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Environmental radioactivity research on radio-iodine contamination by the Fukushima Daiichi Nuclear Power Plant accident

Research Project

Project/Area Number 18K05205
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeMulti-year Fund
Section一般
Review Section Basic Section 34030:Green sustainable chemistry and environmental chemistry-related
Research InstitutionGakushuin University

Principal Investigator

Takeshi Ohno  学習院大学, 理学部, 教授 (40452007)

Project Period (FY) 2018-04-01 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥4,420,000 (Direct Cost: ¥3,400,000、Indirect Cost: ¥1,020,000)
Fiscal Year 2020: ¥910,000 (Direct Cost: ¥700,000、Indirect Cost: ¥210,000)
Fiscal Year 2019: ¥1,820,000 (Direct Cost: ¥1,400,000、Indirect Cost: ¥420,000)
Fiscal Year 2018: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Keywords放射性ヨウ素 / ICP-MS / MS/MS / 原子力発電所事故 / 放射性セシウム / 福島原発事故
Outline of Final Research Achievements

The accident at the Fukushima Daiichi Nuclear Power Plant resulted in a substantial release of radionuclides including Iodine-131, Cesium-134, and Cesium-137 to the atmosphere, and caused significant contamination of the environment. An effective dose estimation of released I-131 is important but difficult due to lack of data on the deposition of I-131. The long-lived radioiodine isotope I-129 is one of the important radionuclides released from nuclear fuel reprocessing plants and nuclear accidents into the environment. In particular, I-129 has been used as a tool to reconstruct the initial distribution of I-131 at nuclear accidents. In this study, the determination of I-129 in enviromental samples by ICP-MS/MS was performed, and the distribution of radioactive iodine released by the Fukushima Daiichi Nuclear Power Plant accident was examined.

Academic Significance and Societal Importance of the Research Achievements

福島第一原子力発電所の事故により、大量の放射性ヨウ素(I-131)が放出された。I-131は体内に入ると甲状腺がんのリスク要因となるため、環境中に含まれるI-131に関する情報は重要である。しかし、事故後数ヶ月でI-131の放射能を調べることは困難となったため、本研究では、事故により同様に放出された長半減期放射性ヨウ素(I-129)を用いてI-131を推定する迅速分析法を開発した。本研究で開発したICP-MS/MS法を用いた分析法は従来法に比べ10倍以上迅速に測定することが可能になった。

Report

(5 results)
  • 2021 Annual Research Report   Final Research Report ( PDF )
  • 2020 Research-status Report
  • 2019 Research-status Report
  • 2018 Research-status Report
  • Research Products

    (10 results)

All 2022 2021 2020 2019 2018

All Journal Article (4 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 4 results) Presentation (6 results)

  • [Journal Article] Temporal change of 236U/238U and 235U/238U isotopic ratios in atmospheric deposition in Tokyo and Akita from 1963 to 19792022

    • Author(s)
      Ohno Takeshi、Sato Naoki、Shikimori Junko、Ijichi Yuta、Fukami Yusuke、Igarashi Yasuhito
    • Journal Title

      Science of The Total Environment

      Volume: 810 Pages: 151292-151292

    • DOI

      10.1016/j.scitotenv.2021.151292

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Simultaneous determination of zircon U?Pb age and titanium concentration using LA-ICP-MS for crystallization age and temperature2020

    • Author(s)
      Yuguchi Takashi、Ishibashi Kozue、Sakata Shuhei、Yokoyama Tatsunori、Itoh Daichi、Ogita Yasuhiro、Yagi Koshi、Ohno Takeshi
    • Journal Title

      Lithos

      Volume: 372-373 Pages: 105682-105682

    • DOI

      10.1016/j.lithos.2020.105682

    • Related Report
      2020 Research-status Report
    • Peer Reviewed
  • [Journal Article] An integrated chemostratigraphic (δ13C-δ18O-87Sr/86Sr-δ15N) study of the Doushantuo Formation in western Hubei Province, South China2019

    • Author(s)
      Lan Zhongwu、Sano Yuji、Yahagi Takuya、Tanaka Kentaro、Shirai Kotaro、Papineau Dominic、Sawaki Yusuke、Ohno Takeshi、Abe Mariko、Yang Hongwei、Liu Hai、Jiang Tao、Wang Teng
    • Journal Title

      Precambrian Research

      Volume: 320 Pages: 232-252

    • DOI

      10.1016/j.precamres.2018.10.018

    • Related Report
      2019 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Determination of strontium 90 in environmental samples by triple quadrupole ICP-MS and its application to Fukushima soil samples2018

    • Author(s)
      Ohno Takeshi、Hirono Mutsumi、Kakuta Shinichiro、Sakata Shuhei
    • Journal Title

      Journal of Analytical Atomic Spectrometry

      Volume: 33 Issue: 6 Pages: 1081-1085

    • DOI

      10.1039/c8ja00017d

    • Related Report
      2018 Research-status Report
    • Peer Reviewed
  • [Presentation] 鉄隕石中のスズ同位体分析法の開発と精製時に起こる非質量依存の同位体分別2021

    • Author(s)
      田中康介、大野剛、深海雄介
    • Organizer
      2021年度日本地球化学会
    • Related Report
      2021 Annual Research Report
  • [Presentation] 光化学反応における水銀同位体分別の波長依存性2021

    • Author(s)
      平野隼、大野剛、深海雄介
    • Organizer
      2021年度日本地球化学会
    • Related Report
      2021 Annual Research Report
  • [Presentation] ICP-MS/MS を用いた極微量放射性同位体分析法が拓く環境放射能研究2021

    • Author(s)
      大野剛、佐藤直輝、佐藤妃奈、福本学、五十嵐康人
    • Organizer
      2021年度日本地球化学会
    • Related Report
      2021 Annual Research Report
  • [Presentation] ICP-MS/MSを用いた極微量放射性同位体分析法の開発と環境放射能研究への応用2020

    • Author(s)
      大野剛, 實籾佑哉, 佐藤妃奈, 深海雄介
    • Organizer
      2020年度日本地球化学会第66回年会
    • Related Report
      2020 Research-status Report
  • [Presentation] ICP-MS/MS を用いた酸化気化導入法による高感度放射性ヨウ素分析法の開発及び環境放射能研究への応用2019

    • Author(s)
      佐藤妃奈、深海雄介、大野剛
    • Organizer
      2019年度日本地球化学会第66回年会
    • Related Report
      2019 Research-status Report
  • [Presentation] ICP-MS/MSを用いた高感度放射性ヨウ素 分析法の開発と環境放射能研究への応用2018

    • Author(s)
      佐藤妃奈、大野剛、坂田周平
    • Organizer
      2018年度日本地球化学会第65回年会
    • Related Report
      2018 Research-status Report

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Published: 2018-04-23   Modified: 2023-01-30  

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