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Development of detritiation system with advanced honeycomb catalyst and adsorbent

Research Project

Project/Area Number 19360416
Research Category

Grant-in-Aid for Scientific Research (B)

Allocation TypeSingle-year Grants
Section一般
Research Field Nuclear fusion studies
Research InstitutionKyushu University

Principal Investigator

MUNAKATA Kenzo  Kyushu University, 工学資源学部, 教授 (70264067)

Co-Investigator(Kenkyū-buntansha) UDA Tatsuhiko  核融合科学研究所, 安全管理センター, 教授 (50280590)
TANAKA Masahiro  核融合科学研究所, 安全管理センター, 助教 (00435520)
Project Period (FY) 2007 – 2009
Project Status Completed (Fiscal Year 2009)
Budget Amount *help
¥14,040,000 (Direct Cost: ¥10,800,000、Indirect Cost: ¥3,240,000)
Fiscal Year 2009: ¥1,430,000 (Direct Cost: ¥1,100,000、Indirect Cost: ¥330,000)
Fiscal Year 2008: ¥1,690,000 (Direct Cost: ¥1,300,000、Indirect Cost: ¥390,000)
Fiscal Year 2007: ¥10,920,000 (Direct Cost: ¥8,400,000、Indirect Cost: ¥2,520,000)
Keywords核融合 / トリチウム / 触媒 / 吸着 / 安全 / 核融合炉 / 安全閉じこめ / ハニカム / 吸着材 / 回収システム / シミュレーション
Research Abstract

Test fabrication of honeycomb catalyst and adsorbent was attempted, of which performance was experimentally investigated. Promising catalyst and adsorbent were found. With regard to promising catalysts, isotope effects were examined using deuterium and tritium. The effect of coexistent water vapor on catalytic activity was investigated as well. In terms of promising adsorbents, adsorption characteristics were thoroughly examined.

Report

(4 results)
  • 2009 Annual Research Report   Final Research Report ( PDF )
  • 2008 Annual Research Report
  • 2007 Annual Research Report
  • Research Products

    (31 results)

All 2010 2009 2008 2007 Other

All Journal Article (21 results) (of which Peer Reviewed: 8 results) Presentation (9 results) Remarks (1 results)

  • [Journal Article] Adsorption of Hydrogen Isotopes on Various Adsorbents at Cryogenic Temperature2009

    • Author(s)
      K. Munakata, T. Takeishi, S. Kajii, T. Wajima, Y. Kawamura
    • Journal Title

      Fusion Science and Technology Vo.56

      Pages: 153-157

    • Related Report
      2009 Final Research Report
  • [Journal Article] Tritium Release from Lithium Orthosilicate Pebbles Deposited with Palladium2009

    • Author(s)
      K. Munakata, T. Shinozaki, K. Inoue, S. Kajii, Y. Shinozaki, R Knitter, N. Bekris, T. Fujii, H. Yamana, K. Okuno
    • Journal Title

      Journal of Nuclear Materials Vol.386-388

      Pages: 1091-1094

    • Related Report
      2009 Final Research Report
  • [Journal Article] Adsorption Capacity of Tritium on Mordenite at Low Temperature2009

    • Author(s)
      Y. Kawamura, Y. Iwai, T. Hayashi, T. Yamanishi, K. Munakata
    • Journal Title

      Fusion Science and Technology Vol.56

      Pages: 168-172

    • Related Report
      2009 Final Research Report
  • [Journal Article] Hydrogen and Methane Oxidation Performances of Hybrid Honeycomb Catalyst for A Tritium Removal System2009

    • Author(s)
      M. Tanaka, T. Uda, Y. Shinozaki, K. Munakata
    • Journal Title

      Fusion Engineering and Design Vol.84

      Pages: 1818-1822

    • Related Report
      2009 Final Research Report
  • [Journal Article] Adsorption of Hydrogen Isotopes on Various Adsorbents at Cryogenic Temperature2009

    • Author(s)
      K.Munakata, et al.
    • Journal Title

      Fusion Science and Technology 56

      Pages: 153-157

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Tritium Release from Lithium Orthosilicate Pebbles Deposited with Palladium2009

    • Author(s)
      K.Munakata, et al.
    • Journal Title

      Journal of Nuclear Materials Vol.386-388

      Pages: 1091-1094

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Hydrogen and Methane Oxidation Performances of Hybrid Honeycomb Catalyst for A Tritium Removal System2009

