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Control of single magnetic spin in a semiconductor dot and its application

Research Project

Project/Area Number 18K18988
Research Category

Grant-in-Aid for Challenging Research (Exploratory)

Allocation TypeMulti-year Fund
Review Section Medium-sized Section 28:Nano/micro science and related fields
Research InstitutionUniversity of Tsukuba

Principal Investigator

Kuroda Shinji  筑波大学, 数理物質系, 教授 (40221949)

Project Period (FY) 2018-06-29 – 2022-03-31
Project Status Completed (Fiscal Year 2021)
Budget Amount *help
¥6,240,000 (Direct Cost: ¥4,800,000、Indirect Cost: ¥1,440,000)
Fiscal Year 2019: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Fiscal Year 2018: ¥3,120,000 (Direct Cost: ¥2,400,000、Indirect Cost: ¥720,000)
Keywords量子ドット / 単一スピン / 交換相互作用 / 光学ポンピング / 表面弾性波 / スピントロニクス / 顕微分光 / スピン‐歪結合 / 格子歪
Outline of Final Research Achievements

We have clarified various aspects of the behavior of a single Cr atom in a CdTe self-assembled dot. We observed the splitting of the exciton emission spectrum due to the exchange interaction with a single Cr spin in the dot, and showed that the distribution of each Cr spin state can be controlled by resonant excitation to the split emission lines. We observed the decay of the distribution of specific Cr spin states generated under resonant excitation (optical pumping) and clarified the transition process between Cr spin states as the origin of the decay. In addition, we found an emission spectrum with a similar shape to that of the exchange splitting of Cr spins, but with different characteristics such as linear polarization properties, which is attributed to the valence fluctuation splitting of Cr ions located near the dots.

Academic Significance and Societal Importance of the Research Achievements

本研究の成果により、CdTe自己形成ドット中の単一Crスピンの種々の特性を明らかにすることができた。特に、共鳴励起の手法により特定のCrスピンの分布が制御できることを示した。この成果は、ドット中の単一Crスピンを量子ビットとして用いた量子情報処理への応用の可能性の探索という点で学術的、社会的意義を有すると考えられる。

Report

(5 results)
  • 2021 Annual Research Report   Final Research Report ( PDF )
  • 2020 Research-status Report
  • 2019 Research-status Report
  • 2018 Research-status Report
  • Research Products

    (41 results)

All 2022 2021 2020 2019 2018 Other

All Int'l Joint Research (4 results) Journal Article (8 results) (of which Int'l Joint Research: 7 results,  Peer Reviewed: 8 results) Presentation (29 results) (of which Int'l Joint Research: 9 results,  Invited: 2 results)

  • [Int'l Joint Research] CNRS, Neel Institut(フランス)

    • Related Report
      2021 Annual Research Report
  • [Int'l Joint Research] CNRS, Neel Institut(フランス)

    • Related Report
      2020 Research-status Report
  • [Int'l Joint Research] Institut Neel, CNRS(フランス)

    • Related Report
      2019 Research-status Report
  • [Int'l Joint Research] CNRS, Institut Neel(フランス)

    • Related Report
      2018 Research-status Report
  • [Journal Article] Hole-Cr+ nanomagnet in a semiconductor quantum dot2021

    • Author(s)
      V. Tiwari, M. Arino, S. Gupta, M. Morita, T. Inoue, D. Caliste, P. Pochet, H. Boukari, S. Kuroda, L. Besombes
    • Journal Title

      Physical Review B

      Volume: 104 Issue: 4

    • DOI

      10.1103/physrevb.104.l041301

    • Related Report
      2021 Annual Research Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Influence of nonequilibrium phonons on the spin dynamics of a single Cr atom2020

    • Author(s)
      Tiwari V.、Makita K.、Arino M.、Morita M.、Kuroda S.、Boukari H.、Besombes L.
    • Journal Title

      Physical Review B

      Volume: 101 Issue: 3 Pages: 1-8

    • DOI

      10.1103/physrevb.101.035305

    • Related Report
      2020 Research-status Report 2019 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Radio-frequency stress-induced modulation of CdTe/ZnTe quantum dots2020

    • Author(s)
      Tiwari V.、Makita K.、Arino M.、Morita M.、Crozes T.、Bellet-Amalric E.、Kuroda S.、Boukari H.、Besombes L.
    • Journal Title

      Journal of Applied Physics

      Volume: 127 Issue: 23 Pages: 234303-234303

    • DOI

      10.1063/5.0011124

    • Related Report
      2020 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Optical control of an individual Cr spin in a semiconductor quantum dot2019

