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Development of new photo/thermo-responsive concentrated slurries for shaping complex and fine structured functional ceramics

Research Project

Project/Area Number 18H01704
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 26020:Inorganic materials and properties-related
Research InstitutionYokohama National University

Principal Investigator

Iijima Motoyuki  横浜国立大学, 大学院環境情報研究院, 准教授 (70513745)

Co-Investigator(Kenkyū-buntansha) 丸尾 昭二  横浜国立大学, 大学院工学研究院, 教授 (00314047)
多々見 純一  横浜国立大学, 大学院環境情報研究院, 教授 (30303085)
Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥16,900,000 (Direct Cost: ¥13,000,000、Indirect Cost: ¥3,900,000)
Fiscal Year 2020: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Fiscal Year 2019: ¥2,600,000 (Direct Cost: ¥2,000,000、Indirect Cost: ¥600,000)
Fiscal Year 2018: ¥11,700,000 (Direct Cost: ¥9,000,000、Indirect Cost: ¥2,700,000)
Keywordsセラミックス / 刺激応答性スラリー / その場固化 / 高精細造形 / 三次元造形 / スラリー / 表面設計 / 分散制御
Outline of Final Research Achievements

Dispersions which ceramic particles were dispersed into solvents in high concentrations and those can be solidified by external stimuli, such as heating and site selective light irradiation, have successfully designed. A new concept which a small amount of organic additives crosslinks the surface modified particles in the dispersions were proposed. After understanding the control factors of slurry solidification behaviors, it was demonstrated that the designed slurry can be applied for shaping complex structured ceramics and further shorten the sintering process compared to the case of using conventional photo/thermo-responsive slurries.

Academic Significance and Societal Importance of the Research Achievements

光や熱刺激で固化する分散液の設計を従来手法と比較して圧倒的に少ない有機添加材量で実現できた点、この分散液の固化性を活用して様々なセラミックス材料の複雑形状体が造形でき、セラミックス材料の焼成時間を格段に短縮する手法を構築した点に高い学術的意義がある。これらの成果は、我々の生活や未来社会を支える構造材料、光学材料、センサー材料などを構成する、特異な形状を有するセラミックス材料の効率的な製造技術として社会に貢献するものである。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (26 results)

All 2021 2020 2019 2018 Other

All Journal Article (5 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 4 results,  Open Access: 1 results) Presentation (19 results) (of which Int'l Joint Research: 6 results,  Invited: 3 results) Remarks (2 results)

  • [Journal Article] 3D structuring of dense alumina ceramics using fiber-based stereolithography with interparticle photo-cross-linkable slurry2021

    • Author(s)
      Seitaro Morita, Motoyuki Iijima, Yuanyi Chen, Taichi Furukawa, Junichi Tatami, Shoji Maruo
    • Journal Title

      Advanced Powder Technology

      Volume: 32 Issue: 1 Pages: 72-79

    • DOI

      10.1016/j.apt.2020.11.016

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Nonaqueous gel casting using multicomponent concentrated slurries through Michael additive reaction for fabricating silicon nitride dense ceramics2021

    • Author(s)
      Motoyuki Iijima, Kenta Hasegawa, Junichi Tatami
    • Journal Title

      Advanced Powder Technology

      Volume: 32 Issue: 2 Pages: 472-479

    • DOI

      10.1016/j.apt.2020.12.028

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 多機能性修飾剤による濃厚系スラリーの分散制御とセラミックスプロセッシング2021

    • Author(s)
      飯島志行、多々見純一
    • Journal Title

      Journal of the Society of Inorganic Materials, Japan

      Volume: 28 Pages: 40-44

    • NAID

      40022456391

    • Related Report
      2020 Annual Research Report
  • [Journal Article] Rapid three-dimensional structuring of transparent SiO2 glass using interparticle photo-cross-linkable suspensions2020

    • Author(s)
      Ryoya Arita, Motoyuki Iijima, Yoko Fujishiro, Seitaro Morita, Taichi Furukawa, Junichi Tatami, Shoji Maruo
    • Journal Title

      Communications Materials

      Volume: 1 Issue: 1

    • DOI

      10.1038/s43246-020-0029-y

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Hetero-assembly of colloidal particles in concentrated non-aqueous suspensions by polymer dispersant design2020

    • Author(s)
      Seitaro Morita, Motoyuki Iijima, Junichi Tatami
    • Journal Title

      Adv. Powder Technol.

      Volume: 31 Issue: 2 Pages: 746-754

    • DOI

      10.1016/j.apt.2019.11.029

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] Design of Interparticle Photo-cross-linkable Alumina Slurries and Application to Fiber-based Stereolithography2021

    • Author(s)
      Motoyuki Iijima, Seitao Morita, Yuanyi Chen, Taichi Furukawa, Junichi Tatami, Shoji Maruo
    • Organizer
      45th International Conference and Expo on Advanced Ceramics and Composites
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] SiO2ナノ粒子を用いた粒子間光架橋スラリーの設計とナノインプリント成形2021

    • Author(s)
      西山健互、飯島志行、多々見純一
    • Organizer
      日本セラミックス協会2021年年会
    • Related Report
      2020 Annual Research Report
  • [Presentation] ヘテロ集積した高濃度スラリーの流動特性に及ぼす粒子径の影響2021

