Development of ambient ionization mass spectrometry using dark current discharge with argon gas
| Project/Area Number |
18K05179
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| Research Category |
Grant-in-Aid for Scientific Research (C)
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| Allocation Type | Multi-year Fund |
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| Section | 一般 |
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| Review Section |
Basic Section 34020:Analytical chemistry-related
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| Research Institution | Yokohama City University |
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Principal Investigator |
Sekimoto Kanako 横浜市立大学, 生命ナノシステム科学研究科(八景キャンパス), 准教授 (40583399)
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| Project Period (FY) |
2018-04-01 – 2021-03-31
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| Project Status |
Completed (Fiscal Year 2020)
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| Budget Amount *help |
¥4,290,000 (Direct Cost: ¥3,300,000、Indirect Cost: ¥990,000)
Fiscal Year 2020: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2019: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2018: ¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
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| Keywords | 質量分析 / アルゴン / 暗流 / DART（リアルタイム直接分析法） / アンビエントイオン化 / アンビエントイオン化法 / DART（リアルタイム直接分析）法 / アンビエント質量分析 / 非持続放電 |
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| Outline of Final Research Achievements |
Direct analysis in real time (DART) is one of ambient ionization mass spectrometry. Although DART has been performed with a great amount of success in various fields, use of helium gas and glow discharge (classified with selfsustaining discharge) causes limitations for utility. In this study, a novel ionization technique using argon gas and atmospheric pressure dark current discharge (classified with non-selfsustaining discharge) has been developed. This technique has ionization efficiency and mechanism comparable to those of conventional DART.
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| Academic Significance and Societal Importance of the Research Achievements |
本研究で見出された「暗流励起アルゴン」によるイオン化は，アンビエント質量分析法の1つであるリアルタイム直接分析法（DART）の問題を抜本的に解決する，安価で・低電力で・どこでも継続的に計測できる質量分析法の要素技術を提供するものである．
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Report
(4 results)
Research Products
(30 results)
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[Journal Article] OH-chemistry of non-methane organic gases (NMOG) emitted from laboratory and ambient biomass burning smoke: evaluating the influence of furans and oxygenated aromatics on ozone and secondary NMOG formation2019
Author(s)
M.M. Coggon, C.Y. Lim, A.R. Koss, K. Sekimoto, B. Yuan, J.B. Gilman, D. Hagan, V. Selimovic, K.J. Zarzana, S.S. Brown, J.M. Roberts, M. Muller, R.J. Yokelson, A. Wisthaler, J. Krechmer, J. Jimenez, C. Cappa, J.H. Kroll, J. de Gouw and C. Warneke
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Journal Title
Atmospheric Chemistry and Physics
Volume: 19
Issue: 23
Pages: 14875-14899
DOI
Related Report
Peer Reviewed / Open Access / Int'l Joint Research
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[Journal Article] Non-methane organic gas emissions from biomass burning: identification, quantification, and emission factors from PTR-ToF during the FIREX 2016 laboratory experiment2018
Author(s)
A. R. Koss, K. Sekimoto, J. B. Gilman, V. Selimovic, M. M. Coggon, K. J. Zarzana, B. Yuan, B. M. Lerner, S. S. Brown, J. L. Jimenez, J. Krechmer, J. M. Roberts, C. Warneke, R. J. Yokelson and J. de Gouw
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Journal Title
Atmospheric Chemistry and Physics
Volume: 18
Issue: 5
Pages: 3299-3319
DOI
Related Report
Peer Reviewed / Open Access / Int'l Joint Research
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[Presentation] High- and low-temperature pyrolysis profiles describe volatile organic compound emissions from western US wildfire fuels2018
Author(s)
◯Kanako Sekimoto, Abigail R. Koss, Jessica B. Gilman, Vanessa Selimovic, Matthew M. Coggon, Kyle J. Zarzana, Bin Yuan, Brian M. Lerner, Steven S. Brown, Carsten Warneke, Robert J. Yokelson, James M. Roberts and Joost de Gouw
Organizer
2018 joint 14th iCACGP Quadrennial Symposium and 15th IGAC Science Conference
Related Report
Int'l Joint Research
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