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Imaging hierarchical structures of surfaces and buried interfaces by using X-ray scattering

Research Project

Project/Area Number 18H03479
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Review Section Basic Section 80040:Quantum beam science-related
Research InstitutionJapan Synchrotron Radiation Research Institute

Principal Investigator

Tajiri Hiroo  公益財団法人高輝度光科学研究センター, 回折・散乱推進室, 主幹研究員 (70360831)

Co-Investigator(Kenkyū-buntansha) 豊川 秀訓  公益財団法人高輝度光科学研究センター, 情報処理推進室, 主幹研究員 (60344397)
Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥17,680,000 (Direct Cost: ¥13,600,000、Indirect Cost: ¥4,080,000)
Fiscal Year 2020: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Fiscal Year 2019: ¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2018: ¥10,140,000 (Direct Cost: ¥7,800,000、Indirect Cost: ¥2,340,000)
Keywords放射光 / 表面・界面 / X線散乱 / 階層構造
Outline of Final Research Achievements

Hierarchical structures of surfaces from an atomic scale to a mesoscopic level have been gathering much interest for deep understanding of corrosion, plating, and self-assembly and so on, where surfaces play an important role intrinsically. Hence, a mesoscopic probe in combination with surface X-ray diffraction (SXRD) has been awaited to provide a new opportunity for studying surface phenomena from the firm basis of its atomic constellation and morphology.
We developed a middle energy-bandwidth monochromator using an asymmetric diffraction geometry at SPring-8, which showed the maximum gain of 2.5. In addition, SXRD with high signal-to-noise ratio was realized using an effective sample cooling system. We also succeeded in image reconstruction of a sample having a fine structure with finer than hundreds of nm resolution by using coherent scattering. These results prove that we have successfully developed a method to probe hierarchical structures of surfaces.

Academic Significance and Societal Importance of the Research Achievements

我々が開発した、結晶表面の原子レベル構造に加えてより大きなスケールの秩序構造すなわち階層構造を可視化できる手法は、これまで解析の難しかった腐食やメッキ加工、自己組織化など表面が重要な役割を果たしている広範な分野に対しても適用可能であり意義深い。研究の過程で実現した、入射光量を最大2.5倍増大させる非対称結晶光学系は表面・界面研究にとどまらず高光量を必要とする放射光実験にも活用できるため広い放射光科学分野への波及効果が期待できる。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (11 results)

All 2020 2019 2018

All Journal Article (2 results) (of which Peer Reviewed: 2 results,  Open Access: 2 results) Presentation (9 results) (of which Int'l Joint Research: 3 results)

  • [Journal Article] Progress in surface X-ray crystallography and the phase problem2020

    • Author(s)
      Tajiri Hiroo
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 59 Issue: 2 Pages: 020503-020503

    • DOI

      10.7567/1347-4065/ab631e

    • NAID

      210000157815

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] A Middle Energy-bandwidth X-ray Monochromator for High-flux Synchrotron Diffraction: Revisiting Asymmetrically cut Silicon Crystals2019

    • Author(s)
      Hiroo Tajiri, Hiroshi Yamazaki, Haruhiko Ohashi, Shunji Goto, Osami Sakata and Tetsuya Ishikawa
    • Journal Title

      Journal of Synchrotron Radiation

      Volume: 印刷中

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access
  • [Presentation] コヒーレント散乱による硬X線インラインホログラフィの試み2020

    • Author(s)
      田尻寛男
    • Organizer
      第75回日本物理学会年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] A middle energy-bandwidth crystal monochromator using asymmetric geometry for high-flux synchrotron X-ray diffraction2019

    • Author(s)
      H. Tajiri, H. Yamazaki, H. Ohashi, S. Goto, O. Sakata, T. Ishikawa
    • Organizer
      Materials Research Meeting 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] a CdTe pixel detector for wide energy range X-ray diffractions2019

    • Author(s)
      H. Toyokawa, C. Saji, M. Kawase, K. Ohara, M. Yonemura, J. Okada, Y. Watanabe, A. Shiro, T. Shobu, K. Suzuki
    • Organizer
      12th International "Hiroshima" Symposium on the Development and Application of Semiconductor Tracking Detectors
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 表面X線構造解析ソフトウェアSISReXの現状2019

    • Author(s)
      田尻寛男
    • Organizer
      第32回日本放射光学会年会・放射光科学合同シンポジウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] 透過X線回折によるシリコン上のビスマス薄膜成長と界面構造のリアルタイム観察2019

    • Author(s)
      田尻寛男
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 多重散乱を取り入れた表面X線構造解析ソフトウェアの開発2019

    • Author(s)
      田尻寛男
    • Organizer
      第74回日本物理学会年会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 多波長ビームを用いた次世代型放射光実験と2次元検出器開発2019

    • Author(s)
      豊川秀訓
    • Organizer
      高エネルギー加速器研究機構第33回 研究会「放射線検出器とその応用」
    • Related Report
      2018 Annual Research Report
  • [Presentation] 多波長弁別型CdTeピクセル検出器開発と放射光応用2019

    • Author(s)
      豊川秀訓
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Dual-energy and energy-dispersive X-ray diffractions using CdTe pixel detector2018

    • Author(s)
      Hidenori Toyokawa
    • Organizer
      International Workshops on Radiation Imaging Detectors (iWoRiD2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research

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Published: 2018-04-23   Modified: 2022-01-27  

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