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Improvement of Thermoelectric Properties and Development of Fabrication Processes for Environmental-friendly Half-Heusler Thermoelectric Materials

Research Project

Project/Area Number 19206073
Research Category

Grant-in-Aid for Scientific Research (A)

Allocation TypeSingle-year Grants
Section一般
Research Field Structural/Functional materials
Research InstitutionTokyo Institute of Technology

Principal Investigator

KIMURA Yoshisato  Tokyo Institute of Technology, 大学院・総合理工学研究科, 准教授 (90262295)

Co-Investigator(Kenkyū-buntansha) MISHIMA Yoshinao  東京工業大学, 大学院・総合理工学研究科, 教授 (00143660)
Project Period (FY) 2007 – 2009
Project Status Completed (Fiscal Year 2009)
Budget Amount *help
¥46,020,000 (Direct Cost: ¥35,400,000、Indirect Cost: ¥10,620,000)
Fiscal Year 2009: ¥10,400,000 (Direct Cost: ¥8,000,000、Indirect Cost: ¥2,400,000)
Fiscal Year 2008: ¥10,140,000 (Direct Cost: ¥7,800,000、Indirect Cost: ¥2,340,000)
Fiscal Year 2007: ¥25,480,000 (Direct Cost: ¥19,600,000、Indirect Cost: ¥5,880,000)
Keywords金属物性 / 環境材料 / 廃熱利用 / 相平衡・状態図 / 材料加工・処理 / 環境エネルギー材料
Research Abstract

We have focused on half-Heusler type compounds MNiSn (M=Ti, Zr, Hf) as environmental-friendly thermoelectric materials which allow us the materials design without depending on toxic elements. Thermoelectric properties of MNiSn were evaluated as their intrinsic physical properties, and the phase separation of TiNiSn from ZrNiSn and HfNiSn, i.e. between the same half-Heusler ordered structure, was determined with related phase equilibria. New fabrication processes were proposed based on the reaction between Sn (liquid) and TiNi (solid) as well as based on the reduction of SnO_2 and oxidization of Ti. Thermoelectric properties were evaluated for TiNiSn/Ti-oxides composite alloys.

Report

(4 results)
  • 2009 Annual Research Report   Final Research Report ( PDF )
  • 2008 Annual Research Report
  • 2007 Annual Research Report
  • Research Products

    (22 results)

All 2010 2009 2008 2007

All Journal Article (4 results) (of which Peer Reviewed: 4 results) Presentation (18 results)

  • [Journal Article] Thermoelectric Performance of Half-Heusler TiNiSn Alloys Fabricated by Solid-Liquid Reaction Sintering2010

    • Author(s)
      Yoshisato Kimura, Chihiro Asami, Yaw.-Wang. Chai, Yoshinao Mishima
    • Journal Title

      Materials Science Forum (in press.)

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Thermoelectric Performance of Half-Heusler TiNiSn Alloys Fabricated by Solid-Liquid Reaction Sintering2010

    • Author(s)
      Y.Kimura, C.Asami, Y.-W.Chai, Y.Mishima
    • Journal Title

      Materials Science Forum (未定)(掲載決定)

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Thermoelectric Properties of Directionally Solidified Half-Heusler (Ma 0. 5, Mb 0. 5)NiSn (Ma, Mb = Hf, Zr, Ti) Alloys2009

    • Author(s)
      Yoshisato Kimura, Hazuki Ueno, Yoshinao Mishima
    • Journal Title

      Journal of Electronic Materials 38

      Pages: 934-939

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Thermoelectric Properties of Directionally Solidified Half-Heusler (M^a_<0.5>, M^b_<0.5>) NiSn (M^a, M^b=Hf, Zr, Ti) Alloys2009

    • Author(s)
      Y. Kimura, H. Ueno, Y. Mishima
    • Journal Title

      Journal of Electronic Materials (印刷中)

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Presentation] Half-Heusler型TINiSn合金の作製プロセス構築のための相平衡2010

    • Author(s)
      大谷真也, 木村好里, 三島良直
    • Organizer
      日本金属学会(第146回大会)
    • Place of Presentation
      筑波大学(つくば市)
    • Year and Date
      2010-03-29
    • Related Report
      2009 Final Research Report
  • [Presentation] Half-Heusler型TiNiSn合金の作製プロセス構築のための相平衡2010

    • Author(s)
      大谷真也、木村好里、三島良直
    • Organizer
      日本金属学会秋期(第146回)大会
    • Place of Presentation
      筑波大学(つくば)
    • Year and Date
      2010-03-29
    • Related Report
      2009 Annual Research Report
  • [Presentation] Phase stability and thermoelectric properties of half-Heusler compounds (Ti, M)NiSn (M = Zr, Hf)2009

    • Author(s)
      Takahiro Kenjo, Yoshisato Kimura, et al.
    • Organizer
      2010 MRS Fall Meeting
    • Place of Presentation
      Boston MA, USA
    • Year and Date
      2009-12-01
    • Related Report
      2009 Final Research Report
  • [Presentation] Phase stability and thermoelectric properties of half-Heusler compounds (Ti, M)NiSn(M=Zr, Hf)2009

    • Author(s)
      T.Kenjo, Y.Kimura, et al.
    • Organizer
      2010 MRS Fall Meeting
    • Place of Presentation
      Boston MA, USA
    • Year and Date
      2009-12-01
    • Related Report
      2009 Annual Research Report
  • [Presentation] SnO2の還元反応を利用した粉末冶金法によるTiNiSn熱電材料の作製プロセスと熱電特性2009

