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鉱物触媒水熱反応を用いた二酸化炭素の地中資源化システム

Research Project

Project/Area Number 18J12695
Research Category

Grant-in-Aid for JSPS Fellows

Allocation TypeSingle-year Grants
Section国内
Research Field Earth system and resources engineering
Research InstitutionTohoku University

Principal Investigator

WANG JIAJIE  東北大学, 環境科学研究科, 特別研究員(DC2)

Project Period (FY) 2018-04-25 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥1,900,000 (Direct Cost: ¥1,900,000)
Fiscal Year 2019: ¥900,000 (Direct Cost: ¥900,000)
Fiscal Year 2018: ¥1,000,000 (Direct Cost: ¥1,000,000)
KeywordsOlivine / Serpentinization / CO2 mineralization / Hydrogen production / serpentinization / carbonation / CO2 storage / Hydrocarbon
Outline of Annual Research Achievements

In this research year, reaction pathways and Fe behaviors during water-olivine-CO2 reactions under different reaction conditions were further summarized and published in the conferences of "17th ICCDU (Germany, 2019)" and 日本地球惑星科学連合大会(2019).
The influences of the most common coexisting minerals (i.e., pyroxenes and spinel) with olivine in peridotite in natural system were clarified. The presence of orthopyroxene or Mg-Al spinel can accelerate olivine alteration in CO2-rich hydrothermal environments and change Fe(II) behaviors without significant influence on the total H2 yield in terms of long-time reaction. However, the mineralization of CO2 could not be enhanced. The role of orthopyroxene and Mg-Al spinel also changed with the reaction time. These findings suggest that using peridotite that contains pyroxenes or spinels for H2 production is also possible; in general, peridotite contains <20 wt% orthopyroxene or >10 wt% Mg-Al spinel is more suitable for H2 production than monomineralic olivine. For another, several ways for elevating H2 production (e.g., including Al sources) were also suggested.
This part of research is a step forward in large-scale application of the new negative-carbon H2 production system. The results have been summarized into 2 papers published in the journal of “International Journal of Hydrogen energy (IF: 4.229)”.

Research Progress Status

令和元年度が最終年度であるため、記入しない。

Strategy for Future Research Activity

令和元年度が最終年度であるため、記入しない。

Report

(2 results)
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (15 results)

All 2020 2019 2018 Other

All Journal Article (4 results) (of which Int'l Joint Research: 3 results,  Peer Reviewed: 4 results,  Open Access: 3 results) Presentation (9 results) (of which Int'l Joint Research: 6 results) Remarks (2 results)

  • [Journal Article] Characteristics of hydrogen production with carbon storage by CO2-rich hydrothermal alteration of olivine in the presence of Mg?Al spinel2020

    • Author(s)
      Wang Jiajie、Watanabe Noriaki、Okamoto Atsushi、Nakamura Kengo、Komai Takeshi
    • Journal Title

      International Journal of Hydrogen Energy

      Volume: in press Issue: 24 Pages: 13163-13175

    • DOI

      10.1016/j.ijhydene.2020.03.032

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Acceleration of hydrogen production during water-olivine-CO2 reactions via high-temperature-facilitated Fe(II) release2019

    • Author(s)
      Wang Jiajie、Watanabe Noriaki、Okamoto Atsushi、Nakamura Kengo、Komai Takeshi
    • Journal Title

      International Journal of Hydrogen Energy

      Volume: 23 Issue: 23 Pages: 11514-11524

    • DOI

      10.1016/j.ijhydene.2019.03.119

    • Related Report
      2019 Annual Research Report 2018 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Pyroxene control of H2 production and carbon storage during water-peridotite-CO2 hydrothermal reactions2019

    • Author(s)
      Wang Jiajie、Watanabe Noriaki、Okamoto Atsushi、Nakamura Kengo、Komai Takeshi
    • Journal Title

      International Journal of Hydrogen Energy

      Volume: 44 Issue: 49 Pages: 26835-26847

    • DOI

      10.1016/j.ijhydene.2019.08.161

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access / Int'l Joint Research
  • [Journal Article] Enhanced hydrogen production with carbon storage by olivine alteration in CO2-rich hydrothermal environments2019

