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Core-level photoionization dynamics with vibronic resolution from fixed-in-space molecules

Research Project

Project/Area Number 19550027
Research Category

Grant-in-Aid for Scientific Research (C)

Allocation TypeSingle-year Grants
Section一般
Research Field Physical chemistry
Research InstitutionHigh Energy Accelerator Research Organization

Principal Investigator

ADACHI Jun-ichi  High Energy Accelerator Research Organization, 物質構造科学研究所, 研究機関講師 (10322629)

Co-Investigator(Renkei-kenkyūsha) YAGISHITA Akira  大学共同利用機関法人高エネルギー加速器研究機構, 物質構造科学研究所, 教授 (80157966)
YAMAZAKI Masakazu  東北大学, 多元物質科学研究所, 助教 (00533465)
FUJIKAWA Takashi  千葉大学, 大学院・融合科学研究科, 教授 (30114987)
Project Period (FY) 2007 – 2009
Project Status Completed (Fiscal Year 2009)
Budget Amount *help
¥4,680,000 (Direct Cost: ¥3,600,000、Indirect Cost: ¥1,080,000)
Fiscal Year 2009: ¥650,000 (Direct Cost: ¥500,000、Indirect Cost: ¥150,000)
Fiscal Year 2008: ¥780,000 (Direct Cost: ¥600,000、Indirect Cost: ¥180,000)
Fiscal Year 2007: ¥3,250,000 (Direct Cost: ¥2,500,000、Indirect Cost: ¥750,000)
Keywords内殻分光 / 光電離ダイナミクス / 光電子回折 / 内殻光電離 / 放射光 / 内殼光電離
Research Abstract

Interaction of the soft x-ray with molecules can lead core-level photoionization. We investigated the core-level photoionization of typical and simple molecules in gas phase by means of a coincidence technique. Molecular-frame photoelectron angular distributions and recoil-frame photoelectron angular distributions were obtained for gaseous molecules. We compared between experimental results and calculated ones with x-ray photoelectron diffraction theory to discuss feasibility of new method to determine geometrical structures of gaseous molecules.

Report

(4 results)
  • 2009 Annual Research Report   Final Research Report ( PDF )
  • 2008 Annual Research Report
  • 2007 Annual Research Report
  • Research Products

    (44 results)

All 2010 2009 2008 2007 Other

All Journal Article (20 results) (of which Peer Reviewed: 18 results) Presentation (18 results) Book (1 results) Remarks (5 results)

  • [Journal Article] Theoretical study of x-ray photoelectron diffraction for fixed-in-space CO molecules2010

    • Author(s)
      M. Kazama, J. Adachi, H. Shinotsuka, M. Yamazaki, Y. Ohoria, A. Yagishita, T. Fujikawa
    • Journal Title

      Chem. Phys. accepted

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Photoemission dynamics in the molecular frame2010

    • Author(s)
      A. Yagishita, J. Adachi, M. Yamazaki
    • Journal Title

      J. Phys. Conf. Ser. 212

      Pages: 12010-12010

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Low kinetic energy photoelectron diffractions for C 1s and O 1s electrons of free CO molecules in the EXAFS region2009

    • Author(s)
      J. Adachi, M. Yamazaki, M. Kazama, Y. Ohori, T. Teramoto, Y. Kimura, A. Yagishita, T. Fujikawa
    • Journal Title

      J. Phys. Conf. Ser. 190

      Pages: 12049-12049

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Theoretical study of focusing and double slit effects in x-ray photoelectron diffraction2009

    • Author(s)
      M. Kazama, M. Yamazaki, J. Adachi, A. Yagishita, T. Fujikawa
    • Journal Title

      J. Phys. Conf. Ser. 190

      Pages: 12048-12048

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Dissociative dynamics of C6H6 and C6H5F molecules following carbon 1s and fluorine 1s photoionization studied by 3D momentum imaging method2009

    • Author(s)
      A. Sugishima, K. Nagaya, H. Iwayama, M. Yao, J. Adachi, Y. Kimura, M. Yamazaki, A. Yagishita
    • Journal Title

      J. Chem. Phys. 113

      Pages: 114309-114309

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] 3D mapping of photoemission from a single oriented H2O molecule2009

    • Author(s)
      M. Yamazaki, J. Adachi, T. Teramoto, A. Yagishita, M. Sterner, P. Decleva
    • Journal Title

      J. Phys. B 42

      Pages: 51001-51001

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] 特別企画検出器シリーズ(6)「タイミングを測るI (MCP検出器)」2009

