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Superconducting mechanism and quantum phase transitions on S-doped FeSe studied via NMR under high pressure

Research Project

Project/Area Number 18H01181
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 13030:Magnetism, superconductivity and strongly correlated systems-related
Research InstitutionKyoto University

Principal Investigator

Fujiwara Naoki  京都大学, 人間・環境学研究科, 准教授 (60272530)

Co-Investigator(Kenkyū-buntansha) 上床 美也  東京大学, 物性研究所, 教授 (40213524)
Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥17,940,000 (Direct Cost: ¥13,800,000、Indirect Cost: ¥4,140,000)
Fiscal Year 2020: ¥2,470,000 (Direct Cost: ¥1,900,000、Indirect Cost: ¥570,000)
Fiscal Year 2019: ¥2,210,000 (Direct Cost: ¥1,700,000、Indirect Cost: ¥510,000)
Fiscal Year 2018: ¥13,260,000 (Direct Cost: ¥10,200,000、Indirect Cost: ¥3,060,000)
Keywords鉄系超伝導体 / 強相関電子系 / 核磁気共鳴 / 高圧下測定 / 量子相転移 / 量子臨界現象 / 高温超伝導 / 鉄系超伝導
Outline of Final Research Achievements

FeSe is a unique high-Tc iron-based superconductor in which nematicity, superconductivity,and magnetism are entangled with each other in the P-T phase diagram. We performed 77Se-nuclear magnetic resonance measurements under pressures of up to 3.9 GPa on 12% S-substituted FeSe, in which the complex overlap between the nematicity and magnetism are resolved. A pressure-induced Lifshitz transition was observed at 1.0 GPa as an anomaly of the density of states and as double superconducting (SC)domes accompanied by different types of antiferromagnetic (AF) fluctuations. The low-Tc SC dome below 1 GPa is accompanied by strong AF fluctuations, whereas the high-Tc SC dome develops above 1 GPa, where AF fluctuations are fairly weak. These results suggest the importance of the dxy orbital and its intra-orbital coupling for the high-Tc superconductivity.

Academic Significance and Societal Importance of the Research Achievements

鉄セレン系超伝導体は、高い超伝導転移点(Tc)をもつ鉄系超伝導体の一つであるが、Tcの起源は解明されたとは言えない。一つには、超伝導、結晶対称性の破れたネマティック秩序、磁性が複雑に関係しているためである。高いTcが4万気圧以上で実現することも問題を難しくしている。本研究では、高圧下でミクロな電子状態を調べるために、キュービックアンビル圧力セルを用いた核磁気共鳴法を開発した。この結果、ネマティック秩序と磁気揺らぎに相関があること、高いTcはネマティック秩序が消滅し、極めて弱い磁気揺らぎ下で実現することが分かった。これは、高温超伝導機構が複数の要因で決まることを示し、起源の多様性を示唆している。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (21 results)

All 2021 2020 2019 2018

All Journal Article (7 results) (of which Int'l Joint Research: 2 results,  Peer Reviewed: 6 results,  Open Access: 3 results) Presentation (13 results) (of which Int'l Joint Research: 3 results,  Invited: 1 results) Book (1 results)

  • [Journal Article] High-Pressure Phase Diagrams of FeSe1-xTex: Correlation between Suppressed Nematicity and Enhanced Superconductivity2021

    • Author(s)
      K. Mukasa, K. Matsuura, M. Qiu, M. Saito, Y. Sugimura, K. Ishida, M. Otani, Y. Onishi, Y. Mizukami, K. Hashimoto, J. Gouchi, R. Kumai, Y. Uwatoko, and T. Shibauchi
    • Journal Title

      Nat. Commun.

