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Studies on an analysis and an emission of halogenated polycyclic aromatic hydrocarbons.

Research Project

Project/Area Number 19350076
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Environmental chemistry
Research InstitutionUniversity of Shizuoka

Principal Investigator

雨谷 敬史  University of Shizuoka, 環境科学研究所 (10244534)

Project Period (FY) 2007 – 2009
Project Status Completed (Fiscal Year 2009)
Budget Amount *help
¥18,200,000 (Direct Cost: ¥14,000,000、Indirect Cost: ¥4,200,000)
Fiscal Year 2009: ¥2,080,000 (Direct Cost: ¥1,600,000、Indirect Cost: ¥480,000)
Fiscal Year 2008: ¥2,990,000 (Direct Cost: ¥2,300,000、Indirect Cost: ¥690,000)
Fiscal Year 2007: ¥13,130,000 (Direct Cost: ¥10,100,000、Indirect Cost: ¥3,030,000)
Keywords有害化学物質 / 有機化学 / 分析化学 / ハロゲン化合物 / 多環芳香族化水素 / 塩化ビニリデン / 塩化ビニル / GC / MS / 負化学イオン化 / 発生機構 / 焼却処理 / ハロゲン化多環芳香族炭化水素 / 発生源 / NCI / 多環芳香族炭化水素
Research Abstract

We have developed an analytical method for halogenated polycyclic aromatic hydrocarbons (PAH-X) by GC/MS with Negative Chemical Ionization method. Sensitivity of 6-chloro-benzo[a]pyrene can be 1,000 times higher than that by GC/MS with Electron Impact ionization method. This method can be used for quantifying phenanthrene and anthracene individually, even if these 2 compounds cannot be separated by GC/MS. We have analyzed PAH-X in the exhaust gas from incinerator, and the results show that PAH-X containing more than 6 halogen molecules cannot be detected. The more halogen molecules PAH-X have, the lower concentration it was. The large amount of hydrogen chloride was emitted from burning of halogenated plastics in an electric furnace, and a little PAH-X can be generated. The results in this study suggest that PAH-X generated both from cyclization of polychloroalkane and halogenation after cyclization of PAH at high temperature.

Report

(4 results)
  • 2009 Annual Research Report   Final Research Report ( PDF )
  • 2008 Annual Research Report
  • 2007 Annual Research Report
  • Research Products

    (36 results)

All 2010 2009 2008 2007 2006 Other

All Journal Article (13 results) (of which Peer Reviewed: 4 results) Presentation (18 results) Book (2 results) Remarks (3 results)

  • [Journal Article] A simple method for screening emission sources of carbonyl compounds in indoor air.2010

    • Author(s)
      Yamashita, S., Kume, K., Horiike, T., Honma, N., Fusaya, M., Ohura T., Amagai, T.
    • Journal Title

      J. Hazard. Materials 178(1-3)

      Pages: 370-376

    • Related Report
      2009 Final Research Report
  • [Journal Article] A methoxyflavonoid, chrysoeriol, selectively inhibits the formation of a carcinogenic estrogen metabolite in MCF-7 breast cancer cells2010

    • Author(s)
      Hitomi Takemura, 他
    • Journal Title

      The Journal of Steroid Biochemistry and Molecular Biology 118

      Pages: 70-76

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Discovery of novel halogenated polycyclic aromatic hydrocarbons in urban particulate matters: Occurrence, photostability, and AhR activity.2009

    • Author(s)
      Ohura, T., Sawada, K., Amagai, T., Shinomiya, M.
    • Journal Title

      Environ. Sci. Technol. 43

      Pages: 2269-2275

    • Related Report
      2009 Final Research Report
  • [Journal Article] Comparative study on indoor air quality in Japan and China: Characteristics of residential indoor and outdoor VOCs.2009

    • Author(s)
      Ohura, T., Amagai, T.,, Shen, X., Li, S., Zhang, P., Zhu, L.
    • Journal Title

