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Scanning tunneling microscopy for the development of ultimate nano-optics

Research Project

Project/Area Number 18H05257
Research Category

Grant-in-Aid for Scientific Research (S)

Allocation TypeSingle-year Grants
Review Section Broad Section D
Research InstitutionInstitute of Physical and Chemical Research

Principal Investigator

金 有洙  国立研究開発法人理化学研究所, 開拓研究本部, 主任研究員 (50373296)

Co-Investigator(Kenkyū-buntansha) 数間 恵弥子  国立研究開発法人理化学研究所, 開拓研究本部, 研究員 (50633864)
今田 裕  国立研究開発法人理化学研究所, 開拓研究本部, 上級研究員 (80586917)
山本 駿玄  国立研究開発法人理化学研究所, 開拓研究本部, 研究員 (50802782)
Project Period (FY) 2018-06-11 – 2023-03-31
Project Status Granted (Fiscal Year 2022)
Budget Amount *help
¥195,780,000 (Direct Cost: ¥150,600,000、Indirect Cost: ¥45,180,000)
Fiscal Year 2022: ¥27,040,000 (Direct Cost: ¥20,800,000、Indirect Cost: ¥6,240,000)
Fiscal Year 2021: ¥22,360,000 (Direct Cost: ¥17,200,000、Indirect Cost: ¥5,160,000)
Fiscal Year 2020: ¥22,360,000 (Direct Cost: ¥17,200,000、Indirect Cost: ¥5,160,000)
Fiscal Year 2019: ¥53,560,000 (Direct Cost: ¥41,200,000、Indirect Cost: ¥12,360,000)
Fiscal Year 2018: ¥70,460,000 (Direct Cost: ¥54,200,000、Indirect Cost: ¥16,260,000)
Keywords近接場光 / 走査トンネル顕微鏡 / 単一分子 / エネルギー移動・変換 / 表面
Outline of Annual Research Achievements

研究項目①~④の各実績の概要は以下の通りであり、順調に研究が進行している。
研究項目①:昨年度はジアリルエテン分子膜のスイッチング挙動について調べ、一部の分子が変化している様子が確認された。詳細を調べるため、ジアリルエテン単一分子のスイッチング挙動について詳細に調べたところ、トンネル電流を印加することで閉環体から開環体と考えられる一方向の変化が観察された。
研究項目②:昨年度に構築した近接場増強フォトルミネッセンスの計測システムを用いて、ドナー分子とアクセプター分子のそれぞれの孤立状態の物性を精査している。さらに独自に開発したCWレーザーでの精密レーザーナノ分光手法と合わせて、空間・エネルギーおよび空間・時間領域で高精度に分子間エネルギー移動を分光計測できるようになった。
研究項目③:昨年度、数psのパルス幅を持つレーザーを励起源として、STM探針先端に局在するプラズモン共鳴による電場増強効果を利用した、非線形光学現象である第二次高調波発生の観測に成功している。現在は二つの同期したパルスレーザーを励起源とした、差周波発生と和周波発生の実験を進めている。
研究項目④:局在表面プラズモンによる光学増強が可能となるスピン偏極STM探針を作製/手法確立するため、貴金属探針の先端を磁性体でコートする探針作製とその評価を行った。これにより、外部から導入した光磁場を増強しつつ磁性観測が可能となると期待できる。現在は、作製したコート探針で生じるプラズモン誘起発光の様子と印加磁場との相関関係を調査している。

Research Progress Status

翌年度、交付申請を辞退するため、記入しない。

Strategy for Future Research Activity

翌年度、交付申請を辞退するため、記入しない。

Assessment Rating
Ex-post Assessment Comments (Rating)

A+: In light of the aim of introducing the research area into the research categories, more research outcomes have been produced than expected.

Assessment Rating
Interim Assessment Comments (Rating)

A: In light of the aim of introducing the research area into the research categories, the expected progress has been made in research.

Report

(9 results)
  • 2023 Ex-post Assessment (Comments) ( PDF )
  • 2021 Annual Research Report
  • 2020 Abstract (Interim Assessment) ( PDF )   Annual Research Report   Interim Assessment (Comments) ( PDF )
  • 2019 Annual Research Report
  • 2018 Abstract ( PDF )   Comments on the Screening Results ( PDF )   Annual Research Report
  • Research Products

    (116 results)

All 2022 2021 2020 2019 Other

All Int'l Joint Research (11 results) Journal Article (22 results) (of which Int'l Joint Research: 11 results,  Peer Reviewed: 20 results,  Open Access: 3 results) Presentation (74 results) (of which Int'l Joint Research: 25 results,  Invited: 37 results) Remarks (8 results) Patent(Industrial Property Rights) (1 results)

