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Itinerant and localized 5d multipoles in the pyrochlore oxides

Research Project

Project/Area Number 18H01169
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
Research InstitutionThe University of Tokyo

Principal Investigator

Hiroi Zenji  東京大学, 物性研究所, 教授 (30192719)

Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥17,940,000 (Direct Cost: ¥13,800,000、Indirect Cost: ¥4,140,000)
Fiscal Year 2020: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Fiscal Year 2019: ¥2,340,000 (Direct Cost: ¥1,800,000、Indirect Cost: ¥540,000)
Fiscal Year 2018: ¥13,000,000 (Direct Cost: ¥10,000,000、Indirect Cost: ¥3,000,000)
Keywordsスピン軌道結合金属 / スピン結合軌道金属 / 多極子秩序 / パイロクロア酸化物 / 空間反転対称性 / 超伝導
Outline of Final Research Achievements

Cd2Re2O7 is a candidate for the spin-orbit-coupled metal (SOCM). SOCM is a metallic system characterized by a centrosymmetric crystal structure and conduction electrons with strong spin-orbit interactions. It has a specific Fermi liquid instability that causes spontaneous inversion symmetry breaking leading to unusual odd-parity multipolar orders. We prepared single crystals with the (001) surface and applied anisotropic stress to control the tetragonal domains. Resistivity measurements using single-domain crystals revealed anisotropy in resistivity as large as 25%, which turned over at Ts2 = 120 K. The origin of the large anisotropy must be spin-dependent scattering in the spin-split Fermi surfaces of the odd parity multipolar orders, which carry important information on the characteristics of the SOCM.

Academic Significance and Societal Importance of the Research Achievements

金属状態を特徴付けるフェルミ面はさまざまなフェルミ液体不安定性を有し、電子系の相転移を誘起する。例えば、電子格子相互作用があれば、フェルミ面に超伝導ギャップが開いて超伝導状態となり、磁気的な不安定性は磁気秩序をもたらす。スピン軌道結合金属ではスピン軌道相互作用に基づく新規なフェルミ液体不安定性が奇パリティ多極子秩序を誘起すると予想されているが、その実験的検証は不十分である。本研究はCd2Re2O7がモデル物質であることを示し、スピン軌道結合金属が物性物理学の教科書に追記されるべき新たな概念であることを示した。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (27 results)

All 2021 2020 2019 2018

All Journal Article (9 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 9 results,  Open Access: 1 results) Presentation (18 results) (of which Int'l Joint Research: 1 results,  Invited: 1 results)

  • [Journal Article] Anomalous changes of electric quadrupole order at low temperatures in the spin-orbit coupled metal Cd2Re2O72020

    • Author(s)
      Uji S.、Sugiura S.、Hirose H. T.、Terashima T.、Matsubayashi Y.、Hirai D.、Hiroi Z.、Hasegawa T.
    • Journal Title

      Physical Review B

      Volume: 102 Issue: 15 Pages: 155131-155131

    • DOI

      10.1103/physrevb.102.155131

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Domain Control by Adjusting Anisotropic Stress in Pyrochlore Oxide Cd2Re2O72020

    • Author(s)
      Tajima Satoshi、Hirai Daigorou、Kinoshita Yuto、Tokunaga Masashi、Akiba Kazuto、Kobayashi Tatsuo C.、Hirose Hishiro T.、Hiroi Zenji
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 89 Issue: 11 Pages: 114711-114711

    • DOI

      10.7566/jpsj.89.114711

    • NAID

      210000158591

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Coexistence of odd-parity and even-parity order parameters in the multipole order phase of the spin-orbit coupled metal Cd2Re2O72020

    • Author(s)
      Matsubayashi Y.、Sugii K.、Hirai D.、Hiroi Z.、Hasegawa T.、Sugiura S.、Hirose H. T.、Terashima T.、Uji S.
    • Journal Title

      Physical Review B

      Volume: 101 Issue: 20 Pages: 205133-205133

    • DOI

      10.1103/physrevb.101.205133

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Variation in Superconducting Symmetry Against Pressure on Noncentrosymmetric Superconductor Cd2Re2O7 Revealed by 185/187Re Nuclear Quadrupole Resonance2020

    • Author(s)
      S. Kitagawa, K. Ishida, T. C. Kobayashi, Y. Matsubayashi, D. Hirai, Z. Hiroi
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 89 Issue: 5 Pages: 53701-53701

    • DOI

      10.7566/jpsj.89.053701

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin-orbit-coupled metal candidate PbRe2O62020

    • Author(s)
      Tajima Satoshi、Hirai Daigorou、Yajima Takeshi、Nishio-Hamane Daisuke、Matsubayashi Yasuhito、Hiroi Zenji
    • Journal Title

      Journal of Solid State Chemistry

      Volume: 288 Pages: 121359-121359

    • DOI

      10.1016/j.jssc.2020.121359

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Split Fermi Surface of the Spin Orbit Coupled Metal Cd2Re2O7 Probed by de Haas-van Alphen Effect2018

    • Author(s)
      Yasuhito Matsubayashi, Kaori Sugii, Hishiro T. Hirose, Daigorou Hirai, Shiori Sugiura, Taichi Terachima, Shinya Uji, Zenji Hiroi
    • Journal Title

      J. Phys. Soc. Jpn.

      Volume: 87 Issue: 5 Pages: 053702-053702

    • DOI

      10.7566/jpsj.87.053702

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Formation and Control of Twin Domains in the Pyrochlore Oxide Cd2Re2O72018

    • Author(s)
      Matsubayashi Yasuhito、Hirai Daigorou、Tokunaga Masashi、Hiroi Zenji
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 87 Issue: 10 Pages: 104604-104604

