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A study on preparation method of room-temperature pure-circular polarization spin LED and its physical mechanims

Research Project

Project/Area Number 18H03878
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Review Section Medium-sized Section 29:Applied condensed matter physics and related fields
Research InstitutionTokyo Institute of Technology

Principal Investigator

Munekata Hiro  東京工業大学, 科学技術創成研究院, 教授 (60270922)

Co-Investigator(Kenkyū-buntansha) 西沢 望  東京工業大学, 科学技術創成研究院, 助教 (80511261)
Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥43,290,000 (Direct Cost: ¥33,300,000、Indirect Cost: ¥9,990,000)
Fiscal Year 2020: ¥11,180,000 (Direct Cost: ¥8,600,000、Indirect Cost: ¥2,580,000)
Fiscal Year 2019: ¥12,480,000 (Direct Cost: ¥9,600,000、Indirect Cost: ¥2,880,000)
Fiscal Year 2018: ¥19,630,000 (Direct Cost: ¥15,100,000、Indirect Cost: ¥4,530,000)
Keywordsスピンフォトニクス / スピントロニクス / 円偏光発光ダイオード / 偏光 / 医療光学 / がん検診 / 光スピントロニクス / スピン発光ダイオード / 円偏光 / 純粋円偏光 / スピン軸変換 / 非線形効果 / 結晶性トンネルバリア / スピン軸転換
Outline of Final Research Achievements

We have challenged reproduction and physical elucidation of pure circular polarization (CP) electroluminescence (EL) from spin LED reported on 2017. Lithography-free new device process and pulsed current/spin injection approach have made it possible to observe the CP enhancement occurring at 30 to 100 A per square cm or higher region, beyond which dynamic reductions in both EL intensity and junction resistance take place simultaneously. These facts suggest that local heating, presumably around oxide barriers in between metal spin injectors and semiconductor layers, enhances CP values as well as alters electronic/optical characteristics of diodes through abrupt generation of phonons. Namely, pulse-injected hot spins whose spin population are initially weakly polarized are strongly CP polarized via non-elastic scattering with phonons. Re-absorption and -emission also assist this scattering process. Optical spin injection experiments have failed because of the lack of excitation power.

Academic Significance and Societal Importance of the Research Achievements

新しい素子化工程とは ① 極薄AlAs結晶層の積極的酸化によるスピン注入バリアの形成、ならびに、② メカニカルマスクによる微小スピン注入電極の直接形成を指すが、基礎研究を小回り良く(少量・多種類)進めることに向いた手法である。電流パルスによるスピン注入実験、こちらは半導体レーザ研究開発において局所加熱を回避する手法であるが、円偏光増大に際してフォノンが寄与する可能性が高いことをえぐり取ったという点で、理論提唱された円偏極フォノン [J. Kishineら, PRL 125, 245302 (2020)] とキャリアスピンとの間の散乱の重要性を示唆する結果であり、今後の波及効果が期待される。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (50 results)

All 2020 2019 2018 Other

All Int'l Joint Research (2 results) Journal Article (15 results) (of which Int'l Joint Research: 5 results,  Peer Reviewed: 14 results,  Open Access: 1 results) Presentation (32 results) (of which Int'l Joint Research: 12 results,  Invited: 3 results) Remarks (1 results)

  • [Int'l Joint Research] Radboud University(オランダ)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] Palestine Technical University(パレスチナ(PLO))

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Recent Progress of Spin-photonic Devices and its Applications2020

    • Author(s)
      Nishizawa Nozomi
    • Journal Title

      IEEJ Transactions on Fundamentals and Materials

      Volume: 140 Issue: 3 Pages: 113-118

    • DOI

      10.1541/ieejfms.140.113

    • NAID

      130007804344

    • ISSN
      0385-4205, 1347-5533
    • Year and Date
      2020-03-01
    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spatial discrimination of cancer using circular polarization of light scattered by biological tissues2020

    • Author(s)
      Nishizawa N.、Kawashima S.、Al-Qadi B.、Kuchimaru T.、Munekata H.
    • Journal Title

      Proceedings of SPIE

      Volume: Vol. 11521 Pages: 11521141-4

    • DOI

      10.1117/12.2573280

    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Journal Article] Magnetic field enhanced detection of coherent phonons in a GaMnAs/GaAs film2020

    • Author(s)
      Brenden A. Magill, Sunil Thapa, Jade Holleman, Stephen McGill, Hiro Munekata, Christopher J. Stanton, Giti A. Khodaparast
    • Journal Title

      Physical Review B

      Volume: 102 Issue: 4 Pages: 0453061-9

    • DOI

      10.1103/physrevb.102.045306

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Modeling and Optimization of Refracting-Facet Spin-Photodiodes based on Ferromagnetic Metal-Insulator-Semiconductor Tunnel Junctions2020

