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Redox-type solid-state ionization chambers and their application to zero-biased wireless radiation sensors

Research Project

Project/Area Number 18H01480
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 21050:Electric and electronic materials-related
Research InstitutionSophia University

Principal Investigator

Toshihiro Nakaoka  上智大学, 理工学部, 教授 (20345143)

Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥17,420,000 (Direct Cost: ¥13,400,000、Indirect Cost: ¥4,020,000)
Fiscal Year 2020: ¥4,810,000 (Direct Cost: ¥3,700,000、Indirect Cost: ¥1,110,000)
Fiscal Year 2019: ¥4,550,000 (Direct Cost: ¥3,500,000、Indirect Cost: ¥1,050,000)
Fiscal Year 2018: ¥8,060,000 (Direct Cost: ¥6,200,000、Indirect Cost: ¥1,860,000)
Keywords放射線センサ / 異常拡散 / 電気化学反応 / カルコゲナイド / 抵抗変化 / 放射線センサー / フォトドーピング / Ag拡散 / レドックス反応
Outline of Final Research Achievements

We proposed a new real-time radiation sensor based on a new operating principle, which can operate at high doses, is compact, and can be wirelessly operated. We have measured the reversible resistance change of about 4% in real time at a high dose of 2 kGy/h.
We proposed a model of the operation mechanism, on the basis of the results of complex impedance measurement, TOF-SIMS, TEM, electron diffraction measurements.
A prototype of an active wireless sensor with a transmission range of 3.5 m was fabricated, and its operation was demonstrated.

Academic Significance and Societal Importance of the Research Achievements

本研究における放射線検出はγ線照射時のAgの異常拡散による導電性領域形成に主に基づく。これまでは,γ線照射に対する不可逆な変化のみ注目されドシメータとして研究されてきたが,本研究ではGe-Sb-Te系アモルファス薄膜においてin-situなリアルタイム測定を行い,可逆な抵抗変化を初めて見出し,リアルタイムセンサとして動作することを実証した。
本素子は抵抗変化型であり無給電で動作する。バッテリーなどは不要であるので放射線耐性が高く,駆動時間の制限がなく,メンテナンスにも有利である。アクティブ型のワイヤレスセンシングを実証することでその有望性を示した。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (22 results)

All 2021 2020 2019 2018 Other

All Journal Article (5 results) (of which Peer Reviewed: 5 results) Presentation (14 results) (of which Invited: 3 results) Remarks (3 results)

  • [Journal Article] Reversible and irreversible resistance changes for gamma-ray irradiation in silver-diffused germanium telluride2020

    • Author(s)
      Park Hyoseong、Watanabe Tatsuya、Yoda Isao、Shohmitsu Yoshinori、Kawasaki Shigeo、Nakaoka Toshihiro
    • Journal Title

      SN Applied Sciences

      Volume: 2 Issue: 12

    • DOI

      10.1007/s42452-020-03927-0

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Single-crystalline Ag2Te nanorods prepared by room temperature sputtering of GeTe2020

    • Author(s)
      Nakaya Kazuki、Nakaoka Toshihiro
    • Journal Title

      SN Applied Sciences

      Volume: 2 Issue: 9

    • DOI

      10.1007/s42452-020-03406-6

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Direct measurement of "ready-made" cations in a Ge2Sb3.4Te6.2 film2019

    • Author(s)
      Yusuke Imanishi, Toshihiro Nakaoka
    • Journal Title

      Journal of Materials Science

      Volume: 54 Issue: 9 Pages: 7072-7077

    • DOI

      10.1007/s10853-019-03405-y

    • Related Report
      2019 Annual Research Report 2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Room temperature growth of silver telluride nanorods by sputtering deposition2018

    • Author(s)
      Yusuke Imanishi and Toshihiro Nakaoka
    • Journal Title

      Applied Physics A

      Volume: 124 Issue: 10

    • DOI

      10.1007/s00339-018-2099-y

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spontaneous room-temperature formation of broccoli-like Ag-GeTe nanostructures assisting filamentary resistive switching2018

    • Author(s)
      Imanishi Yusuke、Hayashi Hitoshi、Nakaoka Toshihiro
    • Journal Title

      Journal of Materials Science

      Volume: 53 Issue: 17 Pages: 12254-12264

    • DOI

      10.1007/s10853-018-2493-z

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] 相変化材料におけるAgの異常拡散ーナノワイヤ形成からガンマ線検出まで2021

    • Author(s)
      中岡俊裕、渡部 達也、朴 孝晟、中谷 和希、依田 功、正光 義則、川﨑 繁男
    • Organizer
      2021年第68回応用物理学会春季学術講演会[17p-Z02-4] (オンライン)シンポジウム内招待講演
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] ffect of Si buffer layer on thermoelectric properties of Sb2Te3 films2020

    • Author(s)
      Ryo Katayama, Hiroki Toyoda, Yuki Matsufuji, Masahiro Nomura, Kazuo Ogata,Takao Mori, and Toshihiro Nakaoka,
    • Organizer
      The 32th Symposium on Phase Change Oriented Science PCOS 2020 [session 2-8]
    • Related Report
      2020 Annual Research Report
  • [Presentation] 相変化材料中の銀イオン伝導を応用した放射線センサーの研究2020

