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Manipulation of optical functionality in strongly coupled organic microcavity

Research Project

Project/Area Number 18H01476
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 21050:Electric and electronic materials-related
Research InstitutionKyoto Institute of Technology

Principal Investigator

Yamashita Kenichi  京都工芸繊維大学, 電気電子工学系, 教授 (00346115)

Co-Investigator(Kenkyū-buntansha) 山雄 健史  京都工芸繊維大学, 材料化学系, 教授 (10397606)
高橋 駿  京都工芸繊維大学, 電気電子工学系, 助教 (60731768)
Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥17,680,000 (Direct Cost: ¥13,600,000、Indirect Cost: ¥4,080,000)
Fiscal Year 2020: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Fiscal Year 2019: ¥5,460,000 (Direct Cost: ¥4,200,000、Indirect Cost: ¥1,260,000)
Fiscal Year 2018: ¥9,620,000 (Direct Cost: ¥7,400,000、Indirect Cost: ¥2,220,000)
Keywordsポラリトン / 有機半導体結晶 / 微小共振器 / ペロブスカイト / 有機結晶 / マイクロキャビティ
Outline of Final Research Achievements

In this study, we comprehensively investigated the photon-exciton interaction in a microcavity using an organic semiconductor materials and their coherent emission phenomenon. As materials, organic crystals having a strong molecular orientation and lead halide perovskite crystals were mainly used. We have succeeded in producing a microcavity using these materials with a high quality factors. Furthermore, by measuring the angle-resolved emission characteristics and the time-resolved emission characteristics, the coupling strength between the photon and exciton modes in the cavity systems and the relaxation mechanism of the excited species to the polariton state were clarified. These results were based on the international collaborations.

Academic Significance and Societal Importance of the Research Achievements

光と物質の混成状態であるポラリトン状態は、そのボーズ粒子的性質から様々な量子デバイス応用が期待されている。有機半導体などの使用により、このポラリトン状態の室温での利用可能性が指摘されている。本研究では、これらの有機系ポラリトン状態を安定して作成するための基礎的物性を様々な側面から明らかにしている。将来的には、低消費電力で動作可能な量子コンピュータやレーザ光源などの実現につながると期待される。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (51 results)

All 2021 2020 2019 2018 Other

All Int'l Joint Research (4 results) Journal Article (11 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 11 results,  Open Access: 1 results) Presentation (36 results) (of which Int'l Joint Research: 12 results,  Invited: 4 results)

  • [Int'l Joint Research] ケンブリッジ大学(英国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] 中国科学院(中国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] University of Cambridge(英国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] University of Cambridge(英国)

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Comprehensive Photophysical Properties of Thiophene/Phenylene Co-oligomers Investigated by Theoretical and Experimental Studies2020

    • Author(s)
      Kong Jie、Zhang Wei、Guo Yuanyuan、Niu Xinmiao、Yamao Takeshi、Yamashita Kenichi、Xia Andong
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 124 Issue: 35 Pages: 18946-18955

    • DOI

      10.1021/acs.jpcc.0c06311

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Dry-wet hybrid deposition of wide-bandgap mixed-halide perovskites for tandem solar cell applications2020

    • Author(s)
      Kanbe Shota、Kagae Junta、Murota Ayane、Hara Yuya、Fujiwara Kentaro、Yamashita Kenichi
    • Journal Title

      Applied Physics Letters

      Volume: 117 Issue: 17 Pages: 171901-171901

    • DOI

      10.1063/5.0029784

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] A polymer film with ultra-broadband optical gain characteristics2020

    • Author(s)
      Yuya Hara, Youtaro Higase, Marie Taguchi, Shun Takahashi, Fumio Sasaki, Kenichi Yamashita
    • Journal Title

      Applied Physics Letters

      Volume: 116 Issue: 6 Pages: 063301-063301

    • DOI

      10.1063/1.5129477

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Excitation dynamics in layered lead halide perovskite crystal slabs and microcavities2020

    • Author(s)
      K. Fujiwara, S.Zhang, S. Takahashi, L. Ni, A. Rao, and K. Yamashita
    • Journal Title