      Atmos. Environ. 43(40)

      Pages: 6352-6359

    • Related Report
      2009 Final Research Report
  • [Journal Article] Pollution level, phase distribution and source analysis of polycyclic aromatic hydrocarbons in residential air in Hangzhou, China.2009

    • Author(s)
      Zhu, L., Lu, H., Chen, S., Amagai, T.
    • Journal Title

      J. Hazard. Materials 162(2-3)

      Pages: 1165-1170

    • Related Report
      2009 Final Research Report
  • [Journal Article] Discovery of novel halogenated polycyclic aromatic hydrocarbons in urban particulate matters : Occurrence, photostability, and AR activity2009

    • Author(s)
      Takeshi Ohura, 他
    • Journal Title

      Environmental Science & Technology 43

      Pages: 2269-2275

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Chlorinated Polycyclic Aromatic Hydrocarbons in the Atmosphere: Seasonal Levels, Gas-Particle Partitioning, and Origin.2008

    • Author(s)
      Ohura, T., Fujima, S., Amagai T., Shinomiya, M.
    • Journal Title

      Environ. Sci. Technol. 42(9)

      Pages: 3296-3302

    • Related Report
      2009 Final Research Report
  • [Journal Article] Field monitoring of volatile organic compounds using passive air samplers in an industrial city in Japan.2008

    • Author(s)
      Kume, K., Ohura, T., Amagai, T., Fusaya, M.
    • Journal Title

      Environ. Pollution 153(3)

      Pages: 649-657

    • Related Report
      2009 Final Research Report
  • [Journal Article] Behavior and prediction of photochemical degradation of chlorinated polycyclic aromatic hydrocarbons in cyclohexane.2008

    • Author(s)
      Ohura, T., Amagai, T., Makino, M.
    • Journal Title

      Chemosphere 70(11)

      Pages: 2110-2117

    • Related Report
      2009 Final Research Report
  • [Journal Article] Studies on a Simultaneous Analytical Method of Urinary Nicotine and its Metabolites, and their Half-Lives in Urine.2008

    • Author(s)
      Matsuki, H., Hashimoto, K., Arashidani, K., Akiyama, Y., Amagai, T., Ishizu, Y., Matsushita, H.
    • Journal Title

      J. Univ. Occup. Environ. Health 30(3)

      Pages: 235-252

    • NAID

      110006880862

    • Related Report
      2009 Final Research Report
  • [Journal Article] Chlorinated Polycyclic Aromatic Hydrocarbons in the Atmosphere : Seasonal Levels, Gas-Particle Partitioning, and Origin.2008

    • Author(s)
      Takeshi Ohura, Shohoko Fujima, Takashi Amagai, Mino Shinomiya
    • Journal Title

      Environmental Science & Technology 42

      Pages: 3296-3302

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Behavior and prediction of photochemical degradation of chlorinated polycyclic aromatic hydrocarbons in cyclohexane.2008

    • Author(s)
      4. Takeshi Ohura, Takashi Amagai, Masakazu Makino
    • Journal Title

      Chemosphere 70

      Pages: 2110-2117

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Aryl Hydrocarbon Receptor-Mediated Effects of Chlorinated Polycyclic Aromatic Hydrocarbons.2007

    • Author(s)
      Takeshi Ohura, Maki Morita, Masakazu Makino, Takashi Amagai, Kayoko Shimoi
    • Journal Title

      Chem. Res. Toxicol 20(9)

      Pages: 1237-1241

    • Related Report
      2009 Final Research Report
  • [Presentation] 食塩電解過程に由来するダイオキシン類及び類縁化合物.2009