    • Author(s)
      渡部達也,朴 孝晟,依田 功,正光義則, 川﨑 繁男,中岡 俊裕
    • Organizer
      Sophia Open Research Weeks 2020 半導体ナノフォトニクス研究会
    • Related Report
      2020 Annual Research Report
  • [Presentation] GeSbTe薄膜におけるAgの電気化学反応 ーナノ構造形成から応用までー2020

    • Author(s)
      中岡 俊裕, 渡部 達也, 朴 孝晟, 依田 功, 正光 義則, 川崎 繁男
    • Organizer
      2020年第67回応用物理学会春季学術講演会 [13p-A201-5]
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Amplification circuit using a frequency-multiplying Ge-Sb-Te thin film2020

    • Author(s)
      Yifei Yin, Jiawen Xiang, Hyoseong Park, Hitoshi Hayashi Toshihiro Nakaoka
    • Organizer
      第67回応用物理学会春季学術講演会[14a-A407-6]
    • Related Report
      2019 Annual Research Report
  • [Presentation] Cyclic voltammetry and effect of gamma-ray irradiation in GeTe thin films with Ag electrodes2019

    • Author(s)
      Tatsuya Watanabe, Hyoseong Park, Isao Yoda, Yoshinori Shohmitsu, Shigeo Kawasaki, Toshihiro Nakaoka
    • Organizer
      The 31th Symposium on Phase Change Oriented Science PCOS
    • Related Report
      2019 Annual Research Report
  • [Presentation] Electrochemical reaction between Ag and GeTe forming single crystalline Ag2Te nanorods2019

    • Author(s)
      Toshihiro Nakaoka, Kazuki Nakaya, Tatsuya Watanabe, Hyoseong Park,
    • Organizer
      The 31th Symposium on Phase Change Oriented Science PCOS
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] AC Impedance measurement under gamma-ray irradiation on GeTe thin films2019

    • Author(s)
      Hyoseong Park, Tatsuya Watanabe, Isao Yoda, Yoshinori Shohmitsu, Shigeo Kawasaki, Toshihiro Nakaoka
    • Organizer
      2019年第80回応用物理学会秋季学術講演会[19p-PA7-8]
    • Related Report
      2019 Annual Research Report
  • [Presentation] GeTe薄膜におけるサイクリックボルタンメトリーとガンマ線照射の影響2019

    • Author(s)
      渡部 達也, 朴 孝晟, 依田 功, 正光 義則, 川﨑 繁男, 中岡 俊裕
    • Organizer
      2019年第80回応用物理学会秋季学術講演会 [19p-PA7-9]
    • Related Report
      2019 Annual Research Report
  • [Presentation] Ag/Pt電極を用いたGe-(Sb)-Te薄膜におけるガンマ線照射に対する可逆な抵抗変化2019

    • Author(s)
      渡部 達也 , 朴 孝晟 ,依田 功 ,正光 義則 , 川崎 繁男 ,中岡 俊裕
    • Organizer
      2019年 第66回応用物理学会春季学術講演会 [10p-W833-11]
    • Related Report
      2018 Annual Research Report
  • [Presentation] Gamma-ray irradiation induced effects on GeTe thin films,2018

    • Author(s)
      Hyoseong Park, Tatsuya Watanabe, Isao Yoda, Shigeo Kawasaki, and Toshihiro Nakaoka
    • Organizer
      The 30th Symposium on Phase Change Oriented Science PCOS 2018 [P-3],
    • Related Report
      2018 Annual Research Report
  • [Presentation] Kazuki Nakaya and Toshihiro Nakaoka, GeTe nanowire growth at room temperature by RF magnetron sputtering2018

    • Author(s)
      Kazuki Nakaya and Toshihiro Nakaoka,
    • Organizer
      The 30th Symposium on Phase Change Oriented Science, PCOS 2018[P-5]
    • Related Report
      2018 Annual Research Report
  • [Presentation] 気相法によるGeTeナノワイヤの結晶成長2018

    • Author(s)
      中谷 和希、今西 祐典、山口 瑛太、中岡 俊裕
    • Organizer
      2018年第79回応用物理学会秋季学術講演会[19p-231A-6]
    • Related Report
      2018 Annual Research Report
  • [Presentation] Ge-(Sb)-Te薄膜におけるガンマ線照射による抵抗変化のリアルタイム測定2018

    • Author(s)
      朴 孝晟、依田 功、川崎 繁男、中岡 俊裕
    • Organizer
      2018年第79回応用物理学会秋季学術講演会[19p-231A-7]
    • Related Report
      2018 Annual Research Report
  • [Remarks] 上智大学教員データベース

    • URL

      https://rscdb.cc.sophia.ac.jp/Profiles/70/0006956/profile.html

    • Related Report
      2019 Annual Research Report
  • [Remarks] Research map

    • URL

      https://researchmap.jp/read0076935/

    • Related Report
      2019 Annual Research Report
  • [Remarks] 上智大学教員教育研究情報データベース

    • URL

      http://rscdb.cc.sophia.ac.jp/Profiles/70/0006956/profile.html

    • Related Report
      2018 Annual Research Report

URL: 

Published: 2018-04-23   Modified: 2022-01-27  

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