    • Author(s)
      Wang Jiajie、Watanabe Noriaki、Okamoto Atsushi、Nakamura Kengo、Komai Takeshi
    • Journal Title

      Journal of CO2 Utilization

      Volume: 30 Pages: 205-213

    • DOI

      10.1016/j.jcou.2019.02.008

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] Influence of pyroxene on peridotite alteration process and kinetics under CO2-rich hydrothermal conditions2019

    • Author(s)
      Wang Jiajie、Watanabe Noriaki、Okamoto Atsushi、Nakamura Kengo、Komai Takeshi
    • Organizer
      16th International Workshop on Water Dynamics
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Pyroxene control of peridotite alteration pathways and kinetics under CO2-rich hydrothermal conditions2019

    • Author(s)
      Wang Jiajie、Watanabe Noriaki、Okamoto Atsushi、Nakamura Kengo、Komai Takeshi
    • Organizer
      日本地球惑星科学連合 2019年大会
    • Related Report
      2019 Annual Research Report
  • [Presentation] NaHCO3-promoted H2 Production during Water-Olivine Reactions under High-temperature conditions2019

    • Author(s)
      Wang Jiajie、Watanabe Noriaki、Okamoto Atsushi、Nakamura Kengo、Komai Takeshi
    • Organizer
      17th International Conference on Carbon Dioxide Utilization
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] NaHCO3-promoted olivine weathering with H2 generation and CO2 sequestration in alkaline hydrothermal system2019

    • Author(s)
      Wang Jiajie、Watanabe Noriaki、Okamoto Atsushi、Nakamura Kengo、Komai Takeshi
    • Organizer
      9th International Conference on Future Environment and Energy
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Simultaneous olivine alteration and carbonation in CO2-rich geological condition: Mineral change and products investigation2018

    • Author(s)
      Wang Jiajie 、Nakamura Kengo、Watanabe Noriaki、Komai Takeshi
    • Organizer
      15th International workshop on water dynamics
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] CO2の貯蔵を利用したエネルギー生産:地殻リアクターの自然加熱中におけるカンラン石の結晶構造の変化2018

    • Author(s)
      Wang Jiajie 、Nakamura Kengo、Watanabe Noriaki、Komai Takeshi
    • Organizer
      平成30年度 資源・素材学会東北支部春季大会
    • Related Report
      2018 Annual Research Report
  • [Presentation] Simultaneous Olivine Alteration and Carbonation in CO2-Rich Geological Condition2018

    • Author(s)
      Wang Jiajie 、Nakamura Kengo、Watanabe Noriaki、Komai Takeshi
    • Organizer
      International Society of Offshore and Polar Engineers
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] CO2リッチ水熱環境における橄欖石の加速風化を用いた水素生成と炭素固定2018

    • Author(s)
      Wang Jiajie、Watanabe Noriaki、Okamoto Atsushi、Nakamura Kengo、Komai Takeshi
    • Organizer
      日本地熱学会 平成30年学術講演会(東京大会)
    • Related Report
      2018 Annual Research Report
  • [Presentation] Simultaneous H2 production with carbon storage by enhanced olivine weathering in laboratory-scale: An investigation of CO2 effect2018

    • Author(s)
      Wang Jiajie、Watanabe Noriaki、Okamoto Atsushi、Nakamura Kengo、Komai Takeshi
    • Organizer
      The Second International Conference on Materials Chemistry and Environmental Protection
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Remarks] Jiajie Wang (researchmap)

    • URL

      https://researchmap.jp/jiajie_wang1

    • Related Report
      2019 Annual Research Report
  • [Remarks] 駒井-渡邉研究室ホームページ

    • URL

      http://www.kankyo.tohoku.ac.jp/teacher/senshin008.html

    • Related Report
      2018 Annual Research Report

URL: 

Published: 2018-05-01   Modified: 2024-03-26  

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