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太陽光を利用した水中細菌の新規光触媒処理システムの開発

Research Project

Project/Area Number 18J20620
Research Category

Grant-in-Aid for JSPS Fellows

Allocation TypeSingle-year Grants
Section国内
Research Field Hygiene and public health
Research InstitutionUniversity of Tsukuba

Principal Investigator

LIU NA  筑波大学, 生命環境科学研究科, 特別研究員(DC1)

Project Period (FY) 2018-04-25 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥2,200,000 (Direct Cost: ¥2,200,000)
Fiscal Year 2020: ¥700,000 (Direct Cost: ¥700,000)
Fiscal Year 2019: ¥700,000 (Direct Cost: ¥700,000)
Fiscal Year 2018: ¥800,000 (Direct Cost: ¥800,000)
KeywordsPhotocatalyst / Glue immobilization / Water disinfection / Various bacteria / Disinfection mechanism / High stability / Visible-light-driven / Solar-light-driven / Gram-positive / Gram-negative
Outline of Annual Research Achievements

During the third fiscal year of my research, in order to test the practical application potential of the newly developed glue-immobilized P/Ag/Ag2O/Ag3PO4/TiO2 (PAgT) photocatalyst system for continuous-cycle sterilization, the study was carried out through the following three key points. (1) Evaluate the photocatalytic inactivation ability of the glue-immobilized PAgT photocatalyst for different kinds of pathogenic bacteria. (2) Investigate the stability and recyclability of the developed glue-immobilized photocatalyst reactor for the continuous-cycle water sterilization. (3) Clarify the disinfection mechanism involved during the immobilized PAgT photocatalyst system for the efficient water sterilization.
The result showed that the newly developed glue-immobilized PAgT photocatalyst system could effectively inactivate various pathogenic bacteria under light irradiation with excellent stability and reusability. The enhanced antibacterial performance of immobilized PAgT system was due to a synergistic effect of disinfection mechanism combining the improved photocatalysis on the introduction of heterojunction structure, and the mechanical stress driven from the composite sharp edge morphology. The present results reveal the possibility of applying the developed silicone glue-immobilized PAgT system for real water sterilization under solar light to further improve the public health level around the world, especially in the rural areas or at the time of disaster.

Research Progress Status

令和2年度が最終年度であるため、記入しない。

Strategy for Future Research Activity

令和2年度が最終年度であるため、記入しない。

Report

(3 results)
  • 2020 Annual Research Report
  • 2019 Annual Research Report
  • 2018 Annual Research Report
  • Research Products

    (35 results)

All 2021 2020 2019 2018

All Journal Article (7 results) (of which Peer Reviewed: 7 results) Presentation (28 results) (of which Int'l Joint Research: 9 results)

  • [Journal Article] Sol-gel/hydrothermal two-step synthesis strategy for promoting Ag species modified TiO2-based composite activity towards H2 evolution under solar light.2021

    • Author(s)
      Zhu, Q., Liu, N., Ma, Q., Sharma, Aditya, Nagai, D., Sun, X., Zhang, C., Yang, Y. N.
    • Journal Title

      Materials Today Energy.

      Volume: 20 Pages: 100648-100648

    • DOI

      10.1016/j.mtener.2021.100648

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Photon number based anaerobic digestion process for efficient bio-methane conversion from ammonium-rich feedstock: Performance evaluation and practical potential2021

    • Author(s)
      Zhu Yunxin、Zhang Nan、Liu Zhiyuan、Liu Na、Sharma Aditya、Chen Guoping、Yang Yingnan
    • Journal Title

      Energy Conversion and Management

      Volume: 238 Pages: 114155-114155

    • DOI

      10.1016/j.enconman.2021.114155

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed
  • [Journal Article] PEG assisted P/Ag/Ag2O/Ag3PO4/TiO2 photocatalyst with enhanced elimination of emerging organic pollutants in salinity condition under solar light illumination.2020

    • Author(s)
      Sharma, Aditya, Liu, N., Ma, Q., Zheng, H. Y., Kawazoe, N., Chen, G., Yang, Y. N.
    • Journal Title

      Chemical Engineering Journal.

