOI

      10.1103/physrevresearch.2.032014

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Evidence for nematic superconductivity of topological surface states in PbTaSe22020

    • Author(s)
      Le Tian、Sun Yue、Jin Hui-Ke、Che Liqiang、Yin Lichang、Li Jie、Pang Guiming、Xu Chunqiang、Zhao Lingxiao、Kittaka Shunichiro、Sakakibara Toshiro、Machida Kazushige、Sankar Raman、Yuan Huiqiu、Chen Genfu、Xu Xiaofeng、Li Shiyan、Zhou Yi、Lu Xin
    • Journal Title

      Science Bulletin

      Volume: 65 Issue: 16 Pages: 1349-1355

    • DOI

      10.1016/j.scib.2020.04.039

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Fully gapped superconductivity without sign reversal in the topological superconductor PbTaSe22020

    • Author(s)
      Sun Yue、Kittaka Shunichiro、Sakakibara Toshiro、Machida Kazushige、Sankar R.、Xu Xiaofeng、Zhou Nan、Xing Xiangzhuo、Shi Zhixiang、Pyon Sunseng、Tamegai Tsuyoshi
    • Journal Title

      Physical Review B

      Volume: 102 Issue: 2 Pages: 024517-024517

    • DOI

      10.1103/physrevb.102.024517

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Kitaev Spin Liquid Candidate OsxCl3 Comprised of Honeycomb Nano-Domains2020

    • Author(s)
      Kota Kataoka, Daigoro Hirai, Takeshi Yajima, Daisuke Nishio-Hamane, Rieko Ishii, Kwang-Yong Choi, Dirk Wulferding, Peter Lemmens, Shunichiro Kittaka, Toshiro Sakakibara, Hajime Ishikawa, Akira Matsuo, Koichi Kindo, and Zenji Hiroi
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 89 Issue: 11 Pages: 1147091-9

    • DOI

      10.7566/jpsj.89.114709

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Field-Orientation Effect on Ferro-Quadrupole Order in PrTi2Al202020

    • Author(s)
      Kittaka Shunichiro、Taniguchi Takanori、Hattori Kazumasa、Nakamura Shota、Sakakibara Toshiro、Takigawa Masashi、Tsujimoto Masaki、Sakai Akito、Matsumoto Yosuke、Nakatsuji Satoru
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 89 Issue: 4 Pages: 043701-043701

    • DOI

      10.7566/jpsj.89.043701

    • NAID

      40022211746

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Magnetic properties of a spin-1/2 honeycomb lattice antiferromagnet2020

    • Author(s)
      Y. Kono, T. Okabe, N. Uemoto, Y. Iwasaki, Y. Hosokoshi, S. Kittaka, T. Sakakibara, and H. Yamaguchi
    • Journal Title

      Phys. Rev. B

      Volume: 101 Issue: 1 Pages: 014437-014437

    • DOI

      10.1103/physrevb.101.014437

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Heavy Fermion State of YbNi2Si3 without Local Inversion Symmetry2020

    • Author(s)
      Nakamura Shota、Hyodo Kazushi、Matsumoto Yuji、Haga Yoshinori、Sato Hitoshi、Ueda Shigenori、Mimura Kojiro、Saiki Katsuyoshi、Iso Kosei、Yamashita Minoru、Kittaka Shunichiro、Sakakibara Toshiro、Ohara Shigeo
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 89 Issue: 2 Pages: 024705-024705

    • DOI

      10.7566/jpsj.89.024705

    • NAID

      40022155106

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Emergent critical phenomenon in spin-1/2 ferromagnetic-leg ladders: Quasi-one-dimensional Bose-Einstein condensate2019

    • Author(s)
      Kono Y.、Kittaka S.、Yamaguchi H.、Hosokoshi Y.、Sakakibara T.
    • Journal Title

      Physical Review B

      Volume: 100 Issue: 5 Pages: 05442-05442

    • DOI

      10.1103/physrevb.100.054442

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fluctuation-Induced First-Order Transition and Tricritical Point in EuPtSi2019

    • Author(s)
      Sakakibara Toshiro、Nakamura Shota、Kittaka Shunichiro、Kakihana Masashi、Hedo Masato、Nakama Takao、Onuki Yoshichika
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 88 Issue: 9 Pages: 093701-093701

    • DOI

      10.7566/jpsj.88.093701

    • NAID

      40022008704

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Quasiparticle Evidence for the Nematic State above Tc in SrxBi2Se32019

    • Author(s)
      Yue Sun, Shunichiro Kittaka, Toshiro Sakakibara, Kazushige Machida, Jinghui Wang, Jinsheng Wen, Xiangzhuo Xing, Zhixiang Shi, and Tsuyoshi Tamegai
    • Journal Title

      Phys. Rev. Lett.

