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Spin liquid phase emerging from competing interaction

Research Project

Project/Area Number 18H01173
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
Research InstitutionNagoya University

Principal Investigator

Terasaki Ichiro  名古屋大学, 理学研究科, 教授 (30227508)

Co-Investigator(Kenkyū-buntansha) 堀田 知佐  東京大学, 大学院総合文化研究科, 准教授 (50372909)
安井 幸夫  明治大学, 理工学部, 専任教授 (80345850)
Project Period (FY) 2018-04-01 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥17,160,000 (Direct Cost: ¥13,200,000、Indirect Cost: ¥3,960,000)
Fiscal Year 2021: ¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2020: ¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2019: ¥4,160,000 (Direct Cost: ¥3,200,000、Indirect Cost: ¥960,000)
Fiscal Year 2018: ¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Keywordsスピン液体 / 相互作用の競合 / 二量体格子 / 不純物効果
Outline of Final Research Achievements

The principal investigator discovered that Ba3ZnRu2O9 was a spin-liquid candidate. In the present project, we have investigated this spin-liquid-like state both experimentally and theoretically. Experimentally, we have found a tiny anomaly in the specific heat near 100 K accompanied by subtle magnetic reflections in the neutron diffraction. This indicates faint magnetic order below 100 K. We have further found through muSR that this order coexists with liquid-like fluctuating spins. In this respect, this magnetic ground state is quite unique. From a theoretical aspect, we have clarified that this unique magnetic state is theoretically plausible by studying a two-dimensional antiferromagnetic dimer triangular lattice. Moreover, we have discovered a new state of weak ferromagnetism in the Nb substituted samples.

Academic Significance and Societal Importance of the Research Achievements

磁性体の研究は物性物理学の王道である。我が国においては本多光太郎先生以来の長い伝統を持ち、世界的にも優れた成果を発信している分野である。本研究はその伝統に連なるものであり、磁性の源となるスピンがペアで3次元格子を作ったとき、どのような磁性が生じるかを実験的・理論的に明らかにした。本研究を通じて我々が見出した状態は、液体のように揺らぐスピンと、きちんと向きが固まって固体のように振る舞うスピンが共存した状態である。これはこれまでに知られていない新しい磁気基底状態であり、磁気物理、統計物理、固体量子論の進展に貢献できる成果である。さらに、乱れを導入することで、弱い強磁性相が生じることも発見した。

Report

(5 results)
  • 2021 Annual Research Report   Final Research Report ( PDF )
  • 2020 Annual Research Report
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (27 results)

All 2022 2021 2020 2019 2018 Other

All Int'l Joint Research (2 results) Journal Article (9 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 9 results,  Open Access: 1 results) Presentation (16 results) (of which Int'l Joint Research: 4 results,  Invited: 4 results)

  • [Int'l Joint Research] University of Edinburgh(英国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] Aalto University(フィンランド)

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Nontrivial Spin Dimer in the Hexagonal Ruthenate Ba3CaRu2O9 Revealed by Nonmagnetic Ion Substitution2021

    • Author(s)
      Nishihara Daiki、Kimura Akinori、Nakano Akitoshi、Taniguchi Hiroki、Terasaki Ichiro
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 90 Issue: 11 Pages: 114706-114706

    • DOI

      10.7566/jpsj.90.114706

    • NAID

      210000159422

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dimensional reduction in quantum spin-1/2 system on a 1/7-depleted triangular lattice2021

    • Author(s)
      Makuta Ryo、Hotta Chisa
    • Journal Title

      Physical Review B

      Volume: 104 Issue: 22 Pages: 224415-224415

    • DOI

      10.1103/physrevb.104.224415

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Sine-square deformation applied to classical Ising models2021

    • Author(s)
      Hotta Chisa、Nakamaniwa Takashi、Nakamura Tota
    • Journal Title

      Physical Review E

      Volume: 104 Issue: 3 Pages: 034133-034133

    • DOI

      10.1103/physreve.104.034133

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Finite temperature thermodynamic properties of the spin-1 nematics in an applied magnetic field2020

    • Author(s)
      Katsuhiro Tanaka, Chisa Hotta
    • Journal Title

      Phys. Rev. B

      Volume: 102 Issue: 14 Pages: 140401-140401

    • DOI

      10.1103/physrevb.102.140401

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Comparative study of the density matrix embedding theory for the Hubbard models2020

    • Author(s)
      Masataka Kawano, Chisa Hotta
    • Journal Title

      Phys. Rev. B

      Volume: 102 Issue: 23 Pages: 235111-235111

    • DOI

      10.1103/physrevb.102.235111

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Entanglement spectrum as a marker for phase transitions in the density embedding theory for interacting spinless fermionic models2020

    • Author(s)
      Xavier Plat, Chisa Hotta
    • Journal Title

      Phys. Rev. B

      Volume: 102 Issue: 14 Pages: 140410-140410

    • DOI

      10.1103/physrevb.102.140410

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Multiple quadrupolar or nematic phases driven by the Heisenberg interactions in a spin-1 dimer system forming a bilayer2020