      Volume: 12 Issue: 1 Pages: 381-381

    • DOI

      10.1038/s41467-020-20621-2

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Internal and External Pressure Effects on Superconductivity in FeTexSe1-x (x=0.46, 0.54) Single Crystals2021

    • Author(s)
      G. Lingannan, K. Ganesan, S. Mariappan, R. Sankar, Y. Uwatoko and S. Arumugam
    • Journal Title

      J Supercond Nov Magn

      Volume: 34 Issue: 3 Pages: 725-731

    • DOI

      10.1007/s10948-020-05790-x

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Fabrication and evaluation via nuclear quadrupole resonance of a palm cubic-anvil pressure cell2020

    • Author(s)
      S. Nakagawa, J. Gochi, T. Kuwayama, S. Nagasaki, T. Takahashi, J. Cheng, Y. Uwatoko and N. Fujiwara
    • Journal Title

      Review of Scientific Instruments

      Volume: 91 Issue: 7 Pages: 0739071-6

    • DOI

      10.1063/5.0012015

    • NAID

      120006870877

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] NMR study under pressure on the iron-based superconductor FeSe1-xSx (x = 0.12 and 0.23): Relationship between nematicity and AF fluctuations2020

    • Author(s)
      Kuwayama T.、Matsuura K.、Mizukami Y.、Kasahara S.、Matsuda Y.、Shibauchi T.、Uwatoko Y.、Fujiwara N.
    • Journal Title

      Modern Physics Letters B

      Volume: 34 Issue: 19n20 Pages: 2040048-2040048

    • DOI

      10.1142/s0217984920400485

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Pressure-induced Lifshitz transition in FeSe0.88S0.12 probed via 77Se-NMR2019

    • Author(s)
      T. Kuwayama, K. Matsuura, Y. Mizukami, S. Kasahara, Y. Matsuda, T. Shibauchi, Y. Uwatoko and N. Fujiwara,
    • Journal Title

      Papers in Physics

      Volume: 11 Pages: 1100031-4

    • DOI

      10.4279/pip.110003

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] 77Se-NMR Study under Pressure on 12%-S Doped FeSe2019

    • Author(s)
      Kuwayama Takanori、Matsuura Kohei、Mizukami Yuta、Kasahara Shigeru、Matsuda Yuji、Shibauchi Takasada、Uwatoko Yoshiya、Fujiwara Naoki
    • Journal Title

      Journal of the Physical Society of Japan

      Volume: 88 Issue: 3 Pages: 033703-033703

    • DOI

      10.7566/jpsj.88.033703

    • NAID

      210000135114

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Magnetic fluctuations under pressure on S-doped FeSe studied via 77Se NMR2018

    • Author(s)
      T. Kuwayama, K. Matsuura, Y. Mizukami, S. Kasahara, Y. Matsuda, T. Shibauchi, Y. Uwatoko, and N. Fujiwara
    • Journal Title

      AIP Advances

      Volume: 8 Issue: 10 Pages: 1013081-5

    • DOI

      10.1063/1.5042570

    • Related Report
      2018 Annual Research Report
  • [Presentation] FeSe1-xSx (x = 0.18)における高圧下77Se-NMR測定2020

    • Author(s)
      中村昂矢, 桑山昂典, 松浦康平, 水上雄太, 笠原成, 松田祐司, 芝内孝禎, 上床美也, 藤原直樹
    • Organizer
      日本物理学会 秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] FeSe1-xSx (x = 0.05)における高圧下77Se-NMR測定2020

    • Author(s)
      猪股和也, 中村昂矢, 桑山昂典, 松浦康平, 水上雄太, 笠原成, 松田祐司, 芝内孝禎, 上床美也, 藤原直樹
    • Organizer
      日本物理学会 秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] FeSe1-xSx (x=0.05) の磁気揺らぎと超伝導2020

    • Author(s)
      猪股 和也, 桑山 昂典, 中村 昂矢, 松浦 康平, 水上 雄太, 笠原 成, 松田 裕司, 芝内 孝禎, 上床 美也 , 藤 原 直樹
    • Organizer
      日本高圧力学会 高圧討論会
    • Related Report
      2020 Annual Research Report
  • [Presentation] PALM 型キュービックアンビルセルによる Cu2O の NQR 測定2020