      Volume: 385 Pages: 123765-123765

    • DOI

      10.1016/j.cej.2019.123765

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Polyethylene glycol (PEG)-modified Ag/Ag2O/Ag3PO4/Bi2WO6 photocatalyst film with enhanced efficiency and stability under solar light2020

    • Author(s)
      Ma, Q., Hu, X., Liu, N., Sharma, Aditya, Zhang, C., Kawazoe, N., Chen, G., Yang, Y. N.
    • Journal Title

      Journal of Colloid and Interface Science.

      Volume: 569 Pages: 101-113

    • DOI

      10.1016/j.jcis.2020.02.064

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Layered Ag/Ag2O/BiPO4/Bi2WO6 heterostructures by two-step method for enhanced photocatalysis2020

    • Author(s)
      Hu Xiaohong、Ma Qiansu、Wang Xinlong、Yang Yingjun、Liu Na、Zhang Cheng、Kawazoe Naoki、Chen Guoping、Yang Yingnan
    • Journal Title

      Journal of Catalysis

      Volume: 387 Pages: 28-38

    • DOI

      10.1016/j.jcat.2020.04.002

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Superior disinfection effect of Escherichia coli by hydrothermal synthesized TiO2-based composite photocatalyst under LED irradiation: Influence of environmental factors and disinfection mechanism2019

    • Author(s)
      Liu Na、Zhu Qi、Zhang Nan、Zhang Cheng、Kawazoe Naoki、Chen Guoping、Negishi Nobuaki、Yang Yingnan
    • Journal Title

      Environmental Pollution

      Volume: 247 Pages: 847-856

    • DOI

      10.1016/j.envpol.2019.01.082

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Development of Solar-light-driven Photocatalyst for energy and environmental application2019

    • Author(s)
      Liu, N, Zhu Q., Zhang, N., Wang, J., Yang, Y. N.
    • Journal Title

      Materials Science and Engineering

      Volume: 印刷中

    • Related Report
      2018 Annual Research Report
    • Peer Reviewed
  • [Presentation] Photocatalytic disinfection of novel composites Ag/Ag2O/BiPO4/Bi2WO6 under solar light irradiation2021

    • Author(s)
      Ming, J., Liu, N., Ma, Q., Yang, Y. N.
    • Organizer
      第9回日本生物工学会東日本支部コロキウム
    • Related Report
      2020 Annual Research Report
  • [Presentation] Highly Efficient Inactivation of Harmful Pathogenic Bacteria by a Stable Visible-light-driven TiO2-based Photocatalyst2020

    • Author(s)
      Liu, N., Ma, Q., Sharma, A., Ming, J., Yang, Y. N.
    • Organizer
      Water and Environment Technology (WET) Conference 2020-online
    • Related Report
      2020 Annual Research Report
  • [Presentation] Effective Elimination of Seawater Pollutants Using Surfactant Modified Using TiO2-based Composite Under Solar Light Illumination2020

    • Author(s)
      Sharma, A., Liu, N., Ma, Q. S., Yano, M., Yang, Y. N.
    • Organizer
      Water and Environment Technology (WET) Conference 2020-online
    • Related Report
      2020 Annual Research Report
  • [Presentation] Photocatalytic Inactivation of Escherichia coli by Ag/Ag2O/BiPO4/Bi2WO6 under Solar Light Irradiation: Effect of Environmental Factors and Disinfection Mechanism2020

    • Author(s)
      Ming, J., Liu, N., Ma, Q. S., Yang, Y. N.
    • Organizer
      Water and Environment Technology (WET) Conference 2020-online
    • Related Report
      2020 Annual Research Report
  • [Presentation] Development of an Adjustable Solar Light Tracking Reactor for Superior Photocatalytic Wastewater Treatment2020

    • Author(s)
      Zhang, C., Liu, N., Ming, J., Ma, Q. S., Yang, Y. N.
    • Organizer
      Water and Environment Technology (WET) Conference 2020-online
    • Related Report
      2020 Annual Research Report
  • [Presentation] Efficient destruction of different pathogenic microorganisms by a novel visible-light-driven TiO2-based photocatalyst2020