    • Author(s)
      山本央, 東野和雄, 大浦健, 雨谷敬史, 嶽盛公昭, 高菅卓三, 橋本俊次, 柏木宣久, 佐々木裕子
    • Organizer
      第18回環境化学討論会
    • Place of Presentation
      つくば
    • Related Report
      2009 Final Research Report
  • [Presentation] 塩素化多環芳香族炭化水素の土壌汚染と発生源に関する研究.2009

    • Author(s)
      大浦健, 山本央, 東野和雄, 雨谷敬史, 四ノ宮美保, 佐々木裕子
    • Organizer
      第18回環境化学討論会
    • Place of Presentation
      つくば
    • Related Report
      2009 Final Research Report
  • [Presentation] 大浦健, 山本央, 東野和雄, 雨谷敬史, 四ノ宮美保, 佐々木裕子:塩素化多環芳香族炭化水素の土壌汚染と発生源に関する研究2009

    • Author(s)
      大浦健, 他
    • Organizer
      第18回環境化学討論会
    • Place of Presentation
      つくば
    • Related Report
      2009 Annual Research Report
  • [Presentation] GC/MS/NCIによる塩素化多環芳香族炭化水素の分析法の開発2008

    • Author(s)
      雨谷敬史
    • Organizer
      第49回大気環境学会
    • Place of Presentation
      金沢大学
    • Year and Date
      2008-09-19
    • Related Report
      2008 Annual Research Report
  • [Presentation] 塩素化多環芳香族炭化水素類のAhR活性能の比較.2008

    • Author(s)
      森田真紀, 榊原啓之, 大浦健, 久留戸涼子, 内藤博敬, 大橋典男, 雨谷敬史, 下位香代子
    • Organizer
      2008年度日本農芸化学会
    • Place of Presentation
      名古屋
    • Related Report
      2009 Final Research Report
  • [Presentation] Chlorinated polycyclic aromatic hydrocarbons in the atmosphere: Levels, gas-particle partitioning, and fates.2008

    • Author(s)
      Ohura, T., Fujima, S., Amagai, T., Shinomiya, M.
    • Organizer
      5th SETAC World Congress
    • Place of Presentation
      Sydney, Australia
    • Related Report
      2009 Final Research Report
  • [Presentation] GC/MS/NCIによる塩素化多環芳香族炭化水素の分析法の開発.2008

    • Author(s)
      雨谷敬史, 唐亮, 山口太地, 大浦健
    • Organizer
      第49回大気環境学会年会
    • Place of Presentation
      金沢
    • Related Report
      2009 Final Research Report
  • [Presentation] Personal exposure and indoor concentrations of benzene and its derivatives in Shizuoka.2008

    • Author(s)
      Amagai, T., Ohura, T.
    • Organizer
      The 2nd China-Japan International Symposium on Indoor Air Pollution and Control.
    • Place of Presentation
      Shizuoka
    • Related Report
      2009 Final Research Report
  • [Presentation] A simple method for determining indoor emission rates of volatile organic compounds.2008

    • Author(s)
      Yamashita, S., Kume, K., Horiike, T., Honma, N., Fusaya, M., Ohura, T., Amagai, T.
    • Organizer
      The 2nd China-Japan International Symposium on Indoor Air Pollution and Control.
    • Place of Presentation
      Shizuoka
    • Related Report
      2009 Final Research Report
  • [Presentation] A comparative study of aldehyde concentrations at public space in Japan.2008

    • Author(s)
      Kamoi, M., Ohura, T., Amagai, T.
    • Organizer
      The 2nd China-Japan International Symposium on Indoor Air Pollution and Control.
    • Place of Presentation
      Shizuoka
    • Related Report
      2009 Final Research Report
  • [Presentation] ハロゲン化多環芳香族炭化水素によるAhRおよびERクロストークを介した遺伝子発現.2008

    • Author(s)
      平林賢, 大浦健, 森田真紀, 久留戸涼子, 榊原啓之, 雨谷敬史, 下位香代子
    • Organizer
      日本環境変異原学会第37回大会
    • Place of Presentation
      沖縄
    • Related Report
      2009 Final Research Report
  • [Presentation] 塩素化多環芳香族炭化水素類の変異原性評価.2008