      ACS Photonics

      Volume: 7 Issue: 3 Pages: 845-852

    • DOI

      10.1021/acsphotonics.0c00038

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Cooperative Behaviors in Amplified Emission from Single Microcrystals of Thiophene/Phenylene Co-Oligomers toward Organic Polariton Laser2019

    • Author(s)
      Hisao Yanagi, Fumio Sasaki, Kenichi Yamashita
    • Journal Title

      Advanced Optical Materials

      Volume: 7 Issue: 17 Pages: 1900136-1900136

    • DOI

      10.1002/adom.201900136

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Strong Exciton-photon Coupling in Organic Microcavity Electroluminescence Devices with Thiophene/Phenylene Co-oligomer Derivatives2019

    • Author(s)
      S. Dokiya, H. Mizuno, H. Mizuno, H. Katsuki, K. Yamashita, F. Sasaki, H. Yanagi
    • Journal Title

      Appl. Phys. Express

      Volume: 12 Issue: 11 Pages: 111002-111002

    • DOI

      10.7567/1882-0786/ab47b9

    • NAID

      120006766862

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Compact solid-state organic laser with fine and broadband wavelength tunability2019

    • Author(s)
      M. Taguchi, Y. Higase, and K. Yamashita
    • Journal Title

      Optics Express

      Volume: 27 Issue: 24 Pages: 35548-35554

    • DOI

      10.1364/oe.27.035548

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] High-gain and wide-band optical amplifications induced by a coupled excited state of organic dye molecules co-doped in polymer waveguide2018

    • Author(s)
      Higase Youtaro、Morita Shinya、Fujii Toshiyuki、Takahashi Shun、Yamashita Kenichi、Sasaki Fumio
    • Journal Title

      Optics Letters

      Volume: 43 Issue: 8 Pages: 1714-1717

    • DOI

      10.1364/ol.43.001714

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ultrafast Dynamics of Polariton Cooling and Renormalization in an Organic Single-Crystal Microcavity under Nonresonant Pumping2018

    • Author(s)
      Yamashita Kenichi、Huynh Uyen、Richter Johannes、Eyre Lissa、Deschler Felix、Rao Akshay、Goto Kaname、Nishimura Takumi、Yamao Takeshi、Hotta Shu、Yanagi Hisao、Nakayama Masaaki、Friend Richard H.
    • Journal Title

      ACS Photonics

      Volume: 印刷中 Issue: 6 Pages: 2182-2188

    • DOI

      10.1021/acsphotonics.8b00041

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Design principle of high-performance organic single-crystal light-emitting devices2018

    • Author(s)
      T. Yamao, S. Higashihara, S. Yamashita, H. Sano, Y. Inada, K. Yamashita, S. Ura, and S. Hotta
    • Journal Title

      Journal of Applied Physics

      Volume: 123 Issue: 23 Pages: 235501-235501

    • DOI

      10.1063/1.5030486

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Modification of dry/wet hybrid fabrication method for preparing a perovskite absorption layer on a PCBM electron transport layer2018

    • Author(s)
      J. Kagae, T. Yamanaka, S. Takahashi, and K. Yamashita
    • Journal Title

      RSC Advances

      Volume: 8 Issue: 68 Pages: 39047-39052

    • DOI

      10.1039/c8ra08022d

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] 鉛ハライドペロブスカイト微小共振器における励起状態ダイナミクス2021

    • Author(s)
      山下兼一
    • Organizer
      レーザー学会学術講演会第41回年次大会
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] 有機発光材料によるオープンキャビティVCSELの動的波長チューニング2021

    • Author(s)
      平尾司、 田口巴里絵、原優也、山下兼一
    • Organizer
      レーザー学会学術講演会第41回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 小型波長可変レーザーへの応用のためのグラフェン量子ドットにおける広帯域光増幅効果2021

    • Author(s)
      原優也、長房司、山下兼一
    • Organizer
      レーザー学会学術講演会第41回年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 全無機ペロブスカイト単結晶を活性層とする微小共振器の発光特性2020

    • Author(s)
      上田悠介、榎本柊生、田上智哉、藤原健太郎、高橋駿、山下兼一
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 有機系光機能材料による微小共振器科学の新展開2020

    • Author(s)
      山下兼一
    • Organizer
      筑波大学物質科学・学術融合セミナー
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] 光学顕微鏡マイクロマニピュレーターで作製したカイラルフォトニック結晶における量子ドット円偏光放射の観測2020