  • [Int'l Joint Research] University of the Philippines Diliman(フィリピン)

    • Related Report
      2021 Annual Research Report
  • [Int'l Joint Research] University of Illinois Chicago(米国)

    • Related Report
      2021 Annual Research Report
  • [Int'l Joint Research] University of Ulsan/Seoul National University/GIST(韓国)

    • Related Report
      2021 Annual Research Report
  • [Int'l Joint Research] University of the Philippines(フィリピン)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] University of Illinois Chicago/UC Santa Barbara(米国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] University of Ulsan/Seoul National University/GIST(韓国)

    • Related Report
      2020 Annual Research Report
  • [Int'l Joint Research] University of Ulsan/GIST/UNIST(韓国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] University of Illinois Chicago(米国)

    • Related Report
      2019 Annual Research Report
  • [Int'l Joint Research] CNRS(フランス)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] University of Illinois Chicago(米国)

    • Related Report
      2018 Annual Research Report
  • [Int'l Joint Research] University of Ulsan(韓国)

    • Related Report
      2018 Annual Research Report
  • [Journal Article] Orbital-resolved visualization of single-molecule photocurrent channels2022

    • Author(s)
      Imai-Imada Miyabi、Imada Hiroshi、Miwa Kuniyuki、Tanaka Yusuke、Kimura Kensuke、Zoh Inhae、Jaculbia Rafael B.、Yoshino Hiroko、Muranaka Atsuya、Uchiyama Masanobu、Kim Yousoo
    • Journal Title

      Nature

      Volume: 603 Issue: 7903 Pages: 829-834

    • DOI

      10.1038/s41586-022-04401-0

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Dissociation of Single O <sub>2</sub> Molecules on Ag(110) by Electrons, Holes, and Localized Surface Plasmons2022

    • Author(s)
      Lee Minhui、Kazuma Emiko、Jung Jaehoon、Trenary Michael、Kim Yousoo
    • Journal Title

      The Chemical Record

      Volume: e202200011 Issue: 6

    • DOI

      10.1002/tcr.202200011

    • Related Report
      2021 Annual Research Report
  • [Journal Article] Visualization of Frontier Molecular Orbital Separation of a Single Thermally Activated Delayed Fluorescence Emitter by STM2021

    • Author(s)
      Zoh Inhae、Imai-Imada Miyabi、Bae Jaehyun、Imada Hiroshi、Tsuchiya Youichi、Adachi Chihaya、Kim Yousoo
    • Journal Title

      The Journal of Physical Chemistry Letters

      Volume: 12 Issue: 31 Pages: 7512-7518

    • DOI

      10.1021/acs.jpclett.1c02140

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Single-molecule laser nanospectroscopy with micro-electron volt energy resolution2021

    • Author(s)
      H. Imada, M. Imai-Imada, K. Miwa, H. Yamane, T. Iwasa, Y. Tanaka, N. Toriumi, K. Kimura, N. Yokoshi, A. Muranaka, M. Uchiyama, T. Taketsugu, Y. K. Kato, H. Ishihara, Y. Kim
    • Journal Title

      Science

      Volume: 373(6550) Issue: 6550 Pages: 95-98

    • DOI

      10.1126/science.abg8790

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Dissociation Mechanism of a Single O<sub>2</sub> Molecule Chemisorbed on Ag(110)2021

    • Author(s)
      Lee Minhui、Kazuma Emiko、Zhang Chi、Trenary Michael、Takeya Jun、Jung Jaehoon、Kim Yousoo
    • Journal Title

      The Journal of Physical Chemistry Letters

      Volume: 12 Issue: 40 Pages: 9868-9873

    • DOI

      10.1021/acs.jpclett.1c02456

    • Related Report
      2021 Annual Research Report
  • [Journal Article] Terahertz-Field-Driven Scanning Tunneling Luminescence Spectroscopy2021

    • Author(s)
      Kimura Kensuke、Morinaga Yuta、Imada Hiroshi、Katayama Ikufumi、Asakawa Kanta、Yoshioka Katsumasa、Kim Yousoo、Takeda Jun
    • Journal Title

      ACS Photonics

      Volume: 8 Issue: 4 Pages: 982-987

    • DOI

      10.1021/acsphotonics.0c01755

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Tunable Optical Transition in 2H-MoS<sub>2</sub> via Direct Electrochemical Engineering of Vacancy Defects and Surface SC Bonds2020

    • Author(s)
      Park Younghee、Shin Seunghyun、An Youngjoon、Ahn Jong-Guk、Shin Geumbi、Ahn Chaehyeon、Bang Jiwon、Baik Jaeyoon、Kim Yousoo、Jung Jaehoon、Lim Hyunseob
    • Journal Title