    • Author(s)
      大浦健, 小田美光, 山田雅巳, 能美健彦, 雨谷敬史, 下位香代子
    • Organizer
      日本環境変異原学会第37回大会
    • Place of Presentation
      沖縄
    • Related Report
      2009 Final Research Report
  • [Presentation] 塩素化および臭素化多環芳香族炭化水素類によるAhR-ERクロストークを介した遺伝子発現について.2008

    • Author(s)
      平林賢, 大浦健, 森田真紀, 久留戸涼子, 榊原啓之, 雨谷敬史, 下位香代子
    • Organizer
      富士山麓アカデミック&サイエンスフェア2008
    • Place of Presentation
      静岡
    • Related Report
      2009 Final Research Report
  • [Presentation] Occurrences and photostabilities of particulate brominated polycyclic aromatic hydrocarbons in urban air.2007

    • Author(s)
      Ohura, T., Sawada, K., Amagai, T., Shinomiya, M.
    • Organizer
      SETAC North America 28th Annual Meeting
    • Place of Presentation
      Milwaukee, USA
    • Related Report
      2009 Final Research Report
  • [Presentation] Personal, indoor and outdoor concentrations of carbonyl compounds: Estimation of the personal exposure levels, sources and risks.2007

    • Author(s)
      Ohura, T., Kamoi, M., Kume, K., Amagai, T.
    • Organizer
      The China-Japan International Symposium on Indoor Air Pollution and Control
    • Place of Presentation
      Hangzhou, China
    • Related Report
      2009 Final Research Report
  • [Presentation] Personal, indoor and outdoor concentrations of polycyclic aromatic hydrocarbons (PAHs): Analytical methods for personal exposure, and sources and risks of PAHs.2007

    • Author(s)
      Ohura, T., Amagai, T.
    • Organizer
      The China-Japan International Symposium on Indoor Air Pollution and Control
    • Place of Presentation
      Hangzhou, China
    • Related Report
      2009 Final Research Report
  • [Presentation] 臭素化多環芳香族炭化水素の大気環境動態2007

    • Author(s)
      大浦健, 澤田恵一, 雨谷敬史, 四ノ宮美保
    • Organizer
      第16回環境化学討論会
    • Place of Presentation
      北九州
    • Related Report
      2009 Final Research Report
  • [Presentation] Evaluation of personal inhalation exposure to carcinogenic compounds.2006

    • Author(s)
      Takashi Amagai, Takeshi Ohura
    • Organizer
      第7回日中健康科学シンポジウム
    • Place of Presentation
      静岡
    • Related Report
      2009 Final Research Report
  • [Book] Chlorinated phenanthrenes induce CYP1A1 through aryl hydrocarbon receptor activation.2007

    • Author(s)
      Morita M, Ohura T, Kuruto-Niwa R, Sakakibara H, Amagai T, Shimoi K
    • Related Report
      2009 Final Research Report
  • [Book] Relationships between halogenated polycyclic aromatic hydrocarbons and dioxins in urban air and incinerators.2007

    • Author(s)
      Ohura T, Kitazawa A, Sawada K, Amagai T, Shinomiya M
    • Related Report
      2009 Final Research Report
  • [Remarks]

    • URL

      http://atmos.u-shizuoka-ken.ac.jp/lab/page1.html

    • Related Report
      2009 Final Research Report
  • [Remarks]

    • URL

      http://atmos.u-shizuoka-ken.ac.jp/lab/pagel.html

    • Related Report
      2009 Annual Research Report
  • [Remarks]

    • URL

      http://atmos.u-shizuoka-ken.ac.jp/lab/page1.html

    • Related Report
      2008 Annual Research Report

URL: 

Published: 2007-04-01   Modified: 2016-04-21  

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