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Fundamental study on the orientation dependence of polycrystalline perovskite thin film properties

Research Project

Project/Area Number 18K14120
Research Category

Grant-in-Aid for Early-Career Scientists

Allocation TypeMulti-year Fund
Review Section Basic Section 29020:Thin film/surface and interfacial physical properties-related
Research InstitutionTohoku University

Principal Investigator

Ma Teng  東北大学, 材料科学高等研究所, 助教 (10734543)

Project Period (FY) 2018-04-01 – 2020-03-31
Project Status Completed (Fiscal Year 2019)
Budget Amount *help
¥2,860,000 (Direct Cost: ¥2,200,000、Indirect Cost: ¥660,000)
Fiscal Year 2019: ¥1,170,000 (Direct Cost: ¥900,000、Indirect Cost: ¥270,000)
Fiscal Year 2018: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Keywordsペロブスカイト / 光電変換デバイス / 太陽電池 / フォトルミネッセンス / 結晶方位 / 表面電位 / 表面修飾 / 光電デバイス / 結晶異方性
Outline of Final Research Achievements

In this study, an original film deposition method was utilized to create a perovskite polycrystalline film with uniform morphology and large crystal size. By evaluating the emission spectra and conductivity of perovskite for each crystal, we have been able to determine the correlation between crystal orientation/interfacial stresses and optical/electrical properties. The findings are essential for improving the performance of photovoltaic devices such as solar cells and photodetectors based on perovskite materials. Furthermore, the fast charge transport properties of the large crystals in the parallel direction of the film have been utilized to develop a new type of perovskite solar cells with a structure. The possibility of further increasing the efficiency of perovskite solar cells is demonstrated.

Academic Significance and Societal Importance of the Research Achievements

本研究によって確立された大結晶を有するペロブスカイト薄膜の成膜法は高性能ペロブスカイト光電変換デバイスの形成に新な手法を提供した。また、結晶構造/界面応力とその光・電特性の関係を明らかにし、ペロブスカイト分野において有用な基礎的な知見を得た。

Report

(3 results)
  • 2019 Annual Research Report   Final Research Report ( PDF )
  • 2018 Research-status Report
  • Research Products

    (16 results)

All 2019 2018 Other

All Journal Article (2 results) (of which Int'l Joint Research: 1 results,  Peer Reviewed: 2 results,  Open Access: 1 results) Presentation (13 results) (of which Int'l Joint Research: 10 results,  Invited: 3 results) Remarks (1 results)

  • [Journal Article] Modulation of Photoinduced Transmembrane Currents in a Fullerene-Doped Freestanding Lipid Bilayer by a Lateral Bias2019

    • Author(s)
      Ma Teng、Feng Xingyao、Ohori Takeshi、Miyata Ryusuke、Tadaki Daisuke、Yamaura Daichi、Deguchi Takafumi、Komiya Maki、Kanomata Kensaku、Hirose Fumihiko、Niwano Michio、Hirano-Iwata Ayumi
    • Journal Title

      ACS Omega

      Volume: 4 Issue: 19 Pages: 18299-18303

    • DOI

      10.1021/acsomega.9b02336

    • Related Report
      2019 Annual Research Report
    • Peer Reviewed / Open Access
  • [Journal Article] Unveil the Full Potential of Integrated-Back-Contact Perovskite Solar Cells Using Numerical Simulation2018

    • Author(s)
      Teng Ma, Qingwen Song, Daisuke Tadaki, Michio Niwano, Ayumi Hirano-Iwata
    • Journal Title

      ACS Applied Energy Materials

      Volume: 1 Issue: 3 Pages: 970-975

    • DOI

      10.1021/acsaem.8b00044

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] Self-assembled nanostructure and their applications2019

    • Author(s)
      Teng Ma
    • Organizer
      The 8th International Donghu Forum for Outstanding Young Scholars
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research / Invited
  • [Presentation] In-situ observation of photocatalytic degradation of organic molecules by TiO2 nanotube arrays2019

    • Author(s)
      Teng Ma, Yasuo Kimura, Michio Niwano, Ayumi Hirano-Iwata
    • Organizer
      2019年度電子デバイス研究会(有機デバイス、酸化物デバイス、一般)
    • Related Report
      2019 Annual Research Report
  • [Presentation] New geometry for thin-film perovskite photovoltaics2019

    • Author(s)
      Teng Ma, Michio Niwano, Ayumi Hirano-Iwata
    • Organizer
      19th International Conference on Solid Films and Surfaces
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Photo-decomposition of organic contaminants on TiO2 nanotube surface observed by MIR-IRAS measurement2019

    • Author(s)
      馬騰, 木村康男, 平野愛弓, 庭野道夫
    • Organizer
      日本表面真空学会2019年学術講演会
    • Related Report
      2019 Annual Research Report
  • [Presentation] Lateral structure for stable and highly efficient perovskite photovoltaics2019

    • Author(s)
      Teng Ma, Daisuke Tadaki, Michio Niwano, Ayumi Hirano-Iwata
    • Organizer
      2019 E-MRS Spring Meeting
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Large single-crystal grains for highly efficient integrated back-contact perovskite solar cells2019

    • Author(s)
      Teng Ma, Ayumi Hirano-Iwata
    • Organizer
      2019 MRS Fall Meeting
    • Related Report
      2019 Annual Research Report
    • Int'l Joint Research
  • [Presentation] Structural evolution for highly efficient perovskite solar cells2019

    • Author(s)
      Teng Ma, Ayumi Hirano-Iwata
    • Organizer
      Asia-Pacific International Conference on Perovskite, Organic Photovoltaics and Optoelectronics
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Back-contact structure for highly efficient perovskite solar cells2019

    • Author(s)
      Teng Ma
    • Organizer
      10th International Workshop on Nanostructures & Nanoelectronics
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Nano-molecular devices2019

    • Author(s)
      Teng Ma
    • Organizer
      The 9th Zijin High-level Forum for Foreign Young Scholars
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] The full potential of integrated-back-contacted perovskite solar cells unveiled by numerical simulation technique2018

    • Author(s)
      Teng Ma, Daisuke Tadaki, Michio Niwano and Ayumi Hirano-Iwata
    • Organizer
      2018 MRS Spring Meeting & Exhibit
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Lateral charge transport in perovskite solar cells2018

    • Author(s)
      Teng Ma, Daisuke Tadaki, Michio Niwano, and Ayumi Hirano-Iwata
    • Organizer
      電子デバイス研究会
    • Related Report
      2018 Research-status Report
  • [Presentation] Boosting the performance of the perovskite solar cells by structural optimization2018

    • Author(s)
      Teng Ma, Ayumi Hirano-Iwata
    • Organizer
      E-MRS Spring Meeting 2018
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Advantages of interdigitated structure over traditional sandwich structure for highly efficient perovskite solar cells2018

    • Author(s)
      Teng Ma, Ayumi Hirano-Iwata
    • Organizer
      12th Aseanian Conference on Nano-hybrid Solar Cells (NHSC)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Remarks] 研究室Webページ

    • URL

      http://www.riec.tohoku.ac.jp/~hir-lab/

    • Related Report
      2019 Annual Research Report

URL: 

Published: 2018-04-23   Modified: 2021-02-19  

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