    • Author(s)
      Ronel Christian Roca, Nozomi Nishizawa, Hiro Munekata
    • Journal Title

      SPIN

      Volume: 10 Issue: 03 Pages: 20500171-14

    • DOI

      10.1142/s2010324720500174

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Ultrafast demagnetization of ferromagnetic semiconductor InMnAs by dual terahertz and infrared excitations2020

    • Author(s)
      E. A. Mashkovich, K. A. Grishunin, Hiro Munekata, A. V. Kimel
    • Journal Title

      Applied Physics Letters

      Volume: 117 Issue: 12 Pages: 1224061-5

    • DOI

      10.1063/5.0017778

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Far- and midinfrared excitation of large amplitude spin precession in the ferromagnetic semiconductor InMnAs2020

    • Author(s)
      Gatilova A.、Mashkovich E. A.、Grishunin K. A.、Pogrebna A.、Mikhaylovskiy R. V.、Rasing Th.、Christianen P. M.、Nishizawa N.、Munekata H.、Kimel A. V.
    • Journal Title

      Physical Review B

      Volume: 101 Issue: 2

    • DOI

      10.1103/physrevb.101.020413

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Monte Carlo simulation of scattered circularly polarized light in biological tissues for detection technique of abnormal tissues using spin-polarized light emitting diodes2020

    • Author(s)
      Nishizawa Nozomi、Hamada Atsushi、Takahashi Kazumasa、Kuchimaru Takahiro、Munekata Hiro
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 59 Issue: SE Pages: SEEG03-SEEG03

    • DOI

      10.35848/1347-4065/ab69db

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Low-threshold pure-circular polarization electro-luminescence from spin-light-emitting diodes consisting of oxidized Al/AlAs tunneling barriers2020

    • Author(s)
      Munekata Hiro
    • Journal Title

      SPIE Proceedings

      Volume: 11288 Pages: 28-28

    • DOI

      10.1117/12.2545701

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Imparting memory functionality to planer waveguide structures with photo-magnetic materials2019

    • Author(s)
      Munekata Hiro、Ogawa Shunta、Michihiro Kento、Nishibayashi Kazuhiro、Nishizawa Nozomi
    • Journal Title

      Japanese Journal of Applied Physics

      Volume: 59 Issue: SE Pages: SEEA05-SEEA05

    • DOI

      10.7567/1347-4065/ab658d

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Spin Injection From EuS/Co Multilayers Into GaAs Detected by Polarized Electroluminescence2019

    • Author(s)
      Goschew A.、Roca R. C.、Nishizawa N.、Munekata H.、Delimitis A.、Fumagalli P.
    • Journal Title

      IEEE Transactions on Magnetics

      Volume: Early access Issue: 7 Pages: 1-4

    • DOI

      10.1109/tmag.2019.2895907

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Arbitrary helicity control of circularly polarized light from lateral-type spin-polarized light-emitting diodes at room temperature2018

    • Author(s)
      Nishizawa Nozomi、Aoyama Masaki、Roca Ronel C.、Nishibayashi Kazuhiro、Munekata Hiro
    • Journal Title

      Applied Physics Express

      Volume: 11 Issue: 5 Pages: 053003-053003

    • DOI

      10.7567/apex.11.053003

    • NAID

      210000136194

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Anatomy of interfacial spin-orbit coupling in Co/Pd multilayers using X-ray magnetic circular dichroism and first-principles calculations2018

    • Author(s)
      Okabayashi Jun、Miura Yoshio、Munekata Hiro
    • Journal Title

      Scientific Reports

      Volume: 8 Issue: 1 Pages: 83031-9

    • DOI

      10.1038/s41598-018-26195-w

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] A lateral-type spin-photodiode based on Fe/x-AlOx/p-InGaAs junctions with a refracting-facet side window2018

    • Author(s)
      Roca Ronel Christian、Nishizawa Nozomi、Nishibayashi Kazuhiro、Munekata Hiro
    • Journal Title

      Journal of Applied Physics

      Volume: 123 Issue: 21 Pages: 213903-213903

    • DOI

      10.1063/1.5026511

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Imaging in-plane 90° magnetization switching in a (Ga,Mn)As epitaxial layer2018

    • Author(s)
      Al-Qadi B.、Sakatoku Y.、Nishizawa N.、Munekata H.
    • Journal Title

      Journal of Applied Physics

      Volume: 124 Issue: 6 Pages: 0639011-8

    • DOI

      10.1063/1.5040129

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 光スピントロニクス:基礎と進展2018

    • Author(s)
      宗片比呂夫
    • Journal Title

      J. Optics(光学)

      Volume: 47 Pages: 132-142

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] Line-Scan-Detections of Cancerous Tissues with Circularly-Polarized Light2020