      ACS Applied Materials and Interfaces

      Volume: 12 Issue: 36 Pages: 40870-40878

    • DOI

      10.1021/acsami.0c09096

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] EXPRESS: Controlling the Resonance Raman Effect in Tip-Enhanced Raman Spectroscopy Using a Thin Insulating Film2020

    • Author(s)
      Jaculbia Rafael、Hayazawa Norihiko、Imada Hiroshi、Kim Yousoo
    • Journal Title

      Applied Spectroscopy

      Volume: 11 Issue: 11 Pages: 1391-1397

    • DOI

      10.1177/0003702820938366

    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Single-molecule study of a plasmon-induced reaction for a strongly chemisorbed molecule2020

    • Author(s)
      Emiko Kazuma, Minhui Lee, Jaehoon Jung, Michael Trenary, Yousoo Kim,
    • Journal Title

      Angewandte Chemie International Edition

      Volume: 59 Issue: 20 Pages: 7960-7966

    • DOI

      10.1002/anie.202001863

    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Centimeter-Scale and Highly Crystalline Two-Dimensional Alcohol: Evidence for Graphenol (C<sub>6</sub>OH)2020

    • Author(s)
      Lim Hyunseob、Park Younghee、Lee Minhui、Ahn Jong-Guk、Li Bao Wen、Luo Da、Jung Jaehoon、Ruoff Rodney S.、Kim Yousoo
    • Journal Title

      Nano Letters

      Volume: 20 Issue: 3 Pages: 2107-2112

    • DOI

      10.1021/acs.nanolett.0c00103

    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Single-molecule resonance Raman effect in a plasmonic nanocavity2020

    • Author(s)
      Jaculbia Rafael B.、Imada Hiroshi、Miwa Kuniyuki、Iwasa Takeshi、Takenaka Masato、Yang Bo、Kazuma Emiko、Hayazawa Norihiko、Taketsugu Tetsuya、Kim Yousoo
    • Journal Title

      Nature Nanotechnology

      Volume: 15 Issue: 2 Pages: 105-110

    • DOI

      10.1038/s41565-019-0614-8

    • Related Report
      2020 Annual Research Report 2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Self-Consistent Tip Conditioning for Tip-Enhanced Raman Spectroscopy in an Ambient Environment2020

    • Author(s)
      Yokota Yasuyuki、Hong Misun、Hayazawa Norihiko、Yang Bo、Kazuma Emiko、Kim Yousoo
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 124 Issue: 42 Pages: 23243-23252

    • DOI

      10.1021/acs.jpcc.0c07579

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 走査トンネル顕微鏡で観る単一分子内における励起子形成:三重項励起子を選択的に形成する新たな機構2020

    • Author(s)
      木村謙介, 三輪邦之, 今田裕, 金有洙
    • Journal Title

      固体物理

      Volume: 55 Pages: 149-159

    • NAID

      40022235522

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Homogeneous Dispersion of Aromatic Thiolates in the Binary Self-Assembled Monolayer on Au(111) via Displacement Revealed by Tip-Enhanced Raman Spectroscopy2020

    • Author(s)
      Hong Misun、Yokota Yasuyuki、Hayazawa Norihiko、Kazuma Emiko、Kim Yousoo
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 124 Issue: 24 Pages: 13141-13149

    • DOI

      10.1021/acs.jpcc.0c01507

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Scanning tunneling microscopic investigations for studying conformational change of underlying Cu(111) and Ni(111) during graphene growth2020

    • Author(s)
      Ahn Jong-Guk、Bang Jiwon、Jung Jaehoon、Kim Yousoo、Lim Hyunseob
    • Journal Title

      Surface Science

      Volume: 693 Pages: 121526-121526

    • DOI

      10.1016/j.susc.2019.121526

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Self-Assembly Growth of an Upright Molecular Precursor with a Rigid Framework2019

    • Author(s)
      Chaunchaiyakul Songpol、Zhang Chi、Imada Hiroshi、Kazuma Emiko、Ishiwari Fumitaka、Shoji Yoshiaki、Fukushima Takanori、Kim Yousoo
    • Journal Title

      The Journal of Physical Chemistry C

      Volume: 123 Issue: 51 Pages: 31272-31278

    • DOI

      10.1021/acs.jpcc.9b09948

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Atomic‐Scale Visualization of the Stepwise Metal‐Mediated Dehalogenative Cycloaddition Reaction Pathways: Competition between Radicals and Organometallic Intermediates2019

    • Author(s)
      Zhang Chi、Kazuma Emiko、Kim Yousoo
    • Journal Title

      Angewandte Chemie International Edition

      Volume: 58 Issue: 49 Pages: 17736-17744

    • DOI

      10.1002/anie.201909111

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Scanning probe microscopy for real-space observations of local chemical reactions induced by localized surface plasmon2019