      Volume: 123 Issue: 2 Pages: 027002-027002

    • DOI

      10.1103/physrevlett.123.027002

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] S=1/2 ferromagnetic Heisenberg chain in a verdazyl-based complex2019

    • Author(s)
      Uemoto N.、Kono Y.、Kittaka S.、Sakakibara T.、Yajima T.、Iwasaki Y.、Miyamoto S.、Hosokoshi Y.、Yamaguchi H.
    • Journal Title

      Physical Review B

      Volume: 99 Issue: 9 Pages: 094418-094418

    • DOI

      10.1103/physrevb.99.094418

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Anisotropic magnetic-field response of quantum critical fluctuations in Ni-doped CeCoIn52019

    • Author(s)
      M. Yokoyama, K. Suzuki, K. Tenya, S. Nakamura, Y. Kono, S. Kittaka, and T. Sakakibara
    • Journal Title

      Physical Review B

      Volume: 99 Issue: 5

    • DOI

      10.1103/physrevb.99.054506

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Unconventional Field-Induced Spin Gap in an S=1/2 Chiral Staggered Chain2019

    • Author(s)
      Liu J.、Kittaka S.、Johnson R. D.、Lancaster T.、Singleton J.、Sakakibara T.、Kohama Y.、van Tol J.、Ardavan A.、Williams B. H.、Blundell S. J.、Manson Z. E.、Manson J. L.、Goddard P. A.
    • Journal Title

      Physical Review Letters

      Volume: 122 Issue: 5 Pages: 0572071-0572076

    • DOI

      10.1103/physrevlett.122.057207

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Field-induced quantum magnetism in the verdazyl-based charge-transfer salt [o-MePy-V-(p-Br)2]FeCl42018

    • Author(s)
      Iwasaki Y.、Kida T.、Hagiwara M.、Kawakami T.、Kono Y.、Kittaka S.、Sakakibara T.、Hosokoshi Y.、Yamaguchi H.
    • Journal Title

      Physical Review B

      Volume: 98 Issue: 22 Pages: 224411-224411

    • DOI

      10.1103/physrevb.98.224411

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Metamagnetic crossover in the quasikagome Ising Kondo-lattice compound CeIrSn2018

    • Author(s)
      S. Tsuda, C. L. Yang, Y. Shimura, K. Umeo, H. Fukuoka, Y. Yamane, T. Onimaru, T. Takabatake, N. Kikugawa, T. Terashima, H. T. Hirose, S. Uji, S. Kittaka, T. Sakakibara
    • Journal Title

      Phys. Rev B.

      Volume: 98 Issue: 15 Pages: 155147-155147

    • DOI

      10.1103/physrevb.98.155147

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Low-Temperature Magnetization Measurements with Precise Two-Axis Alignment of the Sample Orientation2018

    • Author(s)
      Nakamura Shota、Kasahara Akira、Kittaka Shunichiro、Kono Yohei、Onuki Yoshichika、Sakakibara Toshiro
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 87 Issue: 11 Pages: 114001-114001

    • DOI

      10.7566/jpsj.87.114001

    • NAID

      210000134999

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Field-enhanced quantum fluctuation in an S=1/2 frustrated square lattice2018

    • Author(s)
      Yamaguchi H.、Sasaki Y.、Okubo T.、Yoshida M.、Kida T.、Hagiwara M.、Kono Y.、Kittaka S.、Sakakibara T.、Takigawa M.、Iwasaki Y.、Hosokoshi Y.
    • Journal Title

      Physical Review B

      Volume: 98 Issue: 9 Pages: 094402-094402

    • DOI

      10.1103/physrevb.98.094402

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Disorder-sensitive nodelike small gap in FeSe2018

    • Author(s)
      Sun Yue、Kittaka Shunichiro、Nakamura Shota、Sakakibara Toshiro、Zhang Peng、Shin Shik、Irie Koki、Nomoto Takuya、Machida Kazushige、Chen Jingting、Tamegai Tsuyoshi
    • Journal Title

      Physical Review B

      Volume: 98 Issue: 6

    • DOI

      10.1103/physrevb.98.064505

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Searching for gap zeros in Sr2RuO4 via field-angle-dependent specific-heat measurement2018

    • Author(s)
      Shunichiro Kittaka, Shota Nakamura, Toshiro Sakakibara, Naoki Kikugawa, Taichi Terashima, Shinya Uji, Dmitry A. Sokolov, Andrew P. Mackenzie, Koki Irie, Yasumasa Tsutsumi, Katsuhiro Suzuki, and Kazushige Machida
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 87 Issue: 9 Pages: 0937031-5

    • DOI

      10.7566/jpsj.87.093703

    • NAID

      210000134938

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Field-rotational Magnetocaloric Effect: A New Experimental Technique for Accurate Measurement of the Anisotropic Magnetic Entropy2018

    • Author(s)
      Kittaka Shunichiro、Nakamura Shota、Kadowaki Hiroaki、Takatsu Hiroshi、Sakakibara Toshiro
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 87 Issue: 7 Pages: 073601-073601

    • DOI

      10.7566/jpsj.87.073601

    • NAID

      210000134879

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Presentation] (一般シンポジウム講演)角度回転比熱測定からの超伝導ギャップ構造2020

