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Observation of voltage-induced large magnetocapacitance effect in magnetic tunnel junctions

Research Project

Project/Area Number 18H01485
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 21060:Electron device and electronic equipment-related
Research InstitutionKeio University (2019-2020)
Hokkaido University (2018)

Principal Investigator

KAIJU Hideo  慶應義塾大学, 理工学部(矢上), 准教授 (70396323)

Co-Investigator(Kenkyū-buntansha) 西井 準治  北海道大学, 電子科学研究所, 教授 (60357697)
長浜 太郎  北海道大学, 工学研究院, 准教授 (20357651)
Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥17,290,000 (Direct Cost: ¥13,300,000、Indirect Cost: ¥3,990,000)
Fiscal Year 2020: ¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000)
Fiscal Year 2019: ¥5,590,000 (Direct Cost: ¥4,300,000、Indirect Cost: ¥1,290,000)
Fiscal Year 2018: ¥6,110,000 (Direct Cost: ¥4,700,000、Indirect Cost: ¥1,410,000)
Keywordsスピントロニクス / 磁性薄膜 / 誘電体 / 交流インピーダンス特性 / 電気容量 / 表面・界面物性 / ナノ構造
Outline of Final Research Achievements

Magnetocapacitance (MC) effect has attracted much attention due to their potential applications as highly-sensitive magnetic sensors, high-frequency devices and energy storage materials. The MC effect has been observed in multiferroic materials, spintronic devices and magnetic supercapacitors. Here we focus on magnetic tunnel junctions (MTJs) in spintronic devices, and we report a new phenomenon, in which the tunneling magnetocapacitance (TMC) increases with biasing voltage in MgO-based MTJs. We have observed a maximum TMC value of beyond 300%, which is the largest voltage-induced TMC effect ever reported for MTJs. We have found excellent agreement between theory and experiment using extended Debye-Frohlich model. Based on our calculation, we predict that the TMC ratio could reach 1000% in MTJs. Our work has provided a new understanding on AC spin-dependent transports in spintronic devices, and the results reported here may open a novel pathway for spintronics applications.

Academic Significance and Societal Importance of the Research Achievements

本研究成果は、静的なスピン蓄積と交流電場下のスピンダイナミクスに関する新たな学術的知見を提供するとともに、次世代革新的超高性能メモリの実現に向けた重要な設計指針を導くと期待できる。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (46 results)

All 2021 2020 2019 2018 Other

All Int'l Joint Research (3 results) Journal Article (8 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 8 results,  Open Access: 2 results) Presentation (33 results) (of which Int'l Joint Research: 16 results,  Invited: 9 results) Remarks (2 results)

  • [Int'l Joint Research] ブラウン大学(米国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] ブラウン大学(米国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] ブラウン大学(米国)

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Sign Inversion Phenomenon of Voltage-induced Tunnel Magnetocapacitance2021

    • Author(s)
      T. Nakagawa, K. Ogata, Y. Nakayama, G. Xiao, and H. Kaiju
    • Journal Title

      Applied Physics Letter

      Volume: 118

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Principle and Recent Advances in Tunnel Magnetocapacitance Effect2021

    • Author(s)
      H. Kaiju and T. Nagahama
    • Journal Title

      IEEJ Transactions on Fundamentals and Materials

      Volume: 141

    • NAID

      130008033214

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Large Inverse Tunnel Magnetoresistance in Magnetic Tunnel Junctions with an Fe3O4 Electrode2021

    • Author(s)
      Yasui Shoma、Honda Syuta、Okabayashi Jun、Yanase Takashi、Shimada Toshihiro、Nagahama Taro
    • Journal Title

      Physical Review Applied

      Volume: 15 Issue: 3 Pages: 034042-034042

    • DOI

      10.1103/physrevapplied.15.034042

    • NAID

      120007126036

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Voltage-induced Magnetocapacitance Effect in Magnetic Tunnel Junctions2020

    • Author(s)
      H. Kaiju
    • Journal Title

      Materia Japan

      Volume: 59 Issue: 4 Pages: 191-198

    • DOI

      10.2320/materia.59.191

    • NAID

      130007824775

    • ISSN
      1340-2625, 1884-5843
    • Year and Date
      2020-04-01
    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] NiCo2O4 films fabricated by reactive molecular beam epitaxy and annealing in various oxygen atmospheres2020

