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Supersolidity and the quantum spin liquid state in monolayer of helium

Research Project

Project/Area Number 18H01170
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
Research InstitutionThe University of Tokyo

Principal Investigator

FUKUYAMA Hiroshi  東京大学, 低温科学研究センター, 特任研究員 (00181298)

Co-Investigator(Kenkyū-buntansha) 村川 智  東京大学, 低温科学研究センター, 准教授 (90432004)
Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥16,900,000 (Direct Cost: ¥13,000,000、Indirect Cost: ¥3,900,000)
Fiscal Year 2020: ¥3,380,000 (Direct Cost: ¥2,600,000、Indirect Cost: ¥780,000)
Fiscal Year 2019: ¥5,330,000 (Direct Cost: ¥4,100,000、Indirect Cost: ¥1,230,000)
Fiscal Year 2018: ¥8,190,000 (Direct Cost: ¥6,300,000、Indirect Cost: ¥1,890,000)
Keywords量子液晶 / 超固体 / スピン液体 / 単原子層 / 量子スピン液体 / 超個体
Outline of Final Research Achievements

At low temperatures, helium atoms form a monatomic adsorbed layer on a crystalline graphite surface, where atomic motions are restricted to two dimensions (2D). In this 2D quantum system, the novel quantum liquid-crystal (QLC) phase with finite fluidity even at absolute zero is expected to emerge as an intermediate phase between the quantum liquid and solid phases. In this study, by performing simultaneous measurements of mechanical response of the adsorbed helium-4 film under substrate oscillation and specific heat of the film, we have succeeded in observing an anomalous superfluid state, which strongly supports the QLC hypothesis. In addition, we have shown that the novel quantum spin-liquid magnetism observed in the adsorbed film of helium-3, an isotope of helium-4, can be explained by assuming the QLC structure behind. A preliminary but encouraging result of synchrotron radiation X-ray diffraction experiment aiming for structural identification of the QLC phase was also obtained.

Academic Significance and Societal Importance of the Research Achievements

物質が取り得る状態(相)には気体、液体、固体、液晶、アモルファスの5態ある。ヘリウム原子からなる物質系の場合、量子力学効果が顕在化する絶対零度では液体と固体のみが存在し(それぞれ量子固体と量子液体)、後者は粘性のない超流動状態となる。本研究では、表面吸着したヘリウム単原子層膜に「量子液晶」という物質の新たな状態とその超流動相が存在することを強く示唆する結果が得られた。これは人類の自然界の理解をより豊かなものとし、量子計算機の原理である量子もつれと深く関係する「量子スピン液体」磁性など他分野への波及効果もある。高輝度放射光を利用した極低温研究という新分野にも先鞭をつけることができた。

Report

(4 results)
  • 2021 Final Research Report ( PDF )
  • 2020 Annual Research Report
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (50 results)

All 2022 2021 2020 2019 2018 Other

All Journal Article (11 results) (of which Peer Reviewed: 11 results,  Open Access: 3 results) Presentation (36 results) (of which Int'l Joint Research: 12 results,  Invited: 4 results) Remarks (1 results) Patent(Industrial Property Rights) (2 results)

  • [Journal Article] Structural Study of Adsorbed Helium Films: New Approach with Synchrotron Radiation X-rays2022

    • Author(s)
      Yamaguchi Akira、Tajiri Hiroo、Kumashita Atsuki、Usami Jun、Yamane Yu、Sumiyama Akihiko、Suzuki Masaru、Minoguchi Tomoki、Sakurai Yoshiharu、Fukuyama Hiroshi
    • Journal Title

      Journal of Low Temperature Physics

      Volume: online Issue: 5-6 Pages: 1-8

    • DOI

      10.1007/s10909-021-02652-1

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Superconducting Niobium Calorimeter for Studies of Adsorbed Helium Monolayers2021

    • Author(s)
      Usami Jun、Tokeshi Koki、Matsui Tomohiro、Fukuyama Hiroshi
    • Journal Title

      Journal of Low Temperature Physics

      Volume: 203 Issue: 1-2 Pages: 1-10

    • DOI

      10.1007/s10909-020-02558-4

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Negative resistance state in superconducting NbSe 2 induced by surface acoustic waves2020

    • Author(s)
      Masahiko Yokoi, Satoshi Fujiwara, Tomoya Kawamura, Tomonori Arakawa, Kazushi Aoyama, Hiroshi Fukuyama, Kensuke Kobayashi, and Yasuhiro Niimi
    • Journal Title