    • Author(s)
      Emiko Kazuma, Yousoo Kim
    • Journal Title

      Physical Chemistry Chemical Physics

      Volume: 21 Issue: 36 Pages: 19720-19731

    • DOI

      10.1039/c9cp02100k

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Selective triplet exciton formation in a single molecule2019

    • Author(s)
      Kimura Kensuke、Miwa Kuniyuki、Imada Hiroshi、Imai-Imada Miyabi、Kawahara Shota、Takeya Jun、Kawai Maki、Galperin Michael、Kim Yousoo
    • Journal Title

      Nature

      Volume: 570 Issue: 7760 Pages: 210-213

    • DOI

      10.1038/s41586-019-1284-2

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Many-Body State Description of Single-Molecule Electroluminescence Driven by a Scanning Tunneling Microscope2019

    • Author(s)
      Miwa Kuniyuki、Imada Hiroshi、Imai-Imada Miyabi、Kimura Kensuke、Galperin Michael、Kim Yousoo
    • Journal Title

      Nano Letters

      Volume: 19 Issue: 5 Pages: 2803-2811

    • DOI

      10.1021/acs.nanolett.8b04484

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Mechanistic Studies of Plasmon Chemistry on Metal Catalysts2019

    • Author(s)
      Kazuma Emiko、Kim Yousoo
    • Journal Title

      Angewandte Chemie International Edition

      Volume: 58 Issue: 15 Pages: 4800-4808

    • DOI

      10.1002/anie.201811234

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] On‐Surface Evolution of meso ‐Isomerism in Two‐Dimensional Supramolecular Assemblies2019

    • Author(s)
      Park Juyeon、Kim Ju‐Hyung、Bak Sunmi、Tahara Kazukuni、Jung Jaehoon、Kawai Maki、Tobe Yoshito、Kim Yousoo
    • Journal Title

      Angewandte Chemie International Edition

      Volume: 58 Issue: 28 Pages: 9611-9618

    • DOI

      10.1002/anie.201904290

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] 走査トンネル顕微鏡と近接場光学の融合による単一分子ナノ分光2022

    • Author(s)
      今田裕
    • Organizer
      北大理論化学シンポジウム:光と分子の相互作用
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] STM study of overtone-mode induced dissociation of a single O2 molecule chemisorbed on Ag(110)2022

    • Author(s)
      李 民喜, 数間 恵弥子,竹谷 純一,金 有洙
    • Organizer
      NanospecFY2021mini
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 光走査トンネル顕微鏡を用いた単一分子反応の観察2022

    • Author(s)
      数間 恵弥子
    • Organizer
      電気化学会第89回大会
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] プラズモン誘起解離反応の実空間研究2022

    • Author(s)
      数間 恵弥子
    • Organizer
      日本物理学会第77回年次大会
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] Precise investigation of the resonance state of a single molecule in a plasmonic nanocavity2021

    • Author(s)
      Hiroshi Imada
    • Organizer
      Pacifichem 2021
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Orbital-resolved visualization of exciton creation and annihilation in a single molecule2021

    • Author(s)
      Miyabi Imai-Imada, Hiroshi Imada, Kensuke Kimura, Kuniyuki Miwa, Jun Takeya, Yousoo Kim
    • Organizer
      Pacifichem 2021
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] STM Visualization of Frontier Molecular Orbital Separation of a Single TADF Emitter2021

    • Author(s)
      Inhae Zoh, Miyabi Imai-Imada, Jaehyun Bae, Hiroshi Imada, Youichi Tsuchiya, Chihaya Adachi, and Yousoo Kim
    • Organizer
      The 9th International Symposium on Surface Science
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Single-molecule precise laser nanospectroscopy2021

    • Author(s)
      Hiroshi Imada, Miyabi Imai-Imada, Kuniyuki Miwa, Hidemasa Yamane, Takeshi Iwasa, Yusuke Tanaka, Naoyuki Toriumi, Kensuke Kimura, Nobuhiko Yokoshi, Atsuya Muranaka, Masanobu Uchiyama, Tetsuya Taketsugu, Yuichiro K. Kato, Hajime Ishihara, Yousoo Kim
    • Organizer
      The 9th International Symposium on Surface Science
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Atomic-scale investigation of single-molecule photocurrent generation2021

    • Author(s)
      Miyabi Imai-Imada, Hiroshi Imada, Kuniyuki Miwa, Yusuke Tanaka, Kensuke Kimura, Inhae Zoh, Rafael B. Jaculbia, Hiroko Yoshino, Atsuya Muranaka, Masanobu Uchiyama, Yousoo Kim
    • Organizer
      The 9th International Symposium on Surface Science
    • Related Report
      2021 Annual Research Report
  • [Presentation] Single-molecule laser nanospectroscopy using near-field optics with scanning tunneling microscopy2021