    • Author(s)
      Tsujie Asaka、Hara Yoshinori、Yanase Takashi、Shimada Toshihiro、Nagahama Taro
    • Journal Title

      Applied Physics Letters

      Volume: 116 Issue: 23 Pages: 232404-232404

    • DOI

      10.1063/5.0008677

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Tunnel magnetocapacitance in Fe/MgF2 single nanogranular layered films2020

    • Author(s)
      Msiska Robin、Honjo Shusaku、Asai Yuki、Arita Masashi、Tsurumaki-Fukuchi Atsushi、Takahashi Yasuo、Hoshino Norihisa、Akutagawa Tomoyuki、Kitakami Osamu、Fujioka Masaya、Nishii Junji、Kaiju Hideo
    • Journal Title

      Applied Physics Letters

      Volume: 116 Issue: 8 Pages: 082401-082401

    • DOI

      10.1063/1.5139702

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Realization of Novel Nanoscale-Junction Devices using Magnetic Thin-Film Edges2019

    • Author(s)
      H. Kaiju, M. Fujioka and J. Nishii
    • Journal Title

      The Journal of The Institute of Electrical Engineers of Japan

      Volume: 139 Issue: 11 Pages: 730-735

    • DOI

      10.1541/ieejjournal.139.730

    • NAID

      130007740028

    • ISSN
      1340-5551, 1881-4190
    • Year and Date
      2019-11-01
    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Robustness of Voltage-induced Magnetocapacitance2018

    • Author(s)
      H. Kaiju, T. Misawa, T. Nagahama, T. Komine, O. Kitakami, M. Fujioka, J. Nishii, and G. Xiao
    • Journal Title

      Scientific Reports

      Volume: 8 Issue: 1

    • DOI

      10.1038/s41598-018-33065-y

    • NAID

      120006536950

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Presentation] Observation and theoretical calculation of voltage-induced large tunnel magnetocapacitance2021

    • Author(s)
      K. Ogata, Y. Nakayama, G. Xiao, and H. Kaiju
    • Organizer
      The 4th International Symposium for The Core Research Cluster for Spintronics
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 磁気キャパシタンス効果の基礎と最近の新展開2021

    • Author(s)
      海住英生
    • Organizer
      強的秩序とその操作に関わる第12回講演会
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] Fe3O4(001)/MgO(001)/Fe(001)強磁性トンネル接合における大きな負のTMR効果2021

    • Author(s)
      安井彰馬, 本多周太, 岡林潤, 柳瀬隆, 島田敏宏, 長浜太郎
    • Organizer
      第68回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Fe3O4/MgO/Fe磁気トンネル接合におけるトンネル磁気抵抗効果2021

    • Author(s)
      安井 彰馬, 柳瀬 隆, 島田 敏宏, 長浜 太郎
    • Organizer
      第56回応用物理学会北海道支部/第17回日本光学会北海道支部合同学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Voltage-induced large magnetocapacitance effect in MgO-based magnetic tunnel junctions2020

    • Author(s)
      K. Ogata, Y. Nakayama, G. Xiao, and H. Kaiju
    • Organizer
      International Microprocesses and Nanotechnology Conference
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 電圧誘起巨大トンネル磁気キャパシタンス効果の観測と理論的解明2020

    • Author(s)
      緒方健太郎, 中山雄介, Gang Xiao, 海住英生
    • Organizer
      第44回日本磁気学会学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] MgOベース磁気トンネル接合における電圧誘起巨大磁気キャパシタンス効果2020

    • Author(s)
      緒方健太郎, 中山雄介, Gang Xiao, 海住英生
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] NiCo2O4 Thin Films Prepared by Reactive Molecular Beam Epitaxy and Annealing under High Pressure Oxygen Atmosphere2020

    • Author(s)
      Asaka Tsujie, Yoshinori Hara, Takashi Yanase, Toshihiro Shimada, and Taro Nagahama
    • Organizer
      65th Annual Conference on Magnetism and Magnetic Materials
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 反応性MBEで作製したNiCo2O4の磁性と伝導性2020

    • Author(s)
      辻榮朝香、柳瀬隆、島田敏宏、長浜太郎
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 磁気トンネル接合における室温巨大磁気キャパシタンス効果2019

    • Author(s)
      海住英生、長浜太郎、北上修、西井準治、Gang Xiao
    • Organizer
      日本磁気学会第224回研究会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] 磁気キャパシタンス効果の新展開とその学理2019

