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Study on ruthenate superconductors using epitaxy techniques

Research Project

Project/Area Number 18H01866
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 29020:Thin film/surface and interfacial physical properties-related
Research InstitutionTokyo Institute of Technology (2020)
The University of Tokyo (2018-2019)

Principal Investigator

Uchida Masaki  東京工業大学, 理学院, 准教授 (50721726)

Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥18,070,000 (Direct Cost: ¥13,900,000、Indirect Cost: ¥4,170,000)
Fiscal Year 2020: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2019: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2018: ¥13,910,000 (Direct Cost: ¥10,700,000、Indirect Cost: ¥3,210,000)
Keywordsルテニウム酸化物 / 薄膜 / 超伝導体 / 超伝導材料
Outline of Final Research Achievements

Purposes of this study are to realize ruthenium oxide superconductors by epitaxy technique and to elucidate their superconducting states using thin films and junctions. We have succeeded in growing Sr2RuO4 superconducting thin films with a transition temperature exceeding 1.2K, and have discussed possible superconducting symmetries which can be realized in two-dimensional limit by precisely measuring the upper critical magnetic field. We have also succeeded in preparing Sr2RuO4-Sr2RuO4 Josephson junctions, and have clarified that the magnetic field dependence of the Josephson critical current maintains time-reversal symmetry. Furthermore, by growing high-quality RuO2 single crystal thin films on various substrates and controlling epitaxial strain from the substrates, we have succeeded in realizing superconductivity at 1.7 K in RuO2.

Academic Significance and Societal Importance of the Research Achievements

本成果は、転移温度が低く不純物や組成に非常に敏感な酸化物超伝導体の研究において、酸化物分子線エピタキシー技術を用いた新規超伝導体の開拓と、エピタキシャル薄膜やジョセフソン接合を利用した超伝導状態の解明が極めて有効であることを示しており、今後様々な酸化物への応用展開が期待される。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (48 results)

All 2021 2020 2019 2018

All Journal Article (16 results) (of which Int'l Joint Research: 4 results,  Peer Reviewed: 16 results,  Open Access: 5 results) Presentation (32 results) (of which Int'l Joint Research: 14 results,  Invited: 15 results)

  • [Journal Article] Enhancement of spin-orbit coupling in Dirac semimetal Cd3As2 films by Sb doping2021

    • Author(s)
      Y. Nakazawa, M. Uchida, S. Nishihaya, M. Ohno, S. Sato, and M. Kawasaki
    • Journal Title

      Physical Review B

      Volume: 103 Issue: 4 Pages: 045109-045109

    • DOI

      10.1103/physrevb.103.045109

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Quantum transport observed in films of the magnetic topological semimetal EuSb22021

    • Author(s)
      M. Ohno, M. Uchida, R. Kurihara, S. Minami, Y. Nakazawa, S. Sato, M. Kriener, M. Hirayama, A. Miyake, Y. Taguchi, R. Arita, M. Tokunaga, and M. Kawasaki
    • Journal Title

      Physical Review B

      Volume: 103 Issue: 16

    • DOI

      10.1103/physrevb.103.165144

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Molecular beam deposition of a new layered pnictide with distorted Sb square nets2021

    • Author(s)
      M. Ohno, M. Uchida, Y. Nakazawa, S. Sato, M. Kriener, A. Miyake, M. Tokunaga, Y. Taguchi, and M. Kawasaki
    • Journal Title

      APL Materials

      Volume: -

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Intrinsic coupling between spatially-separated surface Fermi-arcs in Weyl orbit quantum Hall states2021

    • Author(s)
      S. Nishihaya, M. Uchida, Y. Nakazawa, M. Kriener, Y. Taguchi, and M. Kawasaki
    • Journal Title

      Nature Communications

      Volume: - Issue: 1

    • DOI

      10.1038/s41467-021-22904-8

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Superconductivity in uniquely strained RuO2 films2020

    • Author(s)
      M. Uchida, T. Nomoto, M. Musashi, R. Arita, and M. Kawasaki
    • Journal Title

      Physical Review Letters

      Volume: 125 Issue: 14 Pages: 147001-147001

    • DOI

      10.1103/physrevlett.125.147001

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Characterization of Sr2RuO4 Josephson junctions made of epitaxial films2020

