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Realization of novel 2D topological insulator materials and its electronic structure analysis by spin-resolved ARPES

Research Project

Project/Area Number 18H01821
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 28030:Nanomaterials-related
Research InstitutionTohoku University

Principal Investigator

Sugawara Katsuaki  東北大学, 理学研究科, 准教授 (70547306)

Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥15,860,000 (Direct Cost: ¥12,200,000、Indirect Cost: ¥3,660,000)
Fiscal Year 2020: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Fiscal Year 2019: ¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
Fiscal Year 2018: ¥9,230,000 (Direct Cost: ¥7,100,000、Indirect Cost: ¥2,130,000)
Keywords2次元トポロジカル絶縁体 / 水素終端処理 / ARPES / MBE / スピン分解ARPES / 2次元トポロジカル絶縁体
Outline of Final Research Achievements

I have fabricated a 2DTI (two-dimensional topological insulator) like Bi monolayer film (called Bismuthene) by using a molecular-beam-epitaxy and characterized the electronic state like Dirac-electron and topological non-trivial edge state by angle-resolved photoemission spectroscopy (ARPES). Firstly, by developing a semiconductor hydrogen-annealing system, I obtained a clean hydrogen-terminated SiC (H-SIC) semiconductor surface. After depositing Bi atoms into H-SiC substrate, I clearly observed not only the superstructure patterns by LEED but also the hole-like dispersive feature by ARPES. These results indicate that we have succeeded in fabricating Bismuthene on H-SiC. In the future, I would clarify the band-gap feature of Dirac electrons and the edge-state in 2DTI. In this study. I also developed a new method for controlling the Dirac electrons by 2DTI heterostructures.

Academic Significance and Societal Importance of the Research Achievements

2DTIを実験的に実現させ近年注目を集めているスピントロニクス分野へ応用展開を行うためには、成長する半導体基板のダングリングボンドを異なる原子で終端させ清浄な基板を得ることと、金属的な性質を持たない基板上に成長させることが強く求められる。本研究では、上記について解決することで、新たな2DTIを生成することが可能であり、2DTI特有のエッジ物性開拓に一つの道を開くことが可能となり、大きな意義を持つと研究者は考えている。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (40 results)

All 2021 2020 2019 2018

All Journal Article (19 results) (of which Int'l Joint Research: 6 results,  Peer Reviewed: 19 results,  Open Access: 8 results) Presentation (19 results) (of which Int'l Joint Research: 11 results,  Invited: 8 results) Book (2 results)

  • [Journal Article] Unusual Temperature Evolution of Quasiparticle Band Dispersion in Electron-Doped FeSe Films2021

    • Author(s)
      Nakayama Kosuke、Shigekawa Koshin、Sugawara Katsuaki、Takahashi Takashi、Sato Takafumi
    • Journal Title

      Symmetry

      Volume: 13 Issue: 2 Pages: 155-155

    • DOI

      10.3390/sym13020155

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Manipulation of Dirac Cone in Topological Insulator/Topological Insulator Heterostructure2021

    • Author(s)
      Sato Takumi、Sugawara Katsuaki、Kato Takemi、Nakata Yuki、Souma Seigo、Yamauchi Kunihiko、Oguchi Tamio、Takahashi Takashi、Sato Takafumi
    • Journal Title

      ACS Applied Electronic Materials

      Volume: 3 Issue: 3 Pages: 1080-1085

    • DOI

      10.1021/acsaelm.0c00918

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Highly Tunable Near‐Room Temperature Ferromagnetism in Cr‐Doped Layered Td‐WTe 22021

    • Author(s)
      Yang Li、Wu Hao、Zhang Liang、Zhang Wenfeng、Li Luying、Kawakami Tappei、Sugawara Katsuaki、Sato Takafumi、Zhang Gaojie、Gao Pengfei、Muhammad Younis、Wen Xiaokun、Tao Boran、Guo Fei、Chang Haixin
    • Journal Title

      Advanced Functional Materials

      Volume: 31 Issue: 13 Pages: 2008116-2008116

    • DOI

      10.1002/adfm.202008116

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dirac Fermion Kinetics in 3D Curved Graphene2020

    • Author(s)
      Yoichi Tanabe, Yoshikazu Ito, Katsuaki Sugawara, Mikito Koshino, Shojiro Kimura, Tomoya Naito, Isaac Johnson, Takashi Takahashi, Mingwei Chen
    • Journal Title