    • Author(s)
      M.Tanaka, T.Uda, Y.Shinozaki, K.Munakata
    • Journal Title

      Fusion Engineering and Design Vol.84

      Pages: 1818-1822

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Tritium Release from Lithium Silicate Pebbles Produced from Lithium Hydroxide2008

    • Author(s)
      K. Munakata, T. Shinozaki, K. Inoue, S. Kajii, Y. Shinozaki, R Knitter, N. Bekris, T. Fujii, H. Yamana, K. Okuno
    • Journal Title

      Fusion Engineering and Design Vol.83

      Pages: 1317-1320

    • Related Report
      2009 Final Research Report
  • [Journal Article] Selective Recovery of Radioactive Carbon Dioxide Released from Nuclear Off-gas by Adsorption2008

    • Author(s)
      K. Munakata, A. Koga
    • Journal Title

      Journal of Power and Energy Systems Vol.2

      Pages: 178-185

    • NAID

      130000072957

    • Related Report
      2009 Final Research Report
  • [Journal Article] Adsorption of Krypton on Adsorbents at Cryogenic Temperatures2008

    • Author(s)
      K. Munakata, T. Shinozaki, H. Okabe
    • Journal Title

      Journal of Power and Energy Systems Vol.2

      Pages: 171-177

    • NAID

      130000072956

    • Related Report
      2009 Final Research Report
  • [Journal Article] Characteristics of Honeycomb Catalysts for Oxidation of Tritiated Hydrogen and Methane Gases2008

    • Author(s)
      T. Uda, M. Tanaka, K. Munakata
    • Journal Title

      Fusion Engineering and Design Vol.83

      Pages: 1715-1720

    • Related Report
      2009 Final Research Report
  • [Journal Article] The background levels of atmospheric tritium concentration in the environment at NIFS Toki site of Japan2008

    • Author(s)
      T. Uda, M. Tanaka, T. Sugiyama, T. Yamaguchi, N. Momoshima
    • Journal Title

      Fusion Science and Technology Vol.54

      Pages: 281-284

    • Related Report
      2009 Final Research Report
  • [Journal Article] Experimental study on electrochemical hydrogen pump of SrZrO_3-based oxide2008

    • Author(s)
      M. Tanaka, Y. Asakura, T. Uda
    • Journal Title

      Fusion Science and Technology Vol.54

      Pages: 479-482

    • Related Report
      2009 Final Research Report
  • [Journal Article] Selective Recovery of Radioactive Carbon Dioxide Released from Nuclear Off-gas by Adsorption2008

    • Author(s)
      Munakata K., et al.
    • Journal Title

      Journal of Power and Energy Systems 20

      Pages: 178-185

    • NAID

      130000072957

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Tritium release from lithium silicate pebbles produced from lithium hydroxide2008

    • Author(s)
      Munakata K., et al.
    • Journal Title

      FUSION ENGINEERING AND DESIGN 83

      Pages: 1317-1320

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Experimental and Simulation Study on Adsorption of Hydrogen Isotopes on MS5A at 77K2007

    • Author(s)
      K. Munakata, S. Beloglazov, N. Bekris, M. Glugla, R. Wagner, E. Fanghanel
    • Journal Title

      Fusion Engineering and Design Vol.82

      Pages: 2303-2310

    • Related Report
      2009 Final Research Report
  • [Journal Article] Vacancy Solution Model Formulated by the NRTL Equation for Correlation of Adsorption Eqilibria2007

    • Author(s)
      K. Munakata
    • Journal Title

      Journal of Chemical Engineering of Japan Vol.40

      Pages: 398-409

    • Related Report
      2009 Final Research Report
  • [Journal Article] Kinetics of Reaction with Water Vapor and ab initio study of Titanium Beryllide2007

    • Author(s)
      K. Munakata, H. Kawamura, M. Uchida
    • Journal Title

      Journal of Nuclear Materials Vol.367-370

      Pages: 1057-1062

    • Related Report
      2009 Final Research Report
  • [Journal Article] Experimental and simulation study on adsorption of hydrogen isotopes on MS5A at 77 K2007

    • Author(s)
      Munakata K, et. al.
    • Journal Title

      FUSION ENGINEERING AND DESIGN 82

      Pages: 2303-2310

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Kinetics of reaction with water vapor and initio study of titanium beryllide2007

    • Author(s)
      Munakata K, et. al.
    • Journal Title

      JOURNAL OF NUCLEAR MATERIALS 367

      Pages: 1057-1062

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Vacancy solution model formulated by the NRTL equation for correlation of adsorption equilibria2007