      Science Advances

      Volume: 6 Issue: 34 Pages: 1-5

    • DOI

      10.1126/sciadv.aba1377

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Performances of a Compact Shielded Superconducting Magnet for Continuous Nuclear Demagnetization Refrigerator2020

    • Author(s)
      Takimoto S.、Toda R.、Murakawa S.、Fukuyama Hiroshi
    • Journal Title

      Journal of Low Temperature Physics

      Volume: - Issue: 1-2 Pages: 179-186

    • DOI

      10.1007/s10909-019-02331-2

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] STM/S observations of graphene on SiC(0001) etched by H-plasma2019

    • Author(s)
      Amend Andre E. B.、Matsui Tomohiro、Hibino Hiroki、Fukuyama Hiroshi
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 58 Issue: SI Pages: SIIA13-SIIA13

    • DOI

      10.7567/1347-4065/ab1b5d

    • NAID

      210000156641

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Hexagonal Nanopits with the Zigzag Edge State on Graphite Surfaces Synthesized by Hydrogen-Plasma Etching2019

    • Author(s)
      Matsui Tomohiro、Sato Hideki、Kita Kazuma、Amend Andre E. B.、Fukuyama Hiroshi
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 123 Issue: 36 Pages: 22665-22673

    • DOI

      10.1021/acs.jpcc.9b06885

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Preface: International Symposium on Quantum Fluids and Solids (QFS2018)2019

    • Author(s)
      Fukuyama Hiroshi、Tsubota Makoto、Takagi Takeo、Choi Hyoungsoon
    • Journal Title

      Journal of Low Temperature Physics

      Volume: 196 Issue: 1-2 Pages: 4-5

    • DOI

      10.1007/s10909-019-02204-8

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] The Role of Substrate Roughness in Superfluid Film Flow Velocity2019

    • Author(s)
      Usami Jun、Kato Nobuyuki、Matsui Tomohiro、Fukuyama Hiroshi
    • Journal Title

      Journal of Low Temperature Physics

      Volume: 印刷中 Issue: 1-2 Pages: 52-59

    • DOI

      10.1007/s10909-018-02119-w

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] STS Studies of Zigzag Graphene Edges Produced by Hydrogen-Plasma Etching2018

    • Author(s)
      Andre E. B. Amend, Tomohiro Matsui, Hideki Sato, Hiroshi Fukuyama
    • Journal Title

      e-Journal of Surface Science and Nanotechnology

      Volume: 16 Issue: 0 Pages: 72-75

    • DOI

      10.1380/ejssnt.2018.72

    • NAID

      130006697170

    • ISSN
      1348-0391
    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Characterization of Pyrolytic Graphite Sheet: A New Type of Adsorption Substrate for Studies of Superfluid Thin Films2018

    • Author(s)
      Nakamura Sachiko、Miyafuji Daisuke、Toda Ryo、Matsui Tomohiro、Fukuyama Hiroshi
    • Journal Title

      Journal of Low Temperature Physics

      Volume: 192 Issue: 5-6 Pages: 330-345

    • DOI

      10.1007/s10909-018-1983-3

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Specific heat, thermal conductivity, and magnetic susceptibility of cyanate ester resins ? An alternative to commonly used epoxy resins2018

    • Author(s)
      Nakamura Sachiko、Fujii Takenori、Matsukawa Shoji、Katagiri Masayuki、Fukuyama Hiroshi
    • Journal Title

      Cryogenics

      Volume: 95 Pages: 76-81

    • DOI

      10.1016/j.cryogenics.2018.09.001

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] 放射光X線散乱による超低温表面の観察手法開発2022

    • Author(s)
      田尻寛男, 山口明, 隈下敦貴, 宇佐美潤, 山根悠, 住山昭彦, 鈴木勝, 蓑口友紀, 福山寛, 櫻井吉晴
    • Organizer
      第35回日本放射光学会年会・放射光科学合同シンポジウム
    • Related Report
      2020 Annual Research Report
  • [Presentation] グラファイト上4He原子層の放射光表面X線回折2022

    • Author(s)
      隈下敦貴, 田尻寛男, 山口明, 宇佐美潤, 住山昭彦, 山根悠, 簑口友紀, 鈴木勝, 櫻井吉晴, 福山寛
    • Organizer
      日本物理学会第77回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Possible coexistence of Superfluidity and Spatial Order in Monolayers of Helium-42021

    • Author(s)
      J. Usami, R. Toda, and Hiroshi Fukuyama
    • Organizer
      APS March Meeting 2021
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Superfluidity Found in the Possible Liquid Crystal Phase of 2D 4He2021