    • Author(s)
      Hiroshi Imada
    • Organizer
      The Eighth NYCU-RIKEN Symposium on Physical and Chemical Sciences
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 先端的光源と走査トンネル顕微鏡の融合による極微分光2021

    • Author(s)
      今田裕
    • Organizer
      第13回放射光学会若手研究会「先端的レーザー分光測定技術の進化とその応用」
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] STM Visualization of Frontier Molecular Orbital Separation of a Single Thermally Activated Delayed Fluorescence Emitter2021

    • Author(s)
      趙仁海, 今井みやび, 裵宰玄, 今田裕, 土屋陽一,安達千波矢, 金有洙
    • Organizer
      表面・界面スペクトロスコピー2021
    • Related Report
      2021 Annual Research Report
  • [Presentation] 光STMを用いた単一分子の精密ナノ分光2021

    • Author(s)
      今田裕
    • Organizer
      2021年日本表面真空学会学術講演会
    • Related Report
      2021 Annual Research Report
    • Invited
  • [Presentation] 半導体GaAsの帯電したドーパント近傍におけるトンネルスピン注入効率の局所変調観察2021

    • Author(s)
      山本駿玄
    • Organizer
      表面界面スペクトロスコピー
    • Related Report
      2021 Annual Research Report
  • [Presentation] Single-molecule studies of plasmon-induced dissociation reactions on metal surfaces using STM2021

    • Author(s)
      Emiko Kazuma, Minhui Lee, Jung, Jaehoon, Michael Trenary, Yousoo Kim
    • Organizer
      Pacifichem 2021
    • Related Report
      2021 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Ag underpotential deposition at thiolate/Au interface on surface-enhanced Raman spectroscopy2021

    • Author(s)
      M. Hong, 横田泰之, R. A. Wong, 早澤紀彦, 数間恵弥子, 金有洙
    • Organizer
      2021年電気化学会第88回大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 大気中探針増強ラマン分光における自己収束的探針先端加工: 増強効果とSTM像への影響2021

    • Author(s)
      横田泰之, M. Hong, 早澤紀彦, 楊波, 数間恵弥子, 金有洙
    • Organizer
      2021年電気化学会第88回大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] STM発光分光法を用いた強磁性体Feと半導体GaAsのトンネル接合におけるエネルギー励起測定2021

    • Author(s)
      山本駿玄, 今田裕, 金有洙
    • Organizer
      2021年第68回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Investigation of luminescence from a localized plasmon induced by THz-field-driven tunneling electrons2021

    • Author(s)
      K. Kimura, Y. Morinaga, H. Imada, I. Kayayama, K. Asakawa, K. Yoshioka, Y. Kim, J. Takeda
    • Organizer
      2021年第68回応用物理学会春季学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 光STMを用いた単一分子内での無輻射緩和過程の実時空間計測2021

    • Author(s)
      今井みやび, 今田裕, 三輪邦之, 木村謙介, I. Zoh, 金有洙
    • Organizer
      日本物理学会2021年第76回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Visualization of frontier molecular orbitals of a TADF emitter at molecular interfaces2021

    • Author(s)
      I. Zoh, M. Imai-Imada, H. Imada, J. Bae, Y. Tsuchiya, C. Adachi, Y. Kim
    • Organizer
      日本物理学会2021年第76回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] 光STMを用いたナフタロシアニン単一分子の光学特性評価2021

    • Author(s)
      今田裕, 今井みやび, 三輪邦之, 金有洙
    • Organizer
      日本物理学会2021年第76回年次大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Single-molecule study of the plasmon-Induced dissociation of O2 molecules2020

    • Author(s)
      E. Kazuma, M. Lee, J. Jung, M. Trenary, Y. Kim
    • Organizer
      The 5th International Workshop on Advanced Nanoscience and Nanomaterials 2020
    • Related Report
      2020 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Tip-enhanced Raman spectroscopy and imaging of a single molecule in ultrahigh vacuum and low temperature environments2020

    • Author(s)
      R. B. Jaculbia, H. Imada, N. Hayazawa, Y. Kim
    • Organizer
      The Philippine-American Academy of Science and Engineering
    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] STM study on electronic structure of TADF emitter2020

    • Author(s)
      I. Zoh, M. Imai-Imada, H. Imada, Y. Kim
    • Organizer
      第14回表面・界面スペクトロスコピー2020
    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Invited
  • [Presentation] 単一酸素分子のプラズモン誘起解離反応の実空間観測2020

    • Author(s)
      数間恵弥子
    • Organizer
      分子研研究会 「ナノ空間で光が織りなす分子操作・化学反応制御の新展開」
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] 単一分子プラズモン誘起解離反応の光STM観測・解析2020