    • Author(s)
      伊藤誠野、高橋駿、山下兼一、舘林潤、岩本敏、荒川泰彦
    • Organizer
      第5回JSAPフォトニクスワークショップ
    • Related Report
      2020 Annual Research Report
  • [Presentation] 広帯域光増幅特性を有するグラフェン量子ドットの作製と評価2020

    • Author(s)
      長房司、原優也、山下兼一
    • Organizer
      第5回JSAPフォトニクスワークショップ
    • Related Report
      2020 Annual Research Report
  • [Presentation] Chiral cavity mode in a GaAs-based three-dimensional photonic crystal fabricated by a micro-manipulation method using an optical microscope2019

    • Author(s)
      Y. Kinuta, S. Takahashi, K. Yamashita, J. Tatebayashi, S. Iwamoto, and Y. Arakawa
    • Organizer
      Compound Semiconductor Week 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Strong light-matter coupling and photoluminescence properties of 2D and quasi-2D perovskite microcavities2019

    • Author(s)
      S. Zhang, L. Ni, A. Rao, and K. Yamashita
    • Organizer
      Compound Semiconductor Week 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Organic single crystal microcavities with strong light-matter coupling2019

    • Author(s)
      K. Yamashita
    • Organizer
      2019 Collaborative Conference on Materials Research (CCMR)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Compact organic solid-state laser with wide wavelength tunability2019

    • Author(s)
      M. Taguchi, Y. Higase, and K. Yamashita
    • Organizer
      10th International Conference on Molecular Electronics & BioElectronics
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Light amplification characteristics of CsPbBr3 single crystal nanoplates2019

    • Author(s)
      S. Enomoto and K, Yamashita
    • Organizer
      10th International Conference on Molecular Electronics & BioElectronics
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Microcavity with organic luminescent material with long exciton lifetime2019

    • Author(s)
      K. Imai and K. Yamashita
    • Organizer
      10th International Conference on Molecular Electronics & BioElectronics
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Dry/wet hybrid growth of FA1-xMAxPbI3-xBrx perovskite films2019

    • Author(s)
      J. Kagae, T. Yamanaka, S. Kanbe, and K. Yamashita
    • Organizer
      10th International Conference on Molecular Electronics & BioElectronics
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photophysics of organic single crystal microcavities2019

    • Author(s)
      K. Yamashita
    • Organizer
      7th International Workshop on Epitaxial Growth and Fundamental Properties of Semiconductor Nanostructures
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 微小光共振器を導入した単層WS2発光デバイス2019

    • Author(s)
      小椋友寛、山田知之、和田尚樹、遠藤尚彦、山下兼一、宮田耕充、蒲江、竹延 大志
    • Organizer
      第57回フラーレン・ナノチューブ・グラフェンシンポジウム
    • Related Report
      2019 Annual Research Report
  • [Presentation] 光学顕微鏡マイクロマニピュレーション法による大面積三次元フォトニック結晶の作製及び光学評価2019

    • Author(s)
      有光佑紀哉、高橋駿、山下兼一、渡邊克之、岩本敏、荒川泰彦
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] (チオフェン/フェニレン)コオリゴマー薄膜を有するマイクロキャビティの作製とその光学特性2019

    • Author(s)
      水野斎、吉田航、豊田健人、香月浩之、佐々木史雄、山下兼一、柳久雄
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 有機半導体単結晶を活性層とする微小共振器の時間分解蛍光特性2019

    • Author(s)
      田上智哉、今井啓太、山下兼一、水野斎、柳久雄
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 層状二次元ペロブスカイト単結晶作製法の検討と光学特性の評価2019

    • Author(s)
      藤原健太郎、張帥、山下兼一
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 有機色素共ドープポリマー薄膜におけるエキサイプレックス発光の利得特性2019

    • Author(s)
      原優也、東瀬陽太郎、田口巴里絵、山下兼一、佐々木史雄
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 光学顕微鏡マイクロマニピュレーション法を用いた半導体カイラルフォトニック結晶における円偏光共振器モードの観測2019

    • Author(s)
      絹田雄三、高橋駿、山下兼一、舘林潤、岩本敏、荒川泰彦
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 三次元カイラルフォトニック結晶の光Weyl点近傍での位相再構成現象の観測2019