      Advanced Materials

      Volume: 32 Issue: 48 Pages: 2005838-2005838

    • DOI

      10.1002/adma.202005838

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Unusual temperature evolution of the band structure of Bi(111) studied by angle-resolved photoemission spectroscopy and density functional theory2020

    • Author(s)
      Sato Takafumi、Yamada Keiko、Kosaka Takao、Souma Seigo、Yamauchi Kunihiko、Sugawara Katsuaki、Oguchi Tamio、Takahashi Takashi
    • Journal Title

      Physical Review B

      Volume: 102 Issue: 8 Pages: 085112-085112

    • DOI

      10.1103/physrevb.102.085112

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Modulation of Dirac electrons in epitaxial Bi2Se3 ultrathin films on van der Waals ferromagnet Cr2Si2Te62020

    • Author(s)
      Kato Takemi、Sugawara Katsuaki、Ito Naohiro、Yamauchi Kunihiko、Sato Takumi、Oguchi Tamio、Takahashi Takashi、Shiomi Yuki、Saitoh Eiji、Sato Takafumi
    • Journal Title

      Physical Review Materials

      Volume: 4 Issue: 8 Pages: 84202-84202

    • DOI

      10.1103/physrevmaterials.4.084202

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Anomalous Hall effect at the spontaneously electron-doped polar surface of PdCoO2 ultrathin films2020

    • Author(s)
      Harada T.、Sugawara K.、Fujiwara K.、Kitamura M.、Ito S.、Nojima T.、Horiba K.、Kumigashira H.、Takahashi T.、Sato T.、Tsukazaki A.
    • Journal Title

      Physical Review Research

      Volume: 2 Issue: 1 Pages: 1-6

    • DOI

      10.1103/physrevresearch.2.013282

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Conversion of a conventional superconductor into a topological superconductor by topological proximity effect2020

    • Author(s)
      Trang C. X.、Shimamura N.、Nakayama K.、Souma S.、Sugawara K.、Watanabe I.、Yamauchi K.、Oguchi T.、Segawa K.、Takahashi T.、Ando Yoichi、Sato T.
    • Journal Title

      Nature Communications

      Volume: 11 Issue: 1 Pages: 1-6

    • DOI

      10.1038/s41467-019-13946-0

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Dichotomy of superconductivity between monolayer FeS and FeSe2019

    • Author(s)
      Shigekawa Koshin、Nakayama Kosuke、Kuno Masato、Phan Giao N.、Owada Kenta、Sugawara Katsuaki、Takahashi Takashi、Sato Takafumi
    • Journal Title

      Proceedings of the National Academy of Sciences

      Volume: 116 Issue: 49 Pages: 24470-24474

    • DOI

      10.1073/pnas.1912836116

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Electronic structure of a Bi2Te3/FeTe heterostructure: Implications for unconventional superconductivity2019

    • Author(s)
      Owada Kenta、Nakayama Kosuke、Tsubono Ryuji、Shigekawa Koshin、Sugawara Katsuaki、Takahashi Takashi、Sato Takafumi
    • Journal Title

      Physical Review B

      Volume: 100 Issue: 6 Pages: 1-5

    • DOI

      10.1103/physrevb.100.064518

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dimensionality reduction and band quantization induced by potassium intercalation in 1T-HfTe22019

    • Author(s)
      Nakata Y.、Sugawara K.、Chainani A.、Yamauchi K.、Nakayama K.、Souma S.、Chuang P.-Y.、Cheng C.-M.、Oguchi T.、Ueno K.、Takahashi T.、Sato T.
    • Journal Title

      Physical Review Materials

      Volume: 3 Issue: 7 Pages: 1-6

    • DOI

      10.1103/physrevmaterials.3.071001

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Monolayer VTe2: Incommensurate Fermi surface nesting and suppression of charge density waves2019

    • Author(s)
      Sugawara Katsuaki、Nakata Yuki、Fujii Kazuki、Nakayama Kosuke、Souma Seigo、Takahashi Takashi、Sato Takafumi
    • Journal Title

      Physical Review B

      Volume: 99 Issue: 24 Pages: 1-6

    • DOI

      10.1103/physrevb.99.241404

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Vortex-induced quantum metallicity in the mono-unit-layer superconductor NbSe22019

    • Author(s)
      Ichinokura Satoru、Nakata Yuki、Sugawara Katsuaki、Endo Yukihiro、Takayama Akari、Takahashi Takashi、Hasegawa Shuji
    • Journal Title