    • Author(s)
      J. Usami, R. Toda, S. Murakawa, and H. Fukuyama
    • Organizer
      International Symposium on Quantum Fluids and Solids (QFS2021)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Pyrolytic graphite for synchrotron X-ray diffraction of two-dimensional helium films2021

    • Author(s)
      A. Kumashita, H. Tajiri, A. Yamaguchi, J. Usami, Y. Yamane, A. Sumiyama, T. Minoguchi, M. Suzuki, Y. Sakurai, and H. Fukuyama
    • Organizer
      International Symposium on Quantum Fluids and Solids (QFS2021)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of a Superconducting Zinc Heat Switch for the Continuous Nuclear Demagnetization Refrigerator2021

    • Author(s)
      R. Toda, S. Takimoto, S. Murakawa, and Hiroshi Fukuyama
    • Organizer
      International Symposium on Quantum Fluids and Solids (QFS2021)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Construction of Continuous Magnetic Cooling Apparatus with Zinc Soldered PrNi5 Nuclear Stages2021

    • Author(s)
      S. Takimoto, R. Toda, S. Murakawa, and Hiroshi Fukuyama
    • Organizer
      International Symposium on Quantum Fluids and Solids (QFS2021)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Structural study of adsorbed helium films: New approach with synchrotron radiation X-rays2021

    • Author(s)
      A. Yamaguchi, H. Tajiri, A. Kumashita, J. Usami, Y. Yamane, A. Sumiyama, M. Suzuki, T. Minoguchi, Y. Sakurai, and H. Fukuyama
    • Organizer
      International Symposium on Quantum Fluids and Solids (QFS2021)
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] グラフェンアンチドット格子における弱局在効果の変調2021

    • Author(s)
      大星和毅、花田尚輝、岩切秀一、松井朋裕、福山寛、小林研介、新見康洋
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 単原子層ヘリウム4における超流動と空間対称性の破れの共存2021

    • Author(s)
      宇佐美潤、戸田亮、村川智、福山寛
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 表面吸着He層の観測に向けた放射光X線回折用冷凍機の製作2021

    • Author(s)
      11.隈下敦貴、山口明、田尻寛男、山根悠、住山昭彦、簑口友紀、鈴木勝、福山寛、櫻井吉晴
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] SiC 基板上のCa インターカレートグラフェンにおける超伝導2021

    • Author(s)
      遠山晴子,秋山了太,橋爪瑞葵,一ノ倉聖,飯盛拓嗣,松井朋裕,堀井健太郎, 佐藤瞬亮,保原麗,遠藤由大,福山寛,平原徹,小森文夫,長谷川修司
    • Organizer
      日本物理学会2021年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] He吸着層観察のための新規グラファイト基板の放射光による構造評価2021

    • Author(s)
      隈下敦貴, 田尻寛男, 山口明, 宇佐美潤, 住山昭彦, 山根悠, 簑口友紀,鈴木勝, 櫻井吉晴, 福山寛
    • Organizer
      日本物理学会2021年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 単原子層ヘリウム4における超流動と空間対称性の破れの共存2020

    • Author(s)
      宇佐美潤、戸田亮、村川智、福山寛
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 亜鉛はんだを用いたPrNi5核ステージの性能評価2020

    • Author(s)
      瀧本翔平、戸田亮、村川智、福山寛
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] エッチンググラフェンのおける弱局在効果の増幅2020

    • Author(s)
      花田尚輝、岩切秀一、浅野拓也、松井朋裕、福山寛、小林研介、新見康洋
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 表面弾性波照射により生じる超伝導NbSe2 薄膜の負抵抗状態の起源2020

    • Author(s)
      横井雅彦、藤原聖士、河村智哉、荒川智紀、青山和司、 福山寛、小林研介、新見康洋
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] ジグザグ端グラフェンの作製及び輸送測定の試み2020

    • Author(s)
      花田尚輝、浅野拓也、鈴木将太、松井朋裕、福山寛、 小林研介、新見康洋
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 小型連続核断熱消磁冷凍機用超伝導熱スイッチの開発2020

    • Author(s)
      戸田亮、瀧本翔平、村川智、福山寛
    • Organizer
      日本物理学会第 75回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 亜鉛はんだを用いたPrNi5 核ステージの製作2020

    • Author(s)
      瀧本翔平、戸田亮、村川智、福山寛
    • Organizer
      日本物理学会第75回 年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] グラファイト上単原子層ヘリウム4 の超流動相図2020