    • Author(s)
      Nozomi Nishizawa, Takahiro Kuchimaru, Hiro MUNEKATA
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Depth Resolution of Cancer Detection with Scattered Circularly-Polarized Light2020

    • Author(s)
      Nozomi Nishizawa, Shinya Kawashima, Takahiro Kuchimaru, Hiro MUNEKATA
    • Organizer
      第81回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 円偏光散乱を用いたがん検出の空間分解能2020

    • Author(s)
      Nozomi Nishizawa, Takahiro Kuchimaru, Hiro MUNEKATA
    • Organizer
      生体医工学シンポジウム2020
    • Related Report
      2020 Annual Research Report
  • [Presentation] 円偏光発光ダイオードとがん検出応用2020

    • Author(s)
      Nozomi Nishizawa, Hiro MUNEKATA
    • Organizer
      令和3年 東北大学電気通信研究所 共同プロジェクト研究会 「固体中のスピン・軌道ダイナミクスとその制御」
    • Related Report
      2020 Annual Research Report
  • [Presentation] Verification of cancer identifications with circular polarized light scattering2020

    • Author(s)
      N. Nishizawa, H. Munekata, B. Al-Qadi, T. Kuchimaru, K. Hara
    • Organizer
      生体医歯工学共同研究拠点 令和2年度成果報告会
    • Related Report
      2020 Annual Research Report
  • [Presentation] 研究の三色旗:自由、寛大、洞察2020

    • Author(s)
      宗片比呂夫
    • Organizer
      第25回半導体スピン工学(大阪)
    • Related Report
      2020 Annual Research Report
  • [Presentation] Low-threshold pure-circular polarization electro-luminescence from spin-light-emitting diodes consisting of oxidized Al/AlAs tunnel barriers2020

    • Author(s)
      Hiro Munekata
    • Organizer
      Photonic West 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 円偏光散乱を用いたがん検出の実証2020

    • Author(s)
      西沢 望, 河島 眞弥, 宗片 比呂夫, Bassam Al-Qadi, 口丸 高弘, 原 和彦
    • Organizer
      令和元年度生体医歯工学共同研究拠点 成果報告会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 円偏光散乱を用いたがん検出2020

    • Author(s)
      西沢 望, Bassam Al-Qadi, 口丸 高弘, 宗片 比呂夫
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Recent progress in spin-LED: realization of pure circular polarization EL at room temperature with current density of 10 A/cm22019

    • Author(s)
      Nozomi Nishizawa and Hiro Munekata
    • Organizer
      SPIE Optics+Photonics 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Imparting Memory Functionality to Planar Wave-Guide Structure with Photo-Magnetic Materials2019

    • Author(s)
      H. Munekata, S. Ogawa, K. Michihiro, K. Nishibayashi, and N. Nishizawa
    • Organizer
      Magnetics and Optics Research International Symposium (MORIS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] An Application of Spin-LED: Unstraining and Non-Invasive Cancer Detection Using Circularly Polarized Light2019

    • Author(s)
      A. Hamada, H. Munekata, and N. Nishizawa
    • Organizer
      Magnetics and Optics Research International Symposium (MORIS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Electrical Circular Polarization Switching at Room Temperature with Spin-Polarized Light Emitting Diodes2019

    • Author(s)
      N. Nishizawa and H. Munekata
    • Organizer
      Magnetics and Optics Research International Symposium (MORIS2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Electroluminescence characteristics and spin dynamics of spin-light-emitting diodes (spin-LEDs) consisting of oxidized Al /AlAs tunneling barriers2019

    • Author(s)
      Ryohei Ito, Nozomi Nishizawa, and Hiro Munekata
    • Organizer
      The 21st International Conference on Electron Dynamics in Semiconductors, Optoelectronics and Nanostructures (EDISON21)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Non-invasive, unstaining, and in vivo diagnosis technique of tumor tissues using circularly polarized light;2019

    • Author(s)
      Nozomi Nishizawa, Kazumasa Takahashi, Atsushi Hamada, Takahiro Kuchimaru, and Hiro Munekata
    • Organizer
      SPIE Optics+Photonics 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Cancer Detection using circular polarization of light scattered by biological tissues2019

    • Author(s)
      N. Nishizawa, B. Al-Qadi, T. Kuchimaru, K. Takahashi, K. Hara, and H. Munekata
    • Organizer
      The 4th International Symposium on Biomedical Engineering (ISBE2019)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Low-threshold pure circular-polarization electroluminescence of spin-LEDs with oxidized Al/AlAs tunnel barriers2019