    • Author(s)
      足立純一, 彦坂泰正
    • Journal Title

      放射光 22巻1号

      Pages: 30-38

    • Related Report
      2009 Final Research Report
  • [Journal Article] Low kinetic energy photoelectron diffractions for C 1s and O 1s electrons of free CO molecules in the EXAFS region2009

    • Author(s)
      ADACHI Jun-ichi, YAMAZAKI Masakazu, KAZAMA Misato, (他5名)
    • Journal Title

      J.Phys.Conf.Ser. 190

      Pages: 12049-12049

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Theoretical study of focusing and double slit effects in x-ray photoelectron diffraction2009

    • Author(s)
      KAZAMA Misato, YAMAZAKI Masakazu, ADACHI Jun-ichi, (他2名)
    • Journal Title

      J.Phys.Conf.Ser. 190

      Pages: 12048-12048

    • Related Report
      2009 Annual Research Report
    • Peer Reviewed
  • [Journal Article] 特別企画検出器シリーズ(6)「タイミングを測るI(MCP検出器)」2009

    • Author(s)
      足立純一, 彦坂泰正
    • Journal Title

      放射光 22

      Pages: 30-38

    • Related Report
      2009 Annual Research Report
  • [Journal Article] 3D mapping of photoemission from a single oriented H_2O molecule2009

    • Author(s)
      YAMAZAKI Masakazu, ADACHI Jun-ichi, 他4名
    • Journal Title

      J. Phys. B 42

      Pages: 51001-51001

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Decay channel dependence of the photoelectron angular distributions in core-level ionization of Ne dimmers2008

    • Author(s)
      M. Yamazaki, J. Adachi, Y. Kimura, A. Yagishita, M. Stener, P. Decleva, N. Kosugi, H. Iwayama, K. Nagaya, M. Yao
    • Journal Title

      Phys. Rev. Lett 101

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Decay Channel Dependence of the Photoelectron Angular Distributions in Core-Level Ionization of Ne Dimers2008

    • Author(s)
      YAMAZAKI Masakazu, ADACHI Jun-ichi, 他8名
    • Journal Title

      Phys. Rev. Lett. 101

      Pages: 43004-43004

    • Related Report
      2008 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Extensive study on the C 1s photoionization of CS2 molecules by multi-coincidence velocity-map imaging spectrometry2007

    • Author(s)
      T. Teramoto, J. Adachi, M. Yamazaki, K. Yamanouchi, M. Stener, P. Decleva, A. Yagishita
    • Journal Title

      J. Phys. B 40

      Pages: 4033-4046

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Photoelectron-photoion-photoion momentum spectroscopy as a direct probe of the core-hole localization in C 1s photoionization of C2H22007

    • Author(s)
      J. Adachi, K. Hosaka, T. Teramoto, M. Yamazaki, N. Watanabe, M. Takahashi, A. Yagishita
    • Journal Title

      J. Phys. B 40

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] New approach for a complete experiment: C1s photoionization in CO2 molecules2007

    • Author(s)
      T. Teramoto, J. Adachi, K. Hosaka, M. Yamazaki, K. Yamanouchi, N.A. Cherepkov, M. Stener, P. Decleva, A. Yagishita
    • Journal Title

      J. Phys. B 40

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Experimental evidence of interatomic resonant Auger electron emission from fixed-in-space NO molecules2007

    • Author(s)
      M. Yamazaki, J. Adachi, T. Teramoto, A. Yagishita
    • Journal Title

      J. Phys. B 40

    • Related Report
      2009 Final Research Report
    • Peer Reviewed
  • [Journal Article] Photoelectron-photoion-photoion momentum spectroscopy as a direct probe of the core-hole localization in C ls photoionization of C_2H_22007

    • Author(s)
      ADACHI Jun-ichi (他6名)
    • Journal Title

      J. Phys. B 40

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] Experimental evidence of interatomic resonant Auger electron emission from fixed-in-space NO molecules2007

    • Author(s)
      YAMAZAKI Masakazu, ADACHI Jun-ichi(他2名)
    • Journal Title

      J. Phys. B 40

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Journal Article] New approach for a complete experiment: Cls photoionization in CO_2 molecules2007

    • Author(s)
      TERAMOTO Takahiro, ADACHI, Jun-ichi(他7名)
    • Journal Title

      J. Phys. B 40

    • Related Report
      2007 Annual Research Report
    • Peer Reviewed
  • [Presentation] EXAFS領域におけるCO分子の分子座標系内殻光電子角度分布2009