    • Author(s)
      Liu, N., Yang, Y. N.
    • Organizer
      第 8 回日本生物工学会東日本支部コロキウム
    • Related Report
      2019 Annual Research Report
  • [Presentation] Solar-light-driven Water Splitting for Hydrogen Evolution by A Novel TiO2 Based Photocatalyst2020

    • Author(s)
      Liu, N., Ma, Q., Ming, J., Negishi, N., Yang, Y. N.
    • Organizer
      85th SCEJ Annual meeting
    • Related Report
      2019 Annual Research Report
  • [Presentation] Characterization and Application of Non-ionic Surfactant Assisted TiO2 Based Composite for Enhanced Degradation of Organic Pollutant in Seawater2020

    • Author(s)
      Sharma A. Ma Q. S. Liu N. Zheng H., Yang, Y. N.
    • Organizer
      85th SCEJ Annual meeting
    • Related Report
      2019 Annual Research Report
  • [Presentation] Development of High Performance Graphene Oxide Modified Bi2WO6 Based Photocatalyst for Wastewater Treatment2020

    • Author(s)
      Ma Q. S. Ming J. Liu N., Zhang C., Yang, Y. N.
    • Organizer
      85th SCEJ Annual meeting
    • Related Report
      2019 Annual Research Report
  • [Presentation] Synergistic Effect of 3D Hierarchical Microsphere TiO2 by Carbon Doping for The Photocatalytic Antibiotic Degradation2020

    • Author(s)
      Sun X. Xu S. Liu N. Qi R., Yang, Y. N.
    • Organizer
      85th SCEJ Annual meeting
    • Related Report
      2019 Annual Research Report
  • [Presentation] Different Inactivation Behaviors of Gram-Positive and Gram-Negative Bacteria in TiO2 Based Photocatalytic Disinfection2019

    • Author(s)
      Liu, N., Zhang, C., Nobuaki, N., Yang, Y. N.
    • Organizer
      71st Society for Biotechnology Annual Meeting
    • Related Report
      2019 Annual Research Report
  • [Presentation] Investigation of Solar Driven Linear Fresnel Photocatalytic Reactor (LFP) for Wastewater Treatment2019

    • Author(s)
      Zhang, C., Liu, N., Ma, Q., Yagi, A., Yang, Y. N.
    • Organizer
      71st Society for Biotechnology Annual Meeting
    • Related Report
      2019 Annual Research Report
  • [Presentation] Green Route for Hydrogen Evolution from Pure Water Splitting Induced by A Solar Light Responsive Photocatalyst2019

    • Author(s)
      Liu, N., Nagai, D., Qi, R., Yang, Y. N.
    • Organizer
      The 2019 International Postgraduate Academic Forum
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Effective Wastewater Treatment with the Developed Liner Fresnel Photocatalytic reactor (LFP) Under Real Solar Light2019

    • Author(s)
      Zhang, C., Liu, N., Yagi, A., Yang, Y. N.
    • Organizer
      The 2019 International Postgraduate Academic Forum
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Characterization and Application of PEG modified TiO2 Based Photocatalyst for Improving Degradation of Organic Pollutant in Seawater2019

    • Author(s)
      Sharma, A., Liu, N., Ma, Q., Zheng, H., Yang, Y. N.
    • Organizer
      The 2019 International Postgraduate Academic Forum
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of Hydrothermal Synthesized Polyethylene Glycol Modified P/Ag/Ag2O/Ag3PO4/TiO2 Photocatalyst with Enhanced Photocatalytic Activity for Wastewater Treatment Under Visible Light Irradiation2019

    • Author(s)
      Yagi, A., Liu, N., Ma, Q., Zhang, C., Yang, Y. N.
    • Organizer
      The 2019 International Postgraduate Academic Forum
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Super-effective visible-light-induced photocatalytic water disinfection by a novel P/Ag/Ag2O/Ag3PO4/TiO2 composite and its mechanism2019

    • Author(s)
      Liu, N., Ma, Q., Zhang, C., Yang, Y. N.
    • Organizer
      International Conference on Environmental Protection and Climate Change 2019
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Insights into photocatalytic inactivation mechanism of a novel hydrothermal synthesized P/Ag/Ag2O/Ag3PO4/TiO2 photocatalyst with superior bactericidal activity2019