    • Author(s)
      H. Munekata, N. Nishizawa, and R. Ito
    • Organizer
      第24回半導体におけるスピン工学の基礎と応用
    • Related Report
      2019 Annual Research Report
  • [Presentation] 室温純粋円偏光発光ダイオードのメカニズム仮説を中心に2019

    • Author(s)
      宗片比呂夫
    • Organizer
      北大学電気通信研究所 共同プロジェクト研究会「固体中のスピン・ダイナミクスの物理と応用」ならびに「スピン軌道相互作用を介した磁化・スピンダイナミクスの電気的操作に関する研究」
    • Related Report
      2018 Annual Research Report
  • [Presentation] 磁化の光励起才差運動が極めて大きな多層積層Co/Pd 構造の作製2019

    • Author(s)
      小川竣太、西沢望、宗片比呂夫
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Co/Pd 多層積層膜の光パルス励起を経由するパーマロイのスピン波生成2019

    • Author(s)
      小野寺蓮太、西沢望、宗片比呂夫
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Imaging in-plane 90° magnetization switching in (Ga,Mn)As;2019

    • Author(s)
      B.Al-Qadi, Y. Sakatoku, N. Nishizawa, and H. Munekata
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Nearly pure circular polarization electroluminescence from spin-LED with significantly reduced current densities2019

    • Author(s)
      N. Nishizawa and H. Munekata
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Experimental evidence for non-thermal aspect of photo-excited precession of magnetization in (Ga,Mn)As2019

    • Author(s)
      Hiro Munekata and Takashi Matsuda
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Consideration on a mechanism of pure circular polarization electroluminescence in a lateral spin-LED2018

    • Author(s)
      H. Munekata and N. Nishizawa
    • Organizer
      Conference on Lasers and Electro-Optics (CLEO 2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of a novel, non-invasive and unstaining diagnosis technique of cancerous tissues using circularly polarized light;2018

    • Author(s)
      N. Nishizawa, K. Takahashi, A. Hamada, T. Kuchimaru, K. Hara, and H. Munekata
    • Organizer
      The 3rd International Symposium on Biomedical Engineering
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Preparation of a Phantom: A Step Toward Application of a Spin-LED for Unstained and Non-Invasive Cancer Detection;2018

    • Author(s)
      N. Nishizawa, K. Takahashi, T. Kuchimaru, and H. Munekata
    • Organizer
      2018 Workshop on Innovative Nanoscale Devices and Systems (WINDS2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Realization of Pure Circular Polarization Electroluminescence at Room Temperature with Spin-LEDs;2018

    • Author(s)
      H. Munekata and N. Nishizawa
    • Organizer
      2018 Workshop on Innovative Nanoscale Devices and Systems (WINDS2018)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Arbitrary helicity control of circular polarization state from lateral-type spin-LED at room temperature2018

    • Author(s)
      N. Nishizawa and H. Munekata
    • Organizer
      第79回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Experimental evidence of non-thermal aspect of photo-excited precession of magnetization in (Ga,Mn)As;2018

    • Author(s)
      H. Munekata and T. Matsuda
    • Organizer
      第23回半導体におけるスピン工学の基礎と応用 (PASPS-23)
    • Related Report
      2018 Annual Research Report
  • [Presentation] パーマロイ表面に形成したCo/Pd極薄多層積層膜の光誘起磁化才差運動2018

    • Author(s)
      小野寺蓮太, 西沢 望, 宗片 比呂夫
    • Organizer
      第23回半導体におけるスピン工学の基礎と応用 (PASPS-23)
    • Related Report
      2018 Annual Research Report
  • [Presentation] Second-generation spin-LEDs having nearly pure circular polarization electroluminescence with x-AlOx/AlAs hybrid tunneling barriers;2018

    • Author(s)
      N. Nishizawa and H. Munekata
    • Organizer
      第23回半導体におけるスピン工学の基礎と応用 (PASPS-23)
    • Related Report
      2018 Annual Research Report
  • [Presentation] Imaging in-plane magnetization switching in a (Ga, Mn)As epitaxial layer;2018

    • Author(s)
      B. Al-Qadi, Y. Sakatoku, N. Nishizawa, and H. Munekata
    • Organizer
      第23回半導体におけるスピン工学の基礎と応用 (PASPS-23)
    • Related Report
      2018 Annual Research Report
  • [Remarks] 室温で発光する円偏光スピンLEDの創製に成功―多分野への応用が期待される光源の登場―

    • URL

      https://www.titech.ac.jp/news/2017/037434.html

    • Related Report
      2018 Annual Research Report

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Published: 2018-04-23   Modified: 2022-01-27  

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