    • Author(s)
      M. Uchida, I. Sakuraba, M. Kawamura, M. Ide, K. S. Takahashi, Y. Tokura, and M. Kawasaki
    • Journal Title

      Physical Review B

      Volume: 101 Issue: 3

    • DOI

      10.1103/physrevb.101.035107

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Quantized surface transport in topological Dirac semimetal films2019

    • Author(s)
      Nishihaya Shinichi、Uchida Masaki、Nakazawa Yusuke、Kurihara Ryosuke、Akiba Kazuto、Kriener Markus、Miyake Atsushi、Taguchi Yasujiro、Tokunaga Masashi、Kawasaki Masashi
    • Journal Title

      Nature Communications

      Volume: 10 Issue: 1 Pages: 2564-2564

    • DOI

      10.1038/s41467-019-10499-0

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Molecular beam epitaxy of three-dimensionally thick Dirac semimetal Cd3As2 films2019

    • Author(s)
      Y. Nakazawa, M. Uchida, S. Nishihaya, S. Sato, A. Nakao, J. Matsuno, and M. Kawasaki
    • Journal Title

      APL Materials

      Volume: 7 Issue: 7 Pages: 071109-071109

    • DOI

      10.1063/1.5098529

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Ballistic transport in periodically modulated MgZnO/ZnO two-dimensional electron systems2019

    • Author(s)
      K. Tanaka, J. Falson, Y. Kozuka, M. Uchida, D. Maryenko, J. T. Ye, Y. Iwasa, A. Tsukazaki, J. H. Smet, and M. Kawasaki
    • Journal Title

      Applied Physics Letters

      Volume: 115 Issue: 15

    • DOI

      10.1063/1.5121005

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Ferromagnetic state above room temperature in a proximitized topological Dirac semimetal2019

    • Author(s)
      M. Uchida, T. Koretsune, S. Sato, M. Kriener, Y. Nakazawa, S. Nishihaya, Y. Taguchi, R. Arita, and M. Kawasaki
    • Journal Title

      Physical Review B

      Volume: 100 Issue: 24 Pages: 245148-245148

    • DOI

      10.1103/physrevb.100.245148

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Anomalous enhancement of upper critical field in Sr2RuO4 thin films2019

    • Author(s)
      M. Uchida, M. Ide, M. Kawamura, K. S. Takahashi, Y. Kozuka, Y. Tokura, M. Kawasaki
    • Journal Title

      Physical Review B

      Volume: 99 Issue: 16

    • DOI

      10.1103/physrevb.99.161111

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Controlling surface carrier density by illumination in the transparent conductor La-doped BaSnO32018

    • Author(s)
      E. B. Lochocki, H. Paik, M. Uchida, D. G. Schlom, and K. M. Shen
    • Journal Title

      Applied Physics Letters

      Volume: 112 Issue: 18

    • DOI

      10.1063/1.5020716

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Gate-tuned quantum Hall states in Dirac semimetal (Cd1-xZnx)3As22018

    • Author(s)
      S. Nishihaya, M. Uchida, Y. Nakazawa, M. Kriener, Y. Kozuka, Y. Taguchi, and M. Kawasaki
    • Journal Title

      Science Advances

      Volume: 4 Issue: 5

    • DOI

      10.1126/sciadv.aar5668

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Negative magnetoresistance suppressed through a topological phase transition in (Cd1?xZnx)3As2 thin films2018

    • Author(s)
      Nishihaya S.、Uchida M.、Nakazawa Y.、Akiba K.、Kriener M.、Kozuka Y.、Miyake A.、Taguchi Y.、Tokunaga M.、Kawasaki M.
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 24 Pages: 245103-245103

    • DOI

      10.1103/physrevb.97.245103

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Signatures of charge-order correlations in transport properties of electron-doped cuprate superconductors2018

    • Author(s)
      H. Matsuoka, M. Nakano, M. Uchida, M. Kawasaki, and Y. Iwasa
    • Journal Title

      Physical Review B

      Volume: 98 Issue: 14 Pages: 144506-144506

    • DOI

      10.1103/physrevb.98.144506

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ferroelectric field control of charge density in oxide films with polarization reversal by electric double layer2018