    • Author(s)
      L. Besombes, H. Boukari, V. Tiwari, A. Lafuente-Sampietro, S. Kuroda, K. Makita
    • Journal Title

      Semiconductor Science and Technology

      Volume: 34 Issue: 6 Pages: 063001-063001

    • DOI

      10.1088/1361-6641/ab13f5

    • Related Report
      2019 Research-status Report 2018 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Charge fluctuations of a Cr atom probed in the optical spectra of a quantum dot2019

    • Author(s)
      L. Besombes, H. Boukari, V. Tiwari, A. Lafuente-Sampietro, M. Sunaga, K. Makita, and S. Kuroda
    • Journal Title

      Physical Review B

      Volume: 99 Issue: 3 Pages: 035309-035309

    • DOI

      10.1103/physrevb.99.035309

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Effect of nitrogen acceptor co-doping on the structural and magnetic properties of (Zn,Fe) Te2019

    • Author(s)
      Indrajit Saha, Takuma Nakamura, Ken Kanazawa, Hiroaki Nitani, Masanori Mitome, Shinji Kuroda
    • Journal Title

      Journal of Crystal Growth

      Volume: 511 Pages: 42-47

    • DOI

      10.1016/j.jcrysgro.2019.01.026

    • Related Report
      2018 Research-status Report
    • Peer Reviewed
  • [Journal Article] Role of hybridization and magnetic effects in massive Dirac cones: Magnetic topological heterostructures with controlled film thickness2019

    • Author(s)
      Yuma Okuyama, Ryo Ishikawa, Shinji Kuroda, Toru Hirahara
    • Journal Title

      Applied Physics Letters

      Volume: 114 Issue: 5 Pages: 051602-051602

    • DOI

      10.1063/1.5083059

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Journal Article] Dynamics of a Cr spin in a semiconductor quantum dot: Hole-Cr flip-flops and spin-phonon coupling2018

    • Author(s)
      A. Lafuente-Sampietro, H. Utsumi, M. Sunaga, K. Makita, H. Boukari, S. Kuroda, and L. Besombes
    • Journal Title

      Physical Review B

      Volume: 97 Issue: 15 Pages: 155301-155301

    • DOI

      10.1103/physrevb.97.155301

    • Related Report
      2018 Research-status Report
    • Peer Reviewed / Int'l Joint Research
  • [Presentation] Cr原子を添加したCdTe/ZnTe量子井戸における零次元励起子の発光スペクトル2022

    • Author(s)
      井上 智貴、森田 真衣、安藤 瞬、黒田 眞司、Vivekanand Tiwari、Herve Boukari、Lucien Besombes
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2021 Annual Research Report
  • [Presentation] Crを添加したCdTe量子井戸の作製と光学特性評価2021

    • Author(s)
      森田 真衣、井上 智貴、安藤 瞬、黒田 眞司、Vivekanand Tiwari、Herve Boukari、Lucien Besombes
    • Organizer
      第82回応用物理学会秋季学術講演会
    • Related Report
      2021 Annual Research Report
  • [Presentation] Crを添加したCdTe量子井戸の作製と光学特性評価2021

    • Author(s)
      森田 真衣、井上 智貴、安藤 瞬、黒田 眞司、Vivekanand Tiwari、Herve Boukari、Lucien Besombes
    • Organizer
      第26回半導体スピン工学の基礎と応用
    • Related Report
      2021 Annual Research Report
  • [Presentation] MBE法によるCr原子1個を含むCdTe 自己形成ドットの作製と光学特性評価2020

    • Author(s)
      森田 真衣、有野 雅史、牧田 憲治、黒田 眞司、Vivekanand Tiwari、Herve Boukari、Lucien Besombes
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2020 Research-status Report
  • [Presentation] 表面弾性波を用いたCdTe量子ドットのPLスペクトルの変調2020

    • Author(s)
      有野 雅史、森田 真衣、牧田 憲治、黒田 眞司、Vivekanand Tiwari、Herve Boukari、Lucien Besombes
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2020 Research-status Report
  • [Presentation] EuS/SnTeヘテロ接合における近接高温強磁性トポロジカル結晶絶縁体界面状態2020

