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Manifacturing room-temperature polariton devices based on organic microcavity

Research Project

Project/Area Number 18H01900
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 30020:Optical engineering and photon science-related
Research InstitutionNara Institute of Science and Technology

Principal Investigator

Katsuki Hiroyuki  奈良先端科学技術大学院大学, 先端科学技術研究科, 准教授 (10390642)

Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥17,550,000 (Direct Cost: ¥13,500,000、Indirect Cost: ¥4,050,000)
Fiscal Year 2020: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2019: ¥6,890,000 (Direct Cost: ¥5,300,000、Indirect Cost: ¥1,590,000)
Fiscal Year 2018: ¥8,970,000 (Direct Cost: ¥6,900,000、Indirect Cost: ¥2,070,000)
Keywords励起子ポラリトン / 超高速分光 / 有機半導体 / ブロッホ表面波 / 強結合状態 / マイクロキャビティ / ポラリトン / コヒーレント制御 / 超高速ダイナミクス / 有機半導体薄膜
Outline of Final Research Achievements

A polaritonic device composed of distributed Bragg reflector pair and thin layer of organic semiconductor is prepared, and its optical characteristics are studied. The formation of polariton condensate is detected with excitation fluence above the threshold. Femtosecond UV pump-white light probe spectroscopy is applied for the same sample under the polariton condensation. The relaxation dynamics of the exciton and polariton states are observed.
Another strong coupling system called Bloch surface wave polariton, composed of a single DBR mirror and thin layer of organic semiconductor, is studied numerically. The relation between the Rabi splitting parameter and the distribution of electric field around the mirror surface is discussed.
A UV pump-THz probe technique is applied for a sub-micron size crystal of MAPbBr3 perovskite, and it is concluded that the thermal excitation from the exciton state to the bottom of the conduction band is not efficient in this material.

Academic Significance and Societal Importance of the Research Achievements

これまでの類似研究では、有機半導体の強結合ポラリトン状態でのポンププローブ実験は行われていたが、本研究では初めてポラリトン凝縮を実際に示す、閾値以上の励起光を入射した状態で、ポンププローブ分光を行うことができた。また、試料をより容易に作成でき、有限な面内運動量を持ったブロッホ表面波ポラリトン状態を保持するための設計指針について提案をすることができた。今後、有機半導体薄膜を利用したポラリトンデバイスを開発するにあたり、これらの結果は有用な情報である。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (28 results)

All 2021 2020 2019 2018 Other

All Journal Article (4 results) (of which Peer Reviewed: 4 results) Presentation (21 results) (of which Int'l Joint Research: 2 results,  Invited: 2 results) Remarks (3 results)

  • [Journal Article] Numerical simulations on strong coupling of Bloch surface waves and excitons in dielectric-organic multilayer structures2020

    • Author(s)
      Christian M. Laurio, Hiroyuki Katsuki, and Hisao Yanagi
    • Journal Title

      J. Phys. Condens. Matter

      Volume: 32 Issue: 41 Pages: 415003-415003

    • DOI

      10.1088/1361-648x/ab9d48

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photon Energy Dependent Ultrafast Photoinduced Terahertz Response in a Microcrystalline Film of CH3NH3PbBr32020

    • Author(s)
      Hiroto Okochi, Hiroyuki Katsuki, Masaaki Tsubouchi, Ryuji Itakura, and Hisao Yanagi
    • Journal Title

      J. Phys. Chem. Lett.

      Volume: 11 Issue: 15 Pages: 6068-6076

    • DOI

      10.1021/acs.jpclett.0c01393

    • NAID

      120007126586

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Mode selective excitation of terahertz vibrations in single crystalline rubrene2019

    • Author(s)
      Yano Keisuke、Katsuki Hiroyuki、Yanagi Hisao
    • Journal Title

      The Journal of Chemical Physics

      Volume: 150 Issue: 5 Pages: 054503-054503

    • DOI

      10.1063/1.5068732

    • NAID

      120006627287

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Incident angle and photon energy dependence of polariton lasing in organic microcavity2019

    • Author(s)
      Mizuno Hideyuki、Akagi Hiroshi、Tsubouchi Masaaki、Itakura Ryuji、Katsuki Hiroyuki、Yanagi Hisao
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 58 Issue: 5 Pages: 052003-052003

    • DOI

      10.7567/1347-4065/ab0507

    • NAID

      120006619182

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] 有機半導体TDAFを用いた励起子ポラリトンにおける緩和過程の時間分解測定2021

    • Author(s)
      松内 秀直, Garrek Stemo, 香月 浩之, 柳 久雄
    • Organizer
      2021年 第68回応用物理学会春季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 強結合ポラリトン状態を利用したコヒーレント光源への応用2021

    • Author(s)
      香月 浩之
    • Organizer
      レーザー学会第41回年次大会
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] 有機半導体におけるコヒーレント輻射光の時間空間コヒーレンス評価2020

    • Author(s)
      田中 誠人, 松尾 匠, 水野 斎, 香月 浩之, 柳 久雄
    • Organizer
      分子科学会オンライン討論会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 有機半導体TDAFを用いた励起子ポラリトンにおける緩和過程の時間分解測定2020