    • Author(s)
      玉置爽真、高橋駿、山下兼一、山口拓也、上田哲也、岩本敏
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Two-step preparation of high quality perovskite film on mesoporous PbI2 underlayer2019

    • Author(s)
      神戸翔太、加賀江純太、山下兼一
    • Organizer
      38th Electronic Materials Symposium
    • Related Report
      2019 Annual Research Report
  • [Presentation] Dry/wet hybrid growth of FA1-xMAxPbI3-yBry perovskite films2019

    • Author(s)
      加賀江純太、山中貴晶、神戸翔太、山下兼一
    • Organizer
      38th Electronic Materials Symposium
    • Related Report
      2019 Annual Research Report
  • [Presentation] Circular dichroism in a three-dimensional chiral photonic crystal fabricated by optical microscope micro-manipulator2019

    • Author(s)
      木村英里香、高橋駿、山下兼一、舘林潤、岩本敏、荒川泰彦
    • Organizer
      38th Electronic Materials Symposium
    • Related Report
      2019 Annual Research Report
  • [Presentation] 光学顕微鏡観察下でのマイクロマニピュレーターを用いたウッドパイル型3次元フォトニック結晶の作製2019

    • Author(s)
      木村英里香、高橋駿、山下兼一、渡邉克之、岩本敏、荒川泰彦
    • Organizer
      第4回JSAPフォトニクスワークショップ
    • Related Report
      2019 Annual Research Report
  • [Presentation] 半導体カイラルフォトニック結晶共振器における円偏光自然放出寿命の数値的検討2019

    • Author(s)
      絹田雄三、高橋駿、山下兼一
    • Organizer
      第4回JSAPフォトニクスワークショップ
    • Related Report
      2019 Annual Research Report
  • [Presentation] 広帯域かつ高精度な波長可変性を有する有機固体レーザーの設計2019

    • Author(s)
      田口巴里絵、平尾司、東瀬陽太郎、山下兼一
    • Organizer
      第540回レーザー学会研究会
    • Related Report
      2019 Annual Research Report
  • [Presentation] CsPbBr3ペロブスカイトマイクロプレートにおける誘導放出とレーザ発振機構の考察2019

    • Author(s)
      榎本柊生、山下 兼一
    • Organizer
      第540回レーザー学会研究会
    • Related Report
      2019 Annual Research Report
  • [Presentation] (チオフェン/フェニレン)コオリゴマー低次元単結晶及びマイクロキャビティの作製とそれらの光学特性2019

    • Author(s)
      水野斎、吉田航、香月浩之、佐々木史雄、山下兼一、柳久雄
    • Organizer
      第540回レーザー学会研究会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 面内分子配向特性を有する有機単結晶微小共振器における発光ダイナミクスとポラリトン緩和過程2019

    • Author(s)
      山下兼一
    • Organizer
      第540回レーザー学会研究会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Control of optical gain band by excited state coupling in polymer thin film co-doped with organic dyes2018

    • Author(s)
      Y. Higase, S. Morita, T. Fujii, K. Yamashita, and F. Sasaki
    • Organizer
      The 12th International Conference on Excitonic and Photonic Peocesses in Condensed Matter and Nano Materials
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Strong coupling formation in organic crystal microcavities2018

    • Author(s)
      T. Nishimura, K. Imai, S. Takahashi, K. Yamashita, H. Yanagi, and M. Nakayama
    • Organizer
      The 12th International Conference on Excitonic and Photonic Peocesses in Condensed Matter and Nano Materials
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Formation of cavity polariton in organic electroluminescence devices with thiophene/phenylene co-oligomer derivatives2018

    • Author(s)
      S. Dokiya, H. Mizuno, H. Katsuki, K. Yamashita, F. Sasaki, and H. Yanagi
    • Organizer
      The 12th International Conference on Excitonic and Photonic Peocesses in Condensed Matter and Nano Materials
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photonics in Organic Crystal Microcavities with Strong Light-Matter Coupling2018

    • Author(s)
      K. Yamashita
    • Organizer
      4th Global Congress & Expo on Material Science and Nanoscience
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited

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Published: 2018-04-23   Modified: 2022-01-27  

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