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Joining of Heat-Resistant Materials Using Isothermal Solidification by Evaporation of Additives in Multi-Element Insert Material

Research Project

Project/Area Number 18K04726
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Review Section Basic Section 26030:Composite materials and interfaces-related
Research InstitutionKyoto Municipal Institute of Industrial Technology and Culture

Principal Investigator

Kohama Kazuyuki  地方独立行政法人京都市産業技術研究所, 京都市産業技術研究所, 次席研究員 (00710287)

Project Period (FY) 2018-04-01 – 2021-03-31
Project Status Completed (Fiscal Year 2020)
Budget Amount *help
¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2020: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2019: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2018: ¥1,560,000 (Direct Cost: ¥1,200,000、Indirect Cost: ¥360,000)
Keywordsセラミックス / ろう接 / 引張強度 / 界面微細組織 / 曲げ強度 / 高温強度 / 状態図 / Si-Mg状態図 / ペースト / 高融点金属
Outline of Final Research Achievements

This study proposes a novel materials-design concept for development of ceramics bonding fillers, for low-temperature joining of ceramics while maintaining the joint’s high-temperature reliability. In the concept, the filler comprises an additive element whose vapor pressure is much higher than that of the filler matrix element. The elemental combination contributes to formation of a molten liquid phase at a low bonding temperature. The additive element is likely to evaporate and be removed from the liquid phase because of its high vapor pressure, and thus, the filler melting point increases gradually toward the inherent melting point of the matrix element during joining.
As a major achievement, sets of ceramic components were successfully joined using a Si-Mg composite filler, showing the practicality of the concept. Investigation on thermo-mechanical properties of the resultant joints led to the conclusion that they were suitable for use in a high-temperature, oxidizing atmosphere.

Academic Significance and Societal Importance of the Research Achievements

本研究で提案した接合用インサート材は,低温で溶融させて接合し,かつ接合後のインサート材の融点を上昇させる手法である。融点を制御するために融点降下元素を添加すること自体は一般的であるが,それを蒸発させて系外に排出するということはこれまでにない極めて独創的な着想である。それが実現可能であることを示しただけでなく,得られた接合体の高温強度特性など優れた特徴を実証した。新たな学術的着想の応用展開を図るという点で,本研究の意義は非常に大きい。セラミックスの大型・複雑形状部材作製の大幅な簡便化と低コスト化につながり,軽量化や燃焼温度の向上によるエンジン低燃費化など社会的貢献につながる。

Report

(4 results)
  • 2020 Annual Research Report   Final Research Report ( PDF )
  • 2019 Research-status Report
  • 2018 Research-status Report
  • Research Products

    (10 results)

All 2021 2020 2019 Other

All Journal Article (2 results) (of which Peer Reviewed: 2 results,  Open Access: 2 results) Presentation (4 results) (of which Int'l Joint Research: 1 results,  Invited: 1 results) Remarks (2 results) Patent(Industrial Property Rights) (2 results) (of which Overseas: 1 results)

  • [Journal Article] Interfacial microstructure characterization and strength evaluation of Si3N4/Si3N4 joints with Si-Mg composite filler for high-temperature applications2021

    • Author(s)
      Kazuyuki Kohama
    • Journal Title

      Ceramics International

      Volume: - Issue: 16 Pages: 22424-22434

    • DOI

      10.1016/j.ceramint.2021.04.252

    • Related Report
      2020 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Joining of alumina ceramics using silicon-magnesium composite filler for high-temperature applications2020

    • Author(s)
      Kazuyuki KOHAMA
    • Journal Title

      Science and Technology of Welding and Joining

      Volume: - Issue: 5 Pages: 1-8

    • DOI

      10.1080/13621718.2020.1714874

    • Related Report
      2019 Research-status Report
    • Peer Reviewed / Open Access
  • [Presentation] Si-Mg混合粉末フィラーによる窒化ケイ素接合体の作製とその高温強度評価2020

    • Author(s)
      小濱和之
    • Organizer
      溶接学会2020年度秋季全国大会
    • Related Report
      2020 Annual Research Report
  • [Presentation] Si基複合粉末フィラーの添加元素蒸発による等温凝固を用いたセラミックスの高耐熱接合2020

    • Author(s)
      小濱和之
    • Organizer
      日本溶接協会2020年度第2回先端材料接合委員会/溶接学会第115回界面接合研究委員会 合同委員会
    • Related Report
      2020 Annual Research Report
    • Invited
  • [Presentation] Mg含有Si基ペーストによるアルミナセラミックスの接合2019

    • Author(s)
      小濱和之
    • Organizer
      一般社団法人溶接学会2019年度秋季全国大会
    • Related Report
      2019 Research-status Report
  • [Presentation] Joining of Alumina Ceramics Using Si-Mg Pastes for High-Temperature Application2019

    • Author(s)
      Kazuyuki KOHAMA
    • Organizer
      The 5th International Symposium on Visualization in Joining & Welding Science through Advanced Measurements and Simulation (Visual-JW2019)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Remarks] 接合後に高融点化する接合用フィラーの新規材料設計とセラミックス高耐熱接合への応用

    • URL

      https://www.youtube.com/watch?v=LK7uvmKM95E&t=5s

    • Related Report
      2020 Annual Research Report
  • [Remarks] 接合後に高融点化する接合用フィラーの新規材料設計とセラミックス高耐熱接合への応用

    • URL

      http://tc-kyoto.or.jp/info/2021/03/chienowa27.pdf

    • Related Report
      2020 Annual Research Report
  • [Patent(Industrial Property Rights)] CERAMIC BONDING MATERIAL2020

    • Inventor(s)
      小濱和之
    • Industrial Property Rights Holder
      京都市産業技術研究所
    • Industrial Property Rights Type
      特許
    • Filing Date
      2020
    • Related Report
      2020 Annual Research Report
    • Overseas
  • [Patent(Industrial Property Rights)] セラミックス接合材2019

    • Inventor(s)
      小濱和之
    • Industrial Property Rights Holder
      京都市産業技術研究所
    • Industrial Property Rights Type
      特許
    • Industrial Property Number
      2019-145396
    • Filing Date
      2019
    • Related Report
      2019 Research-status Report

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Published: 2018-04-23   Modified: 2022-01-27  

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