    • Author(s)
      松内 秀直, Christian M. Laurio, 香月 浩之, 柳 久雄
    • Organizer
      分子科学会オンライン討論会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Photon Energy Dependent Ultrafast Photoinduced Terahertz Response in a Thin Film of CH3NH3PbBr32020

    • Author(s)
      Hiroyuki Katsuki, Hiroto Okochi, Hisao Yanagi, Masaaki Tsubouchi, Ryuji Itakura
    • Organizer
      光・量子ビーム科学合同シンポジウム2020 (OPTO2020)
    • Related Report
      2020 Annual Research Report
  • [Presentation] ハロゲン化鉛ペロブスカイト薄膜の可視ポンプ THz プ ローブ法による過渡透過測定2020

    • Author(s)
      大河内 裕斗, 香月 浩之, 坪内 雅明, 板倉 隆二, 柳久雄
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] One-dimensional photonic crystal as a platform for long-propagating Bloch surface wave polaritons2019

    • Author(s)
      Christian M. Laurio, Hiroyuki Katsuki, and Hisao Yanagi
    • Organizer
      International Conference on Nano-photonics and Nano-optoelectronics 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] ハロゲン化鉛ペロブスカイト薄膜における電子フォノン相互作用の光学測定2019

    • Author(s)
      大河内 裕斗, 香月 浩之, 坪内 雅明, 板倉 隆二, 柳久雄
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 極低温領域におけるルブレン単結晶中のコヒーレントフォノン制御2019

    • Author(s)
      矢野 敬祐, 香月 浩之, 柳 久雄
    • Organizer
      第13回分子科学討論会
    • Related Report
      2019 Annual Research Report
  • [Presentation] フェムト秒ポンプ-プローブ法によるTPCO結晶の励起状態ダイナミクスの研究2019

    • Author(s)
      吉田 航, 大河内 裕斗, 水野 斎, 香月 浩之, 柳 久雄
    • Organizer
      第13回分子科学討論会
    • Related Report
      2019 Annual Research Report
  • [Presentation] フェムト秒紫外ポンプ―白色プローブ法によるTPCO結晶の励起状態ダイナミクスの研究2019

    • Author(s)
      吉田 航, 大河内 裕斗, 香月 浩之, 柳 久雄
    • Organizer
      日本化学会年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 分子性固体中の量子干渉の制御2019

    • Author(s)
      香月浩之
    • Organizer
      日本化学会年会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Ultrafast Relaxation Dynamics of Organic Microcavity Polaritons2018

    • Author(s)
      水野英之、柳久雄、香月浩之、赤木浩、坪内雅明、板倉隆二
    • Organizer
      阪大関西研合同シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] Ultrafast Relaxation Dynamics of Room-temperature Organic Microcavity Polaritons2018

    • Author(s)
      Hideyuki Mizuno, Hisao Yanagi, Hiroshi Akagi, Masaaki Tsubouchi, Ryuji Itakura, and Hiroyuki Katsuki
    • Organizer
      EXCON2018
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 有機薄膜ポラリトンを用いたコヒーレント制御へ向けて2018

    • Author(s)
      香月浩之
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] One-dimensional dielectric multilayer for the investigation of long-propagating Bloch surface wave polaritons2018

    • Author(s)
      C. Laurio, H. Katsuki and H. Yanagi
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 室温における有機半導体キャビティポラリトン誘導散乱過程の観測2018

    • Author(s)
      水野英之, 柳久雄, 香月浩之, 赤木浩, 坪内雅明, 板倉隆二
    • Organizer
      日本物理学会秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 遅延ダブルパルス励起を用いたルブレン結晶のフォノン振幅制御2018

    • Author(s)
      矢野 敬祐,香月 浩之,柳 久雄
    • Organizer
      分子科学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 一次元有機半導体結晶における空間コヒーレンスの評価2018

    • Author(s)
      西脇圭佑,香月浩之,柳久雄
    • Organizer
      分子科学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 強電場レーザーパルスを用いた波束の分散制御2018

    • Author(s)
      香月浩之,大槻幸義,安食徹, 後藤悠, 大森賢治
    • Organizer
      分子科学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 有機半導体を利用したポラリトンのコヒーレント制御を目指して2018

    • Author(s)
      香月浩之
    • Organizer
      分子研研究会
    • Related Report
      2018 Annual Research Report
  • [Remarks] 所属機関のグループホームページ

    • URL

      https://mswebs.naist.jp/LABs/optics/research/detail/85

    • Related Report
      2020 Annual Research Report
  • [Remarks] 研究室個人ページ

    • URL

      https://mswebs.naist.jp/LABs/optics/katsuki/index.html

    • Related Report
      2019 Annual Research Report
  • [Remarks] 個人ホームページ(研究内容について記載)

    • URL

      https://hkatsuki21.wixsite.com/mysite2

    • Related Report
      2018 Annual Research Report

URL: 

Published: 2018-04-23   Modified: 2022-01-27  

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