    • Author(s)
      角田聖那、飯島志行、多々見純一
    • Organizer
      日本セラミックス協会2021年年会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 光架橋性濃厚スラリーの分散状態がシリカガラスの光造形に及ぼす影響2020

    • Author(s)
      飯島志行、有田凌也、藤城陽子、古川太一、多々見純一、丸尾昭二
    • Organizer
      粉体工学会2020年度春期研究発表会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 光硬化性ピッカリングエマルションの設計と複雑形状多孔質シリカ焼結体の作製2020

    • Author(s)
      山野井慶彦、飯島志行、多々見純一
    • Organizer
      粉体工学会2020年度春期研究発表会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 粒子間光架橋性スラリーと光ファイバーを用いたアルミナセラミックスの三次元造形2020

    • Author(s)
      飯島志行、森田聖太郎、陳元依、野田洋平、古川太一、多々見純一、丸尾昭二
    • Organizer
      日本セラミックス協会第33回秋季シンポジウム
    • Related Report
      2020 Annual Research Report
  • [Presentation] 粒子間二元架橋反応により光硬化するスラリーを用いた高強度セラミックス成形体の成形2020

    • Author(s)
      佐藤諒太、飯島志行、多々見純一
    • Organizer
      日本セラミックス協会第33回秋季シンポジウム
    • Related Report
      2020 Annual Research Report
  • [Presentation] 光硬化性ピッカリングエマルションの作製条件が多孔質成形体の微構造に及ぼす影響2020

    • Author(s)
      山野井慶彦、飯島志行、多々見純一
    • Organizer
      粉体工学会2020年度秋期研究発表会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 光硬化性スラリーの粒子間架橋構造制御に基づく成形体の強度向上2020

    • Author(s)
      佐藤 諒太、飯島 志行、多々見 純一
    • Organizer
      日本セラミックス協会2020年年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 光硬化性濃厚SiO2スラリーを用いた多孔質セラミックス成形体の設計2020

    • Author(s)
      山野井 義彦、飯島 志行、多々見 純一
    • Organizer
      日本セラミックス協会2020年年会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Design of functionalized polyethyleneimine as versatile surface modifier for processing nanoparticles in nonaqueous solvents2019

    • Author(s)
      Motoyuki Iijima, Momoko Kataoka, Junichi Tatami
    • Organizer
      The 18th Asian Pacific Confederation of Chemical Engineering Congress
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Polyethyleneimine based multifunctional dispersants: toward versatile approach to control the stability of non-aqueous dispersions2019

    • Author(s)
      Motoyuki Iijima, Seitaro Morita, Ryoya Arita, Junichi Tatami
    • Organizer
      OKINAWA COLLOIDS 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Novel photoresponsive slurry system designed by tailor-made functional dispersants for complex shaped and rapid dewaxable green compacts2019

    • Author(s)
      Motoyuki Iijima, Ryoya Arita, Yoko Fujishiro, Shoji Maruo, Junichi Tatami
    • Organizer
      XVI Conference and Exhibition of the European Ceramic Society
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Processing transparent silica glass with complicated shapes by photo-responsive slurries designed using multifunctional polymer dispersants2019

    • Author(s)
      Motoyuki Iijima, Ryoya Arita, Seitaro Morita, Junichi Tatami
    • Organizer
      EUROMAT2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Processing transparent SiO2 glass by pressureless sintering of green body from photo-curable slurry: effect of particle dispersion2019

    • Author(s)
      Motoyuki Iijima, Ryoya Arita, Junichi Tatami
    • Organizer
      The 13th Pacific Rim Conference of Ceramic Societies
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 多機能性修飾剤を用いた外場応答性スラリーの設計とセラミックスの複雑形状成形プロセスへの応用2019

    • Author(s)
      飯島志行、森田聖太郎、長谷川健太、有田凌也、多々見純一
    • Organizer
      第57回セラミックス基礎科学討論会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 非水系スラリーの分散制御を目的としたポリアクリル酸-オレイルアミン会合体の設計2018

    • Author(s)
      森田聖太郎、飯島志行、多々見純一
    • Organizer
      日本セラミックス協会第31回秋季シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] 反応性高分子分散剤を用いて設計した低樹脂量型光硬化性Al2O3スラリーの硬化挙動制御因子2018

    • Author(s)
      森田聖太郎、飯島志行、多々見純一
    • Organizer
      化学工学会第50回秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] マイケル付加反応を用いた非水系スラリーのその場固化挙動に及ぼす粒子界面と多官能アクリレートの影響2018

    • Author(s)
      長谷川健太、飯島志行、多々見純一
    • Organizer
      第56回粉体に関する討論会
    • Related Report
      2018 Annual Research Report
  • [Remarks] 多々見・飯島研究室ホームページ

    • URL

      http://ceramics.ynu.ac.jp/

    • Related Report
      2019 Annual Research Report
  • [Remarks] 多々見・飯島研究室ホームページ

    • URL

      http://ceramics.ynu.ac.jp/index.html

    • Related Report
      2018 Annual Research Report

URL: 

Published: 2018-04-23   Modified: 2022-01-27  

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