    • Author(s)
      Tanaka Katsuhiro、Hotta Chisa
    • Journal Title

      Physical Review B

      Volume: 101 Issue: 9 Pages: 094422-094422

    • DOI

      10.1103/physrevb.101.094422

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dynamical coupling of dilute magnetic impurities with quantum spin liquid state in the S=3/2 dimer compound Ba3ZnRu2O92018

    • Author(s)
      Yamamoto Takafumi D、Taniguchi Hiroki、Terasaki Ichiro
    • Journal Title

      Journal of Physics: Condensed Matter

      Volume: 30 Issue: 35 Pages: 3558011-6

    • DOI

      10.1088/1361-648x/aad5ac

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin nematics next to spin singlets2018

    • Author(s)
      Yuto Yokoyama, Chisa Hotta
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 18

    • DOI

      10.1103/physrevb.97.180404

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] 固体結晶中の電荷やスピンの量子グラス2022

    • Author(s)
      堀田知佐
    • Organizer
      日本物理学会第77回年次大会
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] Non-equilibrium steady state in the electrical and thermal transport in the Mott insulator Ca2RuO42021

    • Author(s)
      I. Terasaki
    • Organizer
      Oxide Superspin 2021
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Perfect flat band and trimerized charge ordering out of strong spin-orbit interaction2021

    • Author(s)
      Chisa Hotta
    • Organizer
      IBS Workshop
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] スピンギャップ系Ru酸化物Ba3CaRu2O9における非磁性元素置換効果2021

    • Author(s)
      西原大貴、木村晃典、中埜彰俊、谷口博基、寺崎一郎
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] スピン液体候補物質Ba3ZnRu2O9における非磁性元素置換による強磁性の発現2021

    • Author(s)
      木村晃典、安井幸夫、中埜彰俊、谷口博基、寺崎一郎
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] ダイマー基底によるスピンネマティック相の記述と 2 マグノン束縛状態2021

    • Author(s)
      田中克大, 戸塚圭介, 堀田知佐
    • Organizer
      日本物理学会第76回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] S=3/2ダイマー反強磁性体Ba3Ca1-xZnxRu2O9の磁気励起2020

    • Author(s)
      浅井晋一郎, 木村晃典, 山本貴史, 中埜彰俊, 谷口博基, 寺崎一郎, 益田隆嗣
    • Organizer
      日本物理学会 2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] ダイマー反強磁性体Ba3Cu1-xZnxRu2O9のスピンダイナミクス2020

    • Author(s)
      浅井晋一郎、木村晃典、山本貴史、 中埜彰俊、谷口博基、寺崎一郎、益田隆嗣
    • Organizer
      日本中性子科学会 第20回年会
    • Related Report
      2020 Annual Research Report
  • [Presentation] スピン 1 ネマティック相の熱力学量に対する外部磁場の効果2020

    • Author(s)
      田中克大, 堀田知佐
    • Organizer
      日本物理学会 2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] スピン 1 ダイマー三角格子におけるスピンネマティック相2020

    • Author(s)
      田中克大, 堀田知佐
    • Organizer
      日本物理学会2020年年次大会、名古屋大学
    • Related Report
      2019 Annual Research Report
  • [Presentation] S=3/2ダイマー反強磁性体Ba3Ca1-xZnxRu2O9の中性子非弾性散乱2020

    • Author(s)
      浅井晋一郎、木村晃典、山本貴史、中埜昭俊、谷口博基、寺崎一郎、増田隆嗣
    • Organizer
      日本物理学会2020年年次大会、名古屋大学
    • Related Report
      2019 Annual Research Report
  • [Presentation] Magnetic properties of Ba3Co1-xCaxRu2O92019

    • Author(s)
      A. Nagaya, A. Horie, Y. Yasui, T. D. Yamamoto, I. Terasaki
    • Organizer
      Annual Conference on Magnetism and Magnetic Materials, Las Vegas, USA
    • Related Report
      2019 Annual Research Report
  • [Presentation] スピン液体候補物質Ba3ZnRu2O9における置換効果2019

    • Author(s)
      木村晃典, 安井幸夫, 中埜彰俊, 谷口博基, 寺崎一郎
    • Organizer
      日本物理学会 2019年秋季大会 岐阜大学
    • Related Report
      2019 Annual Research Report
  • [Presentation] 量子スピン液体候補物質Ba3ZnRu2O9における磁性不純物に対する量子ゆらぎの効果2018

    • Author(s)
      山本貴史, 谷口博基, 寺崎一郎
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Dilute Magnetic Impurity Effect on a Quantum Spin Liquid Candidate Ba3ZnRu2O9 with S = 3/2 Dimer Lattice2018

    • Author(s)
      T. D. Yamamoto, H. Taniguchi and I. Terasaki
    • Organizer
      International Conference on Magnetism (ICM2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Thermodynamic properties of quantum spin systems2018

    • Author(s)
      Chisa Hotta
    • Organizer
      WE-Heraeus-Seminar on TRENDS IN QUANTUM MAGNETISM
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited

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Published: 2018-04-23   Modified: 2023-01-30  

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