    • Author(s)
      海住英生、長浜太郎、北上修、西井準治、Gang Xiao
    • Organizer
      第1回慶大スピントロニクス研究開発センター研究会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] 磁気キャパシタンス効果の新展開2019

    • Author(s)
      海住 英生、長浜 太郎、北上 修、西井 準治、Gang Xiao
    • Organizer
      電気学会 第7回ナノスケール磁性体研究会
    • Related Report
      2019 Annual Research Report 2018 Annual Research Report
    • Invited
  • [Presentation] Magnetocapacitance Effect in Spintronic Devices2019

    • Author(s)
      H. Kaiju, T. Nagahama, O. Kitakami, J. Nishii, and G. Xiao
    • Organizer
      The 6th Japan-Korea International Symposium on Materials Science and Technology 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Experimental and Theoretical Study on Tunnel Magnetocapacitance in Fe/MgF2 Nanogranular Films2019

    • Author(s)
      R. Msiska, S. Honjo, Y. Asai, M. Arita, A. T. Fukuchi, Y. Takahashi, N. Hoshino, T. Akutagawa, O. Kitakami, M. Fujioka, J. Nishii and H. Kaiju
    • Organizer
      The 6th Japan-Korea International Symposium on Materials Science and Technology 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Electric and magnetic properties in Ni78Fe22/Mq3(M=Al, Er)/Ni78Fe22 nanoscale junction devices utilizing magnetic thin-film edges2019

    • Author(s)
      SASAKI, Yuma; MSISKA, Robin; MISAWA, Takahiro; MORI, Sumito; KOMINE, Takashi; HOSHINO, Norihisa; AKUTAGAWA, Tomoyuki; FUJIOKA, Masaya; NISHII, Junji; KAIJU, Hideo
    • Organizer
      The 13th Pacific Rim Conference of Ceramic Societies
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Epitaxial Growth of NiCo2O4 Films by Reactive Molecular Beam Epitaxy Method2019

    • Author(s)
      Asaka Tsujie, Takashi Yanase, Toshihiro Shimada, Taro Nagahama
    • Organizer
      The 3rd Functional Matrial Symposium
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Junction Area and Bias Voltage Dependence of MR Ratio in Ni78Fe22/Mq3(M=Al, Er)/Ni78Fe22 Nanoscale Junction Devices Utilizing Magnetic Thin-film Edges2019

    • Author(s)
      Yuma Sasaki, Robin Msiska, Takahiro Misawa, Sumito Mori, Takashi Komine, Norihisa Hoshino, Tomoyuki Akutagawa, Masaya Fujioka, Melbert Jeem, Madoka Ono, Junji Nishii, and Hideo Kaiju
    • Organizer
      2019 International Symposium of Research Institute for Electronic Science (RIES) Hokkaido University & Center for Emergent Functional Matter Science (CEFMS) National Chiao Tung University
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Molecular nano-spintronic devices utilizing magnetic thin-film edges2019

    • Author(s)
      Y. Sasaki, R. Msiska, T. Misawa, S. Mori, T. Komine, N. Hoshino, T. Akutagawa, M. Fujioka, J. Nishii, H. Kaiju
    • Organizer
      Industry-UCB-UEC-Keio Workshop 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] The crystal structure and magneto-transport properties of NixCo3-xO4 films2019

    • Author(s)
      Asaka Tsujie, Andrea Fernandez, Lora Veneracion, Takashi Yanase, Toshihiro Shimada, Taro Nagahama
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Ni78Fe22/Mq3(M=Al, Er)/Ni78Fe22 nanoscale junction devices utilizing magnetic thin-film edges2019

    • Author(s)
      Y. Sasaki, R. Msiska, T. Misawa, S. Mori, T. Komine, N. Hoshino, T. Akutagawa, M. Fujioka, J. Nishii, and H. Kaiju
    • Organizer
      The 3rd Workshop on Functional Materials Science
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Voltage-induced Magnetocapacitance in Magnetic Tunnel Junctions2019

    • Author(s)
      H. Kaiju, T. Misawa, T. Nagahama, T. Komine, O. Kitakami, M. Fujioka, J. Nishii and G. Xiao
    • Organizer
      2019 Joint MMM-Intermag Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Electric and magnetic properties of Ni78Fe22/Alq3/Ni78Fe22 nanoscale junction devices utilizing magnetic thin-film edges2019

