Science of local optical-to-terahertz wave conversion in low dimensional nanomaterials
Project/Area Number |
18KK0140
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Research Category |
Fund for the Promotion of Joint International Research (Fostering Joint International Research (B))
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Allocation Type | Multi-year Fund |
Review Section |
Medium-sized Section 28:Nano/micro science and related fields
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Research Institution | Osaka University |
Principal Investigator |
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Co-Investigator(Kenkyū-buntansha) |
芹田 和則 大阪大学, レーザー科学研究所, その他 (00748014)
村上 博成 大阪大学, レーザー科学研究所, 准教授 (30219901)
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Project Period (FY) |
2018-10-09 – 2023-03-31
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Project Status |
Completed (Fiscal Year 2022)
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Budget Amount *help |
¥17,940,000 (Direct Cost: ¥13,800,000、Indirect Cost: ¥4,140,000)
Fiscal Year 2020: ¥6,630,000 (Direct Cost: ¥5,100,000、Indirect Cost: ¥1,530,000)
Fiscal Year 2019: ¥7,540,000 (Direct Cost: ¥5,800,000、Indirect Cost: ¥1,740,000)
Fiscal Year 2018: ¥3,770,000 (Direct Cost: ¥2,900,000、Indirect Cost: ¥870,000)
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Keywords | テラヘルツ波 / ナノカーボン / フェムト秒パルスレーザー / 励起子 / 2次元原子層物質 |
Outline of Final Research Achievements |
We have developed an optical switch using semiconducting carbon nanotubes (CNTs), successfully observed terahertz waves with their femtosecond laser excitation, and combined it with non-equilibrium numerical simulations to elucidate the exciton divergence dynamics from its properties, and the extent of the CNT arrangement makes a significant contribution to the excited quasiparticle dynamics, such as the bypassing of its thermalization pathway, was clarified. We also observed and elucidated complex ultrafast dynamics in GaInN/GaN multilayer quantum well structures and bismuth telluride/telluride heterojunctions by terahertz emission spectroscopy. In addition, anisotropic photophysical properties of photo-charges in the surface nano-region of gallium oxide were also clarified.
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Academic Significance and Societal Importance of the Research Achievements |
カーボンナノチューブ(CNT)など低次元ナノ材料の物性は、その構造に由来する特異な素励起に起因する電気的・光学的特性を有しており、これらを活用した新規な機能を持つ次世代デバイスの基礎研究に向けて、光励起電荷ダイナミクスの解明は不可欠である。しかし、従来のフォトルミネッセンスなどでは、光励起の初期過程におけるキャリア・励起子の発生・走行・解離プロセスなどサブピコ秒レベルの高速な電荷走行現象を捉えることは困難であった。本研究では、高速電荷ダイナミクスをテラヘルツ波放射分光により解明することで、テラヘルツ放射科学を世界に展開する波及効果をもたらし、ナノデバイス開発に新たな道を提供するものとなった。
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Report
(6 results)
Research Products
(73 results)
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[Journal Article] The 2023 terahertz science and technology roadmap2023
Author(s)
Leitenstorfer Alfred、Moskalenko Andrey S、Kampfrath Tobias、Kono Junichiro、Castro-Camus Enrique、Peng Kun、Qureshi Naser、Turchinovich Dmitry、Tanaka Koichiro, others
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Journal Title
Journal of Physics D: Applied Physics
Volume: 56
Issue: 22
Pages: 223001-223001
DOI
Related Report
Peer Reviewed / Open Access / Int'l Joint Research
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[Journal Article] Transition from Diffusive to Superdiffusive Transport in Carbon Nanotube Networks via Nematic Order Control2023
Author(s)
Michael Wais, Filchito Renee G. Bagsican, Natsumi Komatsu, Weilu Gao, Kazunori Serita, Hironaru Murakami, Karsten Held, Iwao Kawayama, Junichiro Kono, Marco Battiato, and Masayoshi Tonouchi
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Journal Title
Nano Letters
Volume: In press
Issue: 10
Pages: 4448-4455
DOI
Related Report
Peer Reviewed / Open Access / Int'l Joint Research
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[Journal Article] Terahertz Excitonics in Carbon Nanotubes: Exciton Autoionization and Multiplication2020
Author(s)
Filchito Renee G. Bagsican, Michael Wais, Natsumi Komatsu, Weilu Gao, Lincoln W. Weber, Kazunori Serita, Hironaru Murakami, Karsten Held, Frank A. Hegmann, Masayoshi Tonouchi, Junichiro Kono, Iwao Kawayama, Marco Battiato
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Journal Title
Nano Lett. 2020
Volume: 20
Issue: 1
Pages: 3098-3105
DOI
Related Report
Peer Reviewed / Open Access / Int'l Joint Research
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[Journal Article] Terahertz Excitonics in Carbon Nanotubes: Exciton Autoionization and Multiplication2020