    • Author(s)
      橘高 俊一郎
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Superconducting gap structure of UTe2 studied from field-angle-resolved measurements of its specific heat2020

    • Author(s)
      S. Kittaka
    • Organizer
      UTe2 online workshop
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Sr2RuO4における超伝導多重相の検証2020

    • Author(s)
      橘高 俊一郎
    • Organizer
      J-Physics:多極子伝導系の物理 令和元年度領域全体会議
    • Related Report
      2019 Annual Research Report
  • [Presentation] 極低温精密比熱測定による超伝導ギャップ構造の決定2019

    • Author(s)
      橘高 俊一郎
    • Organizer
      第13回物性科学領域横断研究会 第14回「凝縮系科学賞」受賞講演
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Thermodynamic Evidence for Two Distinct Non-Fermi-Liquid Regimes and a Quantum Critical Line in the Quasi-Kagome Kondo-Lattice CeRhSn2019

    • Author(s)
      S. Kittaka, Y. Kono, S. Tsuda, T. Takabatake, and T. Sakakibara
    • Organizer
      International Conference on Strongly Correlated Electron Systems 2019 (SCES2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Thermodynamic study of the superconducting gap structure of Sr2RuO42019

    • Author(s)
      S. Kittaka
    • Organizer
      J-Physics 2019 International Conference
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 比熱の磁場角度依存性から見たCd2Re2O7の超伝導ギャップ構造とネマティック状態2019

    • Author(s)
      橘高 俊一郎、平井 大悟郎、廣井 善二、町田 一成、榊原 俊郎
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 磁場角度の効果から探るPrTi2Al20とPrIr2Zn20の多極子秩序相2019

    • Author(s)
      橘高 俊一郎
    • Organizer
      J-Physics地域研究会・本郷
    • Related Report
      2019 Annual Research Report
  • [Presentation] Thermodynamic study of the pairing symmetry in Sr2RuO42019

    • Author(s)
      S. Kittaka
    • Organizer
      Strontium Ruthenate - 25 years of a puzzling superconductor
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 擬カゴメ近藤格子CeRhSnにおける量子臨界性の磁場角度依存性2019

    • Author(s)
      橘高 俊一郎、河野 洋平、津田 研、高畠 敏郎、榊原 俊郎
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Field-orientation effect on the hidden-order transition in URu2Si22019

    • Author(s)
      S. Kittaka
    • Organizer
      Symposium:TPFC 2019
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Sr2RuO4の超伝導ギャップ構造の検証:回転磁場下での比熱測定から2019

    • Author(s)
      橘高 俊一郎、中村 翔太、榊原 俊郎、菊川 直樹、寺嶋 太一、宇治 進也、Dmitry A. Sokolov、Andrew P. Mackenzie、入江 光輝、堤 康雅、鈴木 雄大、町田 一成
    • Organizer
      つくば-柏-本郷 超伝導かけはしプロジェクト ワークショップ(2)
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Multiband full-gap superconductivity in heavy-fermion superconductor CeCu2Si2 revealed by specific-heat measurements2019

    • Author(s)
      S. Kittaka
    • Organizer
      Plasma 2019 Workshop
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Thermodynamic study of Sr2RuO4: identification of the superconducting gap structure2018

    • Author(s)
      S. Kittaka, S. Nakamura, T. Sakakibara, N. Kikugawa, T. Terashima, S. Uji, D. A. Sokolov, A. P. Mackenzie, K. Irie, Y. Tsutsumi, K. Suzuki, and K. Machida
    • Organizer
      International Workshop on j-Fermion Physics and Materials
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 磁場角度分解比熱・エントロピー測定からみたPrTi2Al20の四極子秩序2018

    • Author(s)
      橘高 俊一郎、谷口 貴紀、中村 翔太、榊原 俊郎、瀧川 仁、辻本 真規、酒井 明人、松本 洋介、中辻 知
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Towards identification of the superconducting gap structure of Sr2RuO4: evidence for a horizontal line node gap from field-angle dependence of its specific heat2018

    • Author(s)
      S. Kittaka, S. Nakamura, T. Sakakibara, N. Kikugawa, T. Terashima, S. Uji, D. A. Sokolov, A. P. Mackenzie, K. Irie, Y. Tsutsumi, K. Suzuki, and K. Machida
    • Organizer
      International Conference on Magnetism 2018 (ICM2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Remarks] 研究室のホームページ

    • URL

      https://www.phys.chuo-u.ac.jp/labs/kittaka/index.html

    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
  • [Remarks] 個人のホームページ

    • URL

      https://sakaki.issp.u-tokyo.ac.jp/user/kittaka/index.html

    • Related Report
      2018 Annual Research Report
  • [Remarks] 研究室のホームページ

    • URL

      https://sakaki.issp.u-tokyo.ac.jp/

    • Related Report
      2018 Annual Research Report

URL: 

Published: 2018-04-23   Modified: 2022-01-27  

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