    • Author(s)
      加藤秀樹, 木村好里, 三島良直
    • Organizer
      日本金属学会(第145回大会)
    • Place of Presentation
      京都大学(京都)
    • Year and Date
      2009-09-17
    • Related Report
      2009 Final Research Report
  • [Presentation] Half-Heusler型TiNiSn合金の液相反応焼結による作製と熱電特性評価2009

    • Author(s)
      木村好里, 浅見千裕, 三島良直, ら
    • Organizer
      日本金属学会(第145回大会)
    • Place of Presentation
      京都大学(京都)
    • Year and Date
      2009-09-17
    • Related Report
      2009 Final Research Report
  • [Presentation] Half-Heusler型TiNiSn合金の液相反応燒結による作製と熱電特性評価2009

    • Author(s)
      木村好里、浅見千裕、三島良直, ら
    • Organizer
      日本金属学会秋期(第145回)大会
    • Place of Presentation
      京都大学(京都)
    • Year and Date
      2009-09-17
    • Related Report
      2009 Annual Research Report
  • [Presentation] SnO_2の還元反応を利用した粉末冶金法によるTiNiSn熱電材料の作製プロセスと熱電特性2009

    • Author(s)
      加藤秀樹、木村好里、三島良直
    • Organizer
      日本金属学会秋期(第145回)大会
    • Place of Presentation
      京都大学(京都)
    • Year and Date
      2009-09-17
    • Related Report
      2009 Annual Research Report
  • [Presentation] SnO2の還元反応を利用した粉末冶金法によるHalf-Heusler型TiNiSn熱電材料の作製プロセス2009

    • Author(s)
      加藤秀樹, 木村好里, 三島良直
    • Organizer
      日本金属学会(第144回大会)
    • Place of Presentation
      東京工業大学(大岡山)
    • Year and Date
      2009-03-29
    • Related Report
      2009 Final Research Report
  • [Presentation] SnO_2の還元反応を利用した粉末冶金法によるHalf-Heusler型TiNiSn熱電材料の作製プロセス2009

    • Author(s)
      加藤秀樹, 木村好里, 三島良直
    • Organizer
      日本金属学会春期(第144回)大会(講演概要集P. 258)
    • Place of Presentation
      東京工業大学(大岡山)
    • Year and Date
      2009-03-29
    • Related Report
      2008 Annual Research Report
  • [Presentation] Phase Stability and Thermoelectric Properties of Half-Heusler (Ma, Mb)NiSn (Ma, Mb = Hf, Zr, Ti)2008

    • Author(s)
      Yoshisato Kimura, Hazuki Ueno, Takahiro Kenjo, Chihiro Asami, Yoshinao Mishima
    • Organizer
      2008 MRS Fall Meeting
    • Place of Presentation
      Boston MA, USA
    • Year and Date
      2008-12-01
    • Related Report
      2009 Final Research Report
  • [Presentation] Phase Stability and Thermoelectric Properties of Half-Heusler (M^a, M^b) NiSn (M^a, M^b=Hf, Zr, Ti)2008

    • Author(s)
      Yoshisato Kimura, Hazuki Ueno, Takahiro Kenjo, Chihiro Asami, Yoshinao Mishima
    • Organizer
      2008 MRS Fall Meeting
    • Place of Presentation
      Boston, USA
    • Year and Date
      2008-12-01
    • Related Report
      2008 Annual Research Report
  • [Presentation] Half-Heusler型(Ti, Zr)NiSn固溶体における二相分離傾向と熱電特性2008

    • Author(s)
      権丈孝弘, 木村好里, 三島良直
    • Organizer
      日本金属学会(第143回大会)
    • Place of Presentation
      熊本大学(熊本)
    • Year and Date
      2008-09-24
    • Related Report
      2009 Final Research Report
  • [Presentation] Half-Heusler型(Ti, Zr) NiSn固溶体における二相分離傾向と熱電特性2008

    • Author(s)
      権丈孝弘, 木村好里, 三島良直
    • Organizer
      日本金属学会秋期(第143回)大会(講演概要集P. 84)
    • Place of Presentation
      熊本大学(熊本)
    • Year and Date
      2008-09-24
    • Related Report
      2008 Annual Research Report
  • [Presentation] 還元反応を利用した粉末冶金法の金属間化合物作製プロセスへの応用2007

    • Author(s)
      浅見千裕、木村好里、中谷昌史, 寺西利治
    • Organizer
      日本金属学会(第141回大会)
    • Place of Presentation
      岐阜大学(岐阜)
    • Year and Date
      2007-09-19
    • Related Report
      2009 Final Research Report
  • [Presentation] half-Heusler型化合物熱電材料の相平衡と単相合金作製プロセス2007

    • Author(s)
      木村好里, 浅見千裕, 上野葉月, 田村幸雄
    • Organizer
      日本金属学会(第141回大会)
    • Place of Presentation
      岐阜大学(岐阜)
    • Year and Date
      2007-09-19
    • Related Report
      2009 Final Research Report
  • [Presentation] half-Heusler型化合物熱電材料の相平衡と単相合金作製プロセス2007

    • Author(s)
      木村好里、浅見千裕、上野葉月 ら
    • Organizer
      日本金属学会
    • Place of Presentation
      岐阜大学
    • Year and Date
      2007-09-19
    • Related Report
      2007 Annual Research Report
  • [Presentation] 還元反応を利用した粉末冶金法の金属間化合物作製プロセスへの応用2007

    • Author(s)
      浅見千裕、木村好里、寺西利治 ら
    • Organizer
      日本金属学会
    • Place of Presentation
      岐阜大学
    • Year and Date
      2007-09-19
    • Related Report
      2007 Annual Research Report

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Published: 2007-04-01   Modified: 2016-04-21  

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