    • Author(s)
      数間恵弥子
    • Organizer
      ACE Meeting Online II
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] STMを用いた単一分子の精密レーザー分光2020

    • Author(s)
      今田裕, 今井みやび, 三輪邦之, 木村謙介, 金有洙
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
  • [Presentation] STM発光分光法による単一分子励起・脱励起過程の実空間計測2020

    • Author(s)
      今井みやび, 今田裕, 木村謙介, 三輪邦之, 竹谷純一, 金有洙
    • Organizer
      日本物理学会2020年秋季大会
    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
  • [Presentation] プラズモンが誘起する単一分子化学反応の実空間観測2020

    • Author(s)
      数間恵弥子
    • Organizer
      JST ・触媒学会共催オンライン公開シンポジウム-革新的触媒と反応制御の今後-
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] 光STMを用いたプラズモン誘起化学反応の単一分子レベル解析2020

    • Author(s)
      数間恵弥子
    • Organizer
      表面真空学会関東支部の講演会
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] Nanoscale analysis and control of chemical reactions induced by Iocalized surface plasmon2020

    • Author(s)
      数間恵弥子
    • Organizer
      日本化学会第100春季年会(2020)
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] STM発光分光法を用いた選択的な三重項励起子形成の単一分子計測2020

    • Author(s)
      木村謙介, 三輪邦之, 今田裕, 今井みやび, 河原祥太, 竹谷純一, 川合眞紀, マイケル ガルペリン, 金有洙
    • Organizer
      第48回応用物理学会秋季学術講演会
    • Related Report
      2020 Annual Research Report 2019 Annual Research Report
    • Invited
  • [Presentation] Single-molecule study of the plasmon-Induced dissociation of O2 molecules2020

    • Author(s)
      E. Kazuma, M. Lee, J. Jung, M. Trenary, Y. Kim
    • Organizer
      The 5th International Workshop on Advanced Nanoscience and Nanomaterials 2020 (5th IWANN2020)
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] 単一酸素分子のプラズモン誘起解離反応の実空間観測,2020

    • Author(s)
      數間恵弥子
    • Organizer
      分子研研究会 「ナノ空間で光が織りなす分子操作・化学反応制御の新展開」
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] 単一分子プラズモン誘起解離反応の光STM観測・解析2020

    • Author(s)
      數間恵弥子
    • Organizer
      ACE Meeting Online II,
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] 大気中探針増強ラマン分光測定における増強効果失活過程の検証と対策2020

    • Author(s)
      横田泰之, M. Hong, 早澤紀彦, 楊波, 数間恵弥子, 金有洙
    • Organizer
      2020年日本表面真空学会学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] プラズモンが誘起する単一分子化学反応の実空間観測2020

    • Author(s)
      數間恵弥子
    • Organizer
      JST ・触媒学会共催オンライン公開シンポジウム-革新的触媒と反応制御の今後-
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] 光STMを用いたプラズモン誘起化学反応の単一分子レベル解析2020

    • Author(s)
      數間恵弥子
    • Organizer
      表面真空学会関東支部の講演会
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Nanoscale analysis and control of chemical reactions induced by Iocalized surface plasmon2020

    • Author(s)
      數間恵弥子
    • Organizer
      日本化学会第100春季年会(2020)
    • Related Report
      2019 Annual Research Report
    • Invited
  • [Presentation] Tip-enhanced Raman spectroscopy of displacement process in mixed self-assembled monolayers of aromatic thiolates on Au(111)2020

    • Author(s)
      M. Hong, 横田泰之, 早澤紀彦, 數間恵弥子, 金有洙
    • Organizer
      2020年電気化学会第87回大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Nanoscale analysis and control of chemical reactions induced by Iocalized surface plasmon2020

    • Author(s)
      數間恵弥子
    • Organizer
      日本化学会第100春季年会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Single molecule tip-enhanced Resonance Raman spectroscopy in low temperature environments2019

    • Author(s)
      R. B. Jaculbia, H. Imada, K. Miwa, T. Iwasa, M. Takenaka, B. Yang, E. Kazuma, N. Hayazawa, T. Taketsugu, Y. Kim
    • Organizer
      Philippine-Japan Conference on Photonics and Optical materials
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Plasmon-exciton coupling at an STM junction: fundamental and applications for spatially-resolved single-molecule spectroscopy2019

    • Author(s)
      H. Imada
    • Organizer
      27th International Colloquium on Scanning Probe Microscopy (ICSPM27)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Visualization of exciton creation and annihilation in a single molecule2019