      Physical Review B

      Volume: 99 Issue: 22 Pages: 1-7

    • DOI

      10.1103/physrevb.99.220501

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Weak localization in bilayer graphene with Li-intercalation/desorption2018

    • Author(s)
      Y. Endo, S. Ichinokura, R. Akiyama, A. Takayama, K. Sugawara, K. Nomura, T. Takahashi, S. Hasegawa,
    • Journal Title

      J. Phys.: Condens. Matter

      Volume: 30 Issue: 30 Pages: 3057011-7

    • DOI

      10.1088/1361-648x/aaccc4

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Ultrathin Bismuth Film on High-Temperature Cuprate Superconductor Bi2Sr2CaCu2O8+δ as a Candidate of a Topological Superconductor2018

    • Author(s)
      Shimamura Natsumi、Sugawara Katsuaki、Sucharitakul Sukrit、Souma Seigo、Iwaya Katsuya、Nakayama Kosuke、Trang Chi Xuan、Yamauchi Kunihiko、Oguchi Tamio、Kudo Kazutaka、Noji Takashi、Koike Yoji、Takahashi Takashi、Hanaguri Tetsuo、Sato Takafumi
    • Journal Title

      ACS Nano

      Volume: 12 Issue: 11 Pages: 10977-10983

    • DOI

      10.1021/acsnano.8b04869

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Ultrathin Bismuth Film on 1T-TaS2: Structural Transition and Charge-Density-Wave Proximity Effect2018

    • Author(s)
      Yamada Keiko、Souma Seigo、Yamauchi Kunihiko、Shimamura Natsumi、Sugawara Katsuaki、Trang Chi Xuan、Oguchi Tamio、Ueno Keiji、Takahashi Takashi、Sato Takafumi
    • Journal Title

      Nano Letters

      Volume: 18 Issue: 5 Pages: 3235-3240

    • DOI

      10.1021/acs.nanolett.8b01003

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Selective Fabrication of Mott-Insulating and Metallic Monolayer TaSe22018

    • Author(s)
      Y. Nakata, T. Yoshizawa, K. Sugawara, Y. Umezawa, T. Takahashi and T. Sato
    • Journal Title

      ACS Applied Nano Materials

      Volume: 印刷中 Issue: 4 Pages: 1456-1460

    • DOI

      10.1021/acsanm.8b00184

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Anisotropic band splitting in monolayer NbSe2: implications for superconductivity and charge density wave2018

    • Author(s)
      Nakata Yuki、Sugawara Katsuaki、Ichinokura Satoru、Okada Yoshinori、Hitosugi Taro、Koretsune Takashi、Ueno Keiji、Hasegawa Shuji、Takahashi Takashi、Sato Takafumi
    • Journal Title

      npj 2D Materials and Applications

      Volume: 2 Issue: 1 Pages: 1-6

    • DOI

      10.1038/s41699-018-0057-3

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Pseudogap, Fermi arc, and Peierls-insulating phase induced by 3D?2D crossover in monolayer VSe22018

    • Author(s)
      Umemoto Yuki、Sugawara Katsuaki、Nakata Yuki、Takahashi Takashi、Sato Takafumi
    • Journal Title

      Nano Research

      Volume: 12 Issue: 1 Pages: 165-169

    • DOI

      10.1007/s12274-018-2196-4

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] マイクロARPESによる遷移金属ダイカルコゲナイド薄膜の電子状態2021

    • Author(s)
      菅原克明、川上竜平、加藤剛臣、田口大樹、猿田康朗、久保田雄也、坪野竜治、渡辺夏芽、北村未歩、 堀場弘司、組頭広志、上野啓司、中山耕輔、相馬清吾、高橋 隆、佐藤宇史
    • Organizer
      日本物理学会2021年年次大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Selective fabrication of atomic-layer 1H- and 1T’- MoTe2 films2021

    • Author(s)
      K. Sugawara, Y. Saruta, T. Kato, T. Taguchi, T. Takahashi and T. Sato
    • Organizer
      The 4th International Symposium for The Core Research Cluster for Spintronics
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] The electronic state of atomic-layer TMDs studied by high-resolution ARPES2020

    • Author(s)
      K. Sugawara
    • Organizer
      The 6th International Workshop on 2D Materials
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 1T-XSe2(X=Na, Ta)原子層のモット絶縁相制御:高分解能ARPES2020