    • Author(s)
      Munakata K
    • Journal Title

      JOURNAL OF CHEMICAL ENGINEERING OF JAPAN 40

      Pages: 398-409

    • NAID

      10020086680

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Presentation] CHEMICAL STABILITY OF TITANIUM BERYLLIDE AS NEUTRON MULTIPLIER AT HIGH TEMPERATURES UNDER WATER VAPOR2010

    • Author(s)
      K.Munakata
    • Organizer
      Asian CORE Winter School Technical Program
    • Place of Presentation
      札幌
    • Year and Date
      2010-02-22
    • Related Report
      2009 Annual Research Report
  • [Presentation] Adsorption Characteristics of Water Vapor on Honeycomb Adsorbent2009

    • Author(s)
      Wajima, T., Katekari, K., Munakata, K., Takeishi, T., Hara, K., Wada, K., Inoue, K., Shinozaki, Y., Mochizuki, K., Tanaka, M., Uta, T.
    • Organizer
      14th International Conference on Fusion Reactor Materials (ICFRM-14)
    • Place of Presentation
      Sapporo, Japan
    • Related Report
      2009 Final Research Report
  • [Presentation] Tritium release from ceramic breeder materials deposited with noble metals2009

    • Author(s)
      Mochizuki, K., Munakata, K., Wada, K., Wajima, T., Hara, K., Shinozaki, T., Takeishi, T., Knitter, R., Bekris, N., Fujii, T., Yamana, H., Okuno, K.
    • Organizer
      14th International Conference on Fusion Reactor Materials (ICFRM-14)
    • Place of Presentation
      Sapporo, Japan
    • Related Report
      2009 Final Research Report
  • [Presentation] Oxidation of Hydrogen Isotopes over Honeycomb Catalysts2009

    • Author(s)
      Munakata, K., Wajima, T., Hara, K., Wada, K., Shinozaki, Y., Katekari, K., Mochizuki, K., Tanaka, M., Uta, T.
    • Organizer
      14th International Conference on Fusion Reactor Materials (ICFRM-14)
    • Related Report
      2009 Final Research Report
  • [Presentation] Adsorption Characteristics of Water Vapor on Honeycomb Adsorbent2009

    • Author(s)
      Wajima, T., Katekari, K., Munakata, K., Takeishi, T., Hara, K., Wada, K., Inoue, K., Shinozaki, Y., Mochizuki, K., Tanaka, M., Uta, T.
    • Organizer
      9th International Symposium on Fusion Nuclear Technology (ISFNT-9)
    • Related Report
      2009 Final Research Report
  • [Presentation] Study of Isotope Exchange Reactions on Ceramic Breeder Materials Deposited with Nobel Metal2009

    • Author(s)
      Mochizuki, K., Munakata, K., Hara, K., Wajima, T., Wada, K., Shinozaki, T., Takeishi, T., Knitter, R., Bekris, N., Fujii, T., Yamana, H., Okuno, K.
    • Organizer
      9th International Symposium on Fusion Nuclear Technology (ISFNT-9)
    • Related Report
      2009 Final Research Report
  • [Presentation] Tritium Release Experiments with CATS and Numerical Simulation2009

    • Author(s)
      Munakata, K., Wajima, T., Hara, K., Wada, K., Takeishi, T., Shinozaki, Y., Mochizuki, K., Katekari, K., Kobayashi, K., Iwai, Y., Hayashi, T., Yamanishi, T.
    • Organizer
      9th International Symposium on Fusion Nuclear Technology (ISFNT-9)
    • Related Report
      2009 Final Research Report
  • [Presentation] ハニカム型吸着剤における水分吸着挙動の検討2008

    • Author(s)
      宗像 健三
    • Organizer
      日本原子力学会春の大会
    • Place of Presentation
      大阪大学吹田キャンパス
    • Year and Date
      2008-03-27
    • Related Report
      2008 Annual Research Report
  • [Presentation] ハニカム型吸着剤における水分吸着挙動の検討2008

    • Author(s)
      宗像 健三, 井上 敬太, 篠崎 洋平, 宇田 達彦, 田中 将裕
    • Organizer
      日本原子力学会2008年春の年会
    • Place of Presentation
      大阪大学吹田キャンパス
    • Year and Date
      2008-03-27
    • Related Report
      2007 Annual Research Report
  • [Remarks] ホームページ等

    • Related Report
      2009 Final Research Report

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Published: 2007-04-01   Modified: 2016-04-21  

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