    • Author(s)
      秋山了太、渡邉和己、嶋野武、友弘雄太、渡邉拓斗、石川諒、阿久津和宏、飯田一樹、黒田眞司、長谷川修司
    • Organizer
      日本物理学会 2019年秋季大会
    • Related Report
      2020 Research-status Report
  • [Presentation] トポロジカル結晶絶縁体SnTeと磁性絶縁体EuSのヘテロ接合における界面誘起磁化2020

    • Author(s)
      嶋野 武、友弘 雄太、渡邉 拓斗、渡邉 和己、秋山 了太、阿久津 和宏、飯田 一樹、長谷川 修司、黒田 眞司
    • Organizer
      第25回半導体スピン工学の基礎と応用
    • Related Report
      2020 Research-status Report
  • [Presentation] MBE法によりGaAs(001)基板上へ作製したFeTe薄膜の磁化特性の成長温度依存性およびアニール処理の効果2020

    • Author(s)
      安齋 廷玄、金澤 研、黒田 眞司
    • Organizer
      第25回半導体スピン工学の基礎と応用
    • Related Report
      2020 Research-status Report
  • [Presentation] MBE法によるCrを含むCdTe自己形成ドットの作製と光学特性評価2019

    • Author(s)
      牧田 憲治、有野 雅史、森田 真衣、黒田 眞司、ティワリ ビべカナンド、ボウカリ エルベ、ビソンブ ルシアン
    • Organizer
      第80回応用物理学会秋季学術講演会
    • Related Report
      2019 Research-status Report
  • [Presentation] 単一のCr原子を含むCdTe自己形成ドットの作製と光学特性評価2019

    • Author(s)
      有野 雅史、森田 真衣、牧田 憲治、黒田 眞司、ティワリ ビベカナンド、ボウカリ エルベ、ビソンブ ルシアン
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Research-status Report
  • [Presentation] ドット中の単一Crスピンの緩和に対する光励起フォノンの影響2019

    • Author(s)
      牧田 憲治、有野 雅史、森田 真衣、黒田 眞司、ビソンブ ルシアン、ボウカリ エルベ、ティワリ ビベカナンド
    • Organizer
      第67回応用物理学会春季学術講演会
    • Related Report
      2019 Research-status Report
  • [Presentation] Emission spectrum from self-assembled CdTe dots containing a single Cr atom2019

    • Author(s)
      K. Makita, M. Arino, S. Kuroda, A. Lafuente-Sampietro, V. Tiwari, H. Boukari, L. Besombes
    • Organizer
      10th International School and Conference on Spintronics and Quantum Information Technology (Spintech X)
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] Dynamics and control of a Cr spin in a quantum dot2019

    • Author(s)
      L.Besombes, H.Boukari, V.Tiwari, K.Makita, M.Arino, M.Morita, S.Kuroda
    • Organizer
      19th International Conference on II-VI Compounds and Related Materials
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research / Invited
  • [Presentation] Fabrication of self-assembled dots of CdTe containing Cr by MBE and optical characterization2019

    • Author(s)
      K.Makita, M.Arino, M.Morita, S.Kuroda, L.Besombes, H.Boukari, V.Tiwari
    • Organizer
      19th International Conference on II-VI Compounds and Related Materials
    • Related Report
      2019 Research-status Report
    • Int'l Joint Research
  • [Presentation] CdTe自己形成ドットにおけるCrの電荷揺らぎによる発光スペクトルの分裂2019

    • Author(s)
      牧田 憲治、有野 雅史、須永 雅弘、黒田 眞司、ラファンテ-サンピエトロ アルバン、ボウカリ エルベ、ビソンブ ルシアン
    • Organizer
      第65回応用物理学会春季学術講演会
    • Related Report
      2018 Research-status Report
  • [Presentation] トポロジカル結晶絶縁体 (Pb,Sn)Te (111)薄膜のレーザー励起ARPES測定による非占有状態の観測と超高速キャリアダイナミクス2019

    • Author(s)
      伊藤寛史, 大滝祐輔, 友弘雄太, 石田行章, 秋山了太, 木村昭夫, 辛埴, 黒田眞司
    • Organizer
      日本物理学会 第74回年次大会
    • Related Report
      2018 Research-status Report
  • [Presentation] トポロジカル結晶絶縁体SnTe薄膜の表面バンド分散と超高速キャリアダイナミクス2018

    • Author(s)
      伊藤寛史, 大滝祐輔, 石田行章, 秋山了太, 木村昭夫, 辛埴, 黒田眞司
    • Organizer
      日本物理学会 2018年秋季大会
    • Related Report
      2018 Research-status Report
  • [Presentation] 偏極中性子反射率法を用いたFe/SnTeヘテロ構造界面における強磁性近接効果の観測2018