    • DOI

      10.7566/jpsj.87.104604

    • NAID

      210000134981

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] High-pressure Raman study on the superconducting pyrochlore oxide Cd2Re2O72018

    • Author(s)
      Y. Matsubayashi, T. Hasegawa, N. Ogita, J. Yamaura, Z. Hiroi,
    • Journal Title

      Physica B

      Volume: 536 Pages: 600-603

    • DOI

      10.1016/j.physb.2017.10.030

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Pyrochlore Oxide Superconductor Cd2Re2O7 Revisited2018

    • Author(s)
      Zenji Hiroi、Jun-ichi Yamaura、Tatsuo C. Kobayashi、 Yasuhito Matsubayashi、Daigorou Hirai
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 87 Issue: 2 Pages: 024702-024702

    • DOI

      10.7566/jpsj.87.024702

    • NAID

      210000134700

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] スピン軌道結合金属の相転移における構造変化2021

    • Author(s)
      福井敦仁, 平井大悟郎, 佐賀山基A, 広井善二
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Cd2Re2O7における奇パリティ多極子相の異方性について2020

    • Author(s)
      田島聖士, 平井大悟郎, 木下雄斗, 徳永将史, 秋葉和人A, 小林達生A, 廣瀬陽代B, ○広井善二
    • Organizer
      日本物理学会秋季大会2020
    • Related Report
      2020 Annual Research Report
  • [Presentation] パイロクロア酸化物Cd2Re2O7におけるII-III相転移の連続性2020

    • Author(s)
      長谷川巧, 広井善二A
    • Organizer
      日本物理学会秋季大会2020
    • Related Report
      2020 Annual Research Report
  • [Presentation] NMRから見た5d電子系Cd2Re2O7の相転移と秩序相2020

    • Author(s)
      瀧川仁, 武田晃, 平井大悟郎, 広井善二, 長谷川巧A
    • Organizer
      日本物理学会秋季大会2020
    • Related Report
      2020 Annual Research Report
  • [Presentation] Cd2Re2O7の磁場下熱膨張測定による格子歪みの観測2020

    • Author(s)
      金子佑真, 日高宏之, 村田怜也, 柳澤達也, 網塚浩, 田島聖士A, 平井大悟郎A, 廣井善二A
    • Organizer
      日本物理学会秋季大会2020
    • Related Report
      2020 Annual Research Report
  • [Presentation] スピン軌道結合金属Cd2Re2O7の構造相転移と弾性異常 (II)2020

    • Author(s)
      中村一翔, 工藤慎也, 川崎優介, 中村光輝, 吉澤正人, 中西良樹, 平井大悟郎A, 廣井善二A
    • Organizer
      日本物理学会秋季大会2020
    • Related Report
      2020 Annual Research Report
  • [Presentation] PbRe2O6におけるスピン軌道結合金属の可能性2019

    • Author(s)
      田島聖士, 平井大悟郎, 矢島健, 廣井善二
    • Organizer
      日本物理学会秋期大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Cd2Re2O7における電気トロイダル四極子秩序2019

    • Author(s)
      平井大悟郎, 田島聖士, 広井善二
    • Organizer
      日本物理学会秋期大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] スピン軌道結合金属パイロクロアCd2Re2O7における磁気トルク対称性2019

    • Author(s)
      宇治進也, 杉浦栞理, 廣瀬陽代, 寺嶋太一, 長谷川巧, 松林康仁, 平井大悟郎, 広井善二
    • Organizer
      日本物理学会秋期大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 比熱の磁場角度依存性から見たCd2Re2O7の超伝導ギャップ構造とネマティック状態2019

    • Author(s)
      橘高俊一郎, 平井大悟郎, 廣井善二, 町田一成, 榊原俊郎
    • Organizer
      日本物理学会秋期大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Cd2Re2O7における非相反磁気抵抗2019

    • Author(s)
      木俣基, 須藤健太, 平井大悟郎, 松林康仁, 広井善二
    • Organizer
      日本物理学会秋期大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Cd2Re2O7における高圧下ホール効果2019

    • Author(s)
      小林達生, 池山由十, 三井理功, 秋葉和人, 荒木新吾, 山浦淳一, 松林康仁, 廣井善二
    • Organizer
      日本物理学会秋期大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Cd2Re2O7における高圧相のRe-NQR2019

    • Author(s)
      北川俊作, 石田憲二, 松林康仁, 廣井善二
    • Organizer
      日本物理学会秋期大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] パイロクロア酸化物Cd2Re2O7のNMR2019

    • Author(s)
      米良伸義, 武田晃, 瀧川仁, 松林康仁, 平井大悟郎, 広井善二, 長谷川巧
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] パイロクロア酸化物Cd2Re2O7の一軸圧によるドメイン制御2019

    • Author(s)
      田島聖士, 平井大悟郎, 木下雄斗, 徳永将史, 広井善二
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] パイロクロアCd2Re2O7における低温磁気トルク測定2019

    • Author(s)
      宇治進也, 杉浦栞理, 廣瀬陽代, 寺嶋太一, 長谷川巧, 松林康仁, 平井大悟郎, 広井善二
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Cd2Re2O7の高圧ラマン散乱2018

    • Author(s)
      長谷川巧, 松林康仁, 荻田典男, 山浦淳一, 広井善二
    • Organizer
      日本物理学会秋期大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Itinerant multipole orders in the spin-orbit coupled metal Cd2Re2O72018

    • Author(s)
      Z. Hiroi
    • Organizer
      Frustration, Orbital Fluctuations, and Topology in Kondo Lattices and their relatives
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited

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Published: 2018-04-23   Modified: 2022-01-27  

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