    • Author(s)
      Liu, N., Ma, Q., Negishi, N., Yang, Y. N.
    • Organizer
      第7回日本生物工学会東支部コロキウム
    • Related Report
      2018 Annual Research Report
  • [Presentation] Continuous Bio-hydrogen Production by Iron-modified Zeolite Addition in Hybrid Fixed-bed Reactor2019

    • Author(s)
      Zhao, C. Y., Zhang, N., Zheng, H. Y., Liu, N., Sharma, A., Yang, Y. N.
    • Organizer
      The 53rd Annual Conference of JSWE
    • Related Report
      2018 Annual Research Report
  • [Presentation] Enhanced Photocatalytic Activity of Graphene Oxide Modified Visible-light-driven Photocatalysts for Organic Pollutant Degradation2019

    • Author(s)
      Gu, W., Ma, Q. S., Liu, N., Zhang, N., Yang, Y. N.
    • Organizer
      84th SCEJ Annual Meeting
    • Related Report
      2018 Annual Research Report
  • [Presentation] Development of Linear Fresnel Photoreactor (LFP) for Water Purification Under Solar Light Irradiation2019

    • Author(s)
      Zhang, C., Liu, N., Ma, Q. S., Zhang, N., Yang, Y. N.
    • Organizer
      84th SCEJ Annual Meeting
    • Related Report
      2018 Annual Research Report
  • [Presentation] Effective Treatment of Seawater Pollutants Under Simulated Solar Light Using Modified-TiO2 Photocatalyst2019

    • Author(s)
      Sharma, A., Liu, N., Zhang, N., Ma, Q. S., Zhao, C. Y., Yang, Y. N.
    • Organizer
      84th SCEJ Annual Meeting
    • Related Report
      2018 Annual Research Report
  • [Presentation] Fabrication of High Performance and Stability Bi2WO6 Based Photocatalytic Thin Film Doping with Polyethylene Glycol for Wastewater Treatment2019

    • Author(s)
      Ma, Q. S., Liu, N., Sharma, A., Zhang, N., Yang, Y. N.
    • Organizer
      84th SCEJ Annual Meeting
    • Related Report
      2018 Annual Research Report
  • [Presentation] Photocatalytic Disinfection Performance in Gram-Negative/Gram-Positive Bacteria Mixed System by A Novel TiO2-Based Composite2019

    • Author(s)
      Liu, N., Ma, Q. S., Zhang, C., Sharma, A., Yang, Y. N.
    • Organizer
      84th SCEJ Annual Meeting
    • Related Report
      2018 Annual Research Report
  • [Presentation] Comparison of The Photocatalytic Inactivation Between Two Model Microorganisms: Gram-Positive Enterococcus Sp. and Gram-Negative E. coli2018

    • Author(s)
      Liu, N., Zhu, Q., Zhang, N., Ma, Q. S., Negishi, N., Yang, Y. N.
    • Organizer
      The 11th Japan-China-Korea Graduate Student Forum
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Development of Polyethylene Glycol Modified Bi2WO6-based Composite Photocatalytic Thin Film with High Photocatalytic Activity for Wastewater Treatment under Visible Light2018

    • Author(s)
      Ma, Q. S., Liu, N., Zhang, N., Sharma, A., Yang, Y. N.
    • Organizer
      The 11th Japan-China-Korea Graduate Student Forum
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Effect of Salinity on Degradation of Organic Pollutants in Seawater Using TiO2-Based Composite Photocatalyst2018

    • Author(s)
      Sharma, A., Zheng, H. Y., Liu, N., Zhao, C. Y., Zhang, N., Yang, Y. N.
    • Organizer
      The 11th Japan-China-Korea Graduate Student Forum
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Investigating the Effects of Bioreactor Design and Continuous Nutrition Release from Bed Material During the Hydrogen Fermentation2018

    • Author(s)
      Zhao, C. Y., Zhang, N., Zheng, H. Y., Liu, N., Yang, Y. N.
    • Organizer
      The 11th Japan-China-Korea Graduate Student Forum
    • Related Report
      2018 Annual Research Report
    • Int'l Joint Research

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Published: 2018-05-01   Modified: 2024-03-26  

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