    • Author(s)
      足立純一, 山崎優一, (他6名)
    • Organizer
      日本物理学会2009年秋季大会
    • Place of Presentation
      熊本大学黒髪キャンパス(熊本)
    • Year and Date
      2009-09-27
    • Related Report
      2009 Annual Research Report
  • [Presentation] Low kinetic energy photoelectron diffractions for C 1s and O 1s electrons of free CO molecules in the EXAFS region2009

    • Author(s)
      ADACHI Jun-ichi, YAMAZAKI Masakazu, (他6名)
    • Organizer
      14th Intergational Conference on X-ray Absorption Fine Structure
    • Place of Presentation
      Camerino (Italy)
    • Year and Date
      2009-07-30
    • Related Report
      2009 Annual Research Report
  • [Presentation] Evidence of selective bond breaking induced by dynamical core-hole localization : Measurement of O 1s photoelectron angular distributions relative to the dissociation axis for CO_2 molecules2009

    • Author(s)
      足立純一, 山崎優一, 寺本高啓, 木村恭之, 柳下明
    • Organizer
      第25回化学反応討論会
    • Place of Presentation
      大宮ソニックシティ(大宮)
    • Year and Date
      2009-06-01
    • Related Report
      2009 Annual Research Report
  • [Presentation] Interferences and scatterings of photoelectron partial waves in core-level photoionization : Photoelectron angular distributions in coincidence measurements of photoelectrons and photoions2009

    • Author(s)
      ADACHI Jun-ichi
    • Organizer
      The 13th East Asian Workshop on Chemical Reactions
    • Place of Presentation
      Howard International Hotel (台北;台湾)
    • Year and Date
      2009-03-19
    • Related Report
      2008 Annual Research Report
  • [Presentation] 口頭27pZB-2「EXAFS領域におけるCO分子の分子座標系内殻光電子角度分布」2009

    • Author(s)
      足立純一, 山崎優一, 寺本高啓, 木村恭之, 柳下明, 風間美里, 大堀祐輔, 藤川高志
    • Organizer
      日本物理学会2009年秋季大会
    • Place of Presentation
      熊本
    • Related Report
      2009 Final Research Report
  • [Presentation] Poster PS2-191“Low kinetic energy photoelectron diffractions for C 1s and O 1s electrons of free CO molecules in the EXAFS region"2009

    • Author(s)
      J. Adachi, M. Yamazaki, T. Teramoto, Y. Kimura, A. Yagishita, M. Kazama, Y. Ohori, T. Fujikawa
    • Organizer
      14th International Conference on X-ray Absorption Fine Structure, Camerino
    • Place of Presentation
      Italy
    • Related Report
      2009 Final Research Report
  • [Presentation] ポスター1P54“Evidence of selective bond breaking induced by dynamical core-hole localization: Measurement of O 1s photoelectron angular distributions relative to the dissociation axis for CO2 molecules"2009

    • Author(s)
      足立純一, 山崎優一, 寺本高啓, 木村恭之, 柳下明
    • Organizer
      第25回化学反応討論会
    • Place of Presentation
      大宮
    • Related Report
      2009 Final Research Report
  • [Presentation] ポスターP-UG12-05「EXAFS領域における2原子分子の分子座標系光電子角度分布」2009

    • Author(s)
      足立純一, 山崎優一, 木村恭之, 柳下明, 風間美里, 大堀祐輔, 藤川高志
    • Organizer
      第26回PFシンポジウム
    • Place of Presentation
      つくば
    • Related Report
      2009 Final Research Report
  • [Presentation] Interferences and scatterings of photoelectron partial waves in core-level photoionization: Photoelectron angular distributions in coincidence measurements of photoelectrons and photoions2009

    • Author(s)
      J. Adachi
    • Organizer
      13th East Asian Workshop on Chemical Reactions
    • Place of Presentation
      台北(台湾)
    • Related Report
      2009 Final Research Report
  • [Presentation] 気相CO分子についての低速光電子回折パターン測定2008

    • Author(s)
      足立純一, 他7名
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡国際会議場(福岡)
    • Year and Date
      2008-09-27
    • Related Report
      2008 Annual Research Report
  • [Presentation] 口頭4C15「気相CO分子についての低速光電子回折パターン測定」2008

    • Author(s)
      足立純一, 山崎優一, 木村恭之, 風間美里, 大堀祐輔, 篠塚寛志, 藤川高志, 柳下明
    • Organizer
      第2回分子科学討論会
    • Place of Presentation
      福岡
    • Related Report
      2009 Final Research Report
  • [Presentation] ポスターP05「運動エネルギー150 eVまでの直線分子の分子座標系光電子角度分布」2008