    • Author(s)
      Y. Sasaki, R. Msiska, T. Misawa, S. Mori, T. Komine, N. Hoshino, T. Akutagawa, M. Fujioka, J. Nishii, H. Kaiju
    • Organizer
      2019 Joint MMM-Intermag Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 磁気トンネル接合における室温巨大磁気キャパシタンス効果2019

    • Author(s)
      海住 英生、長浜 太郎、北上 修、西井 準治、Gang Xiao
    • Organizer
      磁気学会第224回研究会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Magnetocapacitance effect in magnetic tunnel junctions2018

    • Author(s)
      H. Kaiju, T. Nagahama, O. Kitakami, J. Nishii, and G. Xiao
    • Organizer
      14th Hokkaido University-Nanjing University-NIMS/MANA Joint Symposium
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Molecular nano-spintronic devices utilizing Ni78Fe22 thin-film edges2018

    • Author(s)
      Y. Sasaki, R. Msiska, T. Misawa, S. Mori, T. Komine, N. Hoshino, T. Akutagawa, M. Fujioka, J. Nishii and H. Kaiju
    • Organizer
      14th Hokkaido University-Nanjing University-NIMS/MANA Joint Symposium
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Ni78Fe22/Alq3/Ni78Fe22 nanoscale junction devices utilizing magnetic thin-film edges2018

    • Author(s)
      Y. Sasaki, R. Msiska, T. Misawa, S. Mori, T. Komine, N. Hoshino, T. Akutagawa, M. Fujioka, J. Nishii, and H. Kaiju
    • Organizer
      The 19th RIES-Hokudai International Symposium
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] FABRICATION OF METASTABLE B2 Fe1-xSnx FILMS BY EPITAXIAL GROWTH ON MgO(001)2018

    • Author(s)
      Taro Nagahama, Yuki Goto, Masato Araki, Takashi Yanase, Shimada Toshihiro, Masahito Tsujikawa and Masafumi Shirai
    • Organizer
      23rd International Colloquium on Magnetic Films and Surfaces ICMFS
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 磁性薄膜エッジを利用した分子ナノ接合素子の作製と電気磁気特性2018

    • Author(s)
      佐々木悠馬、Msiska Robin、三澤貴浩、森澄人、小峰啓史、星野哲久、芥川智行、藤岡正弥、西井準治、海住英生
    • Organizer
      日本材料科学会第4回マテリアルズ・インフォマティクス基礎研究会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 強磁性トンネル接合における電圧誘起磁気キャパシタンス効果2018

    • Author(s)
      海住英生、三澤貴浩、長浜太郎、小峰啓史、北上修、藤岡正弥、西井準治、Xiao Gang
    • Organizer
      第42回日本磁気学会学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 磁性薄膜エッジを利用したNi78Fe22/Alq3/Ni78Fe22ナノ接合素子の電気磁気特性2018

    • Author(s)
      佐々木悠馬、Msiska Robin、三澤貴浩、森澄人、小峰啓史、星野哲久、芥川智行、藤岡正弥、西井準治、海住英生
    • Organizer
      第79回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 薄膜エッジを利用した磁性体/分子/磁性体ナノ接合デバイスの創製2018

    • Author(s)
      海住英生、藤岡正弥、西井準治
    • Organizer
      日本化学会第9回分子アーキテクトニクス研究会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] The crystal structure and magnetotransport properties of CoxFe3-xO4 films and CoxFe3-xO4 / MgO or AlOx / FePt multilayers2018

    • Author(s)
      Asaka Tsujie、Takashi Yanase、Toshihiro Shimada、Taro Nagahama
    • Organizer
      第79回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 磁性薄膜エッジを利用したナノ接合分子スピントロニクスデバイス2018

    • Author(s)
      海住 英生、藤岡 正弥、西井 準治
    • Organizer
      ダイナミックアライアンスG1および物質・デバイス領域共同研究拠点事業合同研究会「有機分子集積体の機能設計と精密計測」
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Remarks] 研究室ホームページ

    • URL

      https://www.kaiju.appi.keio.ac.jp

    • Related Report
      2020 Annual Research Report
  • [Remarks] 研究室HP

    • URL

      https://www.kaiju.appi.keio.ac.jp/

    • Related Report
      2019 Annual Research Report

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Published: 2018-04-23   Modified: 2022-01-27  

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