    • Author(s)
      M. Imai-Imada, H. Imada, K. Kimura, K. Miwa, J. Takeya, Y. Kim
    • Organizer
      27th International Colloquium on Scanning Probe Microscopy (ICSPM27)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Nonplanar stereochiral intermolecular interactions between upright molecular precursors2019

    • Author(s)
      S. Chaunchaiyakul, H. Imada, E. Kazuma, F. Ishiwari, Y. Shoji, T. Fukushima, Y. Kim
    • Organizer
      27th International Colloquium on Scanning Probe Microscopy (ICSPM27)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] STM study of exciton creation and annihilation in a single molecule2019

    • Author(s)
      H. Imada
    • Organizer
      The 81st Okazaki Conference "Forefront of Measurement Technologies for Surface Chemistry and Physics in Real-Space, k-Space, and Real-Time"
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Single molecule study of plasmon-induced chemical reactions2019

    • Author(s)
      E. Kazuma
    • Organizer
      The 81st Okazaki Conference "Forefront of Measurement Technologies for Surface Chemistry and Physics in Real-Space, k-Space, and Real-Time"
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Creation of spin singlet and triplet excitons in a single molecule2019

    • Author(s)
      K. Kimura, K. Miwa, H. Imada, M. Imai-Imada, Y. Kim
    • Organizer
      International School and Symposium on Nanoscale Transport and phoTonics (ISNTT2019)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] STM investigations of plasmon-induced single molecule reaction2019

    • Author(s)
      E. Kazuma
    • Organizer
      IBS-RIKEN Joint Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Atomic-scale study of exciton creation and annihilation in a molecular system2019

    • Author(s)
      H. Imada
    • Organizer
      IBS-RIKEN Joint Conference
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Investigation of selective triplet exciton formation in a molecule with an STM2019

    • Author(s)
      K. Kimura, K. Miwa, H. Imada, M. Imai-Imada, S. Kawahara, J. Takeya, M. Kawai, M. Galperin, Y. Kim
    • Organizer
      704.WE-Heraeus-Seminar "Exploring the Limits of Nanoscience with Scanning Probe Methods"
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Single-molecule optical spectroscopy2019

    • Author(s)
      Y. Kim
    • Organizer
      704.WE-Heraeus-Seminar "Exploring the Limits of Nanoscience with Scanning Probe Methods"
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Single-molecule chemistry and spectroscopy with a photon STM2019

    • Author(s)
      Y. Kim
    • Organizer
      The Seventh RIKEN-NCTU Symposium on Physical and Chemical Sciences
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Single-molecule chemistry and spectroscopy at surfaces2019

    • Author(s)
      Y. Kim
    • Organizer
      2019 RIKEN-NCHU Joint Symposium
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] Vibrationally resolved imaging of a single molecule using tip-enhanced Resonance Raman spectroscopy2019

    • Author(s)
      R. Jaculbia, H. Imada, K. Miwa, B. Yang, E. Kazuma, N. Hayazawa, Y. Kim
    • Organizer
      10th International Conference on Advanced Vibrational Spectroscopy (ICAVS10)
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Single-molecule chemistry and spectroscopy by near-field light2019

    • Author(s)
      Y. Kim
    • Organizer
      Annual Meeting of the Physical Society of Taiwan
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] 単一分子におけるエネルギー移動・変換・散逸の実空間計測と制御2019

    • Author(s)
      金有洙
    • Organizer
      第58回玉城嘉十郎教授記念 公開学術講演会 -界面を考える-
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] Atomic-scale visualization of the stepwise metal-mediated dehalogenative cycloaddition reaction pathways2019

    • Author(s)
      C. Zhang, E. Kazuma, Y. Kim
    • Organizer
      第13回 表面・界面スペクトロスコピー 2019
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] STM発光分光法を用いた選択的な三重項励起子形成の単一分子計測2019

    • Author(s)
      木村謙介, 三輪邦之, 今田裕, 今井みやび, 河原祥太, 竹谷純一, 川合眞紀, マイケル ガルペリン, 金有洙
    • Organizer
      第48回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 光STMを用いた単一分子分光2019

    • Author(s)
      今田裕, 三輪邦之, 今井みやび, 河原祥太, 木村謙介, 金有洙
    • Organizer
      2019年日本表面真空学会学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 走査トンネル顕微鏡を用いた単一分子の蛍光分光2019

    • Author(s)
      今田裕, 今井みやび, 木村謙介, 三輪邦之, 金有洙
    • Organizer
      第31回分子科学討論会
    • Related Report
      2018 Annual Research Report
  • [Presentation] STM発光分光法を用いた選択的な三重項励起子形成の単一分子計測2019

    • Author(s)
      木村謙介, 三輪邦之, 今田裕, 今井みやび, 河原祥太, 竹谷純一, 川合眞紀, マイケル ガルペリン, 金有洙
    • Organizer
      2019年第80回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Vibrational symmetry of a single molecule revealed by tip-enhanced Raman spectroscopy2019