    • Author(s)
      足立純一, 山崎優一, 寺本高啓, 木村恭之, 柳下明
    • Organizer
      原子衝突研究協会第33回研究会
    • Place of Presentation
      札幌
    • Related Report
      2009 Final Research Report
  • [Presentation] 直線分子の光電子放出における分子座標系角度分布での干渉パターン2007

    • Author(s)
      足立 純一
    • Organizer
      第1回分子科学討論会
    • Place of Presentation
      東北大学川内北キャンパス
    • Year and Date
      2007-09-20
    • Related Report
      2007 Annual Research Report
  • [Presentation] 口頭22aRF-6「H2CO分子の内殻光電離における解離軸に対する光電子角度分布測定」2007

    • Author(s)
      足立純一, 山崎優一, 岩山洋士, 村上仁, 永谷清信, 八尾誠, 柳下明
    • Organizer
      第62回日本物理学会年次大会
    • Place of Presentation
      札幌
    • Related Report
      2009 Final Research Report
  • [Presentation] 口頭4C03「直線分子の光電子放出における分子座標系角度分布での干渉パターン」2007

    • Author(s)
      足立純一, 山崎優一, 寺本高啓, 穂坂綱一, 柳下明
    • Organizer
      第1回分子科学討論会
    • Place of Presentation
      仙台
    • Related Report
      2009 Final Research Report
  • [Presentation] Oral Mon3-1“Direct observation of core-hole localization in C 1s photoionization of C2H2 by photoelectronphotoion- photoion momentum spectroscopy"2007

    • Author(s)
      J. Adachi, K. Hosaka, T. Teramoto, M. Yamazaki, N. Watanabe, M. Takahashi, A. Yagishita
    • Organizer
      15th International Conference on Vacuum Ultraviolet Radiation Physics, Berlin
    • Place of Presentation
      Germany
    • Related Report
      2009 Final Research Report
  • [Presentation] Poster Tu027“Vector correlations in carbon 1s photoionizations and followed fragmentations for C2H2 molecules"2007

    • Author(s)
      J. Adachi, K. Hosaka, T. Teramoto, M. Yamazaki, N. Watanabe, M. Takahashi, A. Yagishita
    • Organizer
      XXV International Conference on Photonic, Electronic and Atomic Collisions, Freiburg
    • Place of Presentation
      Germany
    • Related Report
      2009 Final Research Report
  • [Presentation] 口頭1A3「D∞h点群分子の内殻光電子放出における分子座標系角度分布での干渉パターン」2007

    • Author(s)
      足立純一, 山崎優一, 寺本高啓, 穂坂綱一, 柳下明
    • Organizer
      第23回化学反応討論会
    • Place of Presentation
      神戸
    • Related Report
      2009 Final Research Report
  • [Book] KEK Proceedings 2008-19(BL-2Cユーザー研究会:PFの挿入光源における新しい研究の探究)2009

    • Author(s)
      手塚泰久, 組頭広志, 足立純一共編
    • Total Pages
      79
    • Related Report
      2009 Final Research Report
  • [Remarks] 足立純一,「放射光による気相分子の内殻分光・ダイナミクス」PF-上智大放射光物質生命理工学研究会(つくば), 9/29,30 (2009).

    • Related Report
      2009 Final Research Report
  • [Remarks] 足立純一,奨励賞受賞講演「気相分子についての軟X線分光手法の開発と光電離・光解離ダイナミクスの研究」,第3回分子科学討論会(名古屋), 9/22 (2009).

    • Related Report
      2009 Final Research Report
  • [Remarks] 足立純一,「強レーザー場中の原子分子の軟X線放射光による観測の試み」,東大物性研究所短期研究会“高輝度VSX光源が切り拓く先端分光と物性研究への展開"(柏) 7/23,24 (2009).

    • Related Report
      2009 Final Research Report
  • [Remarks] 足立純一「放射光による気相分子の光電離・光解離ダイナミクスの研究」,東邦大学理学部2008年度第4回物理学科コロキウム(船橋) 12/19 (2008).

    • Related Report
      2009 Final Research Report
  • [Remarks] 足立純一「分子配向選択した光電子角度分布で探る分子光電離ダイナミクス」,第4回原子分子光科学討論会(調布) 6/8-9 (2007).○受賞2008年9月,分子科学会奨励賞(分子科学会)受賞;研究課題「気相分子についての軟X線分光手法の開発と光電離・光解離ダイナミクスの研究」

    • Related Report
      2009 Final Research Report

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Published: 2007-04-01   Modified: 2018-02-02  

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