Author(s)
Filchito Renee G. Bagsican, Michael Wais, Natsumi Komatsu, Weilu Gao, Lincoln W. Weber, Kazunori Serita, Hironaru Murakami, Karsten Held, Frank A. Hegmann, Masayoshi Tonouchi, Junichiro Kono, Iwao Kawayama, and Marco Battiato
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Journal Title
Nano Lett. 2020
Volume: 20,05
Issue: 5
Pages: 3098-3105
DOI
Related Report
Peer Reviewed / Open Access / Int'l Joint Research
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[Presentation] Contact-free THz nano-seismology in InGaN/GaN Multiple Quantum Wells2019
Author(s)
Abdul Mannan, I. Kawayama, K. Yamahara, F.R. Bagsican, H. Murakami, T. Langer, H. Bremers, U.Rossow, D. Turchinovich, A. Hangleiter, and M. Tonouchi
Organizer
Global Nonophotonics 2019
Related Report
Int'l Joint Research
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[Presentation] Probing photocarrier dyamics in semiconducting carbon nanotubes by terahertz emission spectroscopy2019
Author(s)
Filchito Renee G. Bagsican, Iwao Kawayama, Michael Wais, Natsumi Komatsu, Kazunori Serita, Weilu Gao, Lincoln Weber, Marco Battiato, Hironaru Murakami, Frank A. Hegmann, Junichiro Kono, and Masayoshi Tonouchi
Organizer
2019 International Conference on Advanced Functional Materials and Nanotechnology
Related Report
Int'l Joint Research / Invited
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[Presentation] Terahertz radiation generated by acoustic wavesin InGaN/GaN Multiple Quantum Wells2019
Author(s)
Abdul Mannan, I. Kawayama, K. Yamahara, F.R. Bagsican, H. Murakami, A. Hangleiter, T. Langer, H. Bremers, U. Rossow, D. Turchinovich, M. Tonouchi.
Organizer
The 80th JSAP Autumn Meeting 2019 JSAP-OSA Joint Symposia
Related Report
Int'l Joint Research
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[Presentation] Observation of Bi2Te3/Te striped structures using a laser terahertz emission microscope2019
Author(s)
F. Murakami, K. Serita, H. Murakami, R. Dalipi, A. M. Urbas, A. Materna, M. Buza, D. A. Pawlak, M. Tonouchi, and I. Kawayama
Organizer
44th International Conference on Infrared, Millimeter, and Terahertz Waves
Related Report
Int'l Joint Research
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[Presentation] Terahertz Emission from a Photoconductive Antenna Switch Based on Aligned Single-Chirality Semiconducting Carbon Nanotubes2019
Author(s)
Filchito Renee G. Bagsican, Iwao Kawayama, Michael Wais, Natsumi Komatsu, Kazunori Serita, Weilu Gao, Lincoln Weber, Marco Battiato, Hironaru Murakami, Frank A. Hegmann, Junichiro Kono, and Masayoshi Tonouchi
Organizer
21st International Conference on Electron Dynamics in Semiconductors, Optoelectronics and Nanostructures
Related Report
Int'l Joint Research
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[Presentation] Characteristics of THz emissions from Bi2Te3/Te striped structure2019
Author(s)
F. Murakami, K. Serita, H. Murakami, R. Dalipi, A. M. Urbas, A. Materna, M. Buza, D. A. Pawlak, M. Tonouchi, and I. Kawayama
Organizer
21st International Conference on Electron Dynamics in Semiconductors, Optoelectronics and Nanostructures
Related Report
Int'l Joint Research
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[Presentation] Terahertz radiation from InGaN/GaN Multiple Quantum Wells2019
Author(s)
Abdul Mannan, I. Kawayama, K. Yamahara, F.R. Bagsican, H. Murakami, T. Langer, H. Bremers, U. Rossow, D. Turchinovich, A. Hangleiter, and M. Tonouchi
Organizer
21st International Conference on Electron Dynamics in Semiconductors, Optoelectronics and Nanostructures
Related Report
Int'l Joint Research
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[Presentation] Terahertz emission from photoconductive antenna switches based on highly-aligned and chirality-enriched semiconducting carbon nanotubes2019
Author(s)
Filchito Renee G. Bagsican, Iwao Kawayama, Michael Wais, Natsumi Komatsu, Kazunori Serita, Weilu Gao, Lincoln Weber, Marco Battiato, Hironaru Murakami, Frank A. Hegmann, Junichiro Kono, and Masayoshi Tonouchi,
Organizer
Optical Terahertz Science and Technology2019
Related Report
Int'l Joint Research
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[Presentation] Terahertz emission properties of photoconductive antennas based on semiconducting carbon nanotubes2018
Author(s)
Filchito Renee Bagsican, Iwao Kawayama, Kazunori Serita, Weilu Gao, Natsumi Komatsu, Michael Wais, Lincoln Weber, Marco Battiato, Hironaru Murakami, Frank A. Hegmann, Junichiro Kono, and Masayoshi Tonouchi
Organizer
The Global Nanophotonics 2018
Related Report
Int'l Joint Research
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