    • Author(s)
      R. B. Jaculbia, H. Iamda, K. Miwa, T. Iwasa, M. Takenaka, B. Yang, E. Kazuma, N. Hayazawa, T. Taketsugu, Y. Kim
    • Organizer
      2019年第80回応用物理学会秋季学術講演会
    • Related Report
      2018 Annual Research Report
  • [Presentation] スピン偏極STM発光分光法を用いた原子精度でのスピン注入と磁気二色性の観測2019

    • Author(s)
      山本駿玄, 今田裕, 金有洙
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 単一分子接合系における光電変換に関する理論解析2019

    • Author(s)
      三輪邦之, 今田裕, 木村謙介, 今井みやび, 金有洙, M. Galperin
    • Organizer
      日本物理学会2019年秋季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 走査型トンネル顕微鏡による単一分子化学反応の解析2019

    • Author(s)
      數間惠弥子
    • Organizer
      分子研研究会「単分子有機化学の挑戦」
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 走査トンネル顕微鏡を用いた三重項励起子形成の単一分子計測2019

    • Author(s)
      金有洙
    • Organizer
      日本化学会第99春季年会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] スピン偏極STM発光分光法を用いた原子精度でのスピン注入と磁気二色性の観測2019

    • Author(s)
      山本駿玄, 今田裕, 金有洙
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 走査トンネル顕微鏡を用いた発光/吸収分光の開発と応用2019

    • Author(s)
      今田裕
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Presentation] 多体状態を基底とした単一分子の光電変換に関する理論解析2019

    • Author(s)
      三輪邦之, 今田裕, 木村謙介, 今井みやび, 金有洙, Michael Galperin
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] STMを用いた単一分子内での選択的な三重項励起子形成2019

    • Author(s)
      木村謙介, 今田裕, 三輪邦之, 今井みやび, 河原祥太, 竹谷純一, 川合眞紀, 金有洙
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] STM発光分光法を用いた単一分子での励起子生成・消滅過程の可視化2019

    • Author(s)
      今井みやび, 今田裕, 木村謙介, 三輪邦之, 竹谷純一, 金有洙
    • Organizer
      日本物理学会第74回年次大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] 近接場光と単一分子の相互作用の原子スケール解析:単一分子の光マニピュレーションに向けて2019

    • Author(s)
      今田裕
    • Organizer
      第66回応用物理学会春季学術講演会
    • Related Report
      2018 Annual Research Report
    • Invited
  • [Remarks] 理化学研究所Kim表面界面科学研究室

    • URL

      http://www2.riken.jp/Kimlab/index.html

    • Related Report
      2021 Annual Research Report
  • [Remarks] ナノの光による単一酸素分子の分解

    • URL

      https://www.riken.jp/press/2020/20200323_1/index.html

    • Related Report
      2020 Annual Research Report 2019 Annual Research Report 2018 Annual Research Report
  • [Remarks] 単一分子による共鳴ラマン散乱の可視化に成功

    • URL

      https://www.riken.jp/press/2020/20200217_1/index.html

    • Related Report
      2020 Annual Research Report 2018 Annual Research Report
  • [Remarks] Kim表面界面科学研究室

    • URL

      http://www2.riken.jp/Kimlab/index.html

    • Related Report
      2020 Annual Research Report
  • [Remarks] テラヘルツ光により超高速に操られたトンネル電子が引き起こす発光を初観測

    • URL

      https://www.riken.jp/press/2021/20210128_1/index.html

    • Related Report
      2019 Annual Research Report
  • [Remarks] 科学は人類の財産、未来への希望

    • URL

      https://www.jst.go.jp/pr/jst-news/backnumber/2020/202011/pdf/2020_11_p12.pdf

    • Related Report
      2019 Annual Research Report
  • [Remarks] 有機ELの新たな発光機構を発見

    • URL

      https://www.riken.jp/press/2019/20190606_1/

    • Related Report
      2018 Annual Research Report
  • [Remarks] 単一分子電界発光の機構解明

    • URL

      https://www.riken.jp/press/2019/20190301_1/

    • Related Report
      2018 Annual Research Report
  • [Patent(Industrial Property Rights)] 走査型トンネル顕微鏡及び方法2021

    • Inventor(s)
      今井みやび, 今田裕, 吉野紘子,金有洙
    • Industrial Property Rights Holder
      今井みやび, 今田裕, 吉野紘子,金有洙
    • Industrial Property Rights Type
      特許
    • Filing Date
      2021
    • Acquisition Date
      2021
    • Related Report
      2021 Annual Research Report

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Published: 2018-06-12   Modified: 2024-03-28  

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