    • Author(s)
      R. Nishino, Y. Kozuka, F. Kagawa, M. Uchida, M. Kawasaki
    • Journal Title

      Applied Physics Letters

      Volume: 113 Issue: 14

    • DOI

      10.1063/1.5047558

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] Quantized Transport on Topological Semimetal Fermi Arcs2021

    • Author(s)
      M. Uchida
    • Organizer
      2021 MRS Spring Meeting
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Two-Dimensional Quantum Oscillations Observed in Magnetic Topological Semimetal EuSb2 Films2021

    • Author(s)
      M.Ohno, M. Uchida, R. Kurihara, S. Minami, Y. Nakazawa, S. Sato, M. Kriener, M. Hirayama, A. Miyake, Y. Taguchi, R. Arita, M. Tokunaga, M. Kawasaki
    • Organizer
      2021 MRS Spring Meeting
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Quantum Hall signature of Weyl orbits in dual-gated Dirac semimetal film2021

    • Author(s)
      S. Nishihaya, M. Uchida, Y. Nakazawa, M. Kriener, Y. Taguchi, M. Kawasaki
    • Organizer
      2021 American Physical Society March Meeting
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 分子線エピタキシー法による新物質EuCdSb2の作製2021

    • Author(s)
      大野瑞貴, 打田正輝, 中澤祐介, 佐藤慎, Markus Kriener, 三宅厚志, 徳永将史, 田口康二郎, 川﨑雅司
    • Organizer
      第68回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] トポロジカル半金属における量子ホール伝導2020

    • Author(s)
      打田正輝
    • Organizer
      ワークショップ「超伝導物質、トポロジカル物質」 (SCTM2020)
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] II-V族化合物を基盤としたトポロジカル物質の開拓2020

    • Author(s)
      打田正輝
    • Organizer
      第25回半導体におけるスピン工学の基礎と応用 (PASPS-25)
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] 砒化物ディラック半金属薄膜の量子輸送現象に関する実験的研究2020

    • Author(s)
      打田正輝
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] Quantized Transport in Topological Semimetal Films2020

    • Author(s)
      M. Uchida
    • Organizer
      2nd IIT Guwahati and TokyoTech Joint Workshop on Condensed Matter and High Energy Physics
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 磁性トポロジカル半金属EuSb2薄膜における二次元量子伝導2020

    • Author(s)
      大野瑞貴, 打田正輝, 栗原綾佑, 見波将, 中澤佑介, 佐藤慎, Markus Kriener, 三宅厚志, 田口康二郎, 有田亮太郎, 徳永将史, 川﨑雅司
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Sbドープしたディラック半金属Cd3As2薄膜におけるスピン軌道相互作用の増大2020

    • Author(s)
      中澤佑介, 打田正輝, 西早辰一, 大野瑞貴, 佐藤慎, 川﨑雅司
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Quantization of Surface Conduction in Topological Semimetal Films2019

    • Author(s)
      M. Uchida
    • Organizer
      The Future of Topological Materials
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Quantized Transport in Topological Semimetal Surfaces2019

    • Author(s)
      M. Uchida
    • Organizer
      Strongly Correlated Electron Systems 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Sr2RuO4 Josephson junctions fabricated from epitaxial films2019

    • Author(s)
      M. Uchida
    • Organizer
      Oxide Superspin Workshop 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Quantum Hall Effect in Topological Semimetal Films2019

    • Author(s)
      M. Uchida, Y. Nakazawa, S. Nishihaya, K. Akiba, M. Kriener, Y. Kozuka, A. Miyake, Y. Taguchi, M. Tokunaga, N. Nagaosa, Y. Tokura, and M. Kawasaki
    • Organizer
      The 7th International Workshop on Emergent Phenomena in Quantum Hall Systems
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 砒化物ディラック半金属薄膜の量子輸送現象に関する実験的研究2019

    • Author(s)
      打田正輝
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Quantized Surface Transport in Topological Semimetal Films2019

    • Author(s)
      打田正輝
    • Organizer
      第43回日本磁気学会学術講演会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] トポロジカル半金属表面における量子化伝導現象2019