    • Author(s)
      中田優樹, ◯菅原克明, C. Bao, S. Zhou, P. Y. Chuang, C. -M Cheng, 高橋隆, A. Chainani, S. Y. Zhou, 佐藤宇史
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 原子層TiSe2-xの高分解能ARPES2020

    • Author(s)
      菅原克明, 中田優樹, 川上竜平, 佐藤匠, 田口大樹, 加藤剛臣, 高橋隆, 佐藤宇史
    • Organizer
      日本物理学会2020年年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Electronic structure of monolayer VTe2 film studed by ARPES2020

    • Author(s)
      K. Sugawara, Y. Nakata, K. Fujii, K. Nakayama, Seigo Souma, T. Takahashi, and T. Sato
    • Organizer
      The 3rd Symposium for The Core Research Clusters for Materials Science and Spintronics
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] High-resolution ARPES studies of atomic-layer TMDs controlled crystal structure2019

    • Author(s)
      K. Sugawara
    • Organizer
      Carrier doping in two-dimensional layered materials、Centro Congressi Federico II
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Electronic structure of atomic-layer VSe2 studied by ARPES2019

    • Author(s)
      K. Sugawara, Y. Umemoto, Y. Nakata, T. Takahashi, and T. Sato
    • Organizer
      Recent Progress in Graphene Research 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] VX2(X=Se, Te)原子層薄膜のCDW相転移:高分解能ARPES2019

    • Author(s)
      菅原克明, 中田優樹, 藤井和樹, 中山耕輔, 相馬清吾, 高橋隆, 佐藤宇史
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 原子層VSe2の高分解能ARPES2019

    • Author(s)
      菅原克明, 中田優樹, 梅本侑煇,高橋隆, 佐藤宇史
    • Organizer
      第32回日本放射光学会年会・放射光科学合同シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] Electronic structure of monolayer VSe2 studied by high-resolution ARPES2019

    • Author(s)
      Katsuaki Sugawara, Yuki Umemoto, Yuki Nakata, T. Takahashi, and T. Sato
    • Organizer
      The 2nd Symposium for World Leading Research Centers
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] High-resolution ARPES studies of group-V atomic-layer transition metal dichlcogenides2019

    • Author(s)
      K. Sugawara
    • Organizer
      2nd International Workshop on 2D Materials
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] グラフェン上の遷移金属ダイカルコゲナイド原子層の高分解能ARPES2019

    • Author(s)
      菅原克明
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 2層グラフェン上のTaSe2原子層の高分解能ARPES2018

    • Author(s)
      菅原克明, 中田優樹, 吉澤拓也, 梅本侑煇, 高橋隆, 佐藤宇史
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Electronic structure of monolayer TiSe2 studied by high-resolution ARPES2018

    • Author(s)
      Katsuaki Sugawara, Yuki Nakata, Yuki Umemoto, T. Takahashi, and T. Sato
    • Organizer
      The 14th International Conference on Atomically Controlled Surfaces, Interfaces and Nanostructures and The 26th International Colloquium on Scanning Probe Microscopy
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Superconducting graphene2018

    • Author(s)
      K. Sugawara, T. Takahashi
    • Organizer
      12th International Conference on Materials and Mechanisms of Superconductivity and High Temperature Superconductors
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 遷移金属ダイカルコゲナイド原子層の高分解能ARPES2018

    • Author(s)
      菅原克明
    • Organizer
      第1回新奇二次元デバイス・物質科学ワークショップ
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] High-resolution ARPES studies of 2D materials related superconductors2018

    • Author(s)
      K. Sugawara
    • Organizer
      First International Workshop on 2D Materials
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] High-resolution ARPES studies of atomic-layer transition metal dichlcogenides2018

    • Author(s)
      K. Sugawara
    • Organizer
      3RD-JPAN-EU FLAGSHIP WORKSHOP ON GRAPHENE AND RELATED 2D MATERILS
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Book] グラフェンから広がる二次元物質の新技術と応用2020

    • Author(s)
      菅原 克明,高橋 隆,佐藤 宇史
    • Publisher
      エヌ・ティー・エス
    • Related Report
      2019 Annual Research Report
  • [Book] 放射光利用の手引き、第4部2019

    • Author(s)
      菅原克明, 高橋隆
    • Publisher
      アグネ技術センター
    • Related Report
      2019 Annual Research Report 2018 Annual Research Report

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Published: 2018-04-23   Modified: 2022-01-27  

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