    • Author(s)
      宇佐美潤、戸田亮、松井朋裕、福山寛
    • Organizer
      日本物理学会第75 回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] STM/S study of epitaxial graphene on SiC(000-1) etched by H-plasma2020

    • Author(s)
      Andre E. B. Amend、Tomohiro Matsui、Hiroshi Fukuyama
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Simultaneous Measurements of Superfluidity and Heat-capacities of Novel Phases in 4He Monolayers2019

    • Author(s)
      J. Usami, R. Toda, S. Nakamura, T. Matsui, and Hiroshi Fukuyama
    • Organizer
      International Symposium on Quantum Fluids and Solids (QFS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Performances of a Compact Shielded Superconducting Magnet for Continuous Nuclear Demagnetization Refrigerator2019

    • Author(s)
      S. Takimoto, R. Toda, S. Murakawa, and Hiroshi Fukuyama
    • Organizer
      International Symposium on Quantum Fluids and Solids (QFS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Substrate Corrugation Effects on Self-Binding of 3He in Two Dimensions2019

    • Author(s)
      M. Kamada, K. Ogawa, R. Nakamura, T. Matsui, and Hiroshi Fukuyama
    • Organizer
      International Symposium on Quantum Fluids and Solids (QFS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Niobium Calorimeter for Studies of Adsorbed Helium Monolayers2019

    • Author(s)
      J. Usami, K. Tokeshi, T. Matsui, and Hiroshi Fukuyama
    • Organizer
      International Symposium on Quantum Fluids and Solids (QFS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] グラフェンナノリボンを用いたスピン輸送測定の試み2019

    • Author(s)
      花田尚輝、松井朋裕、鈴木将太、井邊昂志、谷口祐紀、 福山寛、小林研介、新見康洋
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 2 次元ヘリウム4 における比熱と非古典的回転慣性の同時測定III2019

    • Author(s)
      宇佐美潤、戸田亮、松井朋裕、福山寛
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] ヘリウム吸着膜研究のための超伝導ニオブ製熱容量測定セルの開発2019

    • Author(s)
      宇佐美潤、渡慶次孝気、松井朋裕、福山寛
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] グラフェン・ナノリボンにおけるスピン偏極ジグザグ端状態のSTM/S 観測2019

    • Author(s)
      松井朋裕、Andre E. B. Amend、福山寛
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] New Quantum Spin Liquids in 3He Monolayer on Hydrogen Plated Graphite2018

    • Author(s)
      Masahiro Kamada, Ryuji Nakamura, Katsuyoshi Ogawa, Tomohiro Matsui, and Hiroshi Fukuyama
    • Organizer
      International Sympo- sium on Quantum Fluids and Solids (QFS2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Novel quantum phases of helium confined in two dimensions from quantum liquid-crystal to spin-liquid2018

    • Author(s)
      Hiroshi Fukuyama
    • Organizer
      12th International Conference on Cryocrystals and Quantum Crystals
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 単原子層ヘリウム3で見つかった2種類の量子スピン液体状態2018

    • Author(s)
      福山寛
    • Organizer
      日本物理学会第74 回年次大会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 2次元ヘリウム4における比熱と非古典的回転慣性の 同時測定2018

    • Author(s)
      宇佐美潤、戸田亮、中村祥子、松井朋裕、福山寛
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 単原子層ヘリウム3 の量子液晶相と量子スピ ン液体状態2018

    • Author(s)
      福山寛
    • Organizer
      物性研究所短期研究会「量子多体効果が生み出す液晶的電子状態」
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 2次元ヘリウム4における比熱と非古典回転慣性の同 時測定II2018

    • Author(s)
      宇佐美潤、戸田亮、中村祥子、松井朋裕、福山寛
    • Organizer
      日本物理学会第74 回年次大会
    • Related Report
      2018 Annual Research Report
  • [Remarks] http://kelvin.phys.s.u-tokyo.ac.jp/

    • Related Report
      2019 Annual Research Report
  • [Patent(Industrial Property Rights)] ヘリウムコンテナ2021

    • Inventor(s)
      福山寛
    • Industrial Property Rights Holder
      福山寛
    • Industrial Property Rights Type
      特許
    • Filing Date
      2021
    • Related Report
      2020 Annual Research Report
  • [Patent(Industrial Property Rights)] ヘリウム回収装置およびヘリウム回収方法2020

    • Inventor(s)
      福山寛、大越慎一
    • Industrial Property Rights Holder
      福山寛、大越慎一
    • Industrial Property Rights Type
      特許
    • Filing Date
      2020
    • Related Report
      2020 Annual Research Report

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Published: 2018-04-23   Modified: 2023-01-30  

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