    • Author(s)
      打田正輝
    • Organizer
      第11回トポロジー連携研究会「トポロジカル半金属」
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Quantized Surface Transport Observed in Cd3As2 Films2019

    • Author(s)
      M. Uchida, S. Nishihaya, Y. Nakazawa, R. Kurihara, K. Akiba, M. Kriener, A. Miyake, Y. Taguchi, M. Tokunaga, and M. Kawasaki
    • Organizer
      Materials Research Meeting 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Sr2RuO4 superconducting state as revealed by film and junction experiments2019

    • Author(s)
      M. Uchida, I. Sakuraba, M. Kawamura, M. Ide, K. Takahashi, Y. Tokura, M. Kawasaki
    • Organizer
      CEMS Symposium on “Emergent Quantum Materials 2019”
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 磁性半金属EuSb2薄膜の量子輸送現象2019

    • Author(s)
      大野瑞貴, 打田正輝, 栗原綾佑, M.-T. Huebsch, T. Yu, 中澤佑介, 佐藤慎, Markus Kriener, 三宅厚志, 田口康二郎, 有田亮太郎, 徳永将史, 川﨑雅司
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 磁性半金属EuAs薄膜における異常ホール効果の解明2019

    • Author(s)
      佐藤慎, 打田正輝, 栗原綾佑, 中澤佑介, M. Kriener, 三宅厚志, M.S.Bahramy, 田口康二郎, 徳永将史, 川﨑雅司
    • Organizer
      日本物理学会第75回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] r2RuO4薄膜を用いた弱結合ジョセフソン接合の特性評価2019

    • Author(s)
      打田正輝, 桜庭一啓, 川村稔, 井出元晴, 高橋圭, 十倉好紀, 川崎雅司
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] トポロジカル半金属薄膜における量子化表面伝導2019

    • Author(s)
      打田正輝
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Sr2RuO4 Josephson junctions built in epitaxial films2019

    • Author(s)
      M. Uchida, I. Sakuraba, M. Kawamura, M. Ide, K. Takahashi, Y. Tokura, M. Kawasaki
    • Organizer
      2019 American Physical Society March Meeting
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Quantum transport properties of Cd3As2 films with low carrier density2019

    • Author(s)
      Y. Nakazawa, M. Uchida, S. Nishihaya, S. Sato, M. Kawasaki
    • Organizer
      2019 American Physical Society March Meeting
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Weyl orbit quantum Hall states observed in Dirac semimetal Cd3As2 thin films2019

    • Author(s)
      S. Nishihaya, M. Uchida, Y. Nakazawa, R. Kurihara, K. Akiba, M. Kriener, A. Miyake, Y. Taguchi, M. Tokunaga, M. Kawasaki
    • Organizer
      2019 American Physical Society March Meeting
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 新規磁性半導体EuAs薄膜の作製と磁気輸送特性の評価2019

    • Author(s)
      佐藤慎, 打田正輝, 中澤佑介, 西早辰一, 川﨑雅司
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Quantum transport phenomena in topological semimetal films2018

    • Author(s)
      Masaki Uchida
    • Organizer
      8th CEMS Topical Research Camp on ‘Symmetry and Topology’
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 分子線エピタキシー法による新規磁性半導体EuAs薄膜の作製2018

    • Author(s)
      佐藤慎, 打田正輝, 中澤佑介, 西早辰一, 川﨑雅司
    • Organizer
      第79回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 分子線エピタキシー法により作製したCd3As2薄膜の量子輸送特性2018

    • Author(s)
      中澤佑介, 打田正輝, 西早辰一, 佐藤慎, 川﨑雅司
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] ディラック半金属(Cd1-xZnx)3As2薄膜における表面量子輸送現象2018

    • Author(s)
      西早辰一, 打田正輝, 中澤佑介, 栗原綾佑, M. Kriener, 三宅厚志, 田口康二郎, 徳永将史, 川﨑雅司
    • Organizer
      日本物理学会2018年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Domain Wall Conduction at All-in-all-out Antiferromagnetic Iridate Heterointerface2018

    • Author(s)
      Masaki Uchida
    • Organizer
      CIMTEC 2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited

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Published: 2018-04-23   Modified: 2022-01-27  

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