    • Author(s)
      渡邉和己, 石川諒, 秋山了太, 阿久津和宏, 飯田一樹, 黒田眞司, 長谷川修司
    • Organizer
      日本物理学会 2018年秋季大会
    • Related Report
      2018 Research-status Report
  • [Presentation] IV-VI族半導体PbSnTeのテラヘルツサイクロトロン共鳴2018

    • Author(s)
      今中康貴, D. Kindole, 竹端寛治, 大滝祐輔, 伊藤寛史, 秋山了太, 黒田眞司
    • Organizer
      日本物理学会 2018年秋季大会
    • Related Report
      2018 Research-status Report
  • [Presentation] 磁性トポロジカル絶縁体ヘテロ構造における強磁性とサイズ効果の協奏・競合2018

    • Author(s)
      奥山裕磨, 石川諒, 黒田眞司, 平原徹
    • Organizer
      日本物理学会 2018年秋季大会
    • Related Report
      2018 Research-status Report
  • [Presentation] TEM observation of IV-VI diluted magnetic semiconductor (Sn.Mn)Te grown by MBE2018

    • Author(s)
      Ryo Ishikawa、Hiroshi Ito、Yuta Tomohiro、Ryota Akiyama、Shinji Kuroda、Hiroaki Nitani、Masanori Mitome
    • Organizer
      第79回応用物理学会秋季学術講演会
    • Related Report
      2018 Research-status Report
  • [Presentation] MBE法により成長したFeドープ閃亜鉛鉱型MnTe薄膜の磁気特性・構造特性の成長温度依存性2018

    • Author(s)
      加藤 象二郎、金澤 研、黒田 眞司
    • Organizer
      第79回応用物理学会秋季学術講演会
    • Related Report
      2018 Research-status Report
  • [Presentation] トポロジカル結晶絶縁体SnTe薄膜の表面バンド分散と超高速キャリアダイナミクス2018

    • Author(s)
      伊藤寛史、大滝祐輔、友弘雄太、石田行章、秋山了太、木村昭夫、辛埴、黒田眞司
    • Organizer
      第23回半導体スピン工学の基礎と応用
    • Related Report
      2018 Research-status Report
  • [Presentation] Observation of the unoccupied state of SnTe by laser-excited angle resolved photoemission spectroscopy2018

    • Author(s)
      H. Ito, Y. Otaki, Y. Tomohiro, Y. Ishida, R. Akiyama, A. Kimura, S. Shin, S. Kuroda
    • Organizer
      New Trends in Topological Insulators 2018 (NTTI2018)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Optical control of the single Cr spin in a semiconductor quantum dot2018

    • Author(s)
      A. Lafuente-Sampietro, M. Sunaga, K. Makita, H. Boukari, L. Besombes, S. Kuroda
    • Organizer
      10th International School and Conference on Physics and Applications of Spin Phenomena in Solid (PASPS10)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Structural and magnetic properties of IV-VI diluted magnetic semiconductor (Sn,Mn)Te grown by MBE2018

    • Author(s)
      R. Ishikawa, H. Itoh, Y. Tomohiro, R. Akiyama, H. Nitani, and S. Kuroda
    • Organizer
      10th International School and Conference on Physics and Applications of Spin Phenomena in Solid (PASPS10)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Fabrication of CdTe dots containing single Cr atom and optical control of single spin2018

    • Author(s)
      M. Sunaga, K. Makita, A. Lafuente-Sampietro, H. Boukari, L. Besombes, and S. Kuroda
    • Organizer
      20th International Conference on Molecular Beam Epitaxy (MBE2018)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Effect of nitrogen co-doping on the magnetic and structural properties of (Zn,Fe)Te2018

    • Author(s)
      I. Saha, T. Nakamura, K. Kanazawa, H. Nitani, and S. Kuroda
    • Organizer
      20th International Conference on Molecular Beam Epitaxy (MBE2018)
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research
  • [Presentation] Optical detection and manipulation of a single Cr spin in a semiconductor quantum dot2018

    • Author(s)
      A. Lafuente-Sampietro, M. Sunaga, K. Makita, H. Boukari, L. Besombes, S. Kuroda
    • Organizer
      Annual Workshop of Center for Spintronics Research Network (CSRN) Osaka
    • Related Report
      2018 Research-status Report
    • Int'l Joint Research / Invited

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Published: 2018-07-25   Modified: 2023-01-30  

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