    • Author(s)
      桑山 昂典 , 郷地 順, 中川 悟志, 長崎 尚子, 高橋 輝雄, CHENG Jinguang, 上床 美也 , 藤原 直樹
    • Organizer
      日本高圧力学会 高圧討論会
    • Related Report
      2020 Annual Research Report
  • [Presentation] NMR study under pressure on the iron-based superconductor FeSe1-xSx : observation of two types of low-energy AF fluctuations2019

    • Author(s)
      N. Fujiwara, T. Kuwayama, K. Matsuura, Y. Mizukami, S. Kasahara, Y. Matsuda, T. Shibauchi, and Y. Uwatoko4
    • Organizer
      ELECTRON CORRELATION IN SUPERCONDUCTORS and NANOSTRUCTURES ( ECSN-2019 )
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] FeSe1-xSx (x = 0.12) の反強磁性相における高圧下77Se-NMR測定(口頭発表)2019

    • Author(s)
      桑山昂典, 松浦康平, 水上雄太, 笠原成, 松田祐司, 芝内孝禎, 上床美也, 藤原直樹
    • Organizer
      日本物理学会  2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] FeSe1-xSx(x = 0.05, 0.12, 0.23)の常圧での核磁気共鳴(口頭発表)2019

    • Author(s)
      中村昂矢, 桑山昂典, 松浦康平, 水上雄太, 笠原成, 松田祐司, 芝内孝禎, 上床美也, 藤原直樹
    • Organizer
      日本物理学会 2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] FeSe1-xSx (x = 0.12) の圧力誘起反強磁性と超伝導(口頭発表)2019

    • Author(s)
      桑山昂典, 松浦康平, 水上雄太, 笠原成, 松田祐司, 芝内孝禎, 上床美也, 藤原直樹
    • Organizer
      日本高圧力学会 第60回高圧討論会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Superconductivity and magnetism of S-doped FeSe with a high Tc (=25-30K) studied via 77Se-NMR measurements under pressure2019

    • Author(s)
      Naoki Fujiwara,T. Kuwayama, K. Matsuura, Y. Mizukami, S. Kasahara, Y. Matsuda, T. Sibauchi, Y. Uwatoko
    • Organizer
      APS march meeting 2019
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] FeSe1-xSx(x>0.2)における圧力下77Se-NMR 測定2019

    • Author(s)
      桑山昂典、松浦康平、水上雄太、笠原茂、松田裕司、芝内孝禎、上床美也、藤原直樹
    • Organizer
      日本物理学会 74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Relationship between superconductivity and magnetism on FeSe1-xSx (x = 0.12) studied by 77Se-NMR under pressure2018

    • Author(s)
      T. Kuwayama, K. Matsuura, Y. Mizukami, S. Kasahara, Y. Matsuda, T. Sibauchi, Y. Uwatoko, N. Fujiwara
    • Organizer
      International Conference and Workshop on High Pressure Semiconductors & Superconductors Physics (HPSP18&WHS2)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] FeSe1-xSx(x=0.12)の磁気秩序相近傍における高圧下77Se-NMR 測定2018

    • Author(s)
      桑山昂典、松浦康平、水上雄太、笠原茂、松田裕司、芝内孝禎、上床美也、藤原直樹
    • Organizer
      日本物理学会 2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] FeSe1-xSx(x=0.12)の高圧下77Se-NMRによる緩和時間T1の測定2018

    • Author(s)
      桑山昂典、松浦康平、水上雄太、笠原茂、松田裕司、芝内孝禎、上床美也、藤原直樹
    • Organizer
      日本物理学会 73回年次大会
    • Related Report
      2018 Annual Research Report
  • [Book] 日本物理学会誌2020

    • Author(s)
      藤原直樹, 上床美也
    • Total Pages
      7
    • Publisher
      日本物理学会
    • Related Report
      2020 Annual Research Report

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Published: 2